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RESEARCH PAPER · Nature Chemical Engineering · 2025

Catalytic deconstruction of organic additive-containing plastics

Jacqueline Ngu, Sean Najmi, Esun Selvam, Brandon C. Vance, Piaoping Yang, Dionisios G. Vlachos

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Catalytic deconstruction of organic additive-containing plasticsOriginalCan mixed plastics be recycled and upcycled without separation?11Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides26Advancements in Chemical Recycling Catalysts for Plastic Waste in South Korea5MOF Catalysts for Plastic Depolymerization4MOF Catalysts for Plastic Depolymerization52Overcoming limitations in polyolefins upcycling by codesigning endothermic-exothermic magnetocatalytic system8Plastic waste upcycling through electrocatalysis10Beyond Hydroconversion: A Paradigm Shift for Sustainable Plastic Waste Upcycling9The Effect of Impurities in Post-Consumer Plastic Waste on the Cracking of Polyolefins with Zeolite-based Catalysts1Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11Post‐Synthetic Amide Insertion Into Polyethylenes Augments Diverse Physical Properties and Enables Branching‐Dependent Recyclability5Recyclable Biomass-Derived Polyethylene-like Plastics6Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32The role of catalyst acidity and microstructure on light olefin selectivity in polyethylene deconstruction in short contact time pulse Joule-heated reactors3Reliability of milligram-scale high-throughput screening for evaluating polyolefin chemical recycling in the melt with heterogeneous catalysis3Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Photothermal Revolution in Plastic Upcycling24Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals0Catalytic valorization of polyolefins: from catalysts and processes to reactors0Chemoselective depolymerization of polyurethane via solvent-engineered glycolysis0Hydrogen bond regulation to enhance catalytic C–C bond cleavage of polylactic acid wastes in H 2 O to produce H 20Solvent-mediated contaminant removal from plastic waste using thermodynamic modeling4The Nine Lives of Phenomenological Psychology0Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Stepwise hydrogen spillover–engineered synergistic sites enable near-quantitative conversion of waste PET to p-xylene10Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels1Hydrogenolysis Versus Hydrocracking for Polyolefin Upcycling0Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Integrating integrated circuit wastewater into the metal catalyst supply chain1Towards Sustainable Plastics Management: Value Chain Assessment of Pyrolysis Oil Integration in the Petrochemical Industry0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4Towards Sustainable C1 Valorization: Coupling Biomass and Waste Plastics Conversion with Renewable Energy0Solar-Driven Dehalogenation and Upcycling of Brominated Plastic Waste1Aqueous-Based Biomimetic Porphyrin-Catalyzed Surface Oxidation of Polyethylenes for Enhanced 3D-Printability0Atomically precise catalysts design toward efficient waste plastic hydrogenolysis2Catalytic processes for the depolymerization and upcycling of polyethylene terephthalate (PET): A preface0Environmental Identification of Novel Enzymes for Polyurethane and Polyamide Degradation2Environmental Identification of Novel Enzymes for Polyurethane and Polyamide Degradation1Bifunctional nanocatalyst design for polyolefin hydrocracking2Catalyst-free, microdroplet-mediated waste plastic conversion to diacids4Review on evolving lumped kinetic models in plastic pyrolysis for plastic waste valorization: Roadmap for circular future0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Coke poisoning of Lewis acidic Al sites during hydrodechlorination of plastic pyrolysis oil and its mitigation by two-step hydrotreating0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  1. Can mixed plastics be recycled and upcycled without separation?

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  2. Conversion of Compositionally Diverse Plastic Waste over Earth-Abundant Sulfides

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  3. Advancements in Chemical Recycling Catalysts for Plastic Waste in South Korea

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  4. MOF Catalysts for Plastic Depolymerization

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  5. MOF Catalysts for Plastic Depolymerization

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  6. Overcoming limitations in polyolefins upcycling by codesigning endothermic-exothermic magnetocatalytic system

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  7. Plastic waste upcycling through electrocatalysis

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  8. Beyond Hydroconversion: A Paradigm Shift for Sustainable Plastic Waste Upcycling

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  9. The Effect of Impurities in Post-Consumer Plastic Waste on the Cracking of Polyolefins with Zeolite-based Catalysts

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  10. Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes

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  11. Post‐Synthetic Amide Insertion Into Polyethylenes Augments Diverse Physical Properties and Enables Branching‐Dependent Recyclability

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  13. Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy

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  14. The role of catalyst acidity and microstructure on light olefin selectivity in polyethylene deconstruction in short contact time pulse Joule-heated reactors

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  15. Reliability of milligram-scale high-throughput screening for evaluating polyolefin chemical recycling in the melt with heterogeneous catalysis

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  16. Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion

    ACS Catalysis · 2025-12-10

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  17. Photothermal Revolution in Plastic Upcycling

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  18. Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals

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  19. Catalytic valorization of polyolefins: from catalysts and processes to reactors

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  20. Chemoselective depolymerization of polyurethane via solvent-engineered glycolysis

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  21. Hydrogen bond regulation to enhance catalytic C–C bond cleavage of polylactic acid wastes in H 2 O to produce H 2

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  22. Solvent-mediated contaminant removal from plastic waste using thermodynamic modeling

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  23. The Nine Lives of Phenomenological Psychology

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  25. Stepwise hydrogen spillover–engineered synergistic sites enable near-quantitative conversion of waste PET to p-xylene

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  26. Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels

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  35. Atomically precise catalysts design toward efficient waste plastic hydrogenolysis

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