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RESEARCH PAPER · Chemical Society Reviews · 2017

Controlling cation segregation in perovskite-based electrodes for high electro-catalytic activity and durability

Yifeng Li, Wenqiang Zhang, Yun Hong Zheng, Jing Wen Chen, Bo Hao Yu, Yan Chen, Meilin Liu

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Controlling cation segregation in perovskite-based electrodes for high electro-catalytic activity and durabilityOriginalAn In Situ Formed, Dual‐Phase Cathode with a Highly Active Catalyst Coating for Protonic Ceramic Fuel Cells144Nanomaterials and technologies for low temperature solid oxide fuel cells: Recent advances, challenges and opportunities501Designing a protonic ceramic fuel cell with novel electrochemically active oxygen electrodes based on doped Nd 0.5 Ba 0.5 FeO 3−δ45Thermally stable and coking resistant CoMo alloy-based catalysts as fuel electrodes for solid oxide electrochemical cells27Morphologically well-defined Gd0.1Ce0.9O1.95 embedded Ba0.5Sr0.5Co0.8Fe0.2O3-δ nanofiber with an enhanced triple phase boundary as cathode for low-temperature solid oxide fuel cells50Durability and performance of CGO barriers and LSCF cathode deposited by spray-pyrolysis35Highly Active and Stable Cobalt-Free Hafnium-doped SrFe0.9Hf0.1O3−δ Perovskite Cathode for Solid Oxide Fuel Cells50Oxygen Sponges for Electrocatalysis: Oxygen Reduction/Evolution on Nonstoichiometric, Mixed Metal Oxides71A facile surface chemistry approach to bifunctional excellence for perovskite electrocatalysis74Exploration of Co-Fe alloy precipitation and electrochemical behavior hysteresis using Lanthanum and Cobalt co-substituted SrFeO3-δ SOFC anode67Recent Advances in Novel Nanostructuring Methods of Perovskite Electrocatalysts for Energy‐Related Applications407Cation Segregation of A-Site Deficiency Perovskite La0.85FeO3−δ Nanoparticles toward High-Performance Cathode Catalysts for Rechargeable Li-O2 Battery39Oxygen reduction kinetic enhancements of intermediate-temperature SOFC cathodes with novel Nd0.5Sr0.5CoO3-δ/Nd0.8Sr1.2CoO4±δ heterointerfaces82Sr Segregation in Perovskite Oxides: Why It Happens and How It Exists516A novel heterogeneous La0.8Sr0.2CoO3−δ/(La0.5Sr0.5)2CoO4+δ dual‐phase membrane for oxygen separation11Enhanced electrochemical performance of Ca-doped NdBa1-xCaxCoCuO5+δ as cathode material for intermediate-temperature solid oxide fuel cells41Segregation Induced Self‐Assembly of Highly Active Perovskite for Rapid Oxygen Reduction Reaction50Impact of Strain-Induced Changes in Defect Chemistry on Catalytic Activity of Nd2NiO4+δ Electrodes44Gas Humidification Impact on the Properties and Performance of Perovskite‐Type Functional Materials in Proton‐Conducting Solid Oxide Cells133Micro‐/Nanohoneycomb Solid Oxide Electrolysis Cell Anodes with Ultralarge Current Tolerance63Solid Oxide Fuel Cell Materials and Interfaces4Improving the Electrocatalytic Activity and Durability of the La0.6Sr0.4Co0.2Fe0.8O3−δ Cathode by Surface Modification115In situ synthesis of supported metal nanocatalysts through heterogeneous doping101Acceptor-doped La1.9M0.1Ce2O7 (M = Nd, Sm, Dy, Y, In) proton ceramics and in-situ formed electron-blocking layer for solid oxide fuel cells applications44A self-recovering robust electrode for highly efficient CO 2 electrolysis in symmetrical solid oxide electrolysis cells70Anionic defect engineering of transition metal oxides for oxygen reduction and evolution reactions378Controlling surface cation segregation in a nanostructured double perovskite GdBaCo 2 O 5+δ electrode for solid oxide fuel cells32Fundamental Insights On The Electrolysis Of Co2 Using Solid Oxide Electrolysis Cells0Gamma-Bi 4 V 2 O 11 – a layered oxide material for ion exchange in aqueous media11Segregation Resistant Nanocrystalline/Amorphous (La, Sr) CoO3-(La,Sr)2CoO4 Composite Cathodes for IT-SOFCs7Stable high current density operation of La 0.6 Sr 0.4 Co 0.2 Fe 0.8 O 3−δ oxygen electrodes39Surface recrystallization – an underestimated phenomenon affecting oxygen exchange activity30Study of the relationship between the local geometric structure and the stability of La0.6Sr0.4MnO3−δ and La0.6Sr0.4FeO3−δ electrodes10Multifactor performance analysis of reversible solid oxide cells based on proton-conducting electrolytes48Uncovering the Effect of Lattice Strain and Oxygen Deficiency on Electrocatalytic Activity of Perovskite Cobaltite Thin Films235Cation-swapped homogeneous nanoparticles in perovskite oxides for high power density178New insights into element migration on La0.6Sr0.4Co0.2Fe0.8O3-δ cathodes of intermediate temperature solid oxide fuel cells27Stability and electrochemical performance of nanostructured La2CuO4+δ cathodes20Morphology evolution and exsolution mechanism of a partially decomposed anode for intermediate temperature-solid oxide fuel cells29A discussion on mathematical models of proton conducting Solid Oxide Fuel Cells17Nanoengineering of solid oxide electrochemical cell technologies: An outlook30Nickel enriched Ruddlesden-Popper type lanthanum strontium manganite as electrode for symmetrical solid oxide fuel cell54Enhancing catalysis activity of La0.6Sr0.4Co0.8Fe0.2O3-δ cathode for solid oxide fuel cell by a facile and efficient impregnation process63Enhancing coking resistance of Ni/YSZ electrodes: In situ characterization, mechanism research, and surface engineering107A novel multilaminated composite cathode for solid oxide fuel cells11Oxygen Deficient LaMn0.75Co0.25O3−δ Nanofibers as an Efficient Electrocatalyst for Oxygen Evolution Reaction and Zinc–Air Batteries114Improving the Activity for Oxygen Evolution Reaction by Tailoring Oxygen Defects in Double Perovskite Oxides314Re-evaluation of La0.6Sr0.4Co0.2Fe0.8O3-δ hollow fiber membranes for oxygen separation after long-term storage of five and ten years48Enhancement of the SrTiO 3 Surface Reactivity by Exposure to Electric Fields26Surface Reconstruction under the Exposure of Electric Fields Enhances the Reactivity of Donor-Doped SrTiO 333Identifying the Origin of the Limiting Process in a Double Perovskite PrBa 0.5 Sr 0.5 Co 1.5 Fe 0.5 O 5+δ Thin-Film Electrode for Solid Oxide Fuel Cells37Effect of Microstructure on the Degradation of La0.6Sr0.4CoO3–δ Electrodes in Dry and Humid Atmospheres15La 0.6 Sr 0.4 Co 0.2 Fe 0.8 O 3−δ /CeO 2 Heterostructured Composite Nanofibers as a Highly Active and Robust Cathode Catalyst for Solid Oxide Fuel Cells149Co-electrolysis of H2O and CO2 on exsolved Ni nanoparticles for efficient syngas generation at controllable H2/CO ratios94Nickel Exsolution‐Driven Phase Transformation from an n=2 to an n=1 Ruddlesden‐Popper Manganite for Methane Steam Reforming Reaction in SOFC Conditions46Impact of the Sintering Additive Al2O3 on the Electrical Conductivity of Proton-Conducting Electrolyte CaZr0.95Sc0.05O3 – δ5Correlation of Time-Dependent Oxygen Surface Exchange Kinetics with Surface Chemistry of La0.6Sr0.4Co0.2Fe0.8O3−δ Catalysts65Dual core-shell structured g-C3N4@Fe/Sr@g-C3N4 porous nanosphere as high efficient oxygen reduction reaction electrocatalyst in both acidic and alkaline media for fuel cells26Surface modification of SOFC cathodes by Co, Ni, and Pd oxides33Efficient and stable symmetrical electrode La0.6Sr0.4Co0.2Fe0.7Mo0.1O3–δ for direct hydrocarbon solid oxide fuel cells26Heterointerface engineering for enhancing the electrochemical performance of solid oxide cells319Unveiling Lithium Roles in Cobalt‐Free Cathodes for Efficient Oxygen Reduction Reaction below 600 °C16Sistema de baja dimensionalidad para aplicaciones fotovoltaicas y optoelectrónicas0Structural and electrochemical property evolutions of perovskite SOFC anodes: Role of fuel atmosphere in (La0.4Sr0.6)1-Co0.2Fe0.7Nb0.1O3-δ24Revising the role of chromium on the surface of perovskite electrodes: Poison or promoter for the solid oxide electrolysis cell performance?13Catalytic Steam Reforming of Natural Gas over a New Ni Exsolved Ruddlesden‐Popper Manganite in SOFC Anode Conditions16Construction of Heterointerfaces with Enhanced Oxygen Reduction Kinetics for Intermediate-Temperature Solid Oxide Fuel Cells29Control of transition metal–oxygen bond strength boosts the redox ex-solution in a perovskite oxide surface78How an angstrom-thick oxide overcoat enhances durability and activity of nanoparticle-decorated cathodes in solid oxide fuel cells13In situ exsolved Co nanoparticles coupled on LiCoO 2 nanofibers to induce oxygen electrocatalysis for rechargeable Zn–air batteries45Piezotronic-enhanced oxygen evolution reaction enabled by a Au/MoS 2 nanosheet catalyst31Ruddlesden–Popper perovskites in electrocatalysis330Solid Oxide Fuel Cell Materials and Interfaces3Structural evolution, electrochemical kinetic properties, and stability of A-site doped perovskite Sr 1−x Yb x CoO 3−δ28Suitability of strontium and cobalt-free perovskite cathodes with La 9.67 Si 5 AlO 26 apatite electrolyte for intermediate temperature solid oxide fuel cells2Pr2NiO4-Pr0.2Ce0·8O1.9 composite cathode as a potential cathode material for intermediate temperature solid oxide fuel cells46Oxygen vacancies-rich Ce0.9Gd0.1O2-δ decorated Pr0.5Ba0.5CoO3-δ bifunctional catalyst for efficient and long-lasting rechargeable Zn-air batteries117Surface Reorganization on Electrochemically‐Induced Zn–Ni–Co Spinel Oxides for Enhanced Oxygen Electrocatalysis296Surface Reorganization on Electrochemically‐Induced Zn–Ni–Co Spinel Oxides for Enhanced Oxygen Electrocatalysis96Tuning interfacial chemistry and electrochemical properties of solid oxide cells via cation interdiffusion6Polar or not polar? The interplay between reconstruction, Sr enrichment, and reduction at the La0.75Sr0.25MnO3 (001) surface28Silver-Modified Ba 1– x Co 0.7 Fe 0.2 Nb 0.1 O 3−δ Perovskite Performing as a Cathodic Catalyst of Intermediate-Temperature Solid Oxide Fuel Cells35Enhancing Activity and Durability of A-Site-Deficient (La0.6Sr0.4)0.95Co0.2Fe0.8O3−δ Cathode by Surface Modification with PrO2−δ Nanoparticles101Study on Ca Segregation toward an Epitaxial Interface between Bismuth Ferrite and Strontium Titanate12Activation-free supercapacitor electrode based on surface-modified Sr2CoMo1-xNixO6-δ perovskite64In-situ growth of nanoparticles-decorated double perovskite electrode materials for symmetrical solid oxide cells153The role of A-site cation size mismatch in tune the catalytic activity and durability of double perovskite oxides66In situ embedding of CoFe nanocatalysts into Sr3FeMoO7 matrix as high-performance anode materials for solid oxide fuel cells53Self-sustainable protonic ceramic electrochemical cells using a triple conducting electrode for hydrogen and power production497Review on exsolution and its driving forces in perovskites138Exceptional Tunability over Size and Density of Spontaneously Formed Nanoparticles via Nucleation Dynamics38Atomic‐Scale Insight into Exsolution of CoFe Alloy Nanoparticles in La 0.4 Sr 0.6 Co 0.2 Fe 0.7 Mo 0.1 O 3− δ with Efficient CO 2 Electrolysis185Atomic‐Scale Insight into Exsolution of CoFe Alloy Nanoparticles in La0.4Sr0.6Co0.2Fe0.7Mo0.1O3−δ with Efficient CO2 Electrolysis6In Situ Exsolved Metal Nanoparticles: A Smart Approach for Optimization of Catalysts163N doped carbon coated multi-metals nanoparticles decorated perovskite as electrocatalyst for efficient hydrogen evolution reaction33Nickel exsolution effect on the catalytic behavior of ruddlesden-popper manganites in sofc conditions using colombian natural gas0Methane steam reforming in water-deficient conditions on a new Ni-exsolved Ruddlesden-Popper manganite: Coke formation and H2S poisoning24A facile top-down approach for constructing perovskite oxide nanostructure with abundant oxygen defects as highly efficient water oxidation electrocatalyst25Sr- and Mo-deficiency Sr1.95TiMo1−O6– double perovskites as anodes for solid-oxide fuel cells using H2S-containing syngas19Computational approaches to the exsolution phenomenon in perovskite oxides with a view to design highly durable and active anodes for solid oxide fuel cells13Enhanced Cr tolerance of perovskite oxide via Gd0.1Ce0.9O2 surface modifications13Structure and electrochemical properties of titanate perovskite with in situ exsolution as a ceramic electrode material9Surface Segregation in Solid Oxide Cell Oxygen Electrodes: Phenomena, Mitigation Strategies and Electrochemical Properties216Development of Stable Oxygen Carrier Materials for Chemical Looping Processes—A Review151Highly active dry methane reforming catalysts with boosted in situ grown Ni-Fe nanoparticles on perovskite via atomic layer deposition165A highly active and carbon-tolerant anode decorated with in situ grown cobalt nano-catalyst for intermediate-temperature solid oxide fuel cells88Efficient bifunctional electrocatalysts for solid oxide cells based on the structural evolution of perovskites with abundant defects and exsolved CoFe nanoparticles72A comparative study of surface segregation and interface of La0·6Sr0·4Co0·2Fe0·8O3-δ electrode on GDC and YSZ electrolytes of solid oxide fuel cells77A Mini Review on the Application of Proton-Conducting Solid Oxide Cells for CO 2 Conversion32Controlling cation migration and inter-diffusion across cathode/interlayer/electrolyte interfaces of solid oxide fuel cells: A review116Chromium poisoning for prolonged lifetime of electrodes in solid oxide fuel cells - Review81Photocatalyseurs hétérostructurés LaFeO₃/g-C₃N₄ pour la production d’hydrogène0New Insight into the Doped Strontium Titanate Cathode with In Situ Exsolved Nickel Nanoparticles for Electrolysis of Carbon Dioxide26Effects of surface chemical potentials on cation segregation29Nanoparticle Ex-solution for Supported Catalysts: Materials Design, Mechanism and Future Perspectives181Defect engineering of oxide perovskites for catalysis and energy storage: synthesis of chemistry and materials science335Enhancement of the electrocatalytic activity of La0.6Sr0.4Co0.2Fe0.8O3-δ through surface modification by acid etching24Iron-based electrode materials for solid oxide fuel cells and electrolysers129Promotion of oxygen reduction reaction on a double perovskite electrode by a water-induced surface modification132Single-atom catalysis in advanced oxidation processes for environmental remediation1022Study on the strontium segregation behavior of lanthanum strontium cobalt ferrite electrode under compression27Manipulating Surface Termination of Perovskite Manganate for Oxygen Activation44Progress of Exsolved Metal Nanoparticles on Oxides as High Performance (Electro)Catalysts for the Conversion of Small Molecules120Fe2+‐Induced In Situ Intercalation and Cation Exsolution of Co80Fe20(OH)(OCH3) with Rich Vacancies for Boosting Oxygen Evolution Reaction88A review of the chemical compatibility between oxide electrodes and electrolytes in solid oxide fuel cells89Enhancing Oxygen Reduction Activity and Cr Tolerance of Solid Oxide Fuel Cell Cathodes by a Multiphase Catalyst Coating114In situ exsolution of metallic Cu in mixed oxides as battery-type electrode for energy storage devices20An Elementary Kinetic Model for the LSCF and LSCF-CGO Electrodes of Solid Oxide Cells: Impact of Operating Conditions and Degradation on the Electrode Response38In Situ Exsolution of Noble-Metal Nanoparticles on Perovskites as Enhanced Peroxidase Mimics for Bioanalysis59Perovskite Cathode Materials for Low-Temperature Solid Oxide Fuel Cells: Fundamentals to Optimization99High-Performance-Based Perovskite-Supported Nanocomposite for the Development of Green Energy Device Applications: An Overview29Improving the activity and stability of Ni-based electrodes for solid oxide cells through surface engineering: Recent progress and future perspectives34Lattice contraction tailoring in perovskite oxides towards improvement of oxygen electrode catalytic activity65Flat-tubular solid oxide fuel cells and stacks: a review76Effectively Promoting Activity and Stability of a MnCo2O4-Based Cathode by In Situ Constructed Heterointerfaces for Solid Oxide Fuel Cells50Smart Construction of an Intimate Lithium | Garnet Interface for All‐Solid‐State Batteries by Tuning the Tension of Molten Lithium152Atomic Layer Deposition of Iron, Cobalt, and Nickel Chalcogenides: Progress and Outlook28Recent development of perovskite oxide-based electrocatalysts and their applications in low to intermediate temperature electrochemical devices210Cathode infiltration with enhanced catalytic activity and durability for intermediate-temperature solid oxide fuel cells43Recent progress in nanostructured electrodes for solid oxide fuel cells deposited by spray pyrolysis66Perovskite La0.3Sr0.7Fe0.7Cr0.3O3−δ Catalysis Raises the Bar: Preventing Unwanted Near‐Surface Sr Segregation and SrCO3 Precipitation2Strategy to Elucidate the Reaction Mechanism of Electrodes for Realistic Solid Oxide Electrochemical Cells Using a Dense Bulk Material11Modulating Reaction Pathways on Perovskite Cobaltite Nanofibers through Excessive Surface Oxygen Defects for Efficient Water Oxidation13Solid Oxide Fuel Cells: Reactions0Promoting exsolution of RuFe alloy nanoparticles on Sr2Fe1.4Ru0.1Mo0.5O6−δ via repeated redox manipulations for CO2 electrolysis268Comprehensive understanding of alkaline-earth elements effects on electrocatalytic activity and stability of LaFe0.8Ni0.2O3 electrode for high-temperature CO2 electrolysis14Efficient symmetrical electrodes based on LaCrO3 via microstructural engineering14Enhancing the Intrinsic Activity and Stability of Perovskite Cobaltite at Elevated Temperature Through Surface Stress56Enhanced photoelectrocatalytic hydrogen evolution using off-stoichiometry La0.43FeOy films3An Efficient Symmetric Electrolyzer Based On Bifunctional Perovskite Catalyst for Ammonia Electrolysis90

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  4. Thermally stable and coking resistant CoMo alloy-based catalysts as fuel electrodes for solid oxide electrochemical cells

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  36. Cation-swapped homogeneous nanoparticles in perovskite oxides for high power density

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  37. New insights into element migration on La0.6Sr0.4Co0.2Fe0.8O3-δ cathodes of intermediate temperature solid oxide fuel cells

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  39. Morphology evolution and exsolution mechanism of a partially decomposed anode for intermediate temperature-solid oxide fuel cells

    Electrochimica Acta · 2019-02-27

    Jingwei Li, Bo Wei, Xing Yue, Huan Li, Zhe Lü

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  40. A discussion on mathematical models of proton conducting Solid Oxide Fuel Cells

    International Journal of Hydrogen Energy · 2019-03-21

    JAROSLAW MILEWSKI, Arkadiusz Szczęśniak, Łukasz Szabłowski

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  41. Nanoengineering of solid oxide electrochemical cell technologies: An outlook

    Nano Research · 2019-03-30

    Juliana S. A. Carneiro, Eranda Nikolla

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  42. Nickel enriched Ruddlesden-Popper type lanthanum strontium manganite as electrode for symmetrical solid oxide fuel cell

    Journal of Power Sources · 2019-04-10

    Zheqiang Xu, Yihang Li, Yanhong Wan, Shaowei Zhang, Changrong Xia

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  43. Enhancing catalysis activity of La0.6Sr0.4Co0.8Fe0.2O3-δ cathode for solid oxide fuel cell by a facile and efficient impregnation process

    International Journal of Hydrogen Energy · 2019-04-12

    Haocong Wang, Xiong Zhang, Wenwen Zhang, Zhenye Wei, Kai Guan, Junling Meng, Fanzhi Meng, Jian Meng, Xiaojuan Liu

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  44. Enhancing coking resistance of Ni/YSZ electrodes: In situ characterization, mechanism research, and surface engineering

    Nano Energy · 2019-05-11

    Wangxu Yue, Yifeng Li, Yun Hong Zheng, Tong Wu, Chenhuan Zhao, Jia Chang Zhao, Ga Geng, Wenqiang Zhang, Jing Chen, Jianxin Zhu, Bo Hao Yu

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  45. A novel multilaminated composite cathode for solid oxide fuel cells

    Ceramics International · 2019-05-28

    Lucía dos Santos‐Gómez, Jose Manuel Porras-Vázquez, Francisco Martín, José Ramón Ramos-Barrado, Enrique R. Losilla, David Marrero‐López

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  46. Oxygen Deficient LaMn0.75Co0.25O3−δ Nanofibers as an Efficient Electrocatalyst for Oxygen Evolution Reaction and Zinc–Air Batteries

    Inorganic Chemistry · 2019-06-05

    Juanjuan Bian, Zhipeng Li, Nianwu Li, Chunwen Sun

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  47. Improving the Activity for Oxygen Evolution Reaction by Tailoring Oxygen Defects in Double Perovskite Oxides

    Advanced Functional Materials · 2019-06-07

    Yunmin Zhu, Lei Zhang, Bote Zhao, Huijun Chen, Liu Xi, Ran Zhao, Xinwei Wang, Jiang Liu, Yan Chen, Meilin Liu

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  48. Re-evaluation of La0.6Sr0.4Co0.2Fe0.8O3-δ hollow fiber membranes for oxygen separation after long-term storage of five and ten years

    Journal of Membrane Science · 2019-06-10

    Ning Han, Chi Zhang, Xiaoyao Tan, Zhigang Wang, Sibudjing Kawi, Shaomin Liu

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  49. Enhancement of the SrTiO 3 Surface Reactivity by Exposure to Electric Fields

    ChemNanoMat · 2019-06-11

    Kurt Klauke, Buğra Kayaalp, Mattia Biesuz, Alessandro Iannaci, Vincenzo M. Sglavo, Massimiliano D’Arienzo, Siwon Lee, Jongsu Seo, WooChul Jung, Simone Mascotto

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  50. Surface Reconstruction under the Exposure of Electric Fields Enhances the Reactivity of Donor-Doped SrTiO 3

    The Journal of Physical Chemistry C · 2019-06-13

    Buğra Kayaalp, Kurt Klauke, Mattia Biesuz, Alessandro Iannaci, Vincenzo M. Sglavo, Massimiliano D’Arienzo, Heshmat Noei, Siwon Lee, WooChul Jung, Simone Mascotto

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