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RESEARCH PAPER · Chemistry of Materials · 2023

Regulating Eu 2+ Multisite Occupation through Structural Disorder toward Broadband Near-Infrared Emission

Yingze Zhu, Xuesong Wang, Jianwei Qiao, Мaxim S. Моlokeev, Hendrik Christoffel Swart, Lixin Ning, Zhiguo Xia

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Regulating Eu 2+ Multisite Occupation through Structural Disorder toward Broadband Near-Infrared EmissionOriginalA highly thermally stable Y 3 AlGa 4 O 12 :Cr 3+ phosphor for near-infrared pc-LEDs10Color-tunable emissions realized by Tb 3+ to Eu 3+ energy transfer in ZnGdB 5 O 10 under near-UV excitation9Recent Advances in Multi-Site Luminescent Materials: Design, Identification and Regulation20Unraveling Luminescent Energy Transfer Pathways: Futuristic Approach of Miniature Shortwave Infrared Light-Emitting Diode Design66Developing Broadband Cr3+-Substituted Phosphor-Converted Near-Infrared Light Sources38Research progress of rare earth/transition metal ions doped NIR luminescent materials68-Phenylquinoline-Based Tetradentate 6/6/6 Platinum(II) Complexes for Near-Infrared Emitters11Synthesis, spectral characteristics and energy transfer of SrLa2Al2O7:Mn4+, Dy3+31Multiple local site Cr3+emission leading to broadband NIR light in novel SrGa2O4 phosphors30Mechanoluminescence and afterglow modulation of Zr and Mg doped strontium aluminate3Temperature and Pressure Sensing Using an Optical Platform Based on Upconversion Luminescence in NaSrY(MoO4)3 Codoped with Er3+ and Yb3+ Nanophosphors46Improved thermal stability and quantum efficiency of novel cyan phosphors toward full-visible-spectrum lighting15Tunable luminescence spectra of solid solution phosphors Gd3(Sb1-Ta )O7:Bi3+ for ultrahigh color rendering index full-spectrum white light-emitting diodes21SrHfO3:Cr3+ Perovskite Microcubes for Rare-Earth-Free NIR-I Light Emission11Crystal Field Engineering Yields New 3D Layered Solid Solution Phosphors (Ca/Sr)4MgAl2Si3O14:Eu2+ for White-Light-Emitting Diode Full-Spectrum Lighting17Broadband emitting Fe 3+ ‐doped double perovskite‐type antimonates phosphors for NIR spectroscopy applications28Site occupation, emission color tuning and white LED application of Ce3+-activated chloroborate Ca2BO3Cl4Abnormal spectral broadening of ordered-structure near-infrared phosphor La 2 CaHfO 6 :Cr 3+15Achieving a Eu 2+ -doped NIR phosphor via ionic modulation and its multifunctional applications4Development of a novel Eu 2+ activated oxonitridosilicate cyan phosphor for enhancing the color quality of a violet-chip-based white LED9High thermal stability and quantum efficiency of (Sr,Ba)2Ga2SiO7: Eu2+ phosphors for full-spectrum WLEDs17Ions Co-Substitution Strategy Toward Tunable Broadband Near-Infrared Luminescence from Cr3+ Doped Gallium Oxide Based Phosphors0Research progress on Fe 3+ -activated near-infrared phosphor18Tunable broadband near-infrared luminescence from Cr 3+ -doped gallium oxide-based phosphors for advanced sensing and LED applications12Tunable luminescence via Cr 3+ –Yb 3+ /Nd 3+ energy transfer in Cr 3+ and Yb 3+ /Nd 3+ coactivated NIR phosphors for non-destructive analysis22Thermally Stable NIR Emission from Disordered Ba5La3MgAl3O15:Cr3+ with Peak Wavelength Beyond 900 nm36Highlights from 2023 and Chemistry of Materials’ 35th Year0Energy transfer between two luminous centers and tunable emission of La7Nb3W4O30:Dy3+, Eu3+50Key Role of Metal-to-Metal Charge Transfer Transition between Mo6+ and Bi3+ for Enhancement in NIR Luminescence of Gd2MoO6:Bi,Yb Nanophosphor9Sharp-to-Broad Band Energy Transfer in Lithium Aluminate and Gallate Phosphors for SWIR LED5Highly efficient broadband near-infrared luminescence phosphors Ca3MgSn0.5Zr0.5Ge3O12:Pr3+,Cr3+ for multifunctional applications in pc-LEDs field19Luminescence of iron ions in crystals: Site occupancy, valence states, and excited-state properties14Evidence and Practical Applications of Site Occupancy Theory (SOT) of Eu3+ in Scheelite Compounds6An energy transfer strategy towards versatile sensing applications from Cr3+ and Yb3+ codoped near infrared phosphors4Strategy to optimize the broadband near-infrared emission based on Eu2+-doped sulfureted garnet phosphors toward emerging spectroscopy applications28Wide Range Near‐Zero Thermal Quenching of Orange–Yellow Phosphor via Impeding Self‐Oxidation of Eu 2+ for Versatile Optoelectronic Applications20Efficient Broadband Near‐Infrared Emitters in Lead‐Free Metal Halides with Record Photoluminescence Quantum Yield Under Blue Light Excitation39Study on the properties of Sm3+-Doped CaTbAl3O7 phosphors39Absolutely Structural Disorder Boosting Bandwidth toward Full‐Spectrum White Light from Single Occupancy of Activator36Ce3+,Cr3+ co-doped garnet phosphors with yellow and near-infrared emission for white and near-IR dual-mode pc-LEDs16Customized Cyan Phosphors for Efficient Full‐Spectrum Illumination and Fingerprint Detection22Enhancement strategy of thermal stability and photoluminescent intensity of Cr3+ doped Li3+xZn2–2xGaxSbO6 phosphor in a strong crystal field12Low‐Coordination Crystallographic Lattice Engineering to Discover Ce 3+ ‐Activated Ultra‐Wide Visible‐to‐Near‐Infrared Luminescent Materials9Synthesis and spectroscopic analysis of NaCaYF6:Nd3+, Yb3+NIR emitting phosphor26Tailoring of Spectral Behaviors in Ce3+-Activated Ba2Gd8(SiO4)6O2 Cyan-Emitting Phosphors via Site Substitution Engineering for Plant Growth and Full-Spectrum White Light-Emitting Diodes14Prediction and explanation of the self-reduction of Eu3+ → Eu2+ and Mn4+ → Mn2+ using Site Occupancy Theory (SOT)6Recent progress of inorganic phosphors in artificial plant cultivation LEDs46Cr 3+ –Cr 3+ pairing and multi-site engineering in Sr 2 ZnAl 22 O 36 phosphors for broadband near-infrared emissions14Full Red-Band Emitting of Bamgp2o7: Xmn2+ Phosphor for Plant-Growth Illumination0Near-infrared luminescent materials: a review of their practical applications and prospective advancements47Tunable broadband visible emission achieved by phase transformation-driven self-reduction of Eu 3+ to Eu 2+ in a calcium phosphate matrix6Site occupation engineering induced red-shifted luminescence in (Ca, Sr)Sc2O4:Eu2+ phosphor20Lead-free cesium europium bromide perovskite nanocrystals in glass for white light-emitting diode and X-ray imaging16A strategy to obtain highly luminescent MOF-76 based on hydrothermal annealing treatment8Highly Efficient and Thermally Stable NIR‐Emitting Phosphor with Largely Tunable Peak Wavelength and Bandwidth Toward NIR Spectroscopy Applications47Neighboring‐Cation Substitution Engineering Strategy toward High Performance in Near‐Infrared Light Source for Multifunctional Applications13Simultaneously enhanced shortwave infrared emission and thermal stability enabled by efficient resonance energy transfer in Ca3ScHfAlSi2O12: Cr3+, Yb3+ towards emerging spectroscopy applications3Tunable photoluminescence in Eu2+-activated KCaLa(PO4)2 phosphor through structural disorder3Cationic Substitution-Enabled Green-Emitting Gd 2– y Y y LuAl 4 GaO 12 : Ce 3+ Garnet Phosphors with High Quantum Efficiency and Superior Thermal Stability for Advanced WLEDs12Efficient and broadband near-infrared emitting Ca2YHf2Ga3O12: Cr3+ phosphor for anti-counterfeiting applications8Crystallographic site engineering enables long-wavelength broadband near-infrared emission in Ni2+-activated Sr2MNbO6 (M = Ga and Sc) phosphors with improved thermal stability3β-Ca3(PO4)2-type Eu2+-doped Phosphor: Applications in optical thermometry and full-spectrum lighting5Wavelength-Tunable of Broad Red to Near-Infrared Emission in (Sr,Ba)3Sc4O9 :Eu2+ Phosphors: Crystal Field Effects and Thermal Stability6A review of recent advances in Ce3+-activated garnet phosphors for blue-chip-pumped pc-WLEDs81Synthesis and applications of Eu3+, Na+-doped high-color-purity BaSrGa4O8 red phosphors for w-LEDs and the detection of latent fingerprints11Tunable NIR emission in Cr3+ activated (La,Gd)Sc3(BO3)4 based on host crystal engineering strategy6Synthesis, spectral, and thermal properties of K2CaP2O7:Sm3+ phosphors to fill the amber gap in LED applications10Red-emitting Ca3Bi(PO4)3:Eu3+ phosphors excitable by near-UV light with excellent optical properties for white LED applications0Structure and luminescence of Gd3Ga3MgSiO12:Cr3+ garnet phosphor with highly efficient broadband near-infrared emitting toward pc-LED application7Orange-red emitting of Sm3+-doped Ba3Ga2Ge4O14 phosphor with high color rendering index and high color purity for LED applications4Leveraging heavy rare earth elements (H-REEs) in electrodes to boost the efficiency of photoelectrochemical and electrochemical water splitting5Synergistic optimization of luminescence in feldspar-structured blue-cyan phosphors via heterovalent K+ substitution coupled with bandgap engineering0Revolutionary near-infrared phosphors with emerging structures and mechanisms driving next-generation applications32Lattice sites of Eu3+/Sm3+ in Ca3(Ga, Al)2Ge3O12 photoluminescence spectra and applications in plant fill light, W-LEDs, and fingerprint detection1Enhanced luminescence performance of near-infrared phosphor Y2CaAl4SiO12: Fe3+, Yb3+ through energy transfer for anti-counterfeiting applications10Improved NIR luminescence in Y3-Sc Ga3MgSiO12:Cr3+ phosphor via cation substitution for multifunctional spectroscopic applications4A novel narrow-band red-emitting phosphor for lighting and backlight display1Garnet‐Structured Near‐Infrared Luminescent Materials: Luminescence Fundamentals, Regulation and Applications14Broadband near-infrared emission improvement of Cr3+ doped phosphors via co-doping Bi3+ ions6Cationic regulation and broadband near-infrared emission properties of Li 1.6 (MgZn) 1.6 Sn 2.8 O 8 :Cr 3+5Tunable Broadband Red-To-Near-Infrared Emission in Eu 2+ -Activated Sr 1– x Ba x La 2 Sc 2 O 7 Phosphors via Site-Selective Occupation and Cation Substitution3Broadband NIR emission from Y2CaGa4GeO12:Cr3+ phosphors via co-substitution engineering for bioimaging and night-vision0Synthesis and luminescent properties of Eu2+-doped sodalite- and bystrite-type aluminosilicates: Implications for europium incorporation in feldspathoids0When the crucible contributes: serendipitous formation, flux reactivity, and crystal and electronic structures of two aluminium-bearing mixed-metal oxides, Ba 2.1 Pb 0.9 Al 8.8 In 2.2 O 20 and BaAl 1.6 Ga 0.4 O 40Garnet-structured Y2CaGa4ZrO12:Cr3+ NIR phosphor with combined high efficiency and thermal stability toward constructing high-performance pc-NIR-LED1Dual-broadband NIR-I and NIR-II emission from Fe3+/Ni2+ Co-doped SrLaMgSbO60Crystal field engineering and energy transfer strategy for enhancing broadband near-infrared luminescence of Sm2+ activated oxynitride phosphors0Multifunctional Ca14Zn6Ga10O35: Bi3+, Sm3+ phosphors for thermometry, WLED and anti-counterfeiting0Revisiting the Spectrum–Crystal Field Relationship of 3d 3 Ion (Mn 4+ /Cr 3+ )‐Activated Phosphors via a Recalibrated Database0Ligand Engineering Controls Near-Infrared Emission, Quantum Efficiency, and Photoluminescence Lifetimes in Dimetallic Ru(II) Complexes0

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  47. Recent progress of inorganic phosphors in artificial plant cultivation LEDs

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  48. Cr 3+ –Cr 3+ pairing and multi-site engineering in Sr 2 ZnAl 22 O 36 phosphors for broadband near-infrared emissions

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  49. Full Red-Band Emitting of Bamgp2o7: Xmn2+ Phosphor for Plant-Growth Illumination

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  50. Near-infrared luminescent materials: a review of their practical applications and prospective advancements

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