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RESEARCH PAPER · Applied Catalysis B: Environmental · 2022

Solar energy-driven upcycling of plastic waste on direct Z-scheme heterostructure of V-substituted phosphomolybdic acid/g-C3N4 nanosheets

Chuanwang Xing, Guiyang Yu, Jun Zhou, Qi Liu, Ting Chen, Heyuan Liu, Xiyou Li

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Solar energy-driven upcycling of plastic waste on direct Z-scheme heterostructure of V-substituted phosphomolybdic acid/g-C3N4 nanosheetsOriginalNovel "Toast"-Like G-C3n4/Tio2 Composite: How the “Melting” of G-C3n4 Effects the Photocatalytic Oxidation of Bisphenol a Under Visible-Light Illumination0Enhanced photocatalytic performance by polarizing ferroelectric KNbO3 for degradation of plastic wastes under mild conditions60In Situ Assembly of Hydrogen‐Bonded Organic Framework on Metal–Organic Framework: An Effective Strategy for Constructing Core–Shell Hybrid Photocatalyst100Rational design of covalent heptazine framework photocatalysts with high oxidation ability through reaction-dependent strategy9Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Schottky junction with Bi/Bi 2 O 3 core–shell nanoparticle modified g-C 3 N 4 for boosting photocatalytic H 2 O 2 evolution from pure water20State of the art in the photochemical degradation of (micro)plastics: from fundamental principles to catalysts and applications112Visible light driven reform of wasted plastics to generate green hydrogen over mesoporous ZnIn 2 S 446Well-designed MOF-derived hollow octahedral structure TiO2 coupled with ultra-thin porous g-C3N4 to enhance the degradation of real liquor brewing wastewater27Self‐Adaptive Electronic Structure of Amphoteric Conjugated Ligand‐Modified 3 d Metal−C3N4 Smart Electrocatalyst by pH Self‐Response Realizing Electrocatalytic Self‐Adjustment4Construction of Cu7S4@CuCo2O4 Yolk–Shell Microspheres Composite and Elucidation of Its Enhanced Photocatalytic Activity, Mechanism, and Pathway for Carbamazepine Degradation84Dual P-doped-site modified porous g-C3N4 achieves high dissociation and mobility efficiency for photocatalytic H2O2 production77Cu2−xSe/FeSe2 Z-type heterojunction demonstrate versatile boosting photoelectrochemical, electrocatalytic and photocatalytic properties38Enhanced carrier separation in g-C3N4/MoO3-x heterostructures towards efficient phenol removal25Influence of the calcination duration of g-C3N4/TiO2 “veggie-toast-like” photocatalyst on the visible-light triggered photocatalytic oxidation of bisphenol A29Controllably solar-driven C‒C coupling organic synthesis integrated with H2 production over P-doped g-C3N4 with NiS nanoparticles modification18Janus Z-scheme heterostructure of ZnIn2S4/MoSe2/In2Se3 for efficient photocatalytic hydrogen evolution30Rational design of photo− /electro−catalytic systems for the transformation of plastic wastes51Insight into photocatalysis technology as a promising approach to tackle microplastics pollution through degradation and upcycling87Photothermal Catalysis: An Emerging Green Approach to Upcycling Plastic Waste39Precise Defect Engineering on Graphitic Carbon Nitrides for Boosted Solar H2 Production23Synergistic effects of cocatalyst and homojunction/heterojunction with boosted photocatalytic H2 evolution over Zn0.5Cd0.5S/NDs39Novel catalysts in catalytic upcycling of common polymer wastes26Systemically Understanding Aqueous Photocatalytic Upgrading of Microplastic to Fuels11Activation of 2D cobalt hydroxide with 0D cobalt oxide decoration for microplastics degradation and hydrogen evolution23Construction of D-A type porphyrin-phthalocyanine-based polymer hollow tubes for efficient photodegradation and photoelectrochemical sensing of bisphenol A20Recent advancements in synthesis and multi-functional catalytic applications of graphitic carbon nitride9Atomic Ni directional-substitution on ZnIn2S4 nanosheet to achieve the equilibrium of elevated redox capacity and efficient carrier-kinetics performance in photocatalysis36Recent advances in semiconductor heterojunctions: a detailed review of the fundamentals of photocatalysis, charge transfer mechanism and materials537Solar-driven photocatalysis for recycling and upcycling plastics122Encapsulation of carbon-nanodots into metal-organic frameworks for boosting photocatalytic upcycling of polyvinyl chloride plastic80Insights into Photogenerated Carrier Dynamics and Overall Water Splitting of the CrS 3 /GeSe Heterostructure70An innovative 2D/2D Bi5O7Br/NiFe-LDH Z-scheme heterojunction for enhanced photoreduction CO2 activity27Achieving long-lived shallow trapping states in carbon nitride through the n-π*electronic transition for enhanced photocatalytic hydrogen generation99Efficient photocatalytic production of H2O2 and photodegradation of tetracycline by CdS/square tubular g-C3N4 S-scheme heterojunction photocatalyst122S-vacancy-assisted fast charge transport and oriented ReS 2 growth in twin crystal Zn x Cd 1− x S: an atomic-level heterostructure for dual-functional photocatalytic conversion14Excavating the Potential of Photo‐ and Electroupcycling Platforms Toward a Sustainable Future for Waste Plastics11Green synthesis of 3D core–shell SnS 2 /SnS-Cd 0.5 Zn 0.5 S multi-heterojunction for efficient photocatalytic H 2 evolution4Recent advancement on photocatalytic plastic upcycling90Exposure of Facets to Control Built in Electric Field and Boost Efficient Photodegradation of Br-Cu2o@Nife-Ldhs Heterojunction1Photochemical upcycling and recycling of plastics: achievements and future opportunities56Polyoxometalate-encapsulated metal–organic frameworks for photocatalytic uranium isolation33Hierarchical structures of 2D g-C3N4 sheet supported 3D star-shaped flower CuO nanohybrids for improved photoelectrochemical water oxidation and visible light induced photodegradation of antibiotics21Enhanced Generation and Effective Utilization of Cr(V) for Simultaneous Removal of Coexisting Pollutants via MOF@COF Photocatalysts22Plastic Waste Conversion by Leveraging Renewable Photo/Electro‐Catalytic Technologies27Photo- and electrochemical processes to convert plastic waste into fuels and high-value chemicals45A Unified View of Carbon Neutrality: Solar-Driven Selective Upcycling of Waste Plastics30Photoreforming for microplastics recycling: A critical review26Efficient photocatalytic CO2 reduction achieved by constructing Bi4O5Br2/Bi-MOF Z-scheme heterojunction31Oxygen Vacancies Trigger Rapid Charge Transport Channels at the Engineered Interface of S‐Scheme Heterojunction for Boosting Photocatalytic Performance290Oxygen Vacancies Trigger Rapid Charge Transport Channels at the Engineered Interface of S‐Scheme Heterojunction for Boosting Photocatalytic Performance32From biomass to fuel: Advancing biomass upcycling through photocatalytic innovation13Photocatalysis toward Microplastics Conversion: A Critical Review148Recent advances in polyolefinic plastic pyrolysis to produce fuels and chemicals60Single Dispersion of Fe(H2O)2‐Based Polyoxometalate on Polymeric Carbon Nitride for Biomimetic CH4 Photooxidation34An Overview of the Sustainable Depolymerization/Degradation of Polypropylene Microplastics by Advanced Oxidation Technologies33Photorefinery of Biomass and Plastics to Renewable Chemicals using Heterogeneous Catalysts96Photorefinery of Biomass and Plastics to Renewable Chemicals using Heterogeneous Catalysts4Photocatalytic Cracking of non‐Biodegradable Plastics to Chemicals and Fuels1Photocatalytic Cracking of non‐Biodegradable Plastics to Chemicals and Fuels16Photocatalytic Upcycling of Different Types of Plastic Wastes: A Mini Review7How to determine whether an electron transfer channel is type-II or S-scheme in g–C3N4–based photocatalysts? A critical review30Construction of Br-Cu2O@NiFe-LDHs Z-scheme heterojunction and photocatalytic degradation of catechol13Catalytic Upcycling of Polyolefins316Enhancing photocatalytic nitrogen fixation via electrostatic self-assembly Z-scheme PMoV/NH2–MIL-125 heterojunction: Improved carrier separation through built-in electric field and synergistic effects13Progress on Photo‐, Electro‐, and Photoelectro‐Catalytic Conversion of Recalcitrant Polyethylene, Polypropylene, and Polystyrene ‐ A Review11Visible-light driven S-scheme Bi2WO6/graphitic carbon nitride heterojunction for efficient simultaneous removal of TC and Cr(VI)6Lighting the Way to Greener Solutions: Photocatalytic Breakthroughs in Plastic Degradation0Photocatalytic Degradation of Microplastics: Mechanism, Recent Developments, and Associated Threats0Photocatalytic Perception for Degradation of Macro- and Micro-plastics2Photocatalytic Plastic Degradation and Upcycling into Valuable Chemicals1Plastic Degradation and Conversion by Photocatalysis10Plastic Degradation and Conversion by Photocatalysis (Volume 2): From Waste to Wealth3Plastic Degradation by Photocatalysis: Basic Concepts and General Mechanisms8Solar Light-Assisted Photocatalytic Conversion of Plastics into Hydrogen and Value-Added Chemicals0Plastic‐to‐Treasure: Innovative advances in photo/electro‐catalytic upcycling technologies for commodity chemicals and fuels15Polyoxometalate-incorporated ZnIn2S4 z-scheme heterojunction with enhanced light-driven hydrogen production performances5Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4Application of photocatalytic technology in the treatment and disposal of waste plastics: a review12Circular plastic economy for sustainable development: current advances and future perspectives49Photocatalytic upcycling of polylactic acid to alanine by sulfur vacancy-rich cadmium sulfide103Effect of TiO2 Morphology on the Properties and Photocatalytic Activity of g-C3N4/TiO2 Nanocomposites Under Visible-Light Illumination20Selective Liquid Chemical Production in Waste Polyolefin Photorefinery by Controlling Reactive Species26Recycling homocarbon backbone polymers toward a circular materials economy12Catalytic conversion of polymer waste into high-value products for advancing circular economy and eco-sustainability11Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design Principles73A Mind Map to Address the Next Generation of Artificial Photosynthesis Experiments3Photocatalytic conversion of polystyrene under mild conditions using surface-modified BiOBr/g-C3N4 heterojunction with strong interfacial interactions33Plastic pollutants: From wastes to fuels and high-value chemicals8Visible-light driven phosphotungstic acid/tubular C3N4 heterojunction photocatalyst for efficient cleavage of C–C bond in lignin5Photocatalytic Upcycling of Plastic Waste Into Value‐Added Chemicals21Floatable organic-inorganic hybrid-TiO2 unlocks superoxide radicals for plastic photoreforming in neutral solution56The crystal structure of bis(tetramethylammonium) (di-μ2-aqua)hexaaqua-dibarium(II)) decavanadate0Efficient Z -scheme photocatalytic hydrogen production from overall water splitting by M A 2 Z 4 / X Se 2 ( M = Zn , Cd , Hg ; A = Al , Ga , In ; Z = S , Se , Te ; X = Ti , Zr , Hf ) heterostructures15Photoreforming for upcycling of plastics into energy, chemicals and materials: a review7State-of-the-Art Achievements and Challenges in Photochemical Conversion of Plastics to Chemicals and Composites6Ambient solar thermal catalysis for polyolefin upcycling using copper encapsulated in silicon nanosheets and chloroaluminate ionic liquid32Synergistic Engineering of Zinc Vacancies and Er‐Doping in ZnIn 2 S 4 Nanosheets for Enhanced CO 2 Photoreduction via Optimized Charge Dynamics21Solar-driven conversions of plastic waste to valuable chemicals with green hydrogen production4Synergizing Zinc vacancy engineering and electron-rich polyoxometalates in ZnIn2S4 for solar-light-driven hydrogen evolution with boosted charge dynamics5Addressing the plastic waste crisis: Advanced catalytic strategies for upcycling and fuel production6Heterogeneous photocatalysis as an efficient process for degrading MPs/NPs in aqueous media: A systematic review18Sustainable Treatment of Plastic Wastes with Photocatalytic Technologies: A Review7Polyoxometalates modified g-C3N4 promotes efficient photocatalytic cleavage of C−C bond in lignin model compounds3Upcycling C–O Bond Polymers into Value‐Added Chemicals with Air as the Sole Oxidant2Engineering functional nanocomposites for enhanced AOP-mediated microplastic mineralization: From mechanistic insights to water remediation strategies3Trash‐to‐Energy: Shedding Light on Plastic and Biomass Valorization Through Artificial Photosynthesis Towards Sustainability14Advances and Outlook of In Situ Characterization Techniques for Photocatalytic Reforming of Plastic Wastes5MXene photocatalysts for microplastics degradation under simulated solar illumination3Interfacial P-O-Cu Bonds Drive Rapid Z-Scheme Charge Transfer for Efficient Photocatalytic O2 Evolution Synchronized with Cr(VI) Reduction3Polyoxometalate-based donor–acceptor-type photocatalytic-active cluster: Exploring structure–activity relationships in oxidation of alkylbenzene C(sp 3 )–H bond via ligand design10Catalytic cascade depolymerization for sustainable recycling of waste polyvinyl chloride28Degradation and utilization of polyvinyl chloride (PVC): Challenges and opportunities toward a circular economy24Photoinduced metastable-charging of d-orbital electrons of Re centers enhances interfacial charge migration behavior for efficient coupling conversion0Recent advances in photocatalytic plastic degradation and upcycling: Catalysts, experiments, and mechanisms9Synergistic 3d-5d orbital interactions on oxygen vacancy-rich Pt/TiO2 for enhanced photothermal catalytic oxidation of propylene4Direct Z-scheme photocatalytic water splitting in SnC-based chalcogenide heterostructures: mechanistic insights and hydrogen evolution performance8Highly efficient upcycling of plastic waste upon Bi-modified P-doped g-C3N4: Plasmonic effect-dominated Schottky barrier tuning8Cooperatively boosting C–C coupling and proton reduction upon bismuth-based Z-scheme dual-functional photocatalyst1Regulating free radical species towards selective photocatalytic acetic acid synthesis from polylactic acid plastic over sulfur-doped BiVO4/In2S3 S-scheme heterojunction9Photoreforming of plastic waste into value-added chemicals with hydrogen production4Plastic Upcycling via Artificial Photosynthesis: A Green Conversion From Waste to Value‐Added Chemicals3Vertically channeled aerogel supported CoTiO3/CdS S-scheme heterojunction: Enhanced photocatalytic-PMS synergistic degradation toward PET microplastics0Ultrasensitive colorimetric/fluorescence dual-mode sensing platform based on quasi-NENU-5 for specific detection of glyphosate5Enhanced photocatalytic gaseous acetaldehyde degradation over WO3: Oxidizing vs. non-oxidizing calcination atmosphere1Defect-engineered S-scheme heterojunction boosts X–H bonds activation for synergistic hydrogen production and benzyl alcohol oxidation2Photo-driven upcycling of plastics: pathways to value-added products13D Metal‐Organic Framework‐Based Photocatalysts for Environmental Remediation: Structural Features, Mechanistic Insights, and Emerging Strategies3Single‐Atom Photocatalyst as Floatable Artificial Leaf for Upcycling Oceanic Plastic Waste10Cu-Doped ZnIn2S4 with Sulfur Vacancy Expedites Carrier Separation for Efficient Photocatalytic Hydrogen Evolution2Selective Plastic Photo Upcycling to Acetic Acid via Coupled Oxidation and CO 2 Reduction Over an S‐Scheme g‐C 3 N 4 /Fe 2 O 3 Heterojunction1Chlorine Ion-Enhanced Efficient Photocatalysis of Polyethylene Plastics1Indirect electrocatalytic construction of pyrrolo[1,2-a]quinoxalines catalyzed by V-substituted polyoxometalates0Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3A holistic remedy to the plastic era through a high–performance photocatalytic system0A novel g-C3N4@(H/C-CdS) catalyst based on a microinjection titration-stirring strategy for enhanced visible-light photocatalytic degradation of tetracycline02D/2D heterojunction photocatalysts based on organic semiconductor and g-C3N4 for efficient cleavage of C–C bonds in lignin model compounds0From Nano-(Micro)-Plastics to Value-Added Fuels and Chemicals: A Review of Mechanisms and Future Perspectives on Sonication-Assisted Photocatalytic Upgrading0Recent advances in carbon nitride photocatalysts for multi-phase organic pollutant degradation0Visible-light-driven Bi2WO6/PMo12/g-C3N4 dual Z-scheme heterojunction for high-efficiency organic pollutant degradation: Mechanistic insights and reaction pathways0Design and engineering of heterogeneous photocatalysts for plastic degradation and upcycling0

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