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RESEARCH PAPER · ACS Nano · 2022

Basal Planes Unlocking and Interlayer Engineering Endows Proton Doped-MoO2.8F0.2 with Fast and Stable Magnesium Storage

Weixiao Wang, Yalong Jiang, Ya Yang, Fangyu Xiong, Shaohua Zhu, Junjun Wang, Lulu Du, Jinghui Chen, Lianmeng Cui, Jun Lin Xie, Qinyou An, Liqiang Mai

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Basal Planes Unlocking and Interlayer Engineering Endows Proton Doped-MoO2.8F0.2 with Fast and Stable Magnesium StorageOriginalEngineering d-p orbital hybridization through regulation of interband energy separation for durable aqueous Zn//VO2(B) batteries36Regulating solvation sheath by introducing multifunctional fluoride boronic esters for highly efficient magnesium stripping/plating36Cathode Materials and Chemistries for Magnesium Batteries: Challenges and Opportunities120A critical review of inorganic cathode materials for rechargeable magnesium ion batteries29Combining Structural Modification and Electrolyte Regulation to Enable Long‐Term Cyclic Stability of MoO 3‐x @TiO 2 as Cathode for Aqueous Zn‐Ion Batteries28Enabling Ultrafast Single Mg 2+ Insertion Kinetics of Magnesium-Ion Batteries via In Situ Dynamic Catalysis and Re-equilibration Effects14Valence modulation and morphological engineering of MoO3 as high-performance cathode for aqueous zinc ion batteries24Cationic–Anionic Redox Chemistry in Multivalent Metal‐Ion Batteries: Recent Advances, Reaction Mechanism, Advanced Characterization Techniques, and Prospects22Surface‐Redox Pseudocapacitance‐Dominated Charge Storage Mechanism Enabled by the Reconstructed Cathode/Electrolyte Interface for High‐Rate Magnesium Batteries50Double-chain conjugated carbonyl polymer cathode for rechargeable magnesium batteries: Constructing active sites for reversible storage of bivalent magnesium cations32Defect engineering of W6+-doped NiO for high-performance black smart windows47Design of Layer Structure Metal Oxide Material with Dual-Ion Defects for High-Performance Aqueous Zn Ion Batteries11Organic Molecular Intercalation Enabled Anionic Redox Chemistry with Fast Kinetics for High Performance Magnesium Storage11Magnesium Mitigation Behavior in P2-Layered Sodium-Ion Battery Cathode19Chloride-Free Electrolyte Based on Tetrabutylammonium Triflate Additive for Extended Anodic Stability in Magnesium Batteries35Bimetallic sulfide CoNi2S4 hollow nanospheres as a high-performance cathode material for Mg-ion batteries32A new frontier of flexible energy devices: Aqueous proton supercapacitors18Bimetallic Selenide CuFeSe2 as Mg‐Storage Material for Rechargeable Magnesium Batteries7Oxygen Vacancies Boosted Hydronium Intercalation: A Paradigm Shift in Aluminum‐Based Batteries19Oxygen Vacancies Boosted Hydronium Intercalation: A Paradigm Shift in Aluminum‐Based Batteries6References0Graphitic carbons: preparation, characterization, and application on K‐ion batteries14Insoluble Polyquinonyl Sulfide as High-Capacity Cathode Material for Magnesium Battery2Electron-injection-engineering induced dual-phase MoO2.8F0.2/MoO2.4F0.6 heterostructure for magnesium storage11Coupling Manipulation of Interfacial Chemistry and Coordination Structure in Vanadium Oxides Enables Rapid Magnesium Ion Diffusion Kinetics20Coupling Manipulation of Interfacial Chemistry and Coordination Structure in Vanadium Oxides Enables Rapid Magnesium Ion Diffusion Kinetics3Defect Engineering: Can it Mitigate Strong Coulomb Effect of Mg2+ in Cathode Materials for Rechargeable Magnesium Batteries?43The formation of three-dimensional phosphorus-doped MoO2/C nanostructures for high-performance aqueous zinc-ion batteries1Great impetus of microscopic theoretical analyses for the advancement of magnesium-based batteries4Enabling high-performance multivalent metal-ion batteries: current advances and future prospects146Advanced cathode for synergistic anion-cation redox reactions in magnesium-ion batteries — A pathway to fast diffusion/reaction kinetics12High‐Throughput Screening of 1D Chalcogenide Cathode Materials Beyond VS4 for Rechargeable Magnesium‐Ion Batteries0Surface-redox pseudocapacitive charge storage mechanism based on quantum size effect enabling stable and fast magnesium batteries10Boosting anionic-cationic redox chemistry in anion-rich CuSe2 cathode toward high-energy magnesium batteries9Insertion-type cathode materials in magnesium ion batteries: Research progress and application potential4Recent Progress in Interlayer Engineering of Layered Materials for High-Performance Magnesium Ion Batteries5Roadmap for Next-Generation Electrochemical Energy Storage Technologies: Secondary Batteries and Supercapacitors149P2-Type Mn-Based Oxide Cathode for Chlorine-Free Mg–Na Hybrid Battery Devices8Breaking through the bottleneck: In-depth analysis of the magnesium storage mechanism of intercalation-type cathode materials and prospects for modification strategies2Breaking Bond‐Strain Lockstep in Multielectron Anodes0Quantum size effect activating MoO3-x voltage platforms enables high-capacity and long-cycle magnesium-ion batteries3Confinement−Adsorption Synergy in Hybrid Carbon‐Coated Separator Enables Stable High‐Rate Quinone Cathode for Magnesium Batteries3Unlocking Inert Material to Durable Cathode for Magnesium Storage Inspired via Synergistic Spin‐Orbital Reconfiguration and Adaptive Crystal Transformation0Molecular interlayer engineering of VSe 2 enables fast and durable magnesium–lithium hybrid ion storage0Magnesium-ion battery cathode materials: Artificial intelligence applications, research advances, and industrialization0

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  1. Engineering d-p orbital hybridization through regulation of interband energy separation for durable aqueous Zn//VO2(B) batteries

    Chemical Engineering Journal · 2023-04-06

    Wenwei Zhang, Jianfeng Liu, Wanyue Cai, Min Zhou, Wenhui Zhong, Gaofan Xiao, Ping Luo, Yan Zhao, Qinyou An

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  2. Regulating solvation sheath by introducing multifunctional fluoride boronic esters for highly efficient magnesium stripping/plating

    Energy storage materials · 2023-04-24

    Chunfeng Chen, Jinlong Chen, Shuangshuang Tan, Xueting Huang, Yaoyao Du, Bo Shang, Baihua Qu, Guangsheng Huang, Xiaoyuan Zhou, Jingfeng Wang, Lingjie Li, Fusheng Pan

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  3. Cathode Materials and Chemistries for Magnesium Batteries: Challenges and Opportunities

    Advanced Energy Materials · 2023-05-11

    Zhenyou Li, Joachim Häcker, Maximilian Fichtner, Zhirong Zhao‐Karger

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  4. A critical review of inorganic cathode materials for rechargeable magnesium ion batteries

    Journal of Energy Storage · 2023-05-26

    Meiyu Shi, Tianlin Li, Shang Han, De‐Wen Zhang, Huayan Qi, Tianlong Huang, Zelin Xie, Jiqiu Qi, Fuxiang Wei, Qingkun Meng, Bin Xiao, Qing Yin, Yong‐Zhi Li, Danyang Zhao, Xiaolan Xue, Yanwei Sui

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  5. Combining Structural Modification and Electrolyte Regulation to Enable Long‐Term Cyclic Stability of MoO 3‐x @TiO 2 as Cathode for Aqueous Zn‐Ion Batteries

    Small · 2023-06-01

    Wenjie Huang, Hui Wang, Renzong Hu, Jun Liu, Lichun Yang, Min Hua Zhu

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  6. Enabling Ultrafast Single Mg 2+ Insertion Kinetics of Magnesium-Ion Batteries via In Situ Dynamic Catalysis and Re-equilibration Effects

    ACS Applied Materials & Interfaces · 2023-06-01

    Rongrui Deng, Shuangshuang Tan, Zhongting Wang, Rong Li, Guanjie Lu, Baihua Qu, Le Tong, Ronghua Wang, Chaohe Xu, Guangsheng Huang, Jingfeng Wang, Aitao Tang, Xiaoyuan Zhou, Fusheng Pan

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  7. Valence modulation and morphological engineering of MoO3 as high-performance cathode for aqueous zinc ion batteries

    Electrochimica Acta · 2023-08-05

    Yachen He, Hongwei Tang, Yifeng Huang, Kaihao Chen, Guangxia Wang, Guangxia Wang, Dezhou Zheng, Wei Ming Xu, Fuxin Wang, Xihong Lu

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  8. Cationic–Anionic Redox Chemistry in Multivalent Metal‐Ion Batteries: Recent Advances, Reaction Mechanism, Advanced Characterization Techniques, and Prospects

    Advanced Functional Materials · 2023-08-28

    Xiaolan Xue, Tianlong Huang, Yang Zhang, Jiqiu Qi, Fuxiang Wei, Yanwei Sui, Zhong Jin

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  9. Surface‐Redox Pseudocapacitance‐Dominated Charge Storage Mechanism Enabled by the Reconstructed Cathode/Electrolyte Interface for High‐Rate Magnesium Batteries

    Advanced Energy Materials · 2023-09-13

    Dongzheng Wu, Yuanhong Kang, Fei Wang, Jin Yang, Yaoqi Xu, Yichao Zhuang, Jiayue Wu, Jing Hui Zeng, Yang Yang, Jinbao Zhao

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  10. Double-chain conjugated carbonyl polymer cathode for rechargeable magnesium batteries: Constructing active sites for reversible storage of bivalent magnesium cations

    Energy storage materials · 2023-09-24

    Xin Ren, Donggang Tao, Shuai Cui, Ting Li, Yuliang Cao, Fei Jin Xu

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  11. Defect engineering of W6+-doped NiO for high-performance black smart windows

    Nano Research · 2023-09-25

    Yingjun Xiao, Xiang Zhang, Dukang Yan, Jian-Bo Deng, Ming‐Jun Chen, Hulin Zhang, Wenhai Sun, Jiupeng Zhao, Yao Li

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  12. Design of Layer Structure Metal Oxide Material with Dual-Ion Defects for High-Performance Aqueous Zn Ion Batteries

    ACS Sustainable Chemistry & Engineering · 2023-10-09

    Yuying Li, Xinli Guo, Z. Cao, Shaohua Wang, Qiuping Fu, Yanmei Zheng, Junnan Qu, Ruiting Li, Li Zhao, Dan Luo, Zhongwei Chen

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  13. Organic Molecular Intercalation Enabled Anionic Redox Chemistry with Fast Kinetics for High Performance Magnesium Storage

    Small · 2023-11-10

    Rongrui Deng, Zhongting Wang, Shuangshuang Tan, Guanjie Lu, Xueting Huang, Baihua Qu, Guangsheng Huang, Chaohe Xu, Xiaoyuan Zhou, Jingfeng Wang, Fusheng Pan

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  14. Magnesium Mitigation Behavior in P2-Layered Sodium-Ion Battery Cathode

    The Journal of Physical Chemistry Letters · 2023-11-16

    Hui Wan, Shu Li, Xiang-Long Zhang, Lichen Wu, Zhixiao Liu, Guangdong Liu, Caitian Gao, Wei‐Qing Huang, Huiqiu Deng, Wangyu Hu, Fei Gao

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  15. Chloride-Free Electrolyte Based on Tetrabutylammonium Triflate Additive for Extended Anodic Stability in Magnesium Batteries

    Nano Letters · 2023-11-22

    Deviprasath Chinnadurai, Yuanjian Li, Chang Zhang, Gaoliang Yang, Wei Ying Lieu, Sonal Kumar, Zhenxiang Xing, Wei Liu, Zhi Wei Seh

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  16. Bimetallic sulfide CoNi2S4 hollow nanospheres as a high-performance cathode material for Mg-ion batteries

    Chemical Engineering Journal · 2023-12-21

    Yating Fei, Haobo Wang, Yifan Xu, Lili Song, Yuehua Man, Yichen Du, Jianchun Bao, Xiaosi Zhou

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  17. A new frontier of flexible energy devices: Aqueous proton supercapacitors

    Applied Physics Reviews · 2024-01-16

    Jing Liang, Wei Hong Wu

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  18. Bimetallic Selenide CuFeSe2 as Mg‐Storage Material for Rechargeable Magnesium Batteries

    Batteries & Supercaps · 2024-04-05

    Qinghong Kong, Lianmeng Cui, Xiaobin Liao, Ruohan Yu, Yalong Jiang, Junjun Wang, Wenwei Zhang, Yu Wang, Lei Zhang, Qinyou An

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  19. Oxygen Vacancies Boosted Hydronium Intercalation: A Paradigm Shift in Aluminum‐Based Batteries

    Angewandte Chemie International Edition · 2024-04-22

    Chengxiang Huang, Jiang Zhou, Fuxi Liu, Wenwen Li, Qing Liang, Zhenzhen Zhao, Xin Ge, Kexin Song, Lirong Zheng, Xinyan Zhou, Sifan Qiao, Wei Zhang, Weitao Zheng, Weitao Zheng

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  20. Oxygen Vacancies Boosted Hydronium Intercalation: A Paradigm Shift in Aluminum‐Based Batteries

    Angewandte Chemie · 2024-04-22

    Chengxiang Huang, Jiang Zhou, Fuxi Liu, Wenwen Li, Qing Liang, Zhenzhen Zhao, Xin Ge, Kexin Song, Lirong Zheng, Xinyan Zhou, Sifan Qiao, Wei Zhang, Wei Zhang

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  21. References

    Unknown journal · 2024-05-10

    Jianxin Zou, Yanna NuLi, Zhigang Hu, Xi Lin, Qiuyu Zhang

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  22. Graphitic carbons: preparation, characterization, and application on K‐ion batteries

    Rare Metals · 2024-05-23

    Kangzhe Cao, Jiahui Ma, Yu-Lian Dong, Yu Bing Duan, Runtian Zheng, Dharani Bundhooa, Huiqiao Liu, Yong Lei

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  23. Insoluble Polyquinonyl Sulfide as High-Capacity Cathode Material for Magnesium Battery

    Energy & Fuels · 2024-06-12

    Xingyu Gao, Xiquan Qi, Xiangyu Zhao

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  24. Electron-injection-engineering induced dual-phase MoO2.8F0.2/MoO2.4F0.6 heterostructure for magnesium storage

    National Science Review · 2024-07-11

    Weixiao Wang, Fangyu Xiong, Shaohua Zhu, Mengyu Yan, Xiaobin Liao, Kesong Yu, Lianmeng Cui, Jinghui Chen, Junjun Wang, Ruoqi Lan, Jun Xie, Qinyou An, Liqiang Mai

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  25. Coupling Manipulation of Interfacial Chemistry and Coordination Structure in Vanadium Oxides Enables Rapid Magnesium Ion Diffusion Kinetics

    Angewandte Chemie International Edition · 2024-08-30

    Weixiao Wang, Wenwen Wang, Fangyu Xiong, Jiashen Meng, Jinsong Wu, Wei Yang, Juncai Long, Jinghui Chen, Jiajun Chen, Qinyou An

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  26. Coupling Manipulation of Interfacial Chemistry and Coordination Structure in Vanadium Oxides Enables Rapid Magnesium Ion Diffusion Kinetics

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  27. Defect Engineering: Can it Mitigate Strong Coulomb Effect of Mg2+ in Cathode Materials for Rechargeable Magnesium Batteries?

    Nano-Micro Letters · 2024-09-20

    Zhengqing Fan, Ruimin Li, Xin Zhang, Wanyu Zhao, Zhenghui Pan, Xiaowei Yang

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  28. The formation of three-dimensional phosphorus-doped MoO2/C nanostructures for high-performance aqueous zinc-ion batteries

    Journal of Electroanalytical Chemistry · 2024-10-20

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  29. Great impetus of microscopic theoretical analyses for the advancement of magnesium-based batteries

    Energy storage materials · 2024-11-22

    Miao Tian, Zhitao Wang, Hui Ying Yang, Song Chen

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  30. Enabling high-performance multivalent metal-ion batteries: current advances and future prospects

    Chemical Society Reviews · 2025-01-01

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  31. Advanced cathode for synergistic anion-cation redox reactions in magnesium-ion batteries — A pathway to fast diffusion/reaction kinetics

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  32. High‐Throughput Screening of 1D Chalcogenide Cathode Materials Beyond VS4 for Rechargeable Magnesium‐Ion Batteries

    ChemSusChem · 2025-03-26

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  33. Surface-redox pseudocapacitive charge storage mechanism based on quantum size effect enabling stable and fast magnesium batteries

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  34. Boosting anionic-cationic redox chemistry in anion-rich CuSe2 cathode toward high-energy magnesium batteries

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  35. Insertion-type cathode materials in magnesium ion batteries: Research progress and application potential

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  36. Recent Progress in Interlayer Engineering of Layered Materials for High-Performance Magnesium Ion Batteries

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  37. Roadmap for Next-Generation Electrochemical Energy Storage Technologies: Secondary Batteries and Supercapacitors

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  38. P2-Type Mn-Based Oxide Cathode for Chlorine-Free Mg–Na Hybrid Battery Devices

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  39. Breaking through the bottleneck: In-depth analysis of the magnesium storage mechanism of intercalation-type cathode materials and prospects for modification strategies

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  40. Breaking Bond‐Strain Lockstep in Multielectron Anodes

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  41. Quantum size effect activating MoO3-x voltage platforms enables high-capacity and long-cycle magnesium-ion batteries

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  42. Confinement−Adsorption Synergy in Hybrid Carbon‐Coated Separator Enables Stable High‐Rate Quinone Cathode for Magnesium Batteries

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  43. Unlocking Inert Material to Durable Cathode for Magnesium Storage Inspired via Synergistic Spin‐Orbital Reconfiguration and Adaptive Crystal Transformation

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  44. Molecular interlayer engineering of VSe 2 enables fast and durable magnesium–lithium hybrid ion storage

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