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RESEARCH PAPER · Journal of the American Chemical Society · 2022

Robust Spin-Dependent Anisotropy of Circularly Polarized Light Detection from Achiral Layered Hybrid Perovskite Ferroelectric Crystals

Xiaoqi Li, Fafa Wu, Yunpeng Yao, Wentao Wu, Chengmin Ji, Lina Li, Zhihua Sun, Junhua Luo, Xitao Liu

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Robust Spin-Dependent Anisotropy of Circularly Polarized Light Detection from Achiral Layered Hybrid Perovskite Ferroelectric CrystalsOriginalCharge‐Transfer Complex Doped Photothermal Hydrogels for Discriminating Circularly Polarized Near‐Infrared Light38Charge‐Transfer Complex Doped Photothermal Hydrogels for Discriminating Circularly Polarized Near‐Infrared Light3Emerging Halide Perovskite Ferroelectrics161A nickel( ii )-based one-dimensional organic–inorganic halide perovskite ferroelectric with the highest Curie temperature43Circularly polarized luminescence and nonlinear optical harmonic generation based on chiral zinc halides23High stability and moderate second-order nonlinear optical properties of hybrid lead-free perovskite [(CH 3 ) 3 NCH 2 Cl]CdCl 3 bulk crystals12Mixing cage cations in 2D metal-halide ferroelectrics enhances the ferro-pyro-phototronic effect for self-driven photopyroelectric detection14Reversible phase transition and thermochromic response in hybrid copper-based perovskites18Circularly Polarized Light Responsive Materials: Design Strategies and Applications161Recent Advances and Opportunities in Low‐Dimensional Layered Perovskites for Emergent Applications beyond Photovoltaics41Geometrical Designing of a Soft‐Layered Halide Perovskite Improper Photoferroelectric for Boosted Photostriction12Centimeter‐Size Single Crystals of Halide Perovskite Photoferroelectric Solid Solution with Ultrahigh Pyroelectricity Boosted Photodetection28Centimeter‐Size Single Crystals of Halide Perovskite Photoferroelectric Solid Solution with Ultrahigh Pyroelectricity Boosted Photodetection7Achiral Fluorinated Aromatic Ligands Based Chiral Hybrid Antimony Halides with High‐Efficiency Second‐Harmonic Generation18Interlayer Polymerization of 2D Chiral Perovskite Single‐Crystal Films toward High‐Performance Flexible Circularly Polarized Light Detection46Polarization‐Dependent Large Photorefractive Effect In A Wide Bandgap 2D Metal Halide Ferroelectric14Bulk Photovoltaic Effect in Chiral Layered Hybrid Perovskite Enables Highly Sensitive Near-Infrared Circular Polarization Photodetection33Bulk Photovoltaic Effect Along the Nonpolar Axis in Organic‐Inorganic Hybrid Perovskites6Bulk Photovoltaic Effect Along the Nonpolar Axis in Organic‐Inorganic Hybrid Perovskites18Bulk Photovoltaic Effect in Two-Dimensional Distorted MoTe241Enhanced Circular Dichroism and Polarized Emission in an Achiral, Low Band Gap Bismuth Iodide Perovskite Derivative14Chlorine-substituted chiral 2D perovskite microwires with enhanced lattice rigidity for sensitive circularly polarized light detection11Halogen Effect on the Photoluminescence of 1D Hybrid Lead Halide Perovskites with a Bipyridinium Cation6Hybrid perovskite shows temperature-dependent photoluminescence and dielectric response triggered by halogen substitution22Regulating Circularly Polarized Light Detection via Polar‐Phase Transition in Alternating Chiral‐Achiral Cations Intercalation‐Type Hybrid Perovskites26Enhanced photoelectric performance in Cu–Bi double halide perovskite single crystals4Sensing polarized light via switchable Rashba-Dresselhaus spin splitting in a ferroelectric semiconductor212D Molecular Ferroelectric with Large Out‐of‐plane Polarization for In‐Memory Computing18Phase Transitions and Dynamics in Mixed Three- and Low-Dimensional Lead Halide Perovskites134Engineering ferroelectric-nanonet-based heterostructures enables superior photovoltaic effect and asymmetric switchability8Efficient Charge Transport in Inverted Perovskite Solar Cells via 2D/3D Ferroelectric Heterojunction25Controllable Chiral Lattices for 2D ROA Mapping and a Long-term Stable Broadband CPL Detector0Highly Stable MOF‐Type Lead Halide Luminescent Ferroelectrics26Highly Stable MOF‐Type Lead Halide Luminescent Ferroelectrics7Atomically Precise Chiral Metal Nanoclusters for Circularly Polarized Light Detection49Atomically Precise Chiral Metal Nanoclusters for Circularly Polarized Light Detection6Pyro‐Phototronic Circularly Polarized Light Detection Based on Deuterated L‐Alanine Doped Triglycine Sulfate's Bulk Photovoltaic Effect8Coupled Kite-to-Square Distortion Transition and Physical Properties in 2D Lead Halide Perovskite11Polar Alternating Cations Intercalated Hybrid Perovskite with Iodine‐Substituted Spacers Toward Efficient Passive X‐Ray Detection21Chiral Perovskite Heterostructure Films of CsPbBr3 Quantum Dots and 2D Chiral Perovskite with Circularly Polarized Luminescence Performance and Energy Transfer47Organic Ferroelectrics for Regulation of Electronic and Ionic Transport Toward Neuromorphic Applications15Review of Polarized Light‐Spin/Dipole Interactions: Fundamental Physics and Application in Circularly Polarized Detecting25Halogen Substitution Strategy for Exploiting High‐Performance Molecular Ferroelectrics12D and quasi-2D hybrid halide perovskite single crystals: From fundamentals to functionalized photodetectors15Ferroelectric polarization in 2D halide hybrid perovskites: influence on bulk crystals, thin films, and applications17Mechanical Twisting-Induced Enhancement of Second-Order Optical Nonlinearity in a Flexible Molecular Crystal36Recent Advances in Emerging Polarization‐Sensitive Materials: From Linear/Circular Polarization Detection to Neuromorphic Device Applications60Two‐Dimensional Layered Germanium Iodide Perovskite Ferroelectric Semiconductors25Two‐Dimensional Layered Germanium Iodide Perovskite Ferroelectric Semiconductors22D Perovskite Heterojunction‐Based Self‐Powered Polarized Photodetectors with Controllable Polarization Ratio Enabled by Ferro‐Pyro‐Phototronic Effect25Temperature‐Responsive Photoluminescence of 1D Chiral Lead Halide Perovskites with Highly Anisotropic Second Harmonic Generation21Manipulating perovskite structural asymmetry for high-performing self-powered full-stokes polarimetry32Materials innovation for circularly polarized photodetectors3Enantioselective Se lattices for stable chiroptoelectronic processing media6High-sensitivity self-powered circularly polarized light detection based on chiral antimony-based halides with strong polarity15Recent Progress and Future Opportunities for Optical Manipulation in Halide Perovskite Photodetectors8Emerging molecular ferroelectrics for high-performance perovskite optoelectronic devices9Double-headed brush CsPbI3 nanorod assemblies for high non-filtered linear polarization in optical displays5PdSe2/WS2/PdSe2 unipolar barrier photodetector for visible-infrared polarization detection, synaptic plasticity simulation and neuromorphic visual system15Chiral 3D Perovskite Single Crystals Realized by Lattice Expansion6Hybrid Perovskite Ferroelectric Enables Dual‐Polarity Polarization‐Sensitive Photodetection Toward Encrypted Communication7Multifunctional Chiral Halide Perovskites: Advancing Chiro‐Optics, Chiro‐Optoelectronics, and Spintronics33Achieving Efficient Self‐Driven Full‐Stokes Photodetection in Optically Active Ferroelectric4Achieving Efficient Self‐Driven Full‐Stokes Photodetection in Optically Active Ferroelectric1Tailoring chirality in van der Waals crystals for circular polarization encoded pattern recognition0Wettability-Switchable Azobenzene Inverse Opal Film via Interfacial Engineering2Ionotronics‐Enabled Emerging Halide Perovskite Optoelectronic Devices10Dimensional engineering in chiral layered hybrid perovskites for high-anisotropy self-powered circularly polarized light detection0Inch-sized achiral perovskite ferroelectric single crystals for multiaxial passive circularly polarized light response0Integrated Photon Ellipticity Recognition with Chiral Nanomaterials1Insights Into Ferroelectric Phase Transition Mechanism for One‐Dimensional Halide Perovskites to Attain Record‐Performance Self‐Powered X‐Ray Detection4Emerging halide perovskite ferroelectric semiconductors: Structural diversity, chemical design and optoelectronic applications3Dimensionality Engineering: A Pathway to Ferroelectric Halide Perovskites3Circularly polarized luminescence: materials, photophysics, devices, and applications15Harnessing Strong Chiroptical Nonlinearity in Carbene-Copper-Amides through Center-Specific Chirality: An Approach to Amplified Dissymmetry0Perspective on Ferroelectric and Nonferroelectric Low‐Dimensional Metal Halide Perovskites for Memristor Technology1Halogen Engineering Achieving Regulable Polar Axes and Large Spontaneous Polarization in Mixed‐Cation Metal Halide Hybrid Multiferroics0Ultrawide‐Bandgap Rb 2 AgCl 3 Perovskite Single Crystals Enabling Self‐Powered Solar‐Blind UV Polarization‐Sensitive Photodetection for Intelligent Imaging and Encryption1Bilayered Two-Dimensional Hybrid Perovskite with Switchable Dielectric Properties, Persistent Disorder, and Narrow-Band Emission0Oxygen-Controlled Assembly of Chiral [7]-Helicene on ZnO Surfaces0Circularly Polarized Photoluminescence Obtained by Optical Spin Pumping in Achiral Lead-Halide Perovskites: Implications of Interface-Induced Rashba Splitting0Low-Dimensional Perovskites and Metal Halides across Structures and Functions: Connectivity, Dimensionality, and Emerging Principles1Electrically Switchable Circularly Polarized Light Detection in Optically Active Ferroelectric0Electrically Switchable Circularly Polarized Light Detection in Optically Active Ferroelectric0Phase‐Switchable 2D Single‐Crystalline Perovskite With Low‐Temperature Out‐of‐Plane Rashba Splitting and Room‐Temperature Out‐of‐Plane Ferroelectricity for Electrically Reconfigurable Spin‐Photonics0

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