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RESEARCH PAPER · Chemical Reviews · 2023

Photoreforming of Waste Polymers for Sustainable Hydrogen Fuel and Chemicals Feedstock: Waste to Energy

Muhammad Ashraf, Nisar Ullah, Ibrahim Khan, Wolfgang Tremel, Shahzada Ahmad, Muhammad Nawaz Tahir

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Photoreforming of Waste Polymers for Sustainable Hydrogen Fuel and Chemicals Feedstock: Waste to EnergyOriginalEfficient photodegradation of methyl red dye by kaolin clay supported zinc oxide nanoparticles with their antibacterial and antioxidant activities42Shape‐Controlled First‐Row Transition Metal Vanadates for Electrochemical and Photoelectrochemical Water Splitting22Continuous flow synthesis of Ag-PEDOT-COF nanocomposite for sustainable photoreforming of plastic waste and chromium remediation in visible light29Improving catalytic performance and reusability of flower-like Co-B-P amorphous alloy nanobelts for the selective hydrogenation of furfural in water5Robust electrocatalysts decorated three-dimensional laser-induced graphene for selective alkaline OER and HER58Bandgap Engineering of Melon using Highly Reduced Graphene Oxide for Enhanced Photoelectrochemical Hydrogen Evolution33Boosting Electro- and Photo-Catalytic Activities in Atomically Thin Nanomaterials by Heterointerface Engineering3Organic/inorganic metal halide perovskites for solar-driven water splitting: properties, mechanism, and design26C–H Azidation System Induced by Visible Light from Triboelectric Nanogenerators Based on a Cadmium Coordination Polymer19Constructing fast charge separation of ZnIn2S4 @CuCo2S4 p-n heterojunction for efficient photocatalytic hydrogen energy recovery from quinolone antibiotic wastewater172Photoredox Cascade Catalyst for Efficient Hydrogen Production with Biomass Photoreforming24Photoredox Cascade Catalyst for Efficient Hydrogen Production with Biomass Photoreforming3From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100In-situ synthesized oxygen vacancy filled ZnS/Vo-ZnO heterojunction photocatalysts for efficient H2 production23Carbon nitride (C3N3) decorated with non-noble metal Ni2P Co-catalyst based nanocomposites for photocatalytic water splitting13Magnetism-driven iron oxide nanocomposites for energy and environmental solutions: harnessing magnetism11Continuous flow synthesis of visible light-active conjugated porous polymer for pollutant degradation and plastic waste photoreforming13Simultaneous hydrogen production and conversion of plastic wastes into valued chemicals over a Z-scheme photocatalyst40The defective C3N monolayers as high-efficient hydrogen purification membranes: DFT calculations and MD simulations26Photoreduction of Aqueous Protons Coupling with Alcohol Oxidation on a S‐Scheme Heterojunction Photocatalyst MnO/Carbon Nitride40Hydrogen production and value-added chemical recovery from the photo-reforming process using waste plastics23Progress in recovery, recycling and reuse of polymers, biopolymers and their composites12D semiconductor nanosheets for solar photocatalysis119ZIF-67-derived hollow CoS and Mn0·2Cd0·8S to form a type-II heterojunction for boosting photocatalytic hydrogen evolution19Z-Scheme heterojunction WO3/ZnIn2S4 solar absorber for wastewater remediation22Advanced strategies in electrode engineering and nanomaterial modifications for supercapacitor performance enhancement: A comprehensive review317Recent advancement on photocatalytic plastic upcycling90Electrochemical synergy and future prospects: Advancements and challenges in MXene and MOFs composites for hybrid supercapacitors74Biodegradable polymer nanocomposites as packaging materials: A review0Boosting pollutant degradation with simultaneous H 2 O 2 production from its electron delocalization and excitation co-triggered by microelectric field and visible light1Cu-P@silica-CNT-based catalyst for effective electrolytic water splitting in an alkaline medium with hydrazine assistance5Heterostructured electrocatalysts for the oxygen evolution reaction118Hydrogen storage in a sandwich structure by assembly of BNs and MOFs7Recent progress on the photocatalytic hydrogen evolution reaction over a metal sulfide cocatalyst-mediated carbon nitride system26Solar-driven photoelectrochemical conversion of biomass: recent progress, mechanistic insights and potential scalability88The mechanism of water oxidation using transition metal-based heterogeneous electrocatalysts235Recyclable, Reprocessable, Anticorrosive, and Hydrolysis-Resistant Long-Chain Aliphatic Polycarbonates as Polyethylene-like Materials15Atomic interfacial charge and energy transfer paths at MoS2/Pd bonded defect-rich BiOCl interfaces for efficient photocatalysis37H2 production by solar photoreforming of plastic materials using SiC-g-C3N4composites30Photocatalytic biomass conversion for hydrogen and renewable carbon-based chemicals110Recent advances in bismuth oxyfluoride-based photocatalysts for energy and environmental remediation22Pyrolysis of waste oils for biofuel production: An economic and life cycle assessment79Tandem Chemical Depolymerization and Photoreforming of Waste PET Plastic to High-Value-Added Chemicals148Critical upstream technologies for hydrogen energy industry: Research progress on ammonia decomposition catalysts42Photoelectron Migration Boosted by Hollow Double‐Shell Dyads Based on Covalent Organic Frameworks for Highly Efficient Photocatalytic Hydrogen Generation6Photoelectron Migration Boosted by Hollow Double‐Shell Dyads Based on Covalent Organic Frameworks for Highly Efficient Photocatalytic Hydrogen Generation70Unlocking the Potential of High Entropy Alloys in Electrochemical Water Splitting: A Review1212D Ge 2 Se 2 P 4 Monolayer: A Versatile Photocatalyst for Sustainable Water Splitting15Highly dispersed palladium nanoparticles decorated on nitrogen doped graphene for enhanced photoelectrochemical water splitting5Catalyst design and structure control for photocatalytic refineries of cellulosic biomass to fuels and chemicals41Synergistic Approaches for Enhanced Light-Driven Hydrogen Production: A Membrane-Anchoring Protein-Engineered Biohybrid System with Dual Photosensitizers Strategy25Photoreforming for microplastics recycling: A critical review26Upcycling of Plastic Waste Using Photo-, Electro-, and Photoelectrocatalytic Approaches: A Way toward Circular Economy159Light-driven polymer recycling to monomers and small molecules112Band Energy Modulation in an Fe–Mn–ZnO Nanowire–Nanosheet Catalyst for Efficient Overall Water Splitting12Brookite TiO2 as an active photocatalyst for photoconversion of plastic wastes to acetic acid and simultaneous hydrogen production: Comparison with anatase and rutile53Waste-to-Energy: potencialidades e contextualização da sua aplicação no Brasil1Design of CdS/Covalent Organic Framework as an efficient heterojunction photocatalyst for enhanced photocatalytic H2 evolution3Electron-Rich Ru Supported on N-Doped Coffee Biochar for Selective Reductive Amination of Furfural to Furfurylamine12Emerging Photoreforming Process to Hydrogen Production: A Future Energy106Sustainable hydrogen production: Solar-powered biomass conversion explored through (Photo)electrochemical advancements55Biomass to green surfactants: Microwave-assisted transglycosylation of wheat bran for alkyl glycosides production14Selective Photoreforming of Waste Plastics into Diesel Olefins via Single Reactive Oxygen Species51Selective Photoreforming of Waste Plastics into Diesel Olefins via Single Reactive Oxygen Species8Economics and Applications of Dimethyl Ether from Dehydration of Methanol0Solar‐Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges66Synergy of oxygen doping and nitrogen vacancy for promoting photocatalytic hydrogen generation of g-C3N420An Overview of the Sustainable Depolymerization/Degradation of Polypropylene Microplastics by Advanced Oxidation Technologies33Rational Design of Photoanodes to Produce Value‐Added Chemicals Coupled with Hydrogen10Selective Cleavage of C β −O−4 Bond for Lignin Depolymerization via Paired‐Electrolysis in an Undivided Cell2Selective Cleavage of C β −O−4 Bond for Lignin Depolymerization via Paired‐Electrolysis in an Undivided Cell23NiSe2 nanoparticles modified ZnIn2S4 microspheres for boosting photocatalytic hydrogen evolution under visible light irradiation3Human inventions and its environmental challenges, especially artificial intelligence: New challenges require new thinking44Anchoring NiSx (x=0, 1, 2) on porous g-C3N4 (PCN) to enhance photocatalytic H2 production: The effect of S element on H2 evolution7Photoredox Cascade Catalysts for Solar Hydrogen Production From Sustainable Hydrogen Sources3Advancing Recyclable Thermosets through C═C/C═N Dynamic Covalent Metathesis Chemistry36Trimetallic alloy nanoparticles as cocatalyst for improving the photocatalytic performance of graphitic carbon nitride for H2 production9Enhanced Charge Transfer Dynamics in a NiCo 2 S 4 –Zn x Cd 1– x S Photothermal Catalyst for Efficient Photoreforming of Waste Plastic50Fabrication of nickel oxide decorated CNTs/GO nanohybrid: A multifunctional electrocatalyst for overall electrochemical water splitting7Effect of strain engineering on the highly controllable H2 purification performance of graphenylene-like boron nitride membranes: DFT calculations and MD simulations7Regulation charge spatial separation within necklace-like CdS/UiO-66 nanowires for selective photocatalytic oxidation of lignin6Trends and challenges in hydrogen production for a sustainable energy future293D Printing Modulated Polyvinylidene Fluoride Arrays for Enhanced Output of Piezoelectric Energy Harvesters17In Situ Electrochemical Conversion of Biomass-Derived 5‑Hydroxymethylfurfural into 2,5-Furandicarboxylic Acid by Time-Controlled Aerosol-Assisted Chemical Vapor Deposited FeNi Catalyst8Can hydrogen be generated by UV- photodegradation of biomass residues in water media?4Beyond Water Splitting: Developing Economic Friendly Photoelectrochemical Value-added Reactions for Green Solar-to-Chemical Energy Conversions2A review on progress and prospects of diatomaceous earth as a bio-template material for electrochemical energy storage: synthesis, characterization, and applications28Ultramicroporous carbon molecular sieve membrane derived from hyper-crosslinked ionic polymers for efficient H2/CO2 separation9Status and Enhancement Techniques of Plastic Waste Degradation in the Environment: A Review21Circular Economy and Chemical Conversion for Polyester Wastes23Current Advances in the Photoconversion of Plastics: the Catalysts and Reaction Pathways7Isoreticular Squaraine‐Linked Titanium‐Organic Frameworks for Photocatalytic Water Splitting to Hydrogen Under Visible Light5Photoreforming: A Sustainable Pathway for Plastic Waste to Fuel Conversion1Roles and implications of hydrogen economy in Industry 4.0: Perspectives from the nexus of waste-energy-food0Shining Light on the Future: Photoreforming (PR) as a Solution to Plastic Trash: A Brief Review2Building Mo2C/C/TCN heterojunction for efficient noble-metal-free plastic photoreforming and hydrogen generation20Plastic‐to‐Treasure: Innovative advances in photo/electro‐catalytic upcycling technologies for commodity chemicals and fuels15Mineralizing Biofilm towards Sustainable Conversion of Plastic Wastes to Hydrogen5Mineralizing Biofilm towards Sustainable Conversion of Plastic Wastes to Hydrogen5Advancing gel polymer electrolytes for next-generation high-performance solid-state supercapacitors: A comprehensive review63Cascade degradation and electrocatalytic upcycling of waste poly(ethylene terephthalate) to valued products12Photoreforming of Plastic Waste to Sustainable Fuels and Chemicals: Waste to Energy59Sustainable H2 Production from Lignocellulosic Biomass over MoS2 Modified Sulfur Vacancy Enriched ZnIn2S4 Photocatalyst62Photoreforming of plastic waste into valuable products and hydrogen using a high-entropy oxynitride with distorted atomic-scale structure68Hydroxyl Spillover in Fe–Se Dual-Site Catalysts for Mixed Plastics Assay28Solvothermal synthesis of carbon nitride (g-C 3 N 4 ): bandgap engineering for improved photocatalytic performance12Surface Coverage Tuning for Suppressing Over‐Oxidation: A Case of Photoelectrochemical Alcohol‐to‐Aldehyde/Ketone Conversion17Surface Coverage Tuning for Suppressing Over‐Oxidation: A Case of Photoelectrochemical Alcohol‐to‐Aldehyde/Ketone Conversion1Activation Mechanism of the H 2 on Au 6 ‐based Clusters From the Perspective of Chemical Bonding0BiVO 4 /MoS 2 n–n heterojunction for enhanced solar-driven seawater antibiotic degradation and photocatalytic hydrogen evolution6Economical 550 V energy harvesting from plastic and electronic waste using human motions9Electroless-deposited NiFeP catalyst-coated-membrane cathodes for anion exchange membrane water electrolysis12Microbiological Technology to Extract Bioactive Molecules from Agricultural and Industrial Waste0Photocatalytic dissolution of cellulose for hydrogen and nanofiber production: unveiling crucial factors via experiments and informatics4Photocatalytic water splitting for hydrogen generation0Photoelectrochemical valorisation of organic waste for the cogeneration of solar fuels and value-added chemicals17Plastic photoreforming: catalytic production of hydrogen and valuable chemicals15Porous Nanostructured Cationic Conjugated Polyelectrolyte/Titanium Dioxide Nanosheets Heterojunction for Co-Catalyst-Free Photocatalytic Hydrogen Production0Practice and tactics in the construction of novel degradable plastics at polymer and molecular levels1Solar driven conversion of agricultural biomass to H 2 over few-layer MoS 2 modified ultra-small TiO 2 nanoparticle photocatalysts15State-of-the-art and perspectives of hydrogen generation from waste plastics80Sustainable thermochemical plastic valorization towards a circular economy: a critical review27Green synthesis of activated carbon from biomass waste of date palm seeds: A sustainable solution for energy storage and environmental impact39A multifunctional strategy: Lithium recovery and chlorine fixation via co-pyrolysis of spent lithium-ion batteries and chlorinated waste plastics15In situ construction of metal phosphide-anchored Zn0.5Cd0.5S Schottky junction photocatalysts for efficient hydrogen evolution via photocatalytic reforming of plastics29Photoreforming of waste plastic by B‐doped carbon nitride nanotube: Atomic‐level modulation and mechanism insights44Recycling homocarbon backbone polymers toward a circular materials economy12Biomass-derived carbon for solar H2O2 production: Current trends and future directions6H2 production from photocatalytic reforming of PET over Pt/TiO2: The role of terephthalic acid8Construction of hollow TiO2/black phosphorus quantum dots (BPQDs) with cavity reflection associated oriented electron transfer effects for enhanced photocatalytic efficiency7Enhanced hydrogen and 5-hydroxymethylfurfural (5-HMF) production via photoreforming of cotton cellulose: role of cellulose allomorphs in Pt–g-C3N4–Bi3TiNbO9 catalysis0Unlocking the potential of quinoline-based glycopolymers for photoreforming hydrogen production8Highly efficient H 2 separation and purification performance of C 7 N 6 membranes with strain modulation: DFT calculations and MD simulations4Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design Principles73Effects of operating parameters and fluids on the performance of a hydrogen regenerative flow compressor in a proton exchange membrane fuel cell system4Role of synthetically modulated polymers for efficient photoreforming hydrogen fuel1Simultaneously Tailoring Hydrostability and Photoelectroactivity in Heterocluster Metal–Organic Frameworks for Efficient Photocatalytic Hydrogen Production39Mesoporous Single-Crystalline Particles as Robust and Efficient Acidic Oxygen Evolution Catalysts90Comprehensive Insights into Photoreforming of Waste Plastics for Hydrogen Production1Asymmetric Atomic Pt–B Dual-Site Catalyst for Efficient Photoreforming of Waste Polylactic Acid Plastics in Seawater56Catalysts Design and Atomistic Reaction Modulation by Atomic Layer Deposition for Energy Conversion and Storage Applications35Engineering MIL-53(Al) MOF with Carbon Dots for Synergistic Photocatalysis Applications in Organic Dye Degradation7Photocatalytic Upcycling of Plastic Waste Into Value‐Added Chemicals21Comprehensive Insights into Photoreforming of Waste Plastics for Hydrogen Production19S-Scheme Homojunction Carbon Nitride for Photocatalytic Overall Water Splitting114Optimize molecular engineering of high-crystal PTI/PHI homojunctions for enhanced photoreforming of Poly(ethylene terephthalate) plastics into high-value chemicals5Biomass-to-biohydrogen conversion: Comprehensive analysis of processes, environmental, and economic implications16State-of-the-Art Achievements and Challenges in Photochemical Conversion of Plastics to Chemicals and Composites6Photocatalytic Hydrogen Evolution Driven by Advanced Metal Sulfides from Sustainable Multilevel Biomass and Waste Plastics51Improved Solar‐Powered Water‐Splitting Performance of Bi 4 Ti 3 O 12 /TiO 2 Composite with Synergistically Interacted Heterointerfaces Under Platinum Cocatalysis7

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