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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Single Exposed Zn (0002) Plane and Sustainable Zn‐Oriented Growth Achieving Highly Reversible Zinc Metal Batteries

Da Zhang, Ziyang Song, Ling Miao, Yaokang Lv, Hui Duan, Mingfang Li, Lihua Gan, Mingxian Liu

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Single Exposed Zn (0002) Plane and Sustainable Zn‐Oriented Growth Achieving Highly Reversible Zinc Metal BatteriesOriginalHydrogen bonding-stabilized bipolar organic cathode achieved all-round enhancement in zinc batteries12Building a multifunctional Cu 2 Se@biomass carbon composite interfacial layer on a zinc anode for stable aqueous zinc-ion batteries14Effective anode materials for in situ Sn@C nano-lamellar assembly with doped nanotubes in lithium-ion batteries11Multi-H-bonded self-assembled superstructures for ultrahigh-capacity and ultralong-life all-organic ammonium-ion batteries71Unlocking the potential of a multi-electron p-type polyheterocycle cathode: when it meets a small-size and high-charge anion53Mitigating ion flux vortex enables reversible metal electrodeposition0Unveiling the mysteries of anode-free Zn metal batteries: From key challenges to viable solutions31Eliminating electron localization by molecular array induces uniform zinc deposition enabling stable zinc anode9Comprehensive crystallographic engineering for high-efficiency and durable zinc metal anodes69Tea Polyphenol-Derived Zinc-Rich Complexes for Enhanced Interfacial Dynamics in PEO-Based Gel Electrolytes8Zinc‐Seeded PEDOT:PSS Aerogel Host as Highly Reversible Dendrite‐Free Zinc Metal Anode9Revealing active sites storage mechanism of organic C O/C N compounds for ultralong-life aqueous zinc-ion batteries7Disrupting the Crystal Growth of Corrosion Byproducts to Stabilize Aqueous Zn Metal Batteries0Vesicular-like manganese single-atom doped Poly(1,5-Naphthalenediamine) cathode for durable bipolar zinc-organic batteries3Inorganic–Organic Co‐Intercalated [Al 0.16 (C 5 H 14 ON) 0.12 ]V 2 O 5 ·0.39H 2 O Cathode for High‐Performance Aqueous Zinc‐Ion Batteries67Advancements in ion regulation strategies for enhancing the performance of aqueous Zn-ion batteries63Polyacrylic Acid Binder Enabling High Areal Capacity V2O5·nH2O Cathode for Aqueous Zinc‐Ion Batteries10Insights and prospects on the surface modification of zn metal anodes for aqueous rechargeable Zn-ion batteries5Ion distribution regulator enables ultra-long lifespan and ultra-high rate performance of zinc-ion batteries1Dragon-scale-inspired phosphate interface for enhanced stability of Zn powder anodes12Preconditioned Current to Activate Reaction Sites for Uniform Stripping/Plating toward Long-Life Magnesium Metal Anodes7Synergistic alloy interface and Zn(002) texture for stable Zn anodes in aqueous zinc ion batteries14Bionic Nanogel Interfaces Unlock Long‐Term Stability in Zn Metal Electrodeposition‐Based Electrochromic Windows14How Does the Hydroxylated Carbon Chain Length in Polyol Electrolyte Additives Influence the Stability of Zn Anode?2Preferential Texture of Surface Coating on Zn Anodes for Advanced Aqueous Batteries: Small Change but Big Gain4Preferential Texture of Surface Coating on Zn Anodes for Advanced Aqueous Batteries: Small Change but Big Gain19Realizing High Performance Four‐Electron Zinc‐Iodine Batteries with Acidic Eutectic Electrolyte7Realizing High Performance Four‐Electron Zinc‐Iodine Batteries with Acidic Eutectic Electrolyte48Modulating Adsorption Intermediate Metastability for Tip‐Directed Zinc Stripping and Suppressed Vanadium Dissolution Toward Long‐Cycling Zinc–Vanadium Batteries0Modulating Adsorption Intermediate Metastability for Tip‐Directed Zinc Stripping and Suppressed Vanadium Dissolution Toward Long‐Cycling Zinc–Vanadium Batteries16Low-activation-energy bipolar organic nanostructures for high-capacity and ultralong-life aqueous calcium-ion batteries9In Situ Nitrogen‐Rich Interphase Engineering Boosting Zn (002) Plane Texture with High Depth of Discharge for Long‐Term Zinc Metal Batteries9Advances in electrochemical interface regulation toward stable zinc anodes3Binder-free cold-sprayed Ni electrodes: a scalable route toward high performance hydrogen evolution catalyst15Highly zincophilic-hydrophobic polyzwitterionic hydrogel electrolyte with strong electronegative sulfobetaine-carboxyl motifs for ultrastable zinc-ion batteries23Role of Lewis base-type N sites of MOFs in achieving the preferential exposure of Zn(002) and HER-suppressed long-life zinc anodes3Achieving uniform zinc deposition under practical high areal capacity in zinc-ion batteries0Overcoming the Energy–Power Trade‐Off in Fiber Electronics: The Role of Metal‐Ion Hybrid Capacitors3Structural Engineering via In Situ Etching of Metal Surface for a Stabilized Zinc Metal Anode1Bifunctional mechanism of immobilized organic molecule to steer Zn2+ and polyiodides transport kinetics toward ultra-stable aqueous ZnI2 batteries1Deciphering the metallic zinc anode interface: multimodal characterization strategies for zinc-ion batteries3Hexagonal Porous Zincophilic Alloy Interface for Ultrastable Zinc Metal Anode1Mini review: advanced anodes for flexible Zn ion batteries0Arc-wire–sprayed stainless-steel coatings as robust and cost-effective electrocatalysts for the hydrogen evolution reaction (HER)11Two‐Dimensional Six‐Membered‐Ring Substrates as Interfacial Lattice Locking Layer for Stable Zinc (002) Epitaxial Electrodeposition7A bioinspired microdevice unifying energy storage and actuation through hydration control4Electrochromic zinc-ion batteries: recent progress, challenges and perspectives0Synergistic Piezoelectric‐Field and Crystal Plane Manipulation in Composite Solid Electrolytes Toward High‐Rate Zinc Metal Batteries3Unraveling the Design Principles of Crystallographic Orientation for Ultralong, 8500 Cycled Fe‐Ion Battery1Pre-oriented (002) ZnSn alloy anode via element exchange and low-temperature remelting for synergistically stable aqueous zinc-ion batteries0MnCo2O4 spinel as a noble-metal-free electrocatalyst for hydrogen evolution in alkaline media1Thermodynamics and Kinetics in Host Design for Dendrite‐Free Zinc Metal Anodes0Targeted Modulation of Zn Deposition Behavior toward High-Performance Stable Zn Anodes0

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  2. Building a multifunctional Cu 2 Se@biomass carbon composite interfacial layer on a zinc anode for stable aqueous zinc-ion batteries

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  3. Effective anode materials for in situ Sn@C nano-lamellar assembly with doped nanotubes in lithium-ion batteries

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  4. Multi-H-bonded self-assembled superstructures for ultrahigh-capacity and ultralong-life all-organic ammonium-ion batteries

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  5. Unlocking the potential of a multi-electron p-type polyheterocycle cathode: when it meets a small-size and high-charge anion

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  6. Mitigating ion flux vortex enables reversible metal electrodeposition

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  7. Unveiling the mysteries of anode-free Zn metal batteries: From key challenges to viable solutions

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  8. Eliminating electron localization by molecular array induces uniform zinc deposition enabling stable zinc anode

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  9. Comprehensive crystallographic engineering for high-efficiency and durable zinc metal anodes

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  10. Tea Polyphenol-Derived Zinc-Rich Complexes for Enhanced Interfacial Dynamics in PEO-Based Gel Electrolytes

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  11. Zinc‐Seeded PEDOT:PSS Aerogel Host as Highly Reversible Dendrite‐Free Zinc Metal Anode

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  12. Revealing active sites storage mechanism of organic C O/C N compounds for ultralong-life aqueous zinc-ion batteries

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  13. Disrupting the Crystal Growth of Corrosion Byproducts to Stabilize Aqueous Zn Metal Batteries

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  14. Vesicular-like manganese single-atom doped Poly(1,5-Naphthalenediamine) cathode for durable bipolar zinc-organic batteries

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  15. Inorganic–Organic Co‐Intercalated [Al 0.16 (C 5 H 14 ON) 0.12 ]V 2 O 5 ·0.39H 2 O Cathode for High‐Performance Aqueous Zinc‐Ion Batteries

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  16. Advancements in ion regulation strategies for enhancing the performance of aqueous Zn-ion batteries

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  17. Polyacrylic Acid Binder Enabling High Areal Capacity V2O5·nH2O Cathode for Aqueous Zinc‐Ion Batteries

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  22. Synergistic alloy interface and Zn(002) texture for stable Zn anodes in aqueous zinc ion batteries

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  31. Low-activation-energy bipolar organic nanostructures for high-capacity and ultralong-life aqueous calcium-ion batteries

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  32. In Situ Nitrogen‐Rich Interphase Engineering Boosting Zn (002) Plane Texture with High Depth of Discharge for Long‐Term Zinc Metal Batteries

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  33. Advances in electrochemical interface regulation toward stable zinc anodes

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