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RESEARCH PAPER · Advanced Materials · 2022

Activating C–H Bonds by Tuning Fe Sites and an Interfacial Effect for Enhanced Methanol Oxidation

Sheng Huang, Feng Feng, Rong‐Ting Huang, Ting Ouyang, Jinlong Liu, Zhao‐Qing Liu

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Activating C–H Bonds by Tuning Fe Sites and an Interfacial Effect for Enhanced Methanol OxidationOriginalBoosting the photogenerated charge separation of g-C 3 N 4 by constructing a Ni@Ni 2 P cocatalyst with a core–shell structure4Activating bulk nickel foam for the electrochemical oxidization of ethanol by anchoring MnO 2 @Au nanorods15Facile preparation of a methanol catalyst with ultra-high voltage efficiency and super-durability: Pt pollution introduction by composite electrodeposition9Photocatalytic ability of visible-light-responsive hybrid ZrO 2 particles6Plasmon photocatalytic CO 2 reduction reactions over Au particles on various substrates16Efficient CO2 reduction to formate using a Cu-doped BiVO4 electrocathode in a WO3 photoanode-assisted photoelectrocatalytic system30Enhanced Photocatalytic Hydrogen Evolution and Antibacterial Activities of Ternary Chevrel Phases7Photocatalysis-self-Fenton system over edge covalently modified g-C3N4 with high mineralization of persistent organic pollutants69CdS supported on ZIF-67-derived Co-N-C as efficient nano polyhedron photocatalysts for visible light induced hydrogen production39Coral-like B-doped g-C3N4 with enhanced molecular dipole to boost photocatalysis-self-Fenton removal of persistent organic pollutants124Plasmon-Enhanced Photocatalytic Oxidation of Benzyl Alcohol to Benzaldehyde Using BiVO4/BiOBr/Au Nanosheets22Interface engineering of sandwich SiO2@α-Fe2O3@COF core-shell S-scheme heterojunctions for efficient photocatalytic oxidation of gas-phase H2S37Efficient photocatalytic hydrogen evolution reaction promoted via a synergistic strategy of S-scheme heterojunction structure combined with surface plasmon resonance effect28Vacancy engineered BiVO4 photoanode realizes efficient photoelectrochemical CH3OH oxidation in near-neutral media: Active site regulation improves HCHO selectivity17S-Scheme-Heterojunction LaNiO3/CdLa2S4 Photocatalyst for Solar-Driven CO2-to-CO Conversion31Delafossite-based nitrate treatment for fabricating copper-cerium hybridized interface to achieve enhanced methanol oxidation reaction3Highly Selective Activation of C–H Bond and Inhibition of C–C Bond Cleavage by Tuning Strong Oxidative Pd Sites89Rapid dissociation of high concentration excitons between [Bi2O2]2+ slabs with multifunctional N-Bi-O sites for selective photoconversion into CO115Prussian-blue-analogue derived FeNi2S4/NiS nanoframes supported by N-doped graphene for highly efficient methanol oxidation electrocatalysis31Electrosynthesis of α‐Amino Acids from NO and other NO x species over CoFe alloy‐decorated Self‐standing Carbon Fiber Membranes140Electrosynthesis of α‐Amino Acids from NO and other NO x species over CoFe alloy‐decorated Self‐standing Carbon Fiber Membranes21Multi-strategy for constructing Z-scheme porous hollow double-shell Fe2O3@Ov-NiFe2O4 nanorods-arrays photocathode: Bias-free synthesis of H2O2, Zn-H2O2 cell and generation of NaZnPO421Energy-oriented utilization from organic wastewater: Directional photoelectrocatalytic conversion of phenol to C1 fuels4Organic Upgrading through Photoelectrochemical Reactions: Toward Higher Profits37S-scheme Co3(PO4)2/Twinned-Cd0.5Zn0.5S homo-heterojunction for enhanced photocatalytic H2 evolution82Exposing an Environmentally Friendly Gelation Strategy to Fabricate Modern Three-Dimensional M–Ag (M = Pt and Pd) Aerogels with Excellent Green Energy Generation7Recent Advances and Trends in Photoelectrochemical Hybrid Water Electrolysis1Corner‐Sharing Tetrahedrally Coordinated W‐V Dual Active Sites on Cu2V2O7 for Photoelectrochemical Water Oxidation7Selective CO2‐to‐Syngas Conversion Enabled by Bimetallic Gold/Zinc Sites in Partially Reduced Gold/Zinc Oxide Arrays34Selective CO2‐to‐Syngas Conversion Enabled by Bimetallic Gold/Zinc Sites in Partially Reduced Gold/Zinc Oxide Arrays16Intermetallic Nanocrystals for Fuel-Cells-Based Electrocatalysis257Covalent organic frameworks bearing Ni active sites for free radical-mediated photoelectrochemical organic transformations62Plasmon-Driven Reaction Selectivity Tuning for Photoelectrochemical H2O2 Production34Pauling‐Type Adsorption of O 2 Induced by Heteroatom Doped ZnIn 2 S 4 for Boosted Solar‐Driven H 2 O 2 Production15Pauling‐Type Adsorption of O 2 Induced by Heteroatom Doped ZnIn 2 S 4 for Boosted Solar‐Driven H 2 O 2 Production92Modulation of Electronic Synergy to Enhance the Intrinsic Activity of Fe5Ni4S8 Nanosheets in Restricted Space Carbonized Wood Frameworks for Efficient Oxygen Evolution Reaction13TaS2 Nanosheets Decorated with SnS2 Nanosheet/Reduced Graphene Oxide Composites for Broadband Photodetectors7Modification of hydrothermally synthesized α-Fe 2 O 3 nanorods with g-C 3 N 4 prepared from various precursors as photoanodes for hydrogen production2Solar-driven photoelectrochemical conversion of biomass: recent progress, mechanistic insights and potential scalability88Efficient U(VI) capture co-driven by multiple synergistic mechanisms in an advanced asymmetrical photoelectrocatalytic system12Precise Lattice‐Strain Modulation of Hematite Enabled by Gradient Doping of Mn for Enhanced Photoelectrocatalytic Oxidative C─C Bond Scission15Direct generation of high-valent iron-oxo species to eliminate oxytetracycline at circumneutral pH via paper mill sludge ash activating peroxymonosulfate13Efficient Homolytic Cleavage of H 2 O 2 on Hydroxyl‐Enriched Spinel CuFe 2 O 4 with Dual Lewis Acid Sites142Efficient Homolytic Cleavage of H2O2 on Hydroxyl‐Enriched Spinel CuFe2O4 with Dual Lewis Acid Sites14Anchoring Ultrafine β‐Mo 2 C Clusters Inside Porous Co‐NC Using MOFs for Electric‐Powered Coproduction of Valuable Chemicals7Stabilizing BiVO4 Photoanode in Bicarbonate Electrolyte for Efficient Photoelectrocatalytic Alcohol Oxidation5Electronic modulation caused by interfacial Fe-O-Co-O-Fe bonding for boosting highly efficient non-enzymic nitrite sensing23Cycad-leaf-like crystalline-amorphous heterostructures for efficient urea oxidation-assisted water splitting21Bi Quantum Dots Supported on BiOBr Nanoparticles and Loaded on Porous ZnO as a Photocatalyst for Dye Degradation and H 2 Production13Rapid Surface Reconstruction of In 2 S 3 Photoanode via Flame Treatment for Enhanced Photoelectrochemical Performance29Potential-dependent photo-electro-catalysis coupling mechanism for methanol oxidation: A case study over Pt/Cu-Nb2O5 nanorod arrays8Efficient photoanode with a MoS2/TiO2/Au nanoparticle heterostructure for ultraviolet-visible photoelectrocatalysis16Operando spectroelectrochemical insights into the selectivity difference of photoelectrocatalytic alcohol oxidation to aldehyde on hematite and titania7Enhanced Electrocatalytic Performance of the FePt/PPy-C Composite toward Methanol Oxidation5Wood-derived continuously oriented channels coupled with tunable built-in electric fields for efficient oxygen evolution48Designing TiO 2 Nanotubular Arrays with Au-CoO x Core–Shell Nanoparticles for Enhanced Photoelectrochemical Methanol and Lignin Oxidation18Regulation strategy of spinel OER electrocatalyst4Principle Design of C−C Coupling Pathway Towards Highly Selective C2 Products Using Photocatalytic CO2 Reduction:A Review5Synthesis of intermetallic L 1 0 -Fe 40 Ni 5 M 5 Pt 50 (M = Mn, Co, Cu) nanoparticles for electrocatalytic methanol oxidation5Manipulating the electronic state of tungsten carbide using CoNi@N-doped carbon derived from a bimetallic MOF for enhanced electroreduction reactions12Stabilization of a Co( ii ) site via a Co–O–Fe bridging motif for enhanced electro-oxidation of methanol to formate5Distinct Promotion of PEC Water Oxidation of Ta2O5/α-Fe2O3/Co–Ni PBA via Coupling Ni 3d with O 2p12Mesoporous Co-Mn ferrites as highly radical-forming catalysts for wet peroxide oxidation of 4-nitrophenol12Exploiting Antisite Defects in FeWN 2 Nanosheets for Enol Electro‐oxidation Coupled with H 2 Evolution at a Large Current Density0Exploiting Antisite Defects in FeWN 2 Nanosheets for Enol Electro‐oxidation Coupled with H 2 Evolution at a Large Current Density12A novel and efficient In2O3@RhPt catalyst for solvent-free transfer hydrogenation of TDC to HTDC: Catalytic performance and mechanism0Photoelectrocatalytic Transformations of Waste into Value12Solar-driven electrolysis coupled with valuable chemical synthesis15Recent Progress on Photoelectrochemical Organic Upgrading: A Review from Direct and Indirect Charge Transfer Pathway10Advances in design principles of nanostructured heterojunction catalysts for photoelectrochemical hydrogen evolution reactions: a mini-review3Electronic engineering of spinels for advanced electrocatalysis10Zinc Oxide‐Based Nanocomposite Photoelectrodes for Photoelectrochemical Water Splitting: A Review on Structural Modifications and Performance Optimization7Deciphering electronic metal-support interaction in Ce1/ZnO single-atom catalysts for boosting CO2 electroreduction7Synergistic chiral mediation and Ga 3+ doping introduces lattice distortion and defect states to construct an intensified built-in electric field and abundant active sites for enhanced BiOBr photoelectrocatalytic performance0Role of Coordination Cations on the Formation of Spinels from Hot Stainless Steel Slags0Synergistic Defect Engineering and Self‐Assembled Nafion on Photoanodes Enabling Selective Photoelectrochemical Glucose Oxidation Coupled H 2 Production4Elucidating the NH 2 OH–Mediated Pathway for Photoelectrocatalytic C–N Coupling toward Solar-Driven Hexamethylenetetramine Synthesis3Recent Progress on Photoelectrochemical Biomass‐Derived Platform Molecules Conversion Coupled With Hydrogen Evolution0Hydroxide‐Based Catalysts for Alcohol Electrooxidation: From Fundamentals Understanding to Catalyst Design Strategies1Bimetal oxide heterojunction-based electrocatalyst for methanol oxidation reaction3CuInS2-based S-scheme heterojunction photocatalysts for efficient photocatalytic hydrogen evolution9Hydrophobic Microenvironment on Cu–Co Oxides for Dual Promotion of Mass Transfer and Electronic Regulation in Alkyl Aromatic Oxidation0Work‐Function‐Modulated Ag Single‐Atom Catalysts for Amino Alcohol Oxidation0Work‐Function‐Modulated Ag Single‐Atom Catalysts for Amino Alcohol Oxidation1Application of Single-Atom Synergistic Catalysts in Multifield Coupling Reactions0In Situ Generated Asymmetric Charge‐Polarized Pd δ− ‐O δ− ‐Zn Sites for Highly Selective Photocatalytic Oxidation of Methane to Formaldehyde0Synergistic Integration of Thermocatalysis and Electrocatalysis for Isopropanol Dehydrogenation Toward Efficient Hydrogen Production0Synergistic Integration of Thermocatalysis and Electrocatalysis for Isopropanol Dehydrogenation Toward Efficient Hydrogen Production0Dual‐Interface Kinetics Activation Through Dipole‐Induced Dynamic Liquid Crystal Interfacial Engineering for Efficient Solar Water Splitting0

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  2. Activating bulk nickel foam for the electrochemical oxidization of ethanol by anchoring MnO 2 @Au nanorods

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  50. Rapid Surface Reconstruction of In 2 S 3 Photoanode via Flame Treatment for Enhanced Photoelectrochemical Performance

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