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RESEARCH PAPER · Nature Communications · 2024

Single [0001]-oriented zinc metal anode enables sustainable zinc batteries

Xiaotan Zhang, Jiangxu Li, Yanfen Liu, Bingan Lu, Shuquan Liang, Jiang Zhou

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Single [0001]-oriented zinc metal anode enables sustainable zinc batteriesOriginalChallenges and industrial considerations towards stable and high-energy-density aqueous zinc-ion batteries189Guiding uniform Zn deposition with a multifunctional additive for highly utilized Zn anodes41Interfacial chemistry in multivalent aqueous batteries: fundamentals, challenges, and advances113Understanding the structure–activity relationship of additives for durable Zn metal batteries: a case study of aromatic molecules83Crystallographic Manipulation Strategies toward Reversible Zn Anode with Orientational Deposition151Porous zinc metal anodes for aqueous zinc-ion batteries: Advances and prospectives36Multicore–shell bismuth nanoparticles@N-doped porous carbon nanorods for dendrite-free zinc metal anodes1MXene nanomaterials: Synthesis, properties and applications in energy and environment sector88Spontaneous grain refinement effect of rare earth zinc alloy anodes enables stable zinc batteries128Interfacial Biomacromolecular Engineering Toward Stable Ah‐Level Aqueous Zinc Batteries190Pre‐Corrosion of Zinc Metal Anodes for Enhanced Stability and Kinetics21Dual-function protective layer for highly reversible Zn anode46Organic Cations Texture Zinc Metal Anodes for Deep Cycling Aqueous Zinc Batteries155Hydrophobic Ion Barrier‐Enabled Ultradurable Zn (002) Plane Orientation towards Long‐Life Anode‐Less Zn Batteries3Hydrophobic Ion Barrier‐Enabled Ultradurable Zn (002) Plane Orientation towards Long‐Life Anode‐Less Zn Batteries92Corrosion‐Resistant Shape‐Programmable Zn–I 2 Battery28Revisiting the Charging Mechanism of α‐MnO 2 in Mildly Acidic Aqueous Zinc Electrolytes22Stress relief and crystal face transition process contribute to the stability of zinc anodes18Crystallographically textured zinc nucleation and planar electrodeposition for zinc metal batteries via magnetoelectric and magnetization effects19Nonflammable Fluorinated Electrolyte Realizing High Voltage Anode‐Free Zn Dual‐Ion Batteries25Nonflammable Fluorinated Electrolyte Realizing High Voltage Anode‐Free Zn Dual‐Ion Batteries1Interfacial double-coordination effect reconstructing anode/electrolyte interface for long-term and highly reversible Zn metal anodes36Zn-anode stability in additive added perchlorate electrolyte for aqueous Zn-MnO2 battery4Single Exposed Zn (0002) Plane and Sustainable Zn‐Oriented Growth Achieving Highly Reversible Zinc Metal Batteries0Single Exposed Zn (0002) Plane and Sustainable Zn‐Oriented Growth Achieving Highly Reversible Zinc Metal Batteries53Grain Boundary Filling Empowers (002)‐Textured Zn Metal Anodes with Superior Stability81Balancing Ion Diffusion-Reduction in Chlorine-Free Electrolytes Enables Long-Life Mg Metal Batteries36Single‐Crystalline Zn(002) Facet Enables Ultrastable Anode–Electrolyte Interface28Dipole Moment Dictates the Preferential Immobilization in Gel Electrolytes for Ah‐level Aqueous Zinc‐Metal Batteries71Dipole Moment Dictates the Preferential Immobilization in Gel Electrolytes for Ah‐level Aqueous Zinc‐Metal Batteries1De‐Passivation and Surface Crystal Plane Reconstruction via Chemical Polishing for Highly Reversible Zinc Anodes152Stabilizing water and regulating interfacial electrostatic interaction with economical supporting salt for stable Zn metal anode8Design principles of novel Zn fluorocarboxylate protection layer toward durable dendrite-free Zn metal anodes11Innovative Zinc Anodes: Advancing Metallurgy Methods to Battery Applications41Comprehensive Understanding of Steric‐Hindrance Effect on the Trade‐Off Between Zinc Ions Transfer and Reduction Kinetics to Enable Highly Reversible and Stable Zn Anodes80Turning crisis into opportunity: Intrinsically polarised low concentration eutectic electrolytes enable highly reversible zinc anodes5Manipulation in the In Situ Growth Design Parameters of Aqueous Zinc‐Based Electrodes for Batteries: The Fundamentals and Perspectives18Synergetic bifunctional Cu-In alloy interface enables Ah-level Zn metal pouch cells90Achieving Stable Orientational Zinc Deposition for Reversible Zinc Anode through Supramolecular Anchoring Mechanism8Anion-induced optimization of non-aqueous zinc-air battery performance: Insights into OTF− selection4Biomineralization Inspired the Construction of Dense Spherical Stacks for Dendrite-Free Zinc Anodes20Crystallographic Texturing of Electrodeposits for Sustainable Zn Anodes33Concurrent Regulation of Surface Topography and Interfacial Physicochemistry via Trace Chelation Acid Additives toward Durable Zn Anodes9Revealing Epitaxial Deposition in Alkali Metal Batteries4In Situ Electrochemical Polymerized Bipolar-Type Poly(1,5-diaminonaphthalene) Cathode for High-Performance Aqueous Zinc-Organic Batteries13Interactive issues and strategic solutions for aqueous Zn metal anodes27Functional Hydrogels for Aqueous Zinc‐Based Batteries: Progress and Perspectives61A Multifunctional Crosslinked F‐Free Binder for MnO 2 Microparticle Thick Cathode in Aqueous Zinc‐Ion Batteries20Directing Zn Growth with Biased Adsorption of Straight‐chain Molecules for Superior Zn Anode Stability79Directing Zn Growth with Biased Adsorption of Straight‐chain Molecules for Superior Zn Anode Stability11Operando Evolution of a Hybrid Metallic Alloy Interphase for Reversible Aqueous Zinc Batteries46Operando Evolution of a Hybrid Metallic Alloy Interphase for Reversible Aqueous Zinc Batteries7Uncovering Required Molecular Properties for Interface Regulators and Modification Mechanisms for Zn Anode in Aqueous Batteries35Fundamental understanding of texturing electrodeposition metal zinc anodes for practical aqueous Zn‐ion batteries20Biomimetic robust polymeric interphase facilitating stable Zn metal anode13An MBene-based colloidal electrolyte for high depth-of-discharge and energy-density 2 Ah-scale Zn metal batteries22Constructing a gradient soft-coupled SEI film using a dilute ternary electrolyte system towards high-performance zinc-ion batteries with wide temperature stability26Desired spontaneous corrosion via a highly hydrophilic porous layer for aqueous zinc-ion batteries3Enhancing organic cathodes of aqueous zinc-ion batteries via nitro group modification24Eutectic electrolytes enable dendrite-free and ultradurable zinc metal anodes for rechargeable zinc batteries1First principle investigation of Cr doping effect on the stability of NiFe2O45Hybrid superlattice cathodes unlocking diffusion-barrier-free proton storage for high-rate Zn–MnO 2 batteries1Hydrogel electrolytes for zinc dendrite regulation: balancing conductivity and modulus13Non-destructive stripping electrochemistry enables long-life zinc metal batteries22Spontaneous passivation of selective Zn(101) plating via dangling bond saturation and electrostatic interaction regulation for high-utilization, fast-kinetics zinc anodes25Synergistic polypyrrole coating and electrolyte engineering toward high-performance Zn-based batteries2Unlocking the Facet‐Governed Zn Homoepitaxy Growth Induced by Dynamic l ‐Theanine Evolution Process Realized Highly Reversible Zn Anodes11Tyrosine additives with rich-polar functional groups provide multi-protections for ultra-stable zinc metal anodes60Design Strategies for Practical Zinc‐Air Batteries Toward Electric Vehicles and beyond43NH4+-Modulated Cathodic Interfacial Spatial Charge Redistribution for High-Performance Dual-Ion Capacitors44Texturing (002)‐Oriented Zinc Atop a Cotton Cloth for High‐Performance Zn‐Ion Batteries26Sabatier Principle Inspired Bifunctional Alloy Interface for Stable and High‐Depth Discharging Zinc Metal Anodes18Sabatier Principle Inspired Bifunctional Alloy Interface for Stable and High‐Depth Discharging Zinc Metal Anodes4Targeted Docking of Localized Hydrogen Bond for Efficient and Reversible Zinc‐Ion Batteries63Targeted Docking of Localized Hydrogen Bond for Efficient and Reversible Zinc‐Ion Batteries20Inhibiting Interfacial Electron Leakage via An Artificial Rectified Layer for Longevous Zinc Metal Anodes8Inhibiting Interfacial Electron Leakage via An Artificial Rectified Layer for Longevous Zinc Metal Anodes32Electrodissolution-driven enhancement in Zn electrode reversibility19Mechanism and Structural Defects of Zinc Film Deposited on a Copper Substrate: A Study via Molecular Dynamics Simulations3Nickel silicate nanotubes modifying the surface of Zn anode tuning the uniform zinc deposition for high-performance Zn metal battery13Step‐Edge Guided Homoepitaxy Enables Highly Reversible Zn Plating/Stripping20Step‐Edge Guided Homoepitaxy Enables Highly Reversible Zn Plating/Stripping2Bimetallic Ion Intercalation Optimized the Performance of Hydrated Vanadate Cathodes for Aqueous Zinc Ion Batteries8Challenges and strategies for zinc anodes in aqueous Zinc-Ion batteries67Micromechanical cleavage enables neat surface and organic-inorganic interlayer for reversible Zn anodes2Surface Topography Optimization Engineering: Stabilizing Zinc Metal Anode/Aqueous Electrolyte Interfacial Chemistry34Postpone Interfacial Impoverishment of Zn‐Ions via Neodymium‐Based Conversion Films for Stable Zn Metal Anodes21Establishing Ohmic contact with ultra-thin semiconductor layer through magnetron sputtering for dendrite-free Zn metal batteries4Low Strain Mediated Zn (0002) Plane Epitaxial Plating for Highly Stable Zinc Metal Batteries34Low Strain Mediated Zn (0002) Plane Epitaxial Plating for Highly Stable Zinc Metal Batteries1Water-Restrained Hydrogel Electrolytes with Repulsion-Driven Cationic Express Pathways for Durable Zinc-Ion Batteries71Rechargeable Cadmium Metal Batteries Enabled by an Aqueous CdSO4 Electrolyte14Ordered zinc electrodeposition from single-crystal units to polycrystalline stacking within solid-electrolyte interphase in battery anodes89High‐Entropy Deep Eutectic Solvent Achieves Ultra‐Low Polarization Zinc Anode Chemistry8High‐Entropy Deep Eutectic Solvent Achieves Ultra‐Low Polarization Zinc Anode Chemistry28Single (002)-Textured Zinc Anode via Nonepitaxial Electrodeposition with In Situ Texture Maintenance for Stable Aqueous Zinc Batteries50Electrochemical engineering in aqueous metal-ion batteries18Constructing Lipid-Like Biomimetic Structure via Electrolyte Designation for Stable Zinc-Ion Batteries12Directional solidification in gallium under strong magnetic field: NMR studies5Optimizing Amphoteric Cellulose Additives with Complexation–Adsorption Mechanisms to Stabilize the Zn Anode23SnS 2 (001)‐Reinforced Ion/Molecular Sieving Separator Enables High‐Performance Aqueous Zinc‐Organic Batteries5Accordion-structured robust zinc anodes via MXene-guided deposition towards durable zinc-ion batteries5Six-electron-conversion selenium cathodes stabilized by dead-selenium revitalizer for aqueous zinc batteries17Quasi-Solid-State Electrolytes: Bridging the gap between solid and liquid electrolytes for zinc-ion batteries35Zinc-spray-coated carbon fibres as lean anodes for low-cost zinc-ion batteries1Water-shielding electric double layer and stable interphase engineering for durable aqueous zinc-ion batteries138Breaking Performance Limits of Zn Anodes in Aqueous Batteries by Tailoring Anion and Cation Additives26Electron Donation Effect of α‐Boron Nanosheet Enables Highly Stable Zinc Metal Anode92Solid-state eutectic electrolyte via solvation regulation for voltage-elevated and deep-reversible Zn batteries37Synergistic surface adsorption and pH regulation enable highly reversible zinc metal anodes14Regulated dual-network hydrogel with interfacial engineering effect of alkaline zinc surface for flexible zinc-air battery13Epitaxial Zn (002) growth directed by Cu (111): A dual-layer strategy toward stable and reversible Zn metal anodes34Strategies for Strengthening Zn Metal Anodes in Aqueous Zinc-Ion Batteries─Current States and Perspectives15Designing an Anionic Layer in Low‐Concentration Electrolytes to Promote In‐Plane Ion Diffusion for Dendrite‐Free Zinc‐Ion Batteries23Zinc Deposition Behavior in Concentrated Aqueous Potassium Hydroxide Solutions2Ionically Cross‐Linked Composite Hydrogel Modulating an Electrical Double Layer on Zn Metal Anodes for Enhanced Kinetics and Stability7Proton/hydroxide ion dual-pathway interfacial water regulator-assisted surface stabilization in highly reversible Zn metal batteries23Uniaxially oriented zinc metal negative electrodes toward spontaneous dislocation-free homoepitaxy25Synergistic alloy interface and Zn(002) texture for stable Zn anodes in aqueous zinc ion batteries14Grain Boundary Engineering for Reversible Zn Anodes in Rechargeable Aqueous Zn-Ion Batteries1Free-Standing Al–Zn Anode for High-Performance Flexible Al-Organic Aqueous Batteries1A Synchronous Strategy to Zn-Iodine Battery by Polycationic Long-Chain Molecules36Orienting dendrite resistant behavior via heteroatom regulation toward high areal capacity zinc metal anode0Correlation of metal anode reversibility with solvation chemistry and interfacial electron transfer in aqueous electrolytes24Oriented crystallization of metal electrodeposition in aqueous zinc batteries5Dipole-unit mediated Co-solute engineering to construct nanodomain electrolytes for highly reversible and shuttle-free ZnI2 batteries0High-temperature-resistant mullite nanofiber membrane as an ion-sieving interlayer for uniform Zn2+ flux in long-life zinc ion hybrid capacitors1Epitaxial Substrate Engineering Enables Ultrastable Zinc Anodes via Low‐Lattice‐Mismatch Interface‐Induced Dendrite Regulation20Engineering Low‐Coordination Atoms into Zn 2 Ti 3 O 8 for Stable Zn Metal Anodes2Tuning oriented mesocrystalline assembly of NiCo2O4 via substrate interface engineering for enhanced lithium storage stability2Achieving dendrite-free zinc deposition by constructing stress-induced twin structures on zinc anodes for aqueous zinc-ion batteries8Durable Lithium Metal Anodes Enabled by {110}‐Textured Epitaxy on a LiF@Ag Commensurate Heterostructure4Understanding rate-dependent textured growth in zinc electrodeposition via high-throughput in situ x-ray diffraction29Supercritical CO 2 ‐Induced Surface Autogenous Mineralization Enabling Epitaxial Zn Electrodeposition on Weakly Conductive Crystalline Coating4Inner Helmholtz Layer Regulating Additive for Ultrastable Aqueous Zinc Ion Batteries3Self‐Assembled Homogeneous Heterobimetallic‐Oxide Interfaces Enable Synergistic Hydrogen Evolution Passivation for Durable Acidic Zn–Mn Batteries0Self‐Assembled Homogeneous Heterobimetallic‐Oxide Interfaces Enable Synergistic Hydrogen Evolution Passivation for Durable Acidic Zn–Mn Batteries9Failure Mechanisms and Practical Optimizations for Ah‐Scale Aqueous Zinc‐Ion Pouch Cells45Ion-sieving nanolayers for highly reversible zinc-ion batteries6Competitive Rechargeable Zinc Batteries for Energy Storage14Optimizing Interface Multi‐Physical Fields via (R)‐3‐Aminobutyric Acid Cations for Enhanced Zinc Deposition Behavior Realizes the Highly Efficient Zinc‐Iodine Batteries25Data‐Driven Additive Discovery with HOMO‐Descriptor Enables Durable Aqueous Zinc Batteries via Interfacial Kinetics Engineering58Electrodeposited Zinc Alloy Anodes for Aqueous Zinc Metal Batteries40Facet‐Guided in‐Plane Metal Plating via Accelerated Surface Diffusion in Mg Metal Batteries1Aqueous Zinc‐Ion Pouch Cells: From Failure Mechanisms to Practical Solutions15Aqueous Zinc‐Ion Pouch Cells: From Failure Mechanisms to Practical Solutions20Anion‐Type Solvation Structure Enables Freeze‐Tolerant Aqueous Zinc‐Vanadium Batteries18Emerging strategies on structural and constitutional modifications of zinc anode for enhanced performance in aqueous zinc-ion batteries8Single-Crystalline Anode Materials: Growth, Applications, Fabrication, and Recycling9Co-engineering dual Helmholtz planes and (101) facet-selective deposition for ultra-stable Zn metal anodes73

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