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RESEARCH PAPER · Journal of the American Chemical Society · 2023

Solvent-Mediated Separation and Reversible Transformation of 1D Supramolecular Polymorphs Built from [W10O32]4– Templated 48-Nuclei Silver(I) Cluster

Kai Sheng, Zhi Wang, Li Li, Zhiyong Gao, Chen‐Ho Tung, Di Sun

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Solvent-Mediated Separation and Reversible Transformation of 1D Supramolecular Polymorphs Built from [W10O32]4– Templated 48-Nuclei Silver(I) ClusterOriginalVisible to NIR‐II Photoluminescence of Atomically Precise Gold Nanoclusters189A concise guide to chemical reactions of atomically precise noble metal nanoclusters30Three in One: Three Different Molybdates Trapped in a Thiacalix[4]arene Protected Ag72 Nanocluster for Structural Transformation and Photothermal Conversion36Three in One: Three Different Molybdates Trapped in a Thiacalix[4]arene Protected Ag72 Nanocluster for Structural Transformation and Photothermal Conversion1Atomically Precise Silver Clusters Stabilized by Lacunary Polyoxometalates with Photocatalytic CO 2 Reduction Activity103Atomically Precise Silver Clusters Stabilized by Lacunary Polyoxometalates with Photocatalytic CO2 Reduction Activity8Unlocking the Potential of an Atom-Precise Ag12 Cluster Assembled Material as a Highly Efficient SERS Sensor for the Detection of Hg2+ Ions26A bis-aromatic MOF system constructed with a copper iodine cluster and porphyrinic ligand for enhancing near-infrared photothermal conversion5All-catecholate-stabilized black titanium-oxo clusters for efficient photothermal conversion30Assembly of anionic silver nanoclusters with controlled packing structures through site-specific ionic bridges4Development of non-closed silver clusters by transition-metal-coordination-cluster substituted polyoxometalate templates16Polyoxometalate-mediated syntheses of three structurally new silver clusters22Regulating electrical conductivity and Schottky nature of d 10 metal ion-based nanoarchitectonics in coordination polymers1Two structurally new Lindqvist hexaniobate-templated silver thiolate clusters20Eight‐Electron Copper Nanoclusters for Photothermal Conversion20Self‐Adaptive Aromatic Cation‐π Driven Dimensional Polymorphism in Supramolecular Polymers for the Photocatalytic Oxidation and Separation of Aromatic/Cyclic Aliphatic Compounds0Self‐Adaptive Aromatic Cation‐π Driven Dimensional Polymorphism in Supramolecular Polymers for the Photocatalytic Oxidation and Separation of Aromatic/Cyclic Aliphatic Compounds23Electrocatalytic and photocatalytic activities of two alkynyl Ag20 cage clusters involved ligand exchange between PhCOO− and CF3COO−1Solvent-Mediated Hetero/Homo-Phase Crystallization of Copper Nanoclusters and Superatomic Kernel-Related NIR Phosphorescence44Handedness‐Inverted and Stimuli‐Responsive Circularly Polarized Luminescent Nano/Micromaterials Through Pathway‐Dependent Chiral Supramolecular Polymorphism77Diamondoid Ni(II) Coordination Polymer as an Electrocatalyst for Hydrogen and Oxygen Evolution Reactions and Overall Water Splitting8Structural Insights into In Situ Disulfide Bond Formation for Enhancing Schottky Diode Behavior of a Paddle-Wheel Zn-Based Coordination Polymer6Concomitant Near‐Infrared Photothermy and Photoluminescence of Rod‐Shaped Au 52 (PET) 32 and Au 66 (PET) 38 Synthesized Concurrently10Concomitant Near‐Infrared Photothermy and Photoluminescence of Rod‐Shaped Au 52 (PET) 32 and Au 66 (PET) 38 Synthesized Concurrently36Phenanthroline-Mediated Photoelectrical Enhancement in Calix[4]arene-Functionalized Titanium-Oxo Clusters2Tuning up of chromism, luminescence in cadmium-viologen complexes through polymorphism strategy: Inkless erasable printing application9Micro‐Ring Morphology of Ag7NCs and Light‐Induced Reversible Interconversion of FCC Ag14NCs via Cu2+ ions‐Mediated Particle‐Assisted Reversible Interconversion5Micro‐Ring Morphology of Ag7NCs and Light‐Induced Reversible Interconversion of FCC Ag14NCs via Cu2+ ions‐Mediated Particle‐Assisted Reversible Interconversion1Vanadium-Silsesquioxane Nanocages as Heterogeneous Catalysts for Synthesis of Quinazolinones19Integrating Polyoxometalates and Silver Clusters into Atomically Precise Molecular Heterojunction5Guest-Induced Helical Superstructure from a Gold Nanocluster-Based Supramolecular Organic Framework Enables Efficient Catalysis21Atomically Precise Ternary Cluster: Polyoxometalate Cluster Sandwiched by Gold Clusters Protected by N‐Heterocyclic Carbenes1Atomically Precise Ternary Cluster: Polyoxometalate Cluster Sandwiched by Gold Clusters Protected by N‐Heterocyclic Carbenes9Auxiliary ligand-induced assembly of atomically precise silver clusters4Reversible Interconversion between Ag2 and Ag6 Clusters and Their Responsive Optical Properties13Strategic Advancement in Inner Filter Effect Controllable Detection of Tetracyclines and Nitroaromatics in Real-World Matrices by Two-Dimensional Coordination Polymer12Ln III /Cu I Bimetallic Nanoclusters with Enhanced NIR-II Luminescence21Application of Hard and Soft Acid‐base Theory to Construct Heterometallic Materials with Metal‐oxo Clusters52Application of Hard and Soft Acid‐base Theory to Construct Heterometallic Materials with Metal‐oxo Clusters5Epitaxial Growth of Silver Clusters from Ag57 to Ag72 via Laminating Multiple Different Anion Templates15Epitaxial Growth of Silver Clusters from Ag57 to Ag72 via Laminating Multiple Different Anion Templates0A comprehensive review of atomically precise metal nanoclusters with emergent photophysical properties towards diverse applications171Directly imaging the in-situ chemical transformation of nickel cubane nanoclusters for promoting electrocatalytic urea-oxidation-reaction4A new silver–thiolate nanocluster synthesized utilizing pure-inorganic polyoxoniobate as a starting template and its variable-temperature fluorescence properties0Controllable syntheses of two structurally new {AsW 9 O 33 }-mediated silver alkynyl clusters6Development of a boron-doping strategy to activate luminescence in a non-emissive silver-incorporated polyoxoniobate1Light-induced access to a fluorescent Cd7Ag21 nanocluster from a halide-supported Cd8X nanocluster directed by a face-capping macrocyclic metalloligand2Synthesis, characterization and evaluation of the photochemical properties and photothermal conversion capacities of Mo2CTx-MXene@Fuc nanohybrids8From intermediate capture to functional cluster construction: Synthesis of silver clusters and their Br − /I − sensing applications6Near-Infrared Phosphorescent Silver Nanoclusters/Polyethylenimine Nanocomposites for Photothermal Conversion11pH‐Dependent Switching Between Nonlinear‐Optical‐Active Nitrate‐Based Supramolecular Polymorphs27pH‐Dependent Switching Between Nonlinear‐Optical‐Active Nitrate‐Based Supramolecular Polymorphs2Visible-light-mediated oxidation of saturated C(sp3)-H bonds over [W10O32]4−-POMOFs6Maneuvering the Electronic State and Active Site of Assembled-Gold Nanoclusters through Polyoxometalate Implantation for Heterogeneous Green-Light Photocatalysis13Two- and Three-Dimensional Silver Cluster Assemblies: Effect of Argentophilic Interactions in Photoluminescence8Unprecedented stacking-dependent piezoluminescence enhancement in atomically precise superatomic gold nanoclusters11An Atomically Precise Alkynyl‐Functionalized Silver–Polyoxotungstate Nanocluster with Sandwiched Three‐Layer {Ag 13 } 13+ Cluster Architecture and Enhanced Antitumor Activity7An Atomically Precise Alkynyl‐Functionalized Silver–Polyoxotungstate Nanocluster with Sandwiched Three‐Layer {Ag 13 } 13+ Cluster Architecture and Enhanced Antitumor Activity0Controllable syntheses of {SbW9O33}-sandwiched silver clusters induced by external phosphine ligands towards 4-nitrophenol reduction11pH induced crystallization of aminopyridinium templated Strandberg-type cluster: Synthesis-structure-property correlation3Supramolecular Confinement of Cyclodextrin‐Like Host–Guest Polyoxovanadate in Giant Ag 0/I Nanoclusters7Cosmic Blueprint to Nanoscale Design: Hoag’s Object-Like Polyoxovanadate Encapsulated by a Hierarchical Silver Nanocluster16Solvent-triggered reversible transformation of 2D supramolecular polymorphic silver cluster assembled materials for tailoring photoluminescence and photothermal conversion effect1Achieving Dual RTP/TADF Emission in a Bromine-Free 3D Ag(I) Coordination Polymer for High-Efficiency Exciton Utilization00D organic–inorganic hybrid chloroantimonate with thermochromic luminescence for optical temperature detection and anticounterfeiting0Reversible interconversion in atomically precise metal nanoclusters1A bowl-to-bowl programmable hierarchical self-assembly into multidimensional superstructures1A silver alkynyl cluster templated by a dumbbell-shaped selenotungstate1A Single Alkyne‐Induced Core Isomerism in AuCu Clusters and Its Impact on Electronic Structure and Photothermal Response2A Single Alkyne‐Induced Core Isomerism in AuCu Clusters and Its Impact on Electronic Structure and Photothermal Response1Dual-ligand modulated Lego-like supracluster assembly of Ti-In-oxo clusters and Ag-P clusters for optical limiting applications0Surface triphenylphosphine ligands tuning photoluminescence and photothermal properties of two CuI36 clusters1Solvent‐Induced Reverse‐Ostwald Ripening: Structure Conversion from Ag 56 to Ag 45 Clusters and Its Impact on Catalytic Reduction of 4‐Nitrophenol1Biomimetic Gradient‐Porous Carbon Enables Sustainable High‐Loading Lithium–Sulfur Batteries by Regulating Polysulfide Chemistry0Biomimetic Gradient‐Porous Carbon Enables Sustainable High‐Loading Lithium–Sulfur Batteries by Regulating Polysulfide Chemistry11Solvent-induced synthesis of structurally new {PW9O34}-sandwiched silver alkynyl interclusters0Synergistic Regulation of Excited‐State Electrons Enables Sunlight‐Driven C─Br Bond Activation Through In Situ Polymerized Polyoxometalate‐Gold Nanocluster Assemblies0Atomic-level regulation of POMOF homologous isomer for photocatalytic C-H bond oxidation0Design and Control of Supramolecular Structure in Crown Ether–Manganese Thiocyanate Complexes Tuned by Aliphatic Diamine Alkyl Chains: Parity-Dependent Modulation of Dielectric and Electrochemical Properties0Anion-Directed Assembly of Atomically Precise Silver Nanofibers: Tunable Inner Diameters and Mechanical Exfoliation into Subnanometer Nanofibers1Polyoxometalate-templated assembly of homo- and heterometallic silver clusters0Triple-core copper(II) chain-constructed W10-MOFs for efficient photocatalytic activation of benzyl C–H bonds0On‐Stage and Behind‐the‐Scenes: Solvent‐Directed Structural Transformation and Optical Properties of Metal Clusters0Precise single-atom modification of lacunary germanotungstate-encapsulated silver clusters0

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  48. Synthesis, characterization and evaluation of the photochemical properties and photothermal conversion capacities of Mo2CTx-MXene@Fuc nanohybrids

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  49. From intermediate capture to functional cluster construction: Synthesis of silver clusters and their Br − /I − sensing applications

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  50. Near-Infrared Phosphorescent Silver Nanoclusters/Polyethylenimine Nanocomposites for Photothermal Conversion

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