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RESEARCH PAPER · Coordination Chemistry Reviews · 2023

Metal-organic frameworks for C2H2/CO2 separation: Recent development

Xiaokang Wang, Hongyan Liu, Yue Li, Xinlei Yang, Fei Gao, Xiaoqing Wang, Zixi Kang, Weidong Fan, Daofeng Sun

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Metal-organic frameworks for C2H2/CO2 separation: Recent developmentOriginalA viologen-based Cd( ii ) coordination polymer as a multifunctional platform for photochromism, chemochromism and a broad range of fluorescence pH sensing20An Infinite Multi-Walled Ultramicroporous Metal–Organic Framework for Efficient C2h2/Co2 Separation Under Humid Conditions0An ultramicroporous multi-walled metal–organic framework for efficient C 2 H 2 /CO 2 separation under humid conditions19Metal–Organic Frameworks with Lewis Acid-Base Sites as Highly Efficient Catalyst for the Cycloaddition of Carbon Dioxide0Pillar-Layered Strategy to Design and Synthesis of Two Mofs with Excellent C2h2 Capture and C2h2/Co2 Separation Capability0Two Isostructural Metal-Organic Frameworks Based on Tetracarboxylic Ligand for Highly Gas Adsorption and Separation0Pore-structure control in ultramicroporous porous coordination polymers for efficient selective capture of acetylene15Highly Efficient CO2/C2H2 Separation by Porous Graphene via Quadrupole Gating Mechanism9Effective separation of acetylene from carbon dioxide via commensurate adsorption in a microporous metal-organic framework12Fe‐Based Metal‐Organic Frameworks: From Various Synthesis, Diverse Structures to Multifunctional Applications29Synthesis of metal organic frameworks based on multiazole ligands for adsorption and separation of acetylene1Active Sites Decorated Nonpolar Pore‐Based MOF for One‐step Acquisition of C 2 H 4 and Recovery of C 3 H 680Active Sites Decorated Nonpolar Pore‐Based MOF for One‐step Acquisition of C2H4 and Recovery of C3H64Metal-organic framework-based nanomaterials for CO 2 storage: A review28Solvent‐Directed Construction of a Nanoporous Metal‐Organic Framework with Potential in Selective Adsorption and Separation of Gas Mixtures Studied by Grand Canonical Monte Carlo Simulations12Synthesis of a Carbazole-Based Nanoporous Organic Polymer for Efficient Adsorption/Separation of C2H2 and CO211Nanoporous Cu(II)-Adenine-Based Metal–Organic Frameworks for Selective Adsorption of C2H2 from C2H4 and CO226Metal–organic frameworks with Lewis acid-base sites as highly efficient catalyst for the cycloaddition of carbon dioxide20Separation of High-Purity C 2 H 2 from Binary C 2 H 2 /CO 2 Using Robust Al-Based MOFs Comprising Nitrogen-Containing Heterocyclic Dicarboxylate26A Zn( ii ) pillared-layer ultramicroporous metal–organic framework with matching molecular pockets for C 2 H 2 /CO 2 separation0Boosting Acetylene Packing Density within an Isoreticular Metal–Organic Framework for Efficient C2H2/CO2 Separation22Pillar-Layered strategy to design and synthesis of two MOFs with excellent C2H2 capture and C2H2/CO2 separation capability34Thiadiazole-Functionalized Th/Zr-UiO-66 for Efficient C2H2/CO2 Separation21Cu/Fe-MOFs based on mixed ligands: Synthesis, crystal structure and electrocatalytic hydrogen evolution performance14A review on CO2 capture over novel adsorbents: Progress in robust zeolite adsorbent development8Supramolecular Interactions Induce Dynamics in Metal–Organic Layers to Selectively Separate Acetylene from Carbon Dioxide6Efficient C2H2/CO2 separation in two 2-fold interpenetrating metal-organic frameworks with ultrahigh C2H2 packing density15Flow Channel with Wrinkles and Calcium Sites in a Ca-MOF for Direct One-Step Ethylene Purification from C2 Gases and MTO Products Separation14Influence of Pressure and Temperature on the Flexible Behavior of Iron-Based MIL-53 with the CO2 Host: A Comprehensive Experimental and DFT Study8Optimized separation of C2H2 from binary mixtures of C2H2/CO2 and C2H2/C2H4 by coordinative copper(I) metal nodes modified from HKUST-118Cationic Europium–Organic Framework for Chromatographic Column Separation of Ionic Dyes and Stimuli-Responsive Chromic Properties7Deciphering Mechanisms of CO 2 -Selective Recognition over Acetylene within Porous Materials25Reverse Separation of Carbon Dioxide and Acetylene in Two Isostructural Copper Pyridine‐Carboxylate Frameworks15Reverse Separation of Carbon Dioxide and Acetylene in Two Isostructural Copper Pyridine‐Carboxylate Frameworks51Agricultural waste to environmental purifier: Application and mechanism of aminated pomelo peel for adsorption of anionic dyes and Cr(VI)14Extra-High CO2 Adsorption and Controllable C2H2/CO2 Separation Regulated by the Interlayer Stacking in Pillar-Layered Metal–Organic Frameworks15An adenine-based metal-organic framework with tailored pore environment for adsorption separation of C2H2 from C2H4 and CO214Interpenetrated In(III)-MOF with Multiple Recognition Sites for Single-Step Ethylene Purification4Crystal structures, Hirshfeld surface analyses and optical properties of four new Cu(II)-based coordination polymers0Building Stable Pillar-Layered Metal–Organic Frameworks: Introduction of Unsaturated Bonds for Enhanced Efficiency in C2H2/CO2 Separation19Viologen-Based Photochromic Metal–Organic Framework for Antibiotics Detection in Water22A novel “pore-carrier transfer” strategy for preparation of porous liquids toward efficient CO2 capture25Ultrastable Carboxyl‐Functionalized Pore‐Space‐Partitioned Metal‐Organic Frameworks for Gas Separation66Asymmetrical Modification of Cyclopentadienyl Cobalt in Eu-MOF for C2H2/CO2 Separation10Efficient molecular sieving separation of C2H2/CO2 by a flexible interpenetrated metal-organic framework22Mechanochemical “Cage‐on‐MOF” Strategy for Enhancing Gas Adsorption and Separation through Aperture Matching41Mechanochemical “Cage‐on‐MOF” Strategy for Enhancing Gas Adsorption and Separation through Aperture Matching4A microporous fluorinated MOF for efficient separation of C2H2 from C2H2/CO2 and C2H2/C2H4 mixtures21A Stable Layered Microporous MOF Assembled with Y–O Chains for Separation of MTO Products39Controlling Guest Diffusion by Local Dynamic Motion in Soft Porous Crystals to Separate Water Isotopologues and Similar Gases40One sulfate anion-bridged metal–organic framework for adsorptive separation of C2H2 from C2H4 and CO214Functionalization of Covalent Organic Frameworks with Cyclopentadienyl Cobalt for C 2 H 2 /CO 2 Separation31Functionalization of Covalent Organic Frameworks with Cyclopentadienyl Cobalt for C 2 H 2 /CO 2 Separation13Enabling high C 2 H 2 storage and efficient C 2 H 2 /CO 2 separation in a cage-like MOF with multiple supramolecular binding sites10Efficient inverse CO 2 /C 2 H 2 separation driven by difference in rare thermodynamic affinities in a porous MOF9Rational design of stable carbon nitride monolayer membranes for highly controllable CO 2 capture and separation from CH 4 and C 2 H 27Solvent-induced metal-organic framework for enhanced CO2/CH4 separation: Synthesis, characterization, and mechanism analysis1Opposite trends in acetylene/ethylene selectivity change after organic functionalization of Na+- and Cs+-MOR zeolites2A Chemically Robust Microporous Zn‐MOF for C 2 H 2 Separation from CO 2 and Industrially Relevant Four Component Gas Mixtures37A 2d Robust Microporous Cu-Mof for Efficient Separations for C2h2/Co2/Ch4 Mixtures0A Lewis basic site rich metal–organic framework featuring a hydrogen-bonded acetylene nano-trap for the efficient separation of C 2 H 2 /CO 22Construction of indium–organic frameworks with flu -topology for efficient acetylene separation0Integrating Artificial Intelligence in CO2 Capture and Conversion Processes for Sustainable Energy Solutions3Steric hindrance regulation in hydrogen-bonded organic frameworks: from nonporous to microporous5The Adsorption and Light Hydrocarbon Separation Performance for the Scalable Synthesis of Microporous Cu-Mof0Two stable 2D indium(III)/zirconium(IV) metal-organic frameworks for highly efficient C2H2/CO2 separation0Imidazole-Functionalized Zn-MOFs for One-Step C2H4 Purification from C2H2/C2H4/C2H6 Ternary Mixture24Enhancing Ethylene/Acetylene selective separation in hydrogen-bonded organic framework by modulating pore polarity with Bis-Quinoxaline unit5Engineering the Pore Size and Environment of Pillar-Layered Zinc-Azolate-Carboxylate Frameworks for Efficient CH4 Purification and C2H2/CO2 Separation3One new Co-MOF with F sites in the pores for selective C 2 H 2 adsorption over CO 2 and CH 43Single-Step Ethylene Purification and MTO Product Separation in a Nitrogen-Rich Microporous Metal–Organic Framework14Efficient enhancement of CO2 separation and capture of the T-C3N2 membranes with modulations of strain, charge, and their synergistic effect8Reversed CO2/C2H2 separation via combined adsorption kinetics and diffusion differences in MOF-polymer mixed matrix membrane15Effective physical methods for aflatoxin B1 removal in food: A comprehensive review28A pillar-layered MOF bearing N/O sites for one-step purification of C2H4 from the mixtures with C2H6 or C3H616Breakthrough developments in Metal-Organic frameworks (MOFs) for efficient C4 hydrocarbon separation27Solvent Regulation in Layered Zn-MOFs for C2H2/CO2 and CO2/CH4 Separation4Pore environment optimization of In-MOFs by pore space partition strategy for one-step C2H4 purification from C2H6/C2H4 mixtures8Cu-Based Metal–Organic Frameworks Characterized by V-Shaped Ligands and Application to Efficient Separation of C2H2/CO2 and C2H2/CH46Benchmarking selective capture of trace CO2 from C2H2 using an amine-functionalized adsorbent47The adsorption and light hydrocarbon separation performance for the scalable synthesis of microporous Cu-MOF7A stable scandium(III) metal-organic framework with introduced nitrate ions for enhancing C2H6/C2H4 selectivity in the separation of MTO products5A Rigid, Stable, and Scalable Aliphatic MOF Adsorbent for Efficient C 2 H 2 /CO 2 Separation with Record Acetylene Packing Density35A Rigid, Stable, and Scalable Aliphatic MOF Adsorbent for Efficient C2H2/CO2 Separation with Record Acetylene Packing Density10Two novel [CuxIy]n-based MOFs with high BET surface area for efficient MTO products separation15Overlapping-ligand strategy in copper-paddlewheel supramolecular isomers for enhanced stability and efficient C2H2/CO2 separation4Efficient Kinetic Separation of Carbon Dioxide from Acetylene Using Mordenites Featuring Modified 1D Channels with Excellent Selectivity and Diffusion18Metallic deep eutectic solvent derived chiral carbon dots functionalized MOF@silica composite: A new and highly efficient column packing material29Industrially‐Driven Ultramicroporous Physisorbent with a Trifecta of Customized Functions for Upgrading C 2 H 2 /CO 2 Separation Performance10C 2 H 2 /CO 2 Separation by a Carborane Hybrid 2D Metal–Organic Framework6Zero- to One-Dimensional Transformation in a Highly Porous Metal–Organic Framework to Enhance Physicochemical Properties20Bioinspired Water-Stable Sc-MOF with Amino-Barb Vigreux-Type Channels for One-Step Ethylene Purification2Halide-regulated Mercury (II) coordination polymers showing diverse electrochemical biosensing toward penicillin0Adsorptive Separation of C1–C2 Hydrocarbons in COFs by Microenvironment Modulation16Rugged Cages with Narrow Connecting Channels in a Water-Stable Cu-MOF for One-Step Ethylene Purification and MTO Product Separation7Complete Utilization of Ligand Coordination Sites in Co-MOF for C2H2/CO2 Separation9Simultaneously tuning the pore size and structural softness on flexible metal-organic frameworks for enhanced CO2/C2H2 separation15A cage-based MOF with twf-d topology exhibiting selective C H adsorption4Thermally Induced Topological Isomers of Metal–Organic Frameworks for Enhanced C2H2 Separation from CO2 and C2H41Two-in-One Flexible Metal–Organic Framework: One-Step C 2 H 4 Purification via Inverse C 2 H 6 –C 2 H 4 and C 2 H 2 –CO 2 Separations50Unlocking the Comparative Potential of Porous Frameworks: A Review on MOFs and COFs for Gas Sorption11A 2D robust microporous Cu-MOF for efficient separations for C2H2/CO2/CH4 mixtures4Tailoring a sulfonic metal–organic framework with fluorinated ultramicroporous environments for C2H2/CO2 separation3Pore engineering in metal-organic frameworks for one-step ethylene purification from ternary C2H2/C2H4/C2H6 mixtures6An Extraordinary Stable and Ultramicroporous Y-MOF for Propylene/Ethylene Separation and Knoevenagel Condensation5Ultramicroporous Pyridine-Carboxylate MOFs for Temperature-Adaptive C 2 H 2 /CO 2 Separation via Gate-Opening Sieving1Inverse CO 2 ‐C 2 H 2 Separation on the Low‐Silica CHA Zeolite Through Cooperative Cation and Gas Molecule Migration Mechanism1Inverse CO 2 ‐C 2 H 2 Separation on the Low‐Silica CHA Zeolite Through Cooperative Cation and Gas Molecule Migration Mechanism5Covalent Nitrogen Doped Hypercross-Linked Polymer from Waste Plastic for Greenhouse Gas Adsorption0Electrostatic Potential Gradient Modulation by Organic Cations in Zeolite for Efficient C 2 H 2 /CO 2 Separation18Achieving high-performance acetylene/carbon dioxide separation via green and scalable synthesis of high-density cobalt-based MOF7One‐Dimensional Channel with Side Pockets for Rapid Diffusion and Efficient C 2 H 2 Purification5One‐Dimensional Channel with Side Pockets for Rapid Diffusion and Efficient C 2 H 2 Purification2A tetrazole-functionalized Cu-MOF for efficient C 2 H 2 /CO 2 separation0Allyl-Functionalized ZrT-1 for C2H2/CO2 Separation0CO 2 -selective metal–organic frameworks for one-step C 2 H 2 purification2Fluorine-engineered two-dimensional covalent organic frameworks for enhanced C 2 H 2 /CO 2 separation2Functionalization of benzothiadiazole in magnesium-based metal–organic framework for C 2 H 2 /CO 2 separation0Multivariate MOF-303/MIL-160 balancing the trade-off between capacity and selectivity in CO 2 /CH 4 separation2Structural dimensionality governing CO 2 /C 2 H 2 separation in MWW zeolites2Molecular trap construction via pore environment optimization in ultramicroporous MOFs for efficient C2H2 separation2Synthesis and structure of two 2D In(III)/Zr(IV)‑MOFs with highly efficient C2H2/CO2 separation0Precise Pore Engineering of a Pillar-Layered MOF via the Dual-Ligand Strategy for C 2 H 2 /CO 2 Separation4Insights into the adsorptive separation of CO2 from light hydrocarbons in LTA-type zeolites: Density functional theory calculations and classical molecular simulations1An anion-pillared ultra-microporous MOF with synergistic binding sites for efficient C2H2/CO2 separation2Cinnamon sticks-derived N-doped activated carbons with tailored aperture environment for efficient adsorption and separation of C2H2/CO2 and C2H4/CO22Hydroxyl-functionalized Ni7-cluster-based MOF for cost-effective acetylene separation0Tetrazole-Decorated Ultramicroporous MOF Exhibiting Inverse CO 2 Selectivity for Hydrocarbon Purification1A new topological Cu-MOF constructed via ligand desymmetrization strategy for natural gas liquids separation0“Two‐in‐One” Anion Engineering Strategy for One‐Step Ethylene Purification From a Ternary Mixture0“Two‐in‐One” Anion Engineering Strategy for One‐Step Ethylene Purification From a Ternary Mixture1Engineering modulations in a versatile aluminum-based CAU-1 structure for C2H2 separation from C2H2/CO2 gas mixture0Novel Carborane Based Metal Organic Framework for Record Electronic Specialty Gas C 2 F 6 Purification via Molecular Sieving1Novel Carborane Based Metal Organic Framework for Record Electronic Specialty Gas C 2 F 6 Purification via Molecular Sieving0Heptanuclear Fluorido-Bridged Cobalt Metal−Organic Frameworks Containing BF4− Counteranions for Highly Selective C2H2/CO2 Separation0Aqueous-mediated eco-friendly fabrication of furan dicarboxylate Zr-MOF decorated silica stationary phase for advanced chromatographic separations0Solid-state structural transformations and gate-opening adsorption in a flexible cobalt metal-organic framework0Cage-Confined BF4– Counteranions Generate Fluorine-Rich Microenvironments for C2H2/CO2 Separation in Isostructural Co/Ni-MOFs0Temperature-Dependent Gate-Opening Behavior and C2H2/CO2 and C2H2/C2H4 Separation in a 4-Fold Interpenetrated Flexible MOF0A Rigid–Flexible Zn-DMOF with Dynamic Pore Recognition for Enhanced C2H2/CO2 Separation0Pretreatment-free conversion of spent FCC catalyst into low-silica CHA for K+-gated inverse CO2/C2H2 separation0

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  3. An ultramicroporous multi-walled metal–organic framework for efficient C 2 H 2 /CO 2 separation under humid conditions

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  4. Metal–Organic Frameworks with Lewis Acid-Base Sites as Highly Efficient Catalyst for the Cycloaddition of Carbon Dioxide

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  5. Pillar-Layered Strategy to Design and Synthesis of Two Mofs with Excellent C2h2 Capture and C2h2/Co2 Separation Capability

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  7. Pore-structure control in ultramicroporous porous coordination polymers for efficient selective capture of acetylene

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  8. Highly Efficient CO2/C2H2 Separation by Porous Graphene via Quadrupole Gating Mechanism

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  10. Fe‐Based Metal‐Organic Frameworks: From Various Synthesis, Diverse Structures to Multifunctional Applications

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  11. Synthesis of metal organic frameworks based on multiazole ligands for adsorption and separation of acetylene

    Chinese Science Bulletin (Chinese Version) · 2023-09-01

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  12. Active Sites Decorated Nonpolar Pore‐Based MOF for One‐step Acquisition of C 2 H 4 and Recovery of C 3 H 6

    Angewandte Chemie International Edition · 2023-09-07

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  30. Optimized separation of C2H2 from binary mixtures of C2H2/CO2 and C2H2/C2H4 by coordinative copper(I) metal nodes modified from HKUST-1

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  32. Deciphering Mechanisms of CO 2 -Selective Recognition over Acetylene within Porous Materials

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  33. Reverse Separation of Carbon Dioxide and Acetylene in Two Isostructural Copper Pyridine‐Carboxylate Frameworks

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  35. Agricultural waste to environmental purifier: Application and mechanism of aminated pomelo peel for adsorption of anionic dyes and Cr(VI)

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