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RESEARCH PAPER · Angewandte Chemie International Edition · 2021

The First Sulfate‐Pillared Hybrid Ultramicroporous Material, SOFOUR‐1‐Zn, and Its Acetylene Capture Properties

Debobroto Sensharma, Daniel J. O’Hearn, Amin Koochaki, Andrey A. Bezrukov, Naveen Kumar, Benjamin H. Wilson, Matthias Vandichel, Michael John Zaworotko

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The First Sulfate‐Pillared Hybrid Ultramicroporous Material, SOFOUR‐1‐Zn, and Its Acetylene Capture PropertiesOriginalA new boron cluster anion pillared metal organic framework with ligand inclusion and its selective acetylene capture properties33A Review on Anion-Pillared Metal Organic Framework (Apmof) and its Composites with the Balance of Adsorption Capacity and Separation Selectivity for Efficient Gas Separation1Boosting C 2 H 2 /CO 2 separation of metal–organic frameworks via anion exchange and temperature elevation30Recent advances in microporous metal–organic frameworks as promising adsorbents for gas separation83Pore space partition of metal-organic frameworks for gas storage and separation119Exploring the coordination chemistry of a low symmetry, bent dipyridyl ligand1A review on anion-pillared metal–organic frameworks (APMOFs) and their composites with the balance of adsorption capacity and separation selectivity for efficient gas separation102Pillar Modularity in fsc Topology Hybrid Ultramicroporous Materials Based upon Tetra(4-pyridyl)benzene8Screening Hoffman-type metal organic frameworks for efficient C2H2/CO2 separation65Formation of a Polar Flow Channel with Embedded Gas Recognition Pockets in a Yttrium-Based MOF for Enhanced C 2 H 2 /C 2 H 4 and CO 2 Selective Adsorptions6Optimizing Acetylene Sorption through Induced‐fit Transformations in a Chemically Stable Microporous Framework50Optimizing Acetylene Sorption through Induced‐fit Transformations in a Chemically Stable Microporous Framework3A Robust Molecular Porous Material for C2H2/CO2 Separation13Recent progress in metal–organic frameworks for the separation of gaseous hydrocarbons29Solubility‐Boosted Molecular Sieving‐Based Separation for Purification of Acetylene in Core–Shell IL@MOF Composites46Highly scalable acid-base resistant Cu-Prussian blue metal-organic framework for C2H2/C2H4, biogas, and flue gas separations53Fe-MOF with U-Shaped Channels for C2H2/CO2 and C2H2/C2H4 Separation31Engineering Pore Environments of Sulfate‐Pillared Metal‐Organic Framework for Efficient C 2 H 2 /CO 2 Separation with Record Selectivity125Metal-organic frameworks for C2H2/CO2 separation: Recent development142Vertex Strategy in Layered 2D MOFs: Simultaneous Improvement of Thermodynamics and Kinetics for Record C 2 H 2 /CO 2 Separation Performance109Highly Productive C3H4/C3H6 Trace Separation by a Packing Polymorph of a Layered Hybrid Ultramicroporous Material46Effective separation of acetylene from carbon dioxide via commensurate adsorption in a microporous metal-organic framework12Topological Design of Unprecedented Metal‐Organic Frameworks Featuring Multiple Anion Functionalities and Hierarchical Porosity for Benchmark Acetylene Separation103Topological Design of Unprecedented Metal‐Organic Frameworks Featuring Multiple Anion Functionalities and Hierarchical Porosity for Benchmark Acetylene Separation27Programmed fluorine binding engineering in anion-pillared metal-organic framework for record trace acetylene capture from ethylene104Crystal engineering of a new platform of hybrid ultramicroporous materials and their C 2 H 2 /CO 2 separation properties16Crystal Engineering of a New Hexafluorogermanate Pillared Hybrid Ultramicroporous Material Delivers Enhanced Acetylene Selectivity9Sulfate-Pillared Adsorbent for Efficient Acetylene Separation from Carbon Dioxide and Ethylene18Thiadiazole-Functionalized Th/Zr-UiO-66 for Efficient C2H2/CO2 Separation21Enabling C2H2/CO2 Separation Under Humid Conditions with a Methylated Copper MOF52Dinuclear Copper Sulfate-Based Square Lattice Topology Network with High Alkyne Selectivity6Molecular sieving of iso-butene from C4 olefins with simultaneous high 1,3-butadiene and n-butene uptakes27Does the Central Nitrogen Atom Make a Difference? A Comparison of Non‐Coordinating Pyridine and Benzene Spacers in Multitopic Ligands4Recent Advances of Multidentate Ligand-Based Anion-Pillared MOFs for Enhanced Separation and Purification Processes44Cross‐Linking CdSO4‐Type Nets with Hexafluorosilicate Anions to Form an Ultramicroporous Material for Efficient C2H2/CO2 and C2H2/C2H4 Separation7Auxiliary ligand influence on interpenetration and C2H2/CO2 separation in NDI based isoreticular MOFs5Metal–Organic Framework with Space-Partition Pores by Fluorinated Anions for Benchmark C2H2/CO2 Separation137Efficient recovery of acetylene from quaternary mixture by a pillar-layer framework with abundant Lewis basic sites16Mechanochemical “Cage‐on‐MOF” Strategy for Enhancing Gas Adsorption and Separation through Aperture Matching41Mechanochemical “Cage‐on‐MOF” Strategy for Enhancing Gas Adsorption and Separation through Aperture Matching4Guest Cation Functionalized Metal Organic Framework for Highly Efficient C 2 H 2 /CO 2 Separation22Compatible alignment of pore electro-fields for enhanced one-step ethylene purification from ternary gas mixtures19One sulfate anion-bridged metal–organic framework for adsorptive separation of C2H2 from C2H4 and CO214Isoreticular Contraction in Dicopper Paddle‐Wheel‐Based Metal‐Organic Frameworks to Enhance C2H2/CO2 Separation0Enabling high C 2 H 2 storage and efficient C 2 H 2 /CO 2 separation in a cage-like MOF with multiple supramolecular binding sites10Xenon Regeneration by CO2 Removal from Exhaled Anesthetic Gas Mixture by a Hybrid Ultramicroporous Material with Customized Nanotrap14A new type of C 2 H 2 binding site in a cis -bridging hexafluorosilicate ultramicroporous material that offers trace C 2 H 2 capture4Ionic porous materials: from synthetic strategies to applications in gas separation and catalysis45Synthesis and structural characterisation of Cu II -based MOFs constructed by combining functionalised 1,4-bis(1 H -imidazol-1-Yl)benzene ligands with copper sulfate3Pore space optimization of hybrid ultramicroporous material for exceptional one-step C2H4 purification from C2H2/CO2/C2H4 mixture13Tailoring Pore Environments in Metal–Organic Frameworks for Efficient C2H2/CO2 and C2H2/C2H4 Separations14Complete Utilization of Ligand Coordination Sites in Co-MOF for C2H2/CO2 Separation9Tuning Pore Chemistry of Metal–Organic Frameworks Using Anionic Pillars for Humid-Tolerant CO 2 Capture9A stable amino-functionalized fluorinated metal–organic framework for efficient separation of propyne/propylene0The Prototypal Diamondoid Topology Hybrid Ultramicroporous Materials and Their Water Vapor Sorption Properties3Multivariate Metal–Organic Cages for Efficient C 2 H 2 /CO 2 Separation4A Low-Cost and Highly Stable K 2 Zn 3 [Fe(CN) 6 ] 2 Framework for Efficient CO 2 /C 2 H 2 Separation ★0Construction of Octadentate Carboxylate‐Based Metal–Organic Framework for Effective Acetylene Purification3Isoreticular design of charge-assisted hydrogen-bonded metal-organic frameworks for efficient C2H2/CO2 separation2Tethered Zn(II) Porphyrin-Quaternary Ammonium Catalysts for Efficient CO₂ Cycloaddition with Epoxides under Atmospheric Pressure0Crystal Engineering of Chelating Hybrid Ultramicroporous Materials via Pillar Modulation for Energy‐Efficient Acetylene Separation0Hierarchical Microporous Anion Pillared Metal–Organic Frameworks (APMOFs) for Gas Separation2Hydrogen‐Bonded Organic Frameworks (HOFs) for C2 Gas Separation and Purification0Temperature-Dependent Gate-Opening Behavior and C2H2/CO2 and C2H2/C2H4 Separation in a 4-Fold Interpenetrated Flexible MOF0Regeneration‐Optimized Chemisorbents: Evaluating Hybrid Coordination Networks for Atmospheric Water Harvesting0

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  1. A new boron cluster anion pillared metal organic framework with ligand inclusion and its selective acetylene capture properties

    Inorganic Chemistry Frontiers · 2022-01-01

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  2. A Review on Anion-Pillared Metal Organic Framework (Apmof) and its Composites with the Balance of Adsorption Capacity and Separation Selectivity for Efficient Gas Separation

    SSRN Electronic Journal · 2022-01-01

    Xufei Li, Hui Bian, Weiqiu Huang, Baoyou Yan, Xinya Wang, Bing Zhu

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  3. Boosting C 2 H 2 /CO 2 separation of metal–organic frameworks via anion exchange and temperature elevation

    Journal of Materials Chemistry A · 2022-01-01

    Ting Wang, Wei Mei, Pengfei Li, Yun‐Lei Peng, Yao Chen, Jian‐Gong Ma, Peng Cheng, Ming Fang, Kuang Yu, Zhenjie Zhang

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  4. Recent advances in microporous metal–organic frameworks as promising adsorbents for gas separation

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    Jia‐Xin Wang, Congcong Liang, Xiao‐Wen Gu, Hui‐Min Wen, Chenghao Jiang, Bin Li, Guodong Qian, Banglin Chen

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  5. Pore space partition of metal-organic frameworks for gas storage and separation

    EnergyChem · 2022-06-30

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  6. Exploring the coordination chemistry of a low symmetry, bent dipyridyl ligand

    Journal of Coordination Chemistry · 2022-07-18

    Nicholas Kyratzis, David R. Turner

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  7. A review on anion-pillared metal–organic frameworks (APMOFs) and their composites with the balance of adsorption capacity and separation selectivity for efficient gas separation

    Coordination Chemistry Reviews · 2022-07-22

    Xufei Li, Hui Bian, Weiqiu Huang, Baoyou Yan, Xinya Wang, Bing Zhu

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  8. Pillar Modularity in fsc Topology Hybrid Ultramicroporous Materials Based upon Tetra(4-pyridyl)benzene

    Crystal Growth & Design · 2022-08-19

    Debobroto Sensharma, Benjamin H. Wilson, Naveen Kumar, Daniel J. O’Hearn, Michael John Zaworotko

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  9. Screening Hoffman-type metal organic frameworks for efficient C2H2/CO2 separation

    Chemical Engineering Journal · 2022-09-18

    Wushuang Lou, Jiahao Li, Wanqi Sun, Yongqi Hu, Lingyao Wang, Rodrigo Neumann Barros Ferreira, Mathias Bernhard Steiner, Zonglin Gu, Binquan Luan, Yuanbin Zhang

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  10. Formation of a Polar Flow Channel with Embedded Gas Recognition Pockets in a Yttrium-Based MOF for Enhanced C 2 H 2 /C 2 H 4 and CO 2 Selective Adsorptions

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    Mingxing Zhang, Penghui Liu, Rui Dang, Hui−Hui Cui, Guomin Jiang, Jin Wang, Miao Wang, Tongming Sun, Minmin Wang, Guoping Qin, Su Wang, Yanfeng Tang

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  11. Optimizing Acetylene Sorption through Induced‐fit Transformations in a Chemically Stable Microporous Framework

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    Jindou Tian, Qihui Chen, Feilong Jiang, Daqiang Yuan, Maochun Hong

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  12. Optimizing Acetylene Sorption through Induced‐fit Transformations in a Chemically Stable Microporous Framework

    Angewandte Chemie · 2022-12-16

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  13. A Robust Molecular Porous Material for C2H2/CO2 Separation

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  14. Recent progress in metal–organic frameworks for the separation of gaseous hydrocarbons

    Materials Chemistry Frontiers · 2023-01-01

    Jing‐Hong Li, Jun-Xian Chen, Rui‐Biao Lin, Xiao‐Ming Chen

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  15. Solubility‐Boosted Molecular Sieving‐Based Separation for Purification of Acetylene in Core–Shell IL@MOF Composites

    Advanced Functional Materials · 2023-01-20

    Jincai Yang, Minman Tong, Guopeng Han, Miao Chang, Tongan Yan, Yunpan Ying, Qingyuan Yang, Dahuan Liu

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  16. Highly scalable acid-base resistant Cu-Prussian blue metal-organic framework for C2H2/C2H4, biogas, and flue gas separations

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  17. Fe-MOF with U-Shaped Channels for C2H2/CO2 and C2H2/C2H4 Separation

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  18. Engineering Pore Environments of Sulfate‐Pillared Metal‐Organic Framework for Efficient C 2 H 2 /CO 2 Separation with Record Selectivity

    Advanced Materials · 2023-03-01

    Xing Liu, Peixin Zhang, Hanting Xiong, Yan Zhang, Ke Wu, Junhui Liu, Rajamani Krishna, Jingwen Chen, Shixia Chen, Zheling Zeng, Shuguang Deng, Jun Wang

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  19. Metal-organic frameworks for C2H2/CO2 separation: Recent development

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  20. Vertex Strategy in Layered 2D MOFs: Simultaneous Improvement of Thermodynamics and Kinetics for Record C 2 H 2 /CO 2 Separation Performance

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  21. Highly Productive C3H4/C3H6 Trace Separation by a Packing Polymorph of a Layered Hybrid Ultramicroporous Material

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  22. Effective separation of acetylene from carbon dioxide via commensurate adsorption in a microporous metal-organic framework

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  23. Topological Design of Unprecedented Metal‐Organic Frameworks Featuring Multiple Anion Functionalities and Hierarchical Porosity for Benchmark Acetylene Separation

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  24. Topological Design of Unprecedented Metal‐Organic Frameworks Featuring Multiple Anion Functionalities and Hierarchical Porosity for Benchmark Acetylene Separation

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  25. Programmed fluorine binding engineering in anion-pillared metal-organic framework for record trace acetylene capture from ethylene

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  26. Crystal engineering of a new platform of hybrid ultramicroporous materials and their C 2 H 2 /CO 2 separation properties

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  27. Crystal Engineering of a New Hexafluorogermanate Pillared Hybrid Ultramicroporous Material Delivers Enhanced Acetylene Selectivity

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  28. Sulfate-Pillared Adsorbent for Efficient Acetylene Separation from Carbon Dioxide and Ethylene

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  29. Thiadiazole-Functionalized Th/Zr-UiO-66 for Efficient C2H2/CO2 Separation

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  30. Enabling C2H2/CO2 Separation Under Humid Conditions with a Methylated Copper MOF

    Advanced Science · 2024-02-26

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  31. Dinuclear Copper Sulfate-Based Square Lattice Topology Network with High Alkyne Selectivity

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  32. Molecular sieving of iso-butene from C4 olefins with simultaneous high 1,3-butadiene and n-butene uptakes

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  33. Does the Central Nitrogen Atom Make a Difference? A Comparison of Non‐Coordinating Pyridine and Benzene Spacers in Multitopic Ligands

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  34. Recent Advances of Multidentate Ligand-Based Anion-Pillared MOFs for Enhanced Separation and Purification Processes

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  35. Cross‐Linking CdSO4‐Type Nets with Hexafluorosilicate Anions to Form an Ultramicroporous Material for Efficient C2H2/CO2 and C2H2/C2H4 Separation

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  36. Auxiliary ligand influence on interpenetration and C2H2/CO2 separation in NDI based isoreticular MOFs

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  37. Metal–Organic Framework with Space-Partition Pores by Fluorinated Anions for Benchmark C2H2/CO2 Separation

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  38. Efficient recovery of acetylene from quaternary mixture by a pillar-layer framework with abundant Lewis basic sites

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  39. Mechanochemical “Cage‐on‐MOF” Strategy for Enhancing Gas Adsorption and Separation through Aperture Matching

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  40. Mechanochemical “Cage‐on‐MOF” Strategy for Enhancing Gas Adsorption and Separation through Aperture Matching

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  41. Guest Cation Functionalized Metal Organic Framework for Highly Efficient C 2 H 2 /CO 2 Separation

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  42. Compatible alignment of pore electro-fields for enhanced one-step ethylene purification from ternary gas mixtures

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  43. One sulfate anion-bridged metal–organic framework for adsorptive separation of C2H2 from C2H4 and CO2

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  46. Xenon Regeneration by CO2 Removal from Exhaled Anesthetic Gas Mixture by a Hybrid Ultramicroporous Material with Customized Nanotrap

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  47. A new type of C 2 H 2 binding site in a cis -bridging hexafluorosilicate ultramicroporous material that offers trace C 2 H 2 capture

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  48. Ionic porous materials: from synthetic strategies to applications in gas separation and catalysis

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  49. Synthesis and structural characterisation of Cu II -based MOFs constructed by combining functionalised 1,4-bis(1 H -imidazol-1-Yl)benzene ligands with copper sulfate

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  50. Pore space optimization of hybrid ultramicroporous material for exceptional one-step C2H4 purification from C2H2/CO2/C2H4 mixture

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