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RESEARCH PAPER · Science China Materials · 2023

Fast Li+-conducting Zr4+-based oxychloride electrolyte with good thermal and solvent stability

Bing Li, Yutao Li, Hong‐Shen Zhang, Tingting Wu, Sijie Guo, Amin Cao

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Fast Li+-conducting Zr4+-based oxychloride electrolyte with good thermal and solvent stabilityOriginalAmorphous Chloride Solid Electrolytes with High Li-Ion Conductivity for Stable Cycling of All-Solid-State High-Nickel Cathodes160A multi-step charging/discharging protocol enables stable cycling for lithium argyrodite-based all-solid-state lithium batteries8New advances in solid-state electrolytes: from halides to oxyhalides29Revealing unprecedented cathode interface behavior in all-solid-state batteries with oxychloride solid electrolytes44Li3N interlayer enables stable long-term cycling for sulfide-based all-solid-state Li metal batteries34Amorphous Oxyhalide Matters for Achieving Lithium Superionic Conduction186Inorganic lithium-ion conductors for fast-charging lithium batteries: a review9Variation of electrochemical performance of Li2ZrCl6 halide solid electrolyte with Mn substitution for all-solid-state batteries31Overcoming the Na-ion conductivity bottleneck for the cost-competitive chloride solid electrolytes17A Cost‐Effective Sulfide Solid Electrolyte Li 7 P 3 S 7.5 O 3.5 with Low Density and Excellent Anode Compatibility38A Cost‐Effective Sulfide Solid Electrolyte Li7P3S7.5O3.5 with Low Density and Excellent Anode Compatibility3Exploring superionic conduction in lithium oxyhalide solid electrolytes considering composition and structural factors31Mixed conductive layer formed by ZnO–graphite conversion–reaction enables dendrite–free all–solid–state lithium metal batteries26High Li+ Conducting Porous Garnet Enables Fast Li+ Conduction in Polymer/Garnet Composite Electrolyte4Halide-based solid electrolytes: opportunities and challenges in the synergistic development of all-solid-state Li/Na batteries22Deciphering Interfacial Stability of Sulfide and Halide-Based Electrolytes via Operando X-ray Photoelectron Spectroscopy22Scalable Interfacial Engineering with Lithiophilic‐Lithiophobic Layers for High‐Performance All‐Solid‐State Li‐Metal Batteries33Cation‐Anion‐Engineering Modified Oxychloride Zr‐Based Lithium Superionic Conductors for All‐Solid‐State Lithium Batteries2Cation‐Anion‐Engineering Modified Oxychloride Zr‐Based Lithium Superionic Conductors for All‐Solid‐State Lithium Batteries36Recovering the Ionic Conductivity of Oxygen‐Doped Li3.25InCl5.75O0.25 Electrolyte through Heat Treatment: Reconstructing the Structure Damaged by Moisture11Strategy for synergistic binders in sulfide-based solid electrolyte membrane7Enhancing Compatibility of Halide with Sulfide‐Electrolytes via High Oxygen Incorporation for Robust Solid‐State Batteries31Amorphous Nitride‐chloride Solid‐State Electrolytes for High Performance All‐Solid‐State Lithium Batteries14Amorphous Nitride‐chloride Solid‐State Electrolytes for High Performance All‐Solid‐State Lithium Batteries6Interfacial Coordination Engineering to Boost Li‐Ion Conduction in Economic Zr‐Based Halide Electrolytes22Regulated interface conduction in halide solid electrolyte for all-solid-state sodium batteries1Mechanically compliant and cost-effective 1.4Li2O-0.75ZrCl4-0.25AlCl3 solid electrolyte for all-solid-state batteries with improved cycling stability13Advancing Interface Engineering for Non-Close-Packed Halide-Based All-Solid-State Lithium Batteries3Electrochemical Behavior and Interfacial Failure of Li 2.22 Zr 1.11 Cl 5.33 O 0.67 in High-Performance All-Solid-State Batteries1Tunable ionic conductivity in halide electrolytes through cation ion exchange and channel engineering0Design Principles for Aqueous Stability of Lithium Halide and Oxyhalide Solid Electrolytes from First-Principles Pourbaix Analysis0Endowing Metal Oxychloride Solid Electrolytes with Improved Li Compatibility0Mechanochemical regulation of oxygen-doped halide electrolytes for stable interfaces in all-solid-state batteries0

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  1. Amorphous Chloride Solid Electrolytes with High Li-Ion Conductivity for Stable Cycling of All-Solid-State High-Nickel Cathodes

    Journal of the American Chemical Society · 2023-12-11

    Feng Li, Xiaobin Cheng, Gongxun Lu, Yi‐Chen Yin, Ye-Chao Wu, Ruijun Pan, Jin‐Da Luo, Fanyang Huang, Li‐Zhe Feng, Lei‐Lei Lu, Tao Ma, Lirong Zheng, Shuhong Jiao, Ruiguo Cao, Zhi‐Pan Liu, Hongmin Zhou, Xinyong Tao, Cheng Shang, Hong‐Bin Yao

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  2. A multi-step charging/discharging protocol enables stable cycling for lithium argyrodite-based all-solid-state lithium batteries

    Journal of Materials Chemistry A · 2024-01-01

    Pengfei Ren, Xiaodong Wang, Yirui Deng, Zijun Liu, Ruiping Liu

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  3. New advances in solid-state electrolytes: from halides to oxyhalides

    Inorganic Chemistry Frontiers · 2024-01-01

    Qingtao Wang, Zhenyang Shen, Pengfei Du, Yongmei Zhou, Peng Zhang, Ying Liu

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  4. Revealing unprecedented cathode interface behavior in all-solid-state batteries with oxychloride solid electrolytes

    Energy & Environmental Science · 2024-01-01

    Feipeng Zhao, Shumin Zhang, Shuo Wang, Carmen M. Andrei, Hui Yuan, Jigang Zhou, Jian Wang, Zengqing Zhuo, Yu Zhong, Han Su, Jung Tae Kim, Ruizhi Yu, Yingjie Gao, Jinghua Guo, Tsun‐Kong Sham, Yifei Mo, Xueliang Andy Sun

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  5. Li3N interlayer enables stable long-term cycling for sulfide-based all-solid-state Li metal batteries

    Journal of Energy Storage · 2024-01-18

    Pengfei Ren, Xiaodong Wang, Bing Huang, Ze Liu, Ruiping Liu

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  6. Amorphous Oxyhalide Matters for Achieving Lithium Superionic Conduction

    Journal of the American Chemical Society · 2024-01-29

    Shumin Zhang, Feipeng Zhao, Lo‐Yueh Chang, Yu‐Chun Chuang, Zhen Zhang, Yuanmin Zhu, Xiaoge Hao, Jiamin Fu, Jiatang Chen, Jing Li Luo, Minsi Li, Yingjie Gao, Yining Huang, Tsun‐Kong Sham, Meng Danny Gu, Yuanpeng Zhang, Graham King, Xueliang Andy Sun

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  7. Inorganic lithium-ion conductors for fast-charging lithium batteries: a review

    Journal of Solid State Electrochemistry · 2024-02-13

    Ning Xue, Chang Zhang, Wei Liu

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  8. Variation of electrochemical performance of Li2ZrCl6 halide solid electrolyte with Mn substitution for all-solid-state batteries

    Journal of Power Sources · 2024-03-23

    Han-Jin Jeon, Yuvaraj Subramanian, Kwang‐Sun Ryu

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  9. Overcoming the Na-ion conductivity bottleneck for the cost-competitive chloride solid electrolytes

    Journal of Energy Chemistry · 2024-03-25

    Lv Hu, Hui Li, Fang Chen, Yating Liu, Jinzhu Wang, Cheng Ma

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  10. A Cost‐Effective Sulfide Solid Electrolyte Li 7 P 3 S 7.5 O 3.5 with Low Density and Excellent Anode Compatibility

    Angewandte Chemie International Edition · 2024-06-30

    Hui Li, Qiaosong Lin, Jinzhu Wang, Lv Hu, Fang Chen, Zhihua Zhang, Zhihua Zhang, Cheng Ma

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  11. A Cost‐Effective Sulfide Solid Electrolyte Li7P3S7.5O3.5 with Low Density and Excellent Anode Compatibility

    Angewandte Chemie · 2024-07-01

    Hui Li, Qiaosong Lin, Jinzhu Wang, Lv Hu, Fang Chen, Zhihua Zhang, Cheng Ma

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  12. Exploring superionic conduction in lithium oxyhalide solid electrolytes considering composition and structural factors

    npj Computational Materials · 2024-07-14

    Fiaz Hussain, Jinlong Zhu, Yusheng Zhao, Wei Xia

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  13. Mixed conductive layer formed by ZnO–graphite conversion–reaction enables dendrite–free all–solid–state lithium metal batteries

    Nano Energy · 2024-08-15

    Pengfei Ren, Sidong Zhang, Bing Li, Ruiping Liu, Nan Wu, Yutao Li

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  14. High Li+ Conducting Porous Garnet Enables Fast Li+ Conduction in Polymer/Garnet Composite Electrolyte

    ACS Applied Energy Materials · 2024-09-02

    Wei Hu, Po‐Hsiu Chien, Nan Wu, Shengwen Zhong

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  15. Halide-based solid electrolytes: opportunities and challenges in the synergistic development of all-solid-state Li/Na batteries

    EES batteries. · 2025-01-01

    Xiaohan Tang, Fei Xie, Yaxiang Lu, Xiaohui Rong, Liquan Chen, Yong-Sheng Hu

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  16. Deciphering Interfacial Stability of Sulfide and Halide-Based Electrolytes via Operando X-ray Photoelectron Spectroscopy

    Nano Letters · 2025-03-10

    Zhicong Liu, Jianming Tao, Han Jiang, Yubing Wu, Lin Liang, Yanmin Yang, Yue Chen, Zhigao Huang, Yingbin Lin

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  17. Scalable Interfacial Engineering with Lithiophilic‐Lithiophobic Layers for High‐Performance All‐Solid‐State Li‐Metal Batteries

    Advanced Functional Materials · 2025-03-20

    Pengfei Ren, Nicholas Spencer Grundish, Sidong Zhang, Lihai Zhou, Ruiping Liu, Nan Wu, Yutao Li

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  18. Cation‐Anion‐Engineering Modified Oxychloride Zr‐Based Lithium Superionic Conductors for All‐Solid‐State Lithium Batteries

    Angewandte Chemie · 2025-04-01

    Zongnan Li, Yongbiao Mu, Kunxi Lü, Guojian Kang, Ting Yang, Shuping Huang, Mingdeng Wei, Lin Zeng, Yafeng Li

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  19. Cation‐Anion‐Engineering Modified Oxychloride Zr‐Based Lithium Superionic Conductors for All‐Solid‐State Lithium Batteries

    Angewandte Chemie International Edition · 2025-04-01

    Zongnan Li, Yongbiao Mu, Kunxi Lü, Guojian Kang, Ting Yang, Shuping Huang, Mingdeng Wei, Lin Zeng, Lin Zeng, Yafeng Li, Yafeng Li

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  20. Recovering the Ionic Conductivity of Oxygen‐Doped Li3.25InCl5.75O0.25 Electrolyte through Heat Treatment: Reconstructing the Structure Damaged by Moisture

    ChemSusChem · 2025-05-02

    Miao Deng, Shiyu Liu, Siwu Li, Wenwen Hu, Ziyu Lu, Ziling Jiang, Lin Li, Kunpeng Tang, Lei Shi, Qiyue Luo, Haitao Li, Jie Yang, Chen Liu, Chuang Yu

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  21. Strategy for synergistic binders in sulfide-based solid electrolyte membrane

    Tungsten · 2025-05-22

    Peng-Fei Ren, Sidong Zhang, Cheng Chen, Qi Yang, Ruiping Liu

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  22. Enhancing Compatibility of Halide with Sulfide‐Electrolytes via High Oxygen Incorporation for Robust Solid‐State Batteries

    Advanced Functional Materials · 2025-07-01

    Haochang Zhang, Pengcheng Yu, Ziang Cui, Hailun Jin, Wen Tang, Chunlei Zhao, Jiuwei Lei, Shuaika Liang, Zhepu Shi, Jianhui Wang, Ying Li, Fiaz Hussain, Jinlong Zhu, Wei Xia

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  23. Amorphous Nitride‐chloride Solid‐State Electrolytes for High Performance All‐Solid‐State Lithium Batteries

    Angewandte Chemie International Edition · 2025-07-03

    Tingting Wu, Sijie Guo, Hong‐Shen Zhang, Yue Jiang, Jun Zi Wang, Jiacheng Zhu, Xusheng Zhang, Pengfei Wei, Ziyang Hu, Rongzhi Gao, GuanHua Chen, Rui Wen, Xuefeng Wang, Amin Cao

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  24. Amorphous Nitride‐chloride Solid‐State Electrolytes for High Performance All‐Solid‐State Lithium Batteries

    Angewandte Chemie · 2025-07-03

    Tingting Wu, Sijie Guo, Hong‐Shen Zhang, Yue Jiang, Jun Zi Wang, Jiacheng Zhu, Xusheng Zhang, Pengfei Wei, Ziyang Hu, Rongzhi Gao, GuanHua Chen, Rui Wen, Xuefeng Wang, Amin Cao

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  25. Interfacial Coordination Engineering to Boost Li‐Ion Conduction in Economic Zr‐Based Halide Electrolytes

    Advanced Materials · 2025-07-15

    Mengyi Wu, Han Su, Yu Zhong, Fan Zhao, J.P. Tu, Xiuli Wang

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  26. Regulated interface conduction in halide solid electrolyte for all-solid-state sodium batteries

    Tungsten · 2025-08-06

    Li-Hai Zhou, Bing Li, Wei-Ping Li, Sidong Zhang, Cheng Chen, Xue-Feng Wang, Weidong Zhou

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  27. Mechanically compliant and cost-effective 1.4Li2O-0.75ZrCl4-0.25AlCl3 solid electrolyte for all-solid-state batteries with improved cycling stability

    Nature Communications · 2026-01-08

    Lv Hu, Yaolong He, Dong Wang, Wanxia Li, Jingming Yao, Xiaolong Zhang, Jinfeng Zhu, Huaican Chen, Wen Yin, Yanru Wang, Kejun Yan, Jinzhu Wang, Hui Li, Fang Chen, Yating Liu, Junqi Lai, Qi Chen, Jie Ma, Shuhong Jiao, Guorui Wang, Siqi Shi, Liwei Chen, Jianyu Huang, Cheng Ma

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  28. Advancing Interface Engineering for Non-Close-Packed Halide-Based All-Solid-State Lithium Batteries

    ACS Applied Energy Materials · 2026-03-03

    Kai Zhang, Songjia Kong, Keqi Chen, Siwen Zhang, Yanguang Li, Feipeng Zhao

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  29. Electrochemical Behavior and Interfacial Failure of Li 2.22 Zr 1.11 Cl 5.33 O 0.67 in High-Performance All-Solid-State Batteries

    Industrial & Engineering Chemistry Research · 2026-03-16

    J. J. Chen, Miao Deng, Sitong Ren, Siwu Li, Yi Wang, Zhenyu Wang, Chuang Yu

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  30. Tunable ionic conductivity in halide electrolytes through cation ion exchange and channel engineering

    Applied Physics Letters · 2026-06-15

    Zhiwei Peng, Yi-Xiang Wang, Asad Mehboob, Taoda Liu, Zongqing Tian, Yuhang Dou, Tian Ouyang, Yinghua Niu, Weiqiang Lv

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  31. Design Principles for Aqueous Stability of Lithium Halide and Oxyhalide Solid Electrolytes from First-Principles Pourbaix Analysis

    ACS Energy Letters · 2026-06-22

    Yan Li, Zeyu Deng

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  32. Endowing Metal Oxychloride Solid Electrolytes with Improved Li Compatibility

    Journal of the American Chemical Society · 2026-06-23

    LH Hu, Jingming Yao, Changshun Li, Kejun Yan, Jinfeng Zhu, Yi-Xiang Wang, Hui Li, Fengqian Chen, Huaican Chen, Wen Yin, Jie Ma, Jun Jiang, Zhuoying Zhu, Jianyu Huang, Cheng Ma

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  33. Mechanochemical regulation of oxygen-doped halide electrolytes for stable interfaces in all-solid-state batteries

    Journal of Power Sources · 2026-07-22

    Miao Deng, Li Li, Ziyu Lu, Wenqian Tian, Le Chen, Siwu Li, Chuang Yu

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