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RESEARCH PAPER · Journal of the American Chemical Society · 2023

Beyond π–π Stacking: Understanding Inversion Symmetry Breaking in Crystalline Racemates

Yiran Wang, Matthew Lander Nisbet, Kendall R. Kamp, Emily Hiralal, Romain Gautier, P. Shiv Halasyamani, Kenneth Reinhard Poeppelmeier

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Beyond π–π Stacking: Understanding Inversion Symmetry Breaking in Crystalline RacematesOriginalA new infrared nonlinear optical material BaZnGeS 4 with a wide band gap and large nonlinear optical response34Highly Birefringent d 0 Transition Metal Fluoroantimonite in the Mid Infrared Band: Order–Disorder Regulation by Cationic Size84Targeting Oxide Concentration in Tantalum Oxide-Fluoride Anions0Chiral and Polar Duality Design of Heteroanionic Compounds: Sr18Ge9O5S31 Based on [Sr3OGeS3]2+ and [Sr3SGeS3]2+ Groups20Secondary‐Bond‐Driven Construction of a Polar Material Exhibiting Strong Broad‐Spectrum Second‐Harmonic Generation and Large Birefringence9Secondary‐Bond‐Driven Construction of a Polar Material Exhibiting Strong Broad‐Spectrum Second‐Harmonic Generation and Large Birefringence41Dual-Anion Strategy Induces Dual Enhancement Toward Ultrashort Phase-Matching Wavelength in Deep-UV Transparent d0 Transition Metal Oxyfluorides22Chiral Templating in a Hybrid Chromium Chloride Hydrate2Chiral Metal Self‐Assemblies of Zirconium‐Tetrahedra and Their Second Harmonic Generation Activity6Chiral Metal Self‐Assemblies of Zirconium‐Tetrahedra and Their Second Harmonic Generation Activity0Bonding-Type-Driven Structural Transformation toward Novel Fluoroiodosulfates: Achieving Non-Centrosymmetry and Enhanced Optical Properties in K2(IO3F)SO30Chiral Communication between Enantiomeric Sergeants and Achiral Soldiers in Racemic Triblock Copolymers with Heterochiral Cores for Triggering Multiple Helicity Inversions11Chiral Communication between Enantiomeric Sergeants and Achiral Soldiers in Racemic Triblock Copolymers with Heterochiral Cores for Triggering Multiple Helicity Inversions2Exceptional Second Harmonic Generation in Ultraviolet Nonlinear Optical Oxyfluoroniobate Crystals via Structural Fingerprint Optimization of Polar Chains22Exceptional Second Harmonic Generation in Ultraviolet Nonlinear Optical Oxyfluoroniobate Crystals via Structural Fingerprint Optimization of Polar Chains8Crystallographic symmetry and stereochemical behavior of tris(ethane-1,2-diol)-zinc(ii) 2,2',3,3',5,5',6,6'-octafluoro[1,1'-biphenyl]-4,4'-dicarboxylate, a conglomerate with Z’ = 3.01Suppressing antiparallel dipole alignment: A molecular engineering strategy toward sem-organic UV NLO crystals0Bonding-type-driven structural transformation toward novel fluoroiodosulfates: Achieving non-centrosymmetry and enhanced optical properties in K2(IO3F)SO301D Cobalt‐Cytidine Monophosphate Coordination Polymer Exhibiting Efficient Ultraviolet Second‐Harmonic Generation7Predicting and Rationalizing Piezoelectricity in Racemic Bioorganic Molecular Crystals4Predicting and Rationalizing Piezoelectricity in Racemic Bioorganic Molecular Crystals0Co-assembled organic phosphorescent crystals with ultralong phosphorescence in high-temperature and water environment0An Ultra-Wide Bandgap Sulfonate with Two-Step Second-Harmonic Generation Switching2Positional Isomerism Controls Polarity and Nonlinear Optical Properties in One‐Dimensional Hybrid Germanium Halides0Kinetic Trapping of Pressure‐Induced Symmetry Breaking in Hybrid Metal Halides via Fluorine‐Mediated Molecular Locking0Kinetic Trapping of Pressure‐Induced Symmetry Breaking in Hybrid Metal Halides via Fluorine‐Mediated Molecular Locking0Influence of the Cation Size on Symmetry Breaking and Optical Performances in Ae2Mg3(BO3)2F4 (Ae = Sr, Ba)0

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27 direct citing papers saved.

  1. A new infrared nonlinear optical material BaZnGeS 4 with a wide band gap and large nonlinear optical response

    Inorganic Chemistry Frontiers · 2023-01-01

    Hongshan Wang, Xueting Pan, Wang Zhao, Yu Chu, Junjie Li

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  2. Highly Birefringent d 0 Transition Metal Fluoroantimonite in the Mid Infrared Band: Order–Disorder Regulation by Cationic Size

    Journal of the American Chemical Society · 2023-10-26

    Jia-Hang Wu, Chun‐Li Hu, Ting-Kun Jiang, Jiang‐Gao Mao, Fang Kong

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  3. Targeting Oxide Concentration in Tantalum Oxide-Fluoride Anions

    Solid State Sciences · 2023-11-16

    Kendall R. Kamp, Yiran Wang, Kenneth Reinhard Poeppelmeier

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  4. Chiral and Polar Duality Design of Heteroanionic Compounds: Sr18Ge9O5S31 Based on [Sr3OGeS3]2+ and [Sr3SGeS3]2+ Groups

    Advanced Science · 2023-12-08

    Shaoxin Cui, Hongping Wu, Xinkang Dong, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Kenneth Reinhard Poeppelmeier, Hongwei Yu

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  5. Secondary‐Bond‐Driven Construction of a Polar Material Exhibiting Strong Broad‐Spectrum Second‐Harmonic Generation and Large Birefringence

    Angewandte Chemie · 2023-12-20

    Tianhui Wu, Xingxing Jiang, Kaining Duanmu, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  6. Secondary‐Bond‐Driven Construction of a Polar Material Exhibiting Strong Broad‐Spectrum Second‐Harmonic Generation and Large Birefringence

    Angewandte Chemie International Edition · 2023-12-20

    Tianhui Wu, Xingxing Jiang, Kaining Duanmu, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  7. Dual-Anion Strategy Induces Dual Enhancement Toward Ultrashort Phase-Matching Wavelength in Deep-UV Transparent d0 Transition Metal Oxyfluorides

    ACS Materials Letters · 2024-02-23

    Dongdong Chu, Kewang Zhang, Congwei Xie, Keith T. Butler, Zhihua Yang, Shilie Pan

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  8. Chiral Templating in a Hybrid Chromium Chloride Hydrate

    Inorganic Chemistry · 2024-07-04

    Joseph T. Race, Cierra J. Foster, Patrick M. Woodward

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  9. Chiral Metal Self‐Assemblies of Zirconium‐Tetrahedra and Their Second Harmonic Generation Activity

    Angewandte Chemie International Edition · 2024-10-29

    Ermeng Han, Y.J. Li, Tun Wu, Qixia Bai, Zhe Zhang, Jie George Yuan, Wei Liu, Die Liu, Yiming Li, Pingshan Wang

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  10. Chiral Metal Self‐Assemblies of Zirconium‐Tetrahedra and Their Second Harmonic Generation Activity

    Angewandte Chemie · 2024-10-29

    Ermeng Han, Y.J. Li, Tun Wu, Qixia Bai, Zhe Zhang, Jie George Yuan, Wei Liu, Die Liu, Yiming Li, Pingshan Wang

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  11. Bonding-Type-Driven Structural Transformation toward Novel Fluoroiodosulfates: Achieving Non-Centrosymmetry and Enhanced Optical Properties in K2(IO3F)SO3

    SSRN Electronic Journal · 2025-01-01

    Juhui Cui, Junwei Feng, Yu Feng, Minqiang Gai

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  12. Chiral Communication between Enantiomeric Sergeants and Achiral Soldiers in Racemic Triblock Copolymers with Heterochiral Cores for Triggering Multiple Helicity Inversions

    Angewandte Chemie International Edition · 2025-02-11

    Zixiang He, Haotian Ma, Zeyu Tang, Xiaoxiao Cheng, Wei Zhang

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  13. Chiral Communication between Enantiomeric Sergeants and Achiral Soldiers in Racemic Triblock Copolymers with Heterochiral Cores for Triggering Multiple Helicity Inversions

    Angewandte Chemie · 2025-02-11

    Zixiang He, Haotian Ma, Zeyu Tang, Xiaoxiao Cheng, Wei Zhang

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  14. Exceptional Second Harmonic Generation in Ultraviolet Nonlinear Optical Oxyfluoroniobate Crystals via Structural Fingerprint Optimization of Polar Chains

    Angewandte Chemie International Edition · 2025-07-01

    Congcong Jin, Yang Li, Jin Seong Kim, Joshua Lim, Hongbo Huang, Chong‐An Chen, Jihyun Lee, Yejin Heo, Bingbing Zhang, Joon Ik Jang, Kang Min Ok

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  15. Exceptional Second Harmonic Generation in Ultraviolet Nonlinear Optical Oxyfluoroniobate Crystals via Structural Fingerprint Optimization of Polar Chains

    Angewandte Chemie · 2025-07-01

    Congcong Jin, Yang Li, Jin Seong Kim, Joshua Lim, Hongbo Huang, Chong‐An Chen, Jihyun Lee, Yejin Heo, Bingbing Zhang, Joon Ik Jang, Kang Min Ok

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  16. Crystallographic symmetry and stereochemical behavior of tris(ethane-1,2-diol)-zinc(ii) 2,2',3,3',5,5',6,6'-octafluoro[1,1'-biphenyl]-4,4'-dicarboxylate, a conglomerate with Z’ = 3.0

    Structural Chemistry · 2025-07-25

    Ivan Bernal, Roger A. Lalancette

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  17. Suppressing antiparallel dipole alignment: A molecular engineering strategy toward sem-organic UV NLO crystals

    The Innovation Materials · 2026-01-01

    Guangsheng Xu, Xue Bai, Zhihua Yang, Xueling Hou, Jian Han, Shilie Pan

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  18. Bonding-type-driven structural transformation toward novel fluoroiodosulfates: Achieving non-centrosymmetry and enhanced optical properties in K2(IO3F)SO3

    Materials Today Chemistry · 2026-01-16

    Juhui Cui, Junwei Feng, Feng Xia Yu, minqiang gai

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  19. 1D Cobalt‐Cytidine Monophosphate Coordination Polymer Exhibiting Efficient Ultraviolet Second‐Harmonic Generation

    Chemistry - A European Journal · 2026-02-09

    Mubashar Ilyas, Lin Xiong, Li Zhang, Maida, Maroof Ahmad Khan, Muhammad Abbas, Nagesh Manurkar, Mudassar Ilyas, Niu Zhang, Hui Li

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  20. Predicting and Rationalizing Piezoelectricity in Racemic Bioorganic Molecular Crystals

    Angewandte Chemie International Edition · 2026-03-23

    Shubham Vishnoi, Sarah Guerin

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  21. Predicting and Rationalizing Piezoelectricity in Racemic Bioorganic Molecular Crystals

    Angewandte Chemie · 2026-03-25

    Shubham Vishnoi, Sarah Guerin

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  22. Co-assembled organic phosphorescent crystals with ultralong phosphorescence in high-temperature and water environment

    Chemical Engineering Journal · 2026-04-01

    Bin Li, Ziyi Lu, Wensheng Xu, Ruixue Wang, Jianfeng Liu, Linshuo Jiang, Yin Xiao, Jianchao Ma, Yang Li, Xilong Yan, Bowei Wang, Ligong Chen

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  23. An Ultra-Wide Bandgap Sulfonate with Two-Step Second-Harmonic Generation Switching

    Journal of the American Chemical Society · 2026-04-06

    Feiyuan Gong, Yiran Zhang, Guangfeng Wei, Xingxing Jiang, Chao Wu, Zheshuai Lin, Zhipeng Huang, Jinhu Yang, Mark Graeme Humphrey, Chi Zhang

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  24. Positional Isomerism Controls Polarity and Nonlinear Optical Properties in One‐Dimensional Hybrid Germanium Halides

    Angewandte Chemie · 2026-04-29

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  25. Kinetic Trapping of Pressure‐Induced Symmetry Breaking in Hybrid Metal Halides via Fluorine‐Mediated Molecular Locking

    Angewandte Chemie International Edition · 2026-07-29

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  26. Kinetic Trapping of Pressure‐Induced Symmetry Breaking in Hybrid Metal Halides via Fluorine‐Mediated Molecular Locking

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  27. Influence of the Cation Size on Symmetry Breaking and Optical Performances in Ae2Mg3(BO3)2F4 (Ae = Sr, Ba)

    Inorganic Chemistry · 2026-10-05

    Yu Qiu, Haonan Liu, Yujie Zhang, Hongping Wu, Hongwei Yu

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