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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Application of Hard and Soft Acid‐base Theory to Construct Heterometallic Materials with Metal‐oxo Clusters

Xiao Qi, YuLong Xie, Jingyang Niu, Junwei Zhao, Ya‐Min Li, Wei‐Hui Fang, Jian Zhang

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Application of Hard and Soft Acid‐base Theory to Construct Heterometallic Materials with Metal‐oxo ClustersOriginalPerylene tetracarboxylate dye-based colorimetric and fluorometric sensor for ppb-level fluoride detection in water1A Stable Polyoxovanadate‐based Metal−organic Framework Containing Dual Catalytic Sites for Efficient Synthesis of p– benzoquinones11Uniform phosphazene containing porous organic polymer microspheres for highly efficient and selective silver recovery8In Situ Reaction Forms Uniform Mixed Heterometallic LnIII2MnII4 (Ln = DyIII and GdIII) Clusters: Assembly Mechanism and Insights into Performance2Controlled encapsulation of metal aggregates in metal–organic framework architectures2Scalable and facile fabrication of magnetic triazine polyimide for high-efficiency gold recovery from e-waste5Synergistic Enhancement Effects of Heterogeneous Isomorphism Clusters in Response to Irradiation: Sub-10 nm Nanolithography and Nanoscale Etching Transfer19Molecular Platform of Isoskeletal {M 2 II Ln 4 III } Clusters for the Study of the M II (M = Cu, Zn) Effect on the Magnetic Properties3Structure‐Property Relationship of Heterometallic Coordination Systems Based on Lanthanides/Pincer Ligands1High-efficiency and selective lead capture using thermally regenerable MOF-based adsorbent: Role of thermoresponsive polymer14A pH-Responsive Liquid Crystal-Based Sensing Platform for the Detection of Biothiols2A “Signal Relay” Mode Triggered by Bimetallic Synergistic Enhancement in an MOF-Based Multiemission Fluorescence Sensing/Adsorption Platform for Broad-Concentration-Range Tetracycline Antibiotics Visual Detection35Construction of metal cluster-based materials directed by a bifunctional pyridyl tripodal alcohol ligand according to hard and soft acid-base theory1Robust amide covalent organic framework aerogel for selective recovery of gold from e-waste16Inherent relationships in thiourea derivatives: effects of phenyl substitution position and linear alkyl chain length3Regulating mechanism of thiourea additives via N-alkylation and carbon branch chain content2High‐Nuclear Metal–Oxide Cluster Porous Interlayers Enabling Tailored Carrier Transport and Ion‐Exchange Lead Leakage Prevention in Perovskite Solar Cells2Synthesis and Characterization of Bisphosphonate-Functionalized Gadolinium Oxide Nanoparticles as Nonionizing Contrast Agents to Detect Bone Turnover0A cysteamine-modified photonic crystal hydrogel sensor for visual detection of Hg 2+ ions0Mechanistic insights into phosphate-promoted simultaneous adsorption and spatially stratified distribution of Pb(II) and Cu(II) on chitosan goethite bionanocomposite adsorbents5From statistical mixtures to structural insights: characterisation of heterometallic [M 4 L 6 ] 8+ coordination cages using high resolution ion mobility mass spectrometry0Precise Tailoring of the Coordination Environment of Single‐Atom Cu(I) on Trifurcate AlL 3 Supports for Click Chemistry0Removal of Hf(IV) Ions from Zr(IV) Ions in Sulfuric Acid Solution by Solvent Extraction with PC88A0Piezoelectric catalysis for selective recovery of precious metals (Cu and Au) from waste CPUs22Rare 3D Heterometallic–Organic Frameworks Built from [M 6 ] (M = Zr, Hf) and [Cu 2 I 2 ] Clusters for Iodine Vapor Capture3Unlocking internal aluminum reactivity in nanohydrated alumina via amyloid fibril nanoconfinement for highly efficient water defluorination2Dual-Pore Dodecanuclear Al-Oxo Cluster-Based Bimetallic Isonicotinate Frameworks for Selective Propylene/Ethylene Separation5Ultra-high adsorptive removal of dyeing wastewater by salt-tolerant MOGs via green fabrication strategy and mechanism investigations1Synergistic adsorption of ammonia and cadmium on oxychar for sustainable remediation of water and soil1Metal-organic frameworks for sustainable water management: rational design, sorption mechanisms, and emerging applications11Frontiers of advanced multifunctional liquid metal − wood composite materials7Stabilizing Silver Single‐Atom Site via A Pore‐Confined Triphenylphosphine for CO 2 Conversion With High Substrate‐Specificity3“Two-in-one” luminescent MOFs/sodium alginate aerogel beads for sensitive detection of Al3+ and efficient enrichment of Pb2+ in water4An Oxo-Bridged Trinuclear Nickel(II) Cluster Supported by 1,3,4-Thiadiazole-2,5-Diamine: Crystal Structure, Multitechnique Characterization and Antimicrobial Activity5Structure design of magnetic bamboo-based biochar for ultrafast thallium adsorption from complex wastewater and mechanistic analysis2Unraveling the role of coordination stability in selective separation of rare earth elements from aluminum using dicarboxylates0Threading an Aluminum Molecular Ring Onto a Chemically Growing Copper‐Directed Polyrotaxane1A dual zinc-complexation nanozyme performs synergistic chemodynamic-immunotherapy along with additional immunosuppressive microenvironment remodeling and immune evasion inhibition for efficient breast cancer treatment1Formation Mechanism and Enhanced Iodine Capture of Copper-Based Aluminum-Oxo Cluster Bimetallic Organic Frameworks1Giant Enlarged Circular Metallo-Rings0High-Toughness and Antibacterial Hydrogels via Gelatin and Zr 4+ Synergy for Flexible Motion-Monitoring Sensors2Topological Control of Dual Protonic–Electronic Conduction in Metal–Organic Frameworks0Anomalous permeation selectivity of IA and IIA ions in metal organic frameworks controlled by the horizontal cation-edge interaction0Engineering ferritin nanocages for Cd2 + adsorption with magnetic recyclability0Solvent‐Free “ Weaving ” Synthesis of MOF From Waste Plastics for Record‐Efficiency Evaporation Energy Harvesting1Pulsed laser-induced morphological reconstruction and surface oxidation modulation of colloidal MoS₂ for enhanced dye adsorption0Heterometal-driven symmetry breaking in metal-oxo clusters for highly nonlinear optical application0Tuning diffusion modes in micropore reactors enables efficient gas-liquid transport for CO2 electroreduction0Automatisierte, rotationsunterstützte Schicht‐für‐Schicht‐Epitaxie zur Herstellung hochorientierter MOF‐Dünnschichten mit gemischten Linkern0Adsorptive hydrogels for broad-spectrum heavy metal remediation: From coordinated performance optimization to application-oriented design0PCN‐700: A Model Platform for Crystallographic Probing of Coordination Behavior in Metal–Organic Frameworks0

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