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RESEARCH PAPER · Matter · 2023

Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicals

Junliang Chen, Luyao Zhang, Li Wang, Min Kuang, Shaobin Wang, Jianping Yang

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Toward carbon neutrality: Selective conversion of waste plastics into value-added chemicalsOriginalPrecise activation of C–C bonds for recycling and upcycling of plastics81Monomer recycling of polyethylene terephthalate, polycarbonate and polyethers: Scalable processes to achieve high carbon circularity62A polyamide and polyethylene multilayer composite with enhanced barrier and mechanical properties at high temperature9Heterogeneous catalysis for the environment92Self-supported Ni/Ni 3 N 1− x heterostructures with abundant nitrogen vacancies as efficient electrocatalysts for ethylene glycol oxidation23Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst94Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst5A Unified View of Carbon Neutrality: Solar-Driven Selective Upcycling of Waste Plastics30From waste to wealth: The “Blue Circle” vision for a sustainable ocean future6Harnessing photosynthetic microorganisms for enhanced bioremediation of microplastics: A comprehensive review48Electro-Reforming of PET Plastic to C 2 Chemicals with Concurrent Generation of Hydrogen and Electric Energy188Spent Lithium‐Ion Batteries Derived Co 3 O 4 for Electrocatalytic Polyethylene Terephthalate Plastic Recycling22Fine-tune the electronic structure of copper nanowire networks by heteroatom doping toward enhanced Fenton-like reaction2Hydrogen Bubbles: Harmonizing Local Hydrogen Transfer for Efficient Plastic Hydro-Depolymerization19Unveiling synergy of strain and ligand effects in metallic aerogel for electrocatalytic polyethylene terephthalate upcycling117Electrocatalysis‐driven sustainable plastic waste upcycling33Radicals mediated polypropylene waste plastics oxidation into ketone fuel12Production of liquid hydrocarbon fuels through catalytic cracking of high and low-density polyethylene medical wastes using fly ash as a catalyst22Brønsted-acid sites induced photocatalytic cracking of low-polarity polyethylene plastics17Bimetal-carbon engineering for polypropylene conversion into hydrocarbons and ketones in a Fenton-like system10Microplastic detection and remediation through efficient interfacial solar evaporation for immaculate water production122Interstitial Boron Atoms in Pd Aerogel Selectively Switch the Pathway for Glycolic Acid Synthesis from Waste Plastics122Electrocatalytic upcycling of plastic waste: Progress, challenges, and future53Accelerated Solar-Driven Polyolefin Degradation via Self-Activated Hydroxy-Rich ZnIn2S435Catalytic recycling of plastics into value-added products28Upcycling of monomers derived from waste polyester plastics via electrocatalysis38Plasmonic Copper‐Ruthenium Superstructure for Efficient Photothermal Conversion and Plastic Recycling39Efficient Hydrocracking of Waste Polyethylene into Branched Liquid Fuels over Low Pt‐loaded Nb2O5 Catalyst5Universal and scalable synthesis of photochromic single-atom catalysts for plastic recycling42Preparation of NiCo hydroxide by chloride corrosion for electrocatalytic upcycling of polyethylene terephthalate plastic waste24Highly active cobalt oxide-palladium nanohybrid catalyst enables selective electrocatalytic synthesis of glycolic acid21Plastic Waste as a Challenge Cannot Be Ignored: Characteristics, Sources, Impacts, and Unveiling Potential Solutions through Photocatalysis for Environmental Sustainability5Advanced systems for enhanced CO 2 electroreduction72Merger of Single-Atom Catalysis and Photothermal Catalysis for Future Chemical Production40Recent advances of ethylene glycol oxidation reaction: catalytic mechanism, catalyst design and applications97Carbon Dioxide Upgrading to Biodegradable Plastics through Photo/Electro‐Synthetic Biohybrid Systems0Carbon Dioxide Upgrading to Biodegradable Plastics through Photo/Electro‐Synthetic Biohybrid Systems51Construction of Magnetically Recoverable Fe3o4@Ceo2 Core-Shell Photocatalyst for Efficient Upcycling of Plastic Waste0Innovative recycling strategies for non-recycled plastics: advancing the circular economy for a sustainable future22Monolithic, hybrid and particulate lignin-based hydrogels for sustainable CO 2 capture4Rapid degradation of microplastics by catalyst-free gliding arc plasmatron4Sustainable thermochemical plastic valorization towards a circular economy: a critical review27Advanced Catalysts for the Chemical Recycling of Plastic Waste90Trimetallic mesoporous PdCuRu for efficient formate electrosynthesis from polyethylene terephthalate recycling13Transforming Plastics to Single Atom Catalysts for Peroxymonosulfate Activation: Axial Chloride Coordination Intensified Electron Transfer Pathway116Mechanistic Insights into Polypropylene Hydrogenolysis Using Ni/Al2O3 Catalysts17Strategies and technologies for sustainable plastic waste treatment and recycling17Pd-doped CoNi-based bifunctional electrodes for upcycling of PET plastic with ultra-long stability19Photoreforming of waste plastic by B‐doped carbon nitride nanotube: Atomic‐level modulation and mechanism insights44Solving STEM-Relevant Problems: A Study with Prospective Primary School Teachers0Ampere-Level Upgrading of Polyethylene Terephthalate to Glycolate Using Palladium–Copper/Nickel Hydroxide Electrocatalysts51Photocatalytic Upgrading of Plastic Waste into High-Value-Added Chemicals and Fuels: Advances and Perspectives49Recent advances and challenges of double-atom catalysts in diverse environmental applications: A state-of-the-art review33Phase‐Controlled Pd─S Nanosheet Aerogels for Electrocatalytic Upgrading of Waste Plastics21Shell-like Ni(OH)2 loaded with Pd nanoparticle catalyst mediated efficient electrocatalytic upcycling of polyethylene terephthalate plastics to glycolic acid14Boosting Degradation of Polyethylene at Room Temperature4Persulfate-Based Advanced Oxidation Reforming of Polyethylene Terephthalate Fiber into Formate via Singlet Oxygen Activation25Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design Principles73Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19In-situ reconstruction of electrocatalysts for efficient energy and environmental electrocatalytic reactions17Advancements in the Electrochemical Upcycling of Waste Plastics into High-Value Products11Advances in Solar-Driven, Electro/Photoelectrochemical, and Photothermal-Assisted Upcycling of Waste Plastics10Pulsed electrosynthesis of glycolic acid through polyethylene terephthalate upcycling over a mesoporous PdCu catalyst74Environmental impact assessment of carbon-negative bio-based plastics advancing sustainable feedstock utilization0Photocatalytic Upcycling of Plastic Waste Into Value‐Added Chemicals21Synergistic Catalysis for Recycling and Upcycling of Plastics35Machine Learning‐Assisted Design of Multilayer Thermoplastic Composites: Robust Neural Network Prediction and Feature Importance Analysis3Highly selective photoreforming of plastic waste into pyruvate and coupled with hydrogen production from seawater on the defect-rich 2D/2D Cd0.5Zn0.5S/NiPS35Dual-substrate synergistic catalysis of WS2-Fe clusters on recycled plastic-derived N-doped carbon for H2O2 activation9Photoreforming for upcycling of plastics into energy, chemicals and materials: a review7Lattice and electronic structural engineering toward PET waste upcycling over PVP-incorporated Ni(OH)219Recent advances in the preparation of glycolic acid by selective electrocatalytic oxidation of ethylene glycol36Dual‐Site Synergistic Electrocatalysis Enables Highly Selective Upcycling of Real‐World Plastic Waste to Glycolic Acid62Current developments in multifunctional technology for waste plastic chemical recycling and case studies0Hydrophilicity-redox-coupling enhancement by pizza-structure engineering of Ni2P@CePO4@CFC for boosting furfuraldehyde biomass electro-oxidation19Strategies for Electrochemical Recycling of Plastic Polyethylene Terephthalate‐Derived Ethylene Glycol Into High‐Value Chemicals59A comprehensive review of biomass utilization for sustainable biofuel and biocomponent development23Concurrent production of glycolate and H2 via paired electrolysis: Ethylene glycol oxidation and hydrogen evolution from polyethylene terephthalate hydrolysate19Advanced Materials-Based Nanofiltration Membranes for Efficient Removal of Organic Micropollutants in Water and Wastewater Treatment20Electrocatalytic Polyester Waste Upcycling via Lattice Oxygen Redox Activation13Electrocatalytic Polyester Waste Upcycling via Lattice Oxygen Redox Activation2Circular economy strategies for converting waste plastics into surfactants6Photocatalytic Formamide Synthesis from Plastic Waste and Ammonia via C─N Bond Construction Under Mild Conditions4Photocatalytic Formamide Synthesis from Plastic Waste and Ammonia via C─N Bond Construction Under Mild Conditions23Biocarrier-driven enhancement of caproate production via microbial chain elongation: Linking metabolic redirection and microbiome assembly7Catalytic Depolymerization of Plastics to Valuable Products7Advances and Outlook of In Situ Characterization Techniques for Photocatalytic Reforming of Plastic Wastes5Precisely Controlled Relationship between Sulfur Vacancy and Ni Site for Boosting Photocatalytic Conversion of Polyester into Formate16Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12A magnetically recyclable core-shell heterojunction photocatalyst with oxygen vacancies for efficient upcycling of plastic waste6Emerging electrocatalytic conversion of NO x species into value-added nitrogenous chemicals18Energy‐Saving Microwave‐Assisted Catalysis Over SiC@NiFe for Selective Valorization of Plastic Wastes Into H 2 and Carbon Nanotubes4NanoFe3O4-catalyzed low-carbon upcycling of polyethylene microplastics: Mechanistic insights and environmental benefits3Recent Advances in Photocatalytic Conversion of Furfural2Electrochemical recovery and regeneration of polyethylene terephthalate materials7Electronic interaction of highly-dispersed Pd with defect-rich nickel disulfide nanoarrays for selective ethylene glycol-to-glycolate electroconversion9Programmable Photothermal Upcycling of Mixed Polyesters via Light‐Intensity Gating on a Bifunctional Zn/Co‐ZIF‐C Catalyst3Advanced catalyst design and mechanistic insights in electrocatalytic upcycling of PET-derived ethylene glycol and coupled electrolysis systems4Catalytic valorization of polyolefins: from catalysts and processes to reactors0Electronic Structure Modulation via La and Bi Co-Doping for High-Performance Electroreforming of PET Hydrolysate to Formic Acid0Highly efficient photoreforming of plastic waste for hydrogen production: recent advances and prospects1Sulfuric acid-mediated PET-derived carbon quantum dots for smartphone-assisted Fe 3+ screening in biological samples0Triad of electrocatalytic strategies for polymer monomer synthesis0Recovery technology for waste plastics based on electrocatalytic reforming: From mechanism understanding to catalyst design2Bridging Green Chemistry and Circular Economy: A Pathway to Sustainable Polyester Plastics Through Feedstock, Synthesis, and Waste Upcycling13Preparation of carbon nanotubes by catalytic pyrolysis of waste plastics coupled with chemical vapor deposition: Status and challenges3pH-dependent adsorption and reaction pathway regulation in ethylene glycol oxidation on TiO2 photoanode1Process intensification driven by non-conventional energy fields in emerging plastic recycling: A systematic review2A dual-cathode zinc-ethylene glycol/air battery for concurrent electricity generation and plastic waste upcycling3Recent progress in catalyst design for electrocatalytic upcycling of PET to glycolic acid0Photothermal catalysis for plastic upcycling: a review on material design and reaction mechanisms2Two-Dimensional Ferroelectric Materials Enable Controllable Electrocatalysis2Solvent‐ and Hydrogen‐Free Upcycling of Polystyrene by Layered Double Oxides0A holistic remedy to the plastic era through a high–performance photocatalytic system0Waste plastic recycling and upgrading via electro- and photocatalytic C−X bond coupling1Plastic-to-jet conversion of plastic waste: A critical review of pyrolysis oil characteristics and aviation fuel compliance3Challenges and strategies for catalyst coking in catalytic cracking of polyolefins to liquid fuels1Dynamic Self‐Focusing Photothermal Localization Induced Mild Solvent‐Free Upcycling of Polystyrene0Direct polymer-to-polymer upcycling of mixed PET/PBT wastes into biodegradable plastics: an environmental techno-economic assessment0Photoreforming and Photoelectroreforming of Waste‐Derived Feedstocks for Solar‐Driven Production of Fuels and Chemicals0Multicomponent Nanowire Aerogels With Tailored Adsorption Equilibrium for the Upcycling of Polyethylene Terephthalate0Spatial Confinement Nanoreactors Enable Synergistic Catalysis for Polyethylene Terephthalate-Derived Ethylene Glycol Oxidation0Engineering High-Spin Ruthenium Centers via Gradient Orbital Coupling for Electrocatalytic PET Upcycling0Optimal Design of Catalysts for Photoreforming Lactic Acid/Polylactic Acid to Clean Fuels and Value‐Added Chemicals0Electro‐ and Photocatalytic C─X Bond Coupling in Valorization of Waste Plastics/Biomass: Reaction Mechanism and Catalyst Engineering1Iron-Doped Carbon Nanotubes Facilitate ZnO Interfacial Charge Accumulation for Selective Singlet Oxygen Generation in Piezo-Photocatalytic Microplastics Upcycling0Photothermal Catalytic Depolymerization and Glycolytic Regeneration of Polyethylene Terephthalate0Bifunctional Ni3S2/Co4S3 electrocatalysts for high-efficiency electrochemical reforming of PET hydrolysate and oxygen evolution reaction0Machine learning and causal inference Reveal Gas–Liquid yield Regulation and Economic Feasibility in Catalytic plastic pyrolysis0Beyond Oxygen Evolution: Anodic High‐Value Conversion for Energy‐Saving Hydrogen and Chemical Co‐Production0Design and engineering of heterogeneous photocatalysts for plastic degradation and upcycling0EMSI and Alloying Synergistically Enable Selective Electrooxidation of PET‐Derived Ethylene Glycol to Glycolic Acid on PtAu‐Ni(OH) 20In Situ Hydrogen Utilization in Plastic Waste Recycling and Upcycling0

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