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RESEARCH PAPER · Nature Catalysis · 2024

Parahydrogen-enhanced magnetic resonance identification of intermediates in [Fe]-hydrogenase catalysis

Lukas Kaltschnee, Andrey N. Pravdivtsev, Manuel Gehl, Gangfeng Huang, Georgi L. Stoychev, Christoph Riplinger, Maximilian Keitel, Frank Neese, Jan‐Bernd Hövener, Alexander A. Auer, Christian Griesinger, Seigo Shima, Stefan Glöggler

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Parahydrogen-enhanced magnetic resonance identification of intermediates in [Fe]-hydrogenase catalysisOriginal[Fe]-hydrogenase intermediates revealed2Highly active iron catalysts for olefin hydrogenation enable para -hydrogen induced hyperpolarisation of 1 H and 19 F NMR resonances at 1.4 Tesla2Unconventional Parahydrogen-Induced Hyperpolarization Effects in Chemistry and Catalysis: From Photoreactions to Enzymes18N‐Heterocyclic Carbene Functionalization of 2D Transition Metal Dichalcogenides via a Frustrated Lewis Pair Strategy5Reconstitution of [Fe]-Hydrogenase with Model Complexes Reveals Functional Roles of Methyl Groups in the Metallocofactor3Photosynthetic Biohybrid Systems: A Promising Approach for Energy and Environmental Applications28Towards efficient and safe hydrogen storage for green shipping: Progress on critical technical issues of material development and system construction14Real-Time Probing of Electrochemical Intermediates: Mechanistic Insights via Ambient Mass Spectrometry515 N Reaction Monitoring at Low and Inhomogeneous Magnetic Fields Enabled by Hyperpolarization with Parahydrogen3Field Cycling from 10 nT to 9.4 T: A Flexible Gear Rod Design for Nuclear Spin Relaxation and Hyperpolarization Studies5Probing Hydrogen Activation in a Dimetal Dihydride Complex by Symmetric Exchange with Parahydrogen1Microbial enzymes and activity-assisted electrolysis for the production of biohydrogen0Dynamic Proton Sharing and Second-Sphere Gating Control Catalytic States in [NiFe] Hydrogenase0

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  1. [Fe]-hydrogenase intermediates revealed

    Nature Catalysis · 2024-12-20

    Sven Timo Stripp

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  2. Highly active iron catalysts for olefin hydrogenation enable para -hydrogen induced hyperpolarisation of 1 H and 19 F NMR resonances at 1.4 Tesla

    Chemical Communications · 2025-01-01

    Julianna S. Doll, Jan Kergassner, Bingyu Zhang, Christina Marie Thiele, Gerd Buntkowsky, Markus Enders, Torsten Gutmann, Dragoş‐Adrian Roşca

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  3. Unconventional Parahydrogen-Induced Hyperpolarization Effects in Chemistry and Catalysis: From Photoreactions to Enzymes

    ACS Catalysis · 2025-04-04

    Andrey N. Pravdivtsev, Ben. J. Tickner, Stefan Glöggler, Jan‐Bernd Hövener, Gerd Buntkowsky, Simon B. Duckett, Clifford R. Bowers, Vladimir V. Zhivonitko

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  4. N‐Heterocyclic Carbene Functionalization of 2D Transition Metal Dichalcogenides via a Frustrated Lewis Pair Strategy

    Advanced Functional Materials · 2025-05-22

    Gao Jia, Nachuan Li, Bona Dai, Wenjie Yu, Xiaojie Zhou, Chaohuang Chen, Kazunori Fujisawa, Zhenzhen Yang, Sheng Dai, Yifan Sun

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  5. Reconstitution of [Fe]-Hydrogenase with Model Complexes Reveals Functional Roles of Methyl Groups in the Metallocofactor

    Journal of the American Chemical Society · 2025-06-26

    Chao Wang, Haoyu Li, Jinsi Li, Changjiang Wang, Jinmeng Yu, Seigo Shima, Gangfeng Huang, Hui‐Jie Pan

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  6. Photosynthetic Biohybrid Systems: A Promising Approach for Energy and Environmental Applications

    Environmental Science & Technology · 2025-07-30

    Tianyu Zhi, Tian Fu, Haiyin Zhan, Ruiren Zhou, Mengxue Yang, Chao Gao, Pengfei Wang, Sihui Zhan, Qixing Zhou

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  7. Towards efficient and safe hydrogen storage for green shipping: Progress on critical technical issues of material development and system construction

    International Journal of Hydrogen Energy · 2025-08-19

    Huijin Xu, Yidong Zhang, Xuelai Zhang

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  8. Real-Time Probing of Electrochemical Intermediates: Mechanistic Insights via Ambient Mass Spectrometry

    Analytical Chemistry · 2025-08-29

    Lulu Chen, Xiang Zhao, Bingjie Kong, Chaoyue Gu, Bin Cai

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  9. 15 N Reaction Monitoring at Low and Inhomogeneous Magnetic Fields Enabled by Hyperpolarization with Parahydrogen

    Chemistry - A European Journal · 2025-11-04

    Gonzalo Gabriel Rodriguez, Ruhuai Mei, Lisa M. Fries, Stefan Glöggler

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  10. Field Cycling from 10 nT to 9.4 T: A Flexible Gear Rod Design for Nuclear Spin Relaxation and Hyperpolarization Studies

    ACS Measurement Science Au · 2025-12-01

    Josh P. Peters, Charbel D. Assaf, Mathis Côté, Jan‐Bernd Hövener, Andrey N. Pravdivtsev

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  11. Probing Hydrogen Activation in a Dimetal Dihydride Complex by Symmetric Exchange with Parahydrogen

    Journal of the American Chemical Society · 2026-02-12

    Julius Frederik Matz, Lukas Kaltschnee, Sara Ida Mozzi, Gonzalo Gabriel Rodriguez, Anton Römer, Ricardo A. Mata, Ilya Kuprov, Franc Meyer, Stefan Glöggler

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  12. Microbial enzymes and activity-assisted electrolysis for the production of biohydrogen

    Biomass and Bioenergy · 2026-04-13

    Shalu Rawat, Soumya Ranjan Mishra, P. Manikanta, Rohit Rangnath Nikam, Philippe M. Heynderickx, Siddappa A. Patil, Bhari Mallanna Nagaraja

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  13. Dynamic Proton Sharing and Second-Sphere Gating Control Catalytic States in [NiFe] Hydrogenase

    Journal of the American Chemical Society · 2026-07-01

    Shruti Moorthy, Gaurav Joshi, Abhishek Sirohiwal

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