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RESEARCH PAPER · Chemistry of Materials · 2024

Large Mid-Infrared Second-Harmonic Generation in Eu(II)-Based Quaternary Chalcogenides

Subhendu Jana, Eric A. Gabilondo, Machima Mongkhonratanachai, Yujie Zhang, P. Shiv Halasyamani, Paul A. Maggard

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Large Mid-Infrared Second-Harmonic Generation in Eu(II)-Based Quaternary ChalcogenidesOriginalSynthesis, Optical, and Magnetic Properties of the Mixed Chalcogenide Semiconductor Series Eu(II)2SiSexS4-x, Prepared via the Flux-Assisted Boron Chalcogen Mixture Method4Isovalent cation substitution drives structural transformation and infrared nonlinear optical activity in Eu-based chalcogenides11NaCaGa 3 S 6 : a mixed alkali metal and alkaline earth metal sulfide with a distinctive [Ga 5 S 10 ] ∞ layered framework0Eu(II)‐Based Quaternary Chalcogenides with Noncentrosymmetric Structures Stabilized by Site Disorder of d10 Metal Cations4Cation Equivalent Multisubstitution Realizing Structure Transformation and Balanced Nonlinear Optical Performance of Quaternary Eu-Based Chalcogenides8Ternary Antimony Selenide Semiconductors: Synthesis, Crystal Structure, Electronic Structure, and Optical Properties5Magnetic Properties and Large Second-Harmonic Generation Response of a Chiral Ternary Chalcogenide: Eu 2 SiSe 48Dimensional Reduction Guides Electronic Structure Evolution in the A n Cu 4– n SnS 4 Semiconductor Series8From Centrosymmetric Eu 2 Ga 2 S 5 to Noncentrosymmetric EuMg 6 Ga 6 S 16 via Introduction of Distorted MgS 6 Octahedron: Featuring Wide Bandgap and Nonlinear Optical Activity3SrZnSiS4: Shattering the 4.0 eV Threshold toward Dual-Optimized Bandgap and Second-Harmonic Generation5Molecular Modifications of Crystalline Poly(triazine imide) for Advancing Its Structure–Property Relationships in Light-Driven Catalysis1A Homoatomic Heteroleptic Coordination Strategy for Exceptional Infrared Linear and Nonlinear Optical Properties in ANb 2 PS 4 (S 2 ) 3 (A = K,Rb,Cs)3K 2 ZnMoP 2 O 10 : crystal growth, optical characterization, and structure–property insights into phase matching0Polar Antiperovskite Oxides: Promising Mid-Infrared Nonlinear Optical Materials with Strong Second-Harmonic Generation2Structure–Optical Property Relationships in AMM′Q 3 Chalcogenides0From KBa 4 Ge 3 S 10 Cl to ABa 3 EuGe 3 S 11 (A = Na, K) Synthesized by Reactive Flux Assisted Metal Oxide-Boron-Chalcogen (MOBQ) Method: Effect of Cation/Anion Cosubstitution on Crystal Structure and Nonlinear Optical Properties0Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0EuMn6Ga6S16: A Wide Bandgap Europium-Based Nonlinear Optical Sulfide0Where Are Eu? Structural Diversity from Coloring Variants in Tellurides Eu(Al1– x Ga x )2Te40

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  1. Synthesis, Optical, and Magnetic Properties of the Mixed Chalcogenide Semiconductor Series Eu(II)2SiSexS4-x, Prepared via the Flux-Assisted Boron Chalcogen Mixture Method

    Inorganic Chemistry · 2024-12-04

    Gopabandhu Panigrahi, Gregory W. Morrison, Mark D. Smith, Hans‐Conrad zur Loye

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  2. Isovalent cation substitution drives structural transformation and infrared nonlinear optical activity in Eu-based chalcogenides

    Inorganic Chemistry Frontiers · 2025-01-01

    Ping Feng, Shenghua Zhou, Mao‐Yin Ran, Bingxuan Li, Xin-Tao Wu, Hua Lin, Qi‐Long Zhu

    Read original paper ↗ ·

  3. NaCaGa 3 S 6 : a mixed alkali metal and alkaline earth metal sulfide with a distinctive [Ga 5 S 10 ] ∞ layered framework

    Dalton Transactions · 2025-01-01

    Jiale Chen, Haipeng Zhou, Huimin Sha, Jinfeng Liu, Xiu Zhu, Guisheng Xu, Jiankang Wang

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  4. Eu(II)‐Based Quaternary Chalcogenides with Noncentrosymmetric Structures Stabilized by Site Disorder of d10 Metal Cations

    Zeitschrift für anorganische und allgemeine Chemie · 2025-04-14

    Subhendu Jana, Eric A. Gabilondo, Machima Mongkhonratanachai, P. Shiv Halasyamani, Paul A. Maggard

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  5. Cation Equivalent Multisubstitution Realizing Structure Transformation and Balanced Nonlinear Optical Performance of Quaternary Eu-Based Chalcogenides

    Inorganic Chemistry · 2025-05-30

    Fang-Xu Tian, Wen‐Dong Yao, Wenfeng Zhou, Jing Zhu, Sheng‐Ping Guo

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  6. Ternary Antimony Selenide Semiconductors: Synthesis, Crystal Structure, Electronic Structure, and Optical Properties

    Inorganic Chemistry · 2025-06-18

    James Pirez, Subhendu Jana, Eric A. Gabilondo, Scott McGuigan, P. Shiv Halasyamani, Paul A. Maggard

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  7. Magnetic Properties and Large Second-Harmonic Generation Response of a Chiral Ternary Chalcogenide: Eu 2 SiSe 4

    Chemistry of Materials · 2025-07-09

    Shaun O’Donnell, Ian Andreas Leahy, Subhendu Jana, Eric A. Gabilondo, P. Shiv Halasyamani, Paul A. Maggard, Rebecca W. Smaha

    Read original paper ↗ ·

  8. Dimensional Reduction Guides Electronic Structure Evolution in the A n Cu 4– n SnS 4 Semiconductor Series

    Journal of the American Chemical Society · 2025-08-07

    Michael A. Viti, Zhi Li, Chris M. Wolverton, Mercouri G. Kanatzidis

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  9. From Centrosymmetric Eu 2 Ga 2 S 5 to Noncentrosymmetric EuMg 6 Ga 6 S 16 via Introduction of Distorted MgS 6 Octahedron: Featuring Wide Bandgap and Nonlinear Optical Activity

    Inorganic Chemistry · 2025-08-21

    Qiu-Yang Du, Wen‐Dong Yao, Xu-Bin Ni, Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

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  10. SrZnSiS4: Shattering the 4.0 eV Threshold toward Dual-Optimized Bandgap and Second-Harmonic Generation

    Inorganic Chemistry · 2025-09-04

    Huilin Yin, Xia Wu, Shuchang Wu, Changsheng Sun, Chengxiao Wang, Jiaman Sun, Yang Liu, Xiao‐Ming Jiang, Ximeng Lv, Dajiang Mei

    Read original paper ↗ ·

  11. Molecular Modifications of Crystalline Poly(triazine imide) for Advancing Its Structure–Property Relationships in Light-Driven Catalysis

    Chemistry of Materials · 2025-09-18

    Scott McGuigan, Carrie L. Donley, Erika Ortiz, Shaun O’Donnell, Magnus Pauly, William C. Hockaday, Eric A. Stach, Paul A. Maggard

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  12. A Homoatomic Heteroleptic Coordination Strategy for Exceptional Infrared Linear and Nonlinear Optical Properties in ANb 2 PS 4 (S 2 ) 3 (A = K,Rb,Cs)

    Inorganic Chemistry · 2025-12-31

    Yumiao Niu, Yan Chun Xiao, Yidan Chen, Chu Chu, Daqing Yang, Ying Wang, Bingbing Zhang

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  13. K 2 ZnMoP 2 O 10 : crystal growth, optical characterization, and structure–property insights into phase matching

    CrystEngComm · 2026-01-01

    Youbin Wang, Haonan Liu, Yujie Zhang, Hongping Wu, Hongping Wu, Zhanggui Hu

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  14. Polar Antiperovskite Oxides: Promising Mid-Infrared Nonlinear Optical Materials with Strong Second-Harmonic Generation

    Chemistry of Materials · 2026-03-26

    Yunseung Kuk, Kang Min Ok, P. Shiv Halasyamani

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  15. Structure–Optical Property Relationships in AMM′Q 3 Chalcogenides

    Chemistry of Materials · 2026-06-10

    Ayat Tassanov, Huiju Lee, Daniel W. Spainhour, Yi Xia, James M. Hodges

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  16. From KBa 4 Ge 3 S 10 Cl to ABa 3 EuGe 3 S 11 (A = Na, K) Synthesized by Reactive Flux Assisted Metal Oxide-Boron-Chalcogen (MOBQ) Method: Effect of Cation/Anion Cosubstitution on Crystal Structure and Nonlinear Optical Properties

    Inorganic Chemistry · 2026-06-12

    Qiu-Yang Du, Ming-Yang Li, Nan Zhang, Wenfeng Zhou, Ru‐Ling Tang, Sheng‐Ping Guo

    Read original paper ↗ ·

  17. Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects

    Advanced Optical Materials · 2026-07-21

    Xiangran Kong, Jingdong Yan, Zi Wang, Hongwei Leng, Shichao Cheng, Sue Hao, Xiaoran Niu, Zuotao Lei, Chunhui Yang

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  18. EuMn6Ga6S16: A Wide Bandgap Europium-Based Nonlinear Optical Sulfide

    Inorganic Chemistry · 2026-08-16

    Yu‐Xuan Zhang, Jiang-Hui Fan, Zhen‐Cheng Wu, Shao-Peng Gui, Mao‐Yin Ran, Sheng‐Ping Guo

    Read original paper ↗ ·

  19. Where Are Eu? Structural Diversity from Coloring Variants in Tellurides Eu(Al1– x Ga x )2Te4

    Inorganic Chemistry · 2026-10-05

    Pritam Das, Trinanjan Dey, Vidyanshu Mishra, Chloe F. McLeod, Dmitry Vrublevskiy, Zhongqi Lin, A. Mar

    Read original paper ↗ ·
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