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RESEARCH PAPER · Journal of the American Chemical Society · 2025

High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid Sites

Shuheng Tian, Risheng Bai, Zirui Gao, Zhiwei Chen, Maolin Wang, Haoyi Tang, Siyu Lin, Bingjun Xu, Xi Liu, Jihong Yu, Ding Ma

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High-Efficiency Hydrocracking of Polyolefin Plastics by Controlling Intimacy between Pt Clusters and Zeolite Acid SitesOriginalTri-coordinated copper single atoms on SAPO-34 boosts acetic acid production from methane and carbon dioxide2A review of recent advances in thermal-catalytic cracking of plastic waste8Chemical recycling of polyolefin wastes: recent advances and insights into recycling routes0Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Synergistic Metal-Acid Unit for Boosting Tandem Catalysis via Efficient Transformation of the Key Intermediate4Catalytic Oxidation of Commodity Plastics: Advances in Polyethylene and Polystyrene Valorization5Acidified montmorillonite (MMT)-supported ultrafine Ru nanoparticles for polyethylene plastic upcycling0Dual advantages of rapid zeolite channel diffusion and Ni sites: 1Ni/L-DAl zeolite enables efficient polyolefin hydrocracking to liquid fuel1Enhancing aromatic yield by zeolites in polypropylene hydrocracking to jet fuel over Ru 1 -ZrO 2 without forming CH 40Highly selective hydrocracking of polypropylene to gasoline-range fuels over the Pt/MCM-22 catalyst0Mechanochemical strategies for environmental remediation and resource recovery2N-doped Hollow Carbon Spheres Supported Co Nanoparticles for Hydrogen Production from Ammonia Borane5Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Solvent-free recycling of polystyrene waste into valuable mono-aromatics over a Ni/NbO x catalyst0Efficient Hydrogenation of Phenanthrene Enabled by d-Orbital Restructuring: A DFT Study0Acid sites in hydrogen-involved polyolefin upcycling: mechanistic insights and design principles0Aqua‐Oxidation of Polyethylene Into Carboxylic Acids Under Mild Conditions: A Catalyst‐Free Upcycling Strategy for Nonpolar Plastics3Low-Temperature Upcycling of Polyethylene into Fuel-Range Hydrocarbons: An Innovative Approach on the Feed-Catalyst Bed Design1Aqua‐Oxidation of Polyethylene Into Carboxylic Acids Under Mild Conditions: A Catalyst‐Free Upcycling Strategy for Nonpolar Plastics5Rational design of bifunctional catalysts for hydrocracking of polyethylene waste plastics to narrow-distributed liquid fuels4Tandem catalysis for carbon circularity3Acid Site Engineering of Ni/BEA Zeolites Enables Efficient Upcycling of Polyolefin Plastics to Liquid Fuels1Structure–performance relationships in heterogeneous catalysts for polyolefin plastic hydroconversion1Pd@γ-Al2O3-catalyzed ring-expansion rearrangement synthesis of sustainable multiply-alkylated cyclopentanes lubricants0Catalytic Upcycling of Polyolefins and Polystyrene: Integrating Active Site Design With Mass Transfer Considerations4iPDA-Assisted Design of Hierarchical Beta Zeolites for the Sustainable Upcycling of Polyethylene to Naphtha with Ultra-Low Pt Loading1Hydrocracking of LDPE to liquid fuel over HY zeolite supported Ni catalyst: synergistic effect among metal, porosity and acidity1Highly efficient synthesis of high-density aviation fuel over dual-site promoted GaZnZrOx/Znβ catalysts from CO2 hydrogenation coupled with naphthalene alkylation0Synthetic control over proximity of metal and acid dual sites switches the selectivity of acetophenone hydrodeoxygenation2A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Dual redox shuttles drive efficient succinic acid electrosynthesis from plastic and biowaste1Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Ceria‐Based Catalysts for Sustainable Processing of Plastic Waste0From waste to wealth: Advanced strategies and mechanisms for chemical recycling and upcycling of polymeric materials1Promoting CO 2 Conversion With Terminal Alkynes Over ZSM‐5 Zeolite‐Confined Uniform Ag Nanoparticles0Promoting CO 2 Conversion With Terminal Alkynes Over ZSM‐5 Zeolite‐Confined Uniform Ag Nanoparticles0Cage-directed skeleton rearrangement mechanism of hydrogenated polycyclic aromatic hydrocarbons to alkyl adamantanes: reaction network and hydrogen transfer on acid sites0Exceptional CO 2 Hydrogenation to Gasoline Enabled by GaZrO x /Ga‐ZSM‐5 Tandem Catalyst0Extreme Nanoconfinement Dramatically Enhances Small Molecule Solubility in Nonpolar Polymers1Bifunctional nanocatalyst design for polyolefin hydrocracking2Design and Application of Industrial Catalysts for Hydrocracking of PAHs: Catalytic Technology and Metal–Acid Intimacy0Quantitative Polyethylene Upcycling to Liquid Olefins over Ru-Containing Layered Zeolites0Biomimetic Redox-Mediated Proton Relay in Nanoreactors for Photocatalysis0Challenges and strategies for catalyst coking in catalytic cracking of polyolefins to liquid fuels1Coupling Polyolefin Conversion and Methanol Reduction for C 9 –C 10 Alkylaromatic Production1Coupling Polyolefin Conversion and Methanol Reduction for C 9 –C 10 Alkylaromatic Production0Rational construction of multifunctional Pd/Zn-ZSM-5 catalyst for high-yield production of ethanol via glucose hydrogenolysis0Redirecting Reaction Pathway in Tandem Catalysis With Isolated Metal–Acid Architecture0Redirecting Reaction Pathway in Tandem Catalysis With Isolated Metal–Acid Architecture0Comprehensive quantitative analysis of polyolefin hydrogenolysis toward plastic waste management0Confined Isomerization Enables Solar-Thermal Upcycling of Polyolefins into High-Octane Gasoline0Sufficient Metal–Acid Site Matching in Co-Loaded WO x -ZrO2 Catalysts for Polyethylene Hydrocracking0Coke poisoning of Lewis acidic Al sites during hydrodechlorination of plastic pyrolysis oil and its mitigation by two-step hydrotreating0In-situ hydrogen generation via water-gas shift reaction over Ni-Fe3O4/USY: A sustainable pathway for efficient polypropylene hydrogenolysis0Metal-Acid Balance Enables Earth-Abundant Metal Upcycling of Polyolefins to Jet Fuel0Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products0Tandem catalysts for hydroconversion of polyethylene-EVOH multilayer plastics0Optimization of Hydrogen Evolution Performance in ZnIn 2 S 4 Photocatalysts via Ho‐Doped Induced Tensile Strain0A review on selective dealkylation of alkylaromatics: Feedstocks, catalysts, and reaction pathways0Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes0Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes0Programming Iron Nuclearity and Coordination for Hydride‐Mediated Nitroarene Reduction0Frustrated Lewis Pairs Enable Efficient Polyethylene Oxidative Upcycling0Frustrated Lewis Pairs Enable Efficient Polyethylene Oxidative Upcycling0Programming Iron Nuclearity and Coordination for Hydride‐Mediated Nitroarene Reduction0

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