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RESEARCH PAPER · Angewandte Chemie International Edition · 2025

pH‐Dependent Switching Between Nonlinear‐Optical‐Active Nitrate‐Based Supramolecular Polymorphs

Qiao Xia, Xingxing Jiang, Chunbo Jiang, Haijun Zhang, Yilei Hu, Qi Lu, Chao Wu, Guangfeng Wei, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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pH‐Dependent Switching Between Nonlinear‐Optical‐Active Nitrate‐Based Supramolecular PolymorphsOriginalPhase transition engineering to break the symmetry of diamond-like chalcogenide for second-order nonlinear optics2Y(C 6 H 5 SO 3 ) 3 ·9H 2 O: strategic integration of ligand substitution and π-conjugated group linkage in sulfates for enhanced ultraviolet nonlinear optical properties4(CN4H7)H2C3N3S3: Trithiocyanurate Exhibiting Giant Optical Anisotropy via Weak Interaction-Mediated Functional Module Alignment3Enhancing Birefringence via a Planar‐Conformation‐Locking Strategy3From centrosymmetric CN3H6C6H5SO3 to non-centrosymmetric CN3H6C6H4SO3(OH): Hydroxyl introduced hydrogen bond reconstruction to realize strong second harmonic generation3Research on Nonlinear Optical Materials Based on BO 3 and BO 4 Hydroxy Tetraborates4Organic Halogen Substitution-Driven Halogen Bonding Induces Polar 3D Supramolecular Framework and Second-Harmonic-Generation Response7pH‐Regulated Ring‐Opening/Closing Transformation in Polyoxometalates Enables High‐Performance Nonlinear Optical Crystals13Hydroxyl-induced structural reconstruction: two new potassium hepta-borates with deep-UV transparency and enhanced birefringence1Chiral-Unit-Driven Short-Wave Ultraviolet Nonlinear Optical Acetates with Balanced Overall Optical Properties3Design of borate-squarate hybrid crystals with large birefringence by synergistic assembly of planar π-conjugated groups0Halogen-ion-driven polymorphs for high-performance nonlinear optical crystalline materials3Isoniazid nitrate: synergistic dual π-conjugation triggering prominent second-harmonic generation0Stable lead succinate-iodides with strong second-harmonic generation response and large birefringence0Vapochromic methanol recoordination and spin-state switching in square-planar Ni( ii ) complexes derived from trans - and cis -coordinated precursors0The modulation of structural polarity facilitating the gradient enhancement of second harmonic generation effects in hybrid metal halides5The charge transfer mechanism and optimization strategy for two-photon absorption properties of A-π-A symmetric dyes in the near-infrared region0An Ultra-Wide Bandgap Sulfonate with Two-Step Second-Harmonic Generation Switching2Chirality-driven polar lattice engineering for high-performance organic nonlinear optical crystals3Recent Progress in Hg-Based Oxysalt Crystals for Nonlinear Optics and Birefringence Applications5Steric hindrance and hydrogen-bond networks synergistically directing molecular alignment for high-performance ultraviolet birefringent1Reverse Weak Polarity‐Induced Ordered Layer Control for Enhanced Second‐Harmonic Generation in Ultraviolet Nonlinear Optical Crystals2Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals1Symmetry Breaking Induced by Hydration-Number Tuning Enables Second-Order Nonlinear Optical Responses in Lanthanum Sulfate Hydrates0Exceptional Solar‐Blind Birefringence Engineered by Complementary Hydrogen‐Bond Ordering of π‐Conjugated Units0Record Second-Harmonic Generation and Exceptional Optical Anisotropy in High-Symmetry 1D Polar Perovskites1The Parallel Coplanar Alignment of Planar Non‐π‐Conjugated [Pb 3 Br 3 ] Rings for a Stable Ultraviolet Nonlinear Optical Crystal0

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  1. Phase transition engineering to break the symmetry of diamond-like chalcogenide for second-order nonlinear optics

    Inorganic Chemistry Frontiers · 2025-01-01

    Chunlan Tang, Aoge Yao, Wenhao Xing, Wenwen Jiang, Jian Tang, Lei Kang, Jieyun Wu, Wenlong Yin, Bin Kang

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  2. Y(C 6 H 5 SO 3 ) 3 ·9H 2 O: strategic integration of ligand substitution and π-conjugated group linkage in sulfates for enhanced ultraviolet nonlinear optical properties

    Inorganic Chemistry Frontiers · 2025-01-01

    Xiaodong Zhang, Bohui Xu, Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin

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  3. (CN4H7)H2C3N3S3: Trithiocyanurate Exhibiting Giant Optical Anisotropy via Weak Interaction-Mediated Functional Module Alignment

    Inorganic Chemistry · 2025-08-19

    Xia Hao, Y.K. Su, Chensheng Lin, Min Luo, Lingli Wu, Ruijie Wang, Xin Wen, Ning Ye

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  4. Enhancing Birefringence via a Planar‐Conformation‐Locking Strategy

    Laser & Photonics Review · 2025-09-04

    Yaoguo Shen, Jiajia Xiong, Mengqing Wu, M.-R. Li, Yingwu Zhou, Yanjie Zhang

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  5. From centrosymmetric CN3H6C6H5SO3 to non-centrosymmetric CN3H6C6H4SO3(OH): Hydroxyl introduced hydrogen bond reconstruction to realize strong second harmonic generation

    Chinese Journal of Structural Chemistry · 2025-09-04

    Xiaodong Zhang, Bohui Xu, Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin

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  6. Research on Nonlinear Optical Materials Based on BO 3 and BO 4 Hydroxy Tetraborates

    Advanced Optical Materials · 2025-09-15

    Shuai An, Bailin Chen, Fangfang Zhang, Xueling Hou, Shilie Pan

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  7. Organic Halogen Substitution-Driven Halogen Bonding Induces Polar 3D Supramolecular Framework and Second-Harmonic-Generation Response

    Inorganic Chemistry · 2025-09-17

    Mingchang Wang, Jiajia Li, Yan Chen, Ke‐Zhao Du, Jin Chen

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  8. pH‐Regulated Ring‐Opening/Closing Transformation in Polyoxometalates Enables High‐Performance Nonlinear Optical Crystals

    Angewandte Chemie International Edition · 2025-11-06

    Wei Zeng, Jing Zhang, Yao Tian, Hongmei Zeng, Zhien Lin, Liujiang Zhou, Kang Min Ok, Guohong Zou

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  9. Hydroxyl-induced structural reconstruction: two new potassium hepta-borates with deep-UV transparency and enhanced birefringence

    Inorganic Chemistry Frontiers · 2025-11-15

    Meng Cheng, Wenbin Zhang, Wenqi Jin, Артем Ромаевич Оганов, Zhihua Yang, Shilie Pan

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  10. Chiral-Unit-Driven Short-Wave Ultraviolet Nonlinear Optical Acetates with Balanced Overall Optical Properties

    The Journal of Physical Chemistry Letters · 2025-12-26

    Zi-Xuan Zhao, Wei Chen, Hui‐Yan Zhao, Mengjiao Xu, Chao He, Qi Wei, Guo-Ming Wang

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  11. Design of borate-squarate hybrid crystals with large birefringence by synergistic assembly of planar π-conjugated groups

    Dalton Transactions · 2026-01-01

    Haowen Li, X Y Wang, Hui Chai, Fangfang Zhang

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  12. Halogen-ion-driven polymorphs for high-performance nonlinear optical crystalline materials

    Chemical Science · 2026-01-01

    Yuwei Kang, Can Hui Yang, Yunjie Wang, Qi Wu

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  13. Isoniazid nitrate: synergistic dual π-conjugation triggering prominent second-harmonic generation

    Chemical Communications · 2026-01-01

    Yang Chi, Ya-Ping Zhao, Sheng‐Ping Guo

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  14. Stable lead succinate-iodides with strong second-harmonic generation response and large birefringence

    Inorganic Chemistry Frontiers · 2026-01-01

    Yulu Wu, Jialin Zeng, Rui Biao Fu, Wen Jing Yang, Zilong Geng, Senfu Lei, Yiting Luo, Xiaofan Tong, Zuju Ma

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  15. Vapochromic methanol recoordination and spin-state switching in square-planar Ni( ii ) complexes derived from trans - and cis -coordinated precursors

    Inorganic Chemistry Frontiers · 2026-01-01

    Sotaro Kusumoto, Kazuki Nakahama, Kazuki Isaka, Ryo Ohtani, Yuudai Iwai, Yuta Shudo, Kosaku Ohishi, Teruki Motohashi, Kanta Miyake, Masato Tateishi, Hikaru Zenno, Shinya Hayami, Yang Kim, Yoshihiro Koide

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  16. The modulation of structural polarity facilitating the gradient enhancement of second harmonic generation effects in hybrid metal halides

    Science China Chemistry · 2026-01-04

    Ru‐Ling Tang, Die-Xue Yang, Jian-Dong Guo, C. Z. Chen, Wenlong Liu, Sheng‐Ping Guo

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  17. The charge transfer mechanism and optimization strategy for two-photon absorption properties of A-π-A symmetric dyes in the near-infrared region

    Journal of Photochemistry and Photobiology A Chemistry · 2026-03-31

    Linpo Yang, Bingyan Chen, Cheng Zhao, Jia Wei, Yuanzuo Li, Yinglin Song

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  18. An Ultra-Wide Bandgap Sulfonate with Two-Step Second-Harmonic Generation Switching

    Journal of the American Chemical Society · 2026-04-06

    Feiyuan Gong, Yiran Zhang, Guangfeng Wei, Xingxing Jiang, Chao Wu, Zheshuai Lin, Zhipeng Huang, Jinhu Yang, Mark Graeme Humphrey, Chi Zhang

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  19. Chirality-driven polar lattice engineering for high-performance organic nonlinear optical crystals

    Science China Materials · 2026-04-07

    Bo Liu, Jiali Chen, Yu-Peng Han, Qiaohong Li, Shangda Li, Fusong Wang, Jian Zhang

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  20. Recent Progress in Hg-Based Oxysalt Crystals for Nonlinear Optics and Birefringence Applications

    Inorganic Chemistry · 2026-04-15

    Peng-Fei Li, Y Wang, Naifeng Zhuang, Jiannian Yao, Yu‐Wu Zhong

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  21. Steric hindrance and hydrogen-bond networks synergistically directing molecular alignment for high-performance ultraviolet birefringent

    Journal of Molecular Structure · 2026-05-07

    Yuqi Qin, Paipai Zhang, Peng Jiang, Xueling Hou, Hu Jiang, Minqiang Gai

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  22. Reverse Weak Polarity‐Induced Ordered Layer Control for Enhanced Second‐Harmonic Generation in Ultraviolet Nonlinear Optical Crystals

    Advanced Science · 2026-05-11

    Lingli Wu, Chensheng Lin, Bo Li, Huixin Fan, Lingfei Lv, Shunda Yang, Tao Yan, Min Luo

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  23. Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals

    Advanced Functional Materials · 2026-06-01

    Hangwei Jia, Yaqi Jin, Muhammad Arif, Bailin Chen, Zhihua Yang, Xueling Hou, Shilie Pan

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  24. Symmetry Breaking Induced by Hydration-Number Tuning Enables Second-Order Nonlinear Optical Responses in Lanthanum Sulfate Hydrates

    Inorganic Chemistry · 2026-08-04

    Xiuying Zhang, Yebiao Wu, Qiya Huang, Lehui Liu, Peican Chen, Hongming Liu

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  25. Exceptional Solar‐Blind Birefringence Engineered by Complementary Hydrogen‐Bond Ordering of π‐Conjugated Units

    Small · 2026-08-05

    Qianxi Hu, Junwei Feng, Long Chen, Minqiang Gai

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  26. Record Second-Harmonic Generation and Exceptional Optical Anisotropy in High-Symmetry 1D Polar Perovskites

    Journal of the American Chemical Society · 2026-08-12

    Shaohua Xiao, Xingxing Jiang, Xiaotian Zhang, Chunbo Jiang, Wenzhi Song, Yukang Fan, Kaining Duanmu, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  27. The Parallel Coplanar Alignment of Planar Non‐π‐Conjugated [Pb 3 Br 3 ] Rings for a Stable Ultraviolet Nonlinear Optical Crystal

    Advanced Optical Materials · 2026-08-27

    Xiaofan Tong, Zuju Ma, Yulu Wu, Ruibiao Fu, Wenjing Yang, Jiacheng Chen, Qian Zeng

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