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RESEARCH PAPER · Advanced Optical Materials · 2021

Trade‐off Lattice Site Occupancy Engineering Strategy for Near‐Infrared Phosphors with Ultrabroad and Tunable Emission

Tianchun Lang, Mingsheng Cai, Shuangqiang Fang, Tao Han, Shuangshuang He, Qunyi Wang, Guanghui Ge, Jun Wang, Chaozhong Guo, Lingling Peng, Shixiu Cao, Bitao Liu, Vladimir I. Korepanov, Аlexey N. Yakovlev, Jianbei Qiu

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Trade‐off Lattice Site Occupancy Engineering Strategy for Near‐Infrared Phosphors with Ultrabroad and Tunable EmissionOriginalA near-infrared phosphor doped with Cr3+ towards zero-thermal-quenching for high-power LEDs56Spectral engineering and thermometric performance of LiIn(Si2-Ge )O6: Cr3+ phosphor for multi-mode NIR thermometry26Highly Efficient and Stable Near‐Infrared Broadband Garnet Phosphor for Multifunctional Phosphor‐Converted Light‐Emitting Diodes118Multiple Strategies to Approach High-Efficiency Luminescence Controllable in Blue/Cyan/Green-Emitting Bi 3+ -Activated Phosphors30Efficient, Stable, and Ultra‐Broadband Near‐Infrared Garnet Phosphors for Miniaturized Optical Applications89Long persistent luminescence property of green emitting Sr3Ga4O9: Tb3+ phosphor for anti-counterfeiting application20Ultra‐Wide Vis–NIR Mg2Al4Si5O18:Eu2+,Cr3+ Phosphor Containing Unusual NIR Luminescence Induced by Cr3+ Occupying Tetrahedral Coordination for Hyperspectral Imaging66Spectral Regulation and Efficiency Optimization in Cr3+‐Doped Gadolinium Aluminum Gallium Garnet Near‐Infrared Ceramic Phosphors via Crystal‐Field Engineering29Advances in Chromium‐Activated Phosphors for Near‐Infrared Light Sources489Enhanced Thermal Stability and Energy Transfer by Crystal‐Field Engineering in a Garnet Phosphor for Thermometry and NIR‐LED48Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting89Luminescence properties and phase transformation of broadband NIR emitting A2(WO4)3:Cr3+ (A=Al3+, Sc3+) phosphors toward NIR spectroscopy applications16Enhanced cyan emission via competitive site occupancy engineering in Sr2SiO4:Eu2+ phosphor for achieving full-spectrum LED lighting19Site-Selective Occupancy Control of Cr Ions toward Ultrabroad-Band Infrared Luminescence with a Spectral Width up to 419 nm79Site-selective occupation of Cr3+ ions toward ultra-broadband near-infrared emission stannate phosphors23Recent Advances in Chromium‐Doped Near‐Infrared Luminescent Materials: Fundamentals, Optimization Strategies, and Applications252Super Broadband Near‐Infrared Solid Solution Phosphors with Adjustable Peak Wavelengths from 1165 to 875 nm for NIR Spectroscopy Applications41Broadening of the near-infrared emission band of the Mg 2 Al 4 Si 5 O 18 :Cr 3+ phosphor for illumination emission applications12Highly efficient and thermally stable broadband near-infrared emitting garnet Ca 3 Sc 2 Ge 3 O 12 :Cr 3+ ,Ce 3+ phosphors for multiple pc-LED applications33Inducing octahedral distortion to enhance NIR emission in Cr-doped garnet Ca 3 (Al, Sc) 2 Ge 3 O 1249Influence of framework disordering on the luminescence performance of Cr 3+ -doped near-infrared phosphors: a case study of A 3 B 6 O 14 -type hosts8Spectroscopically enhanced far-red phosphor Li 2 Mg 3 TiO 6 :Cr 3+ and its application prospects to the cold resistance of rice6Color tunable (Ba,Ca)ScO2F: Eu2+, Bi3+, K+ perovskite with dependence of excitation wavelength for advanced anti-counterfeiting application9Tunable-Color UV-Excitation Sb3+/(Bi3+, Ag+)-Doped Cs2NaInCl6 Perovskite for High-Color-Rendering Full-Spectrum w-LEDs15Recent Advances in Multi-Site Luminescent Materials: Design, Identification and Regulation20Anti-thermal-quenching in Zn1-Li Ga2O4-δ:Cr3+ phosphor for plant cultivation and optical thermometer based on defect engineering30The co-optimization of efficiency and emission bandwidth in GSAGG:Cr3+ NIR ceramic phosphors19Recent Advances in Light-Conversion Phosphors for Plant Growth and Strategies for the Modulation of Photoluminescence Properties47Near-Infrared LuCa 2 ScZrGa 2 GeO 12 :Cr 3+ Garnet Phosphor with Ultra-broadband Emission for NIR LED Applications60Study on the mechanism of high energy transfer efficiency of blue light excited Cr 3+ , Nd 3+ co-doped near infrared phosphors8Ultra-broadband near-infrared phosphor La2CaTa Zr(1-)O6:Cr3+ for phosphor-converted light-emitting diodes30The ultra-wideband near-infrared luminescence properties and applications of K2SrGe8O18:Cr3+ phosphor26Multiple defects induced near-infrared self-luminescence of (Ca,Sr)LaMgTaO6 double perovskite phosphor29Hetero-valent substitution induced luminescence enhancement of Zn1-Ga2+O4+δ:Cr3+ near infrared phosphors for plant cultivation12Structure modulation induced luminescence improvement in Gd3-Y Ga5O12:Cr3+ deep-red phosphors for dragon fruit cultivation15Optimizing interstitial site luminescence via a sensitizer strategy towards green synthesis of Mn4+-activated fluoride phosphors0Valence conversion and site reconstruction in near-infrared-emitting chromium-activated garnet for simultaneous enhancement of quantum efficiency and thermal stability161High‐Performance NIR Emission in Chromium‐Doped Garnet Phosphors Enabled by Structure and Excitation Regulation67A novel self-activated near-infrared luminescence of BaLaMgTaO6 phosphor13Achieving Luminescence of Sr3Ga1.98In0.02Ge4O14:0.03Cr3+ via [In3+] Substitution [Ga3+] and Its Application to NIR pc-LED in Non-Destructive Testing5Engineering deep-red Al20B4O36:Cr3+ phosphors for photomorphogenesis9Compositional modulation induced broadband NIR luminescence enhancement in A2ScNbO6:Cr3+ (A = Ba, Sr)12High external quantum yield in near-infrared phosphor Bi2Ga4O9:Cr3+ excited by near-ultraviolet or blue light9Small Stokes Shift and Two‐Site Occupation in the ANb2O6:Cr3+ (A = Zn/Mg) Phosphors Toward Highly Efficient Ultra‐Broadband Near‐Infrared Emission for Multifunctional Applications24A post-reduction strategy to enhance near-infrared-II emission from Li 4 SrCa(SiO 4 ) 2 :Cr 4+ phosphors11Broadband short-wave near-infrared-emitting phosphor MgNb 2 O 6 :Cr 3+ for pc -LED applications9Efficient and stable near-infrared Y 2 Mg 2 Al 2 Si 2 O 12 :Cr 3+ phosphor: analysis of the luminescence source by a site elimination strategy35Long-wavelength near-infrared light emitting Ni 2+ -doped double perovskite molybdate-based solid-solution phosphors43Blueshift and Photoluminescence Enhancement in Broadband Near‐Infrared Emitting Phosphor NaSr2(Al/Ga)Ge5O14: Cr3+ Dependence on the Sc/In Substitution40Tailoring the Cr3+ Emission via Combinatorial Management of Crystal‐Field and Energy Transfer for Multiple NIR LEDs30Mechanism analysis on manipulation of long afterglow luminescence properties of Y3Al5-xGaxO12:Ce3+, Cr3+ phosphors10UV- and X-ray-activated broadband NIR garnet-type Ca3Ga2Sn3O12:Fe3+ phosphors with efficient persistent luminescence34Dual substitution of host lattice ions to enhance the luminescence properties of Zn2TiO4:Cr3+ phosphor3Near‐infrared emitting metal halide materials: Luminescence design and applications78Broadband emitting Mg3Lu2Ge3O12:Cr3+ phosphors with garnet structure for high-performance NIR LEDs applications25Ultraviolet-B and Near-Infrared Dual-Band Luminescence in Bi 3+ /Bi 2+ Codoped Persistent Phosphor for Optical Storage Application46Cr3+ activated Gd3Sc2Al3O12 garnet phosphor ceramic with broadband emissions and enhanced thermal stability toward high-power near-infrared LED/LD16Heterostructure anion-groups guided design enabling customizable Eu2+ spectrum behavior in borophosphate7Co-training machine learning enables interpretable discovery of near-infrared phosphors with high performance16A novel highly efficient Eu3+-doped germanate red phosphor for accurate latent fingerprint detection and WLED applications33Achieving a Balance of Good Quantum Efficiency and Thermal Stability in the Y2CaScAl3GeO12:Cr3+ Broadband Phosphor for Multiple NIR Spectroscopy Applications17Developing an efficient garnet-type near-infrared phosphor Na 1.5 Gd 1.5 Sc 2 Ge 3 O 12 :Cr 3+ with relatively long-wavelength emission10Achieving Flat Ultra‐Broadband NIR Emission in Cr 3+ Doped Garnet‐Type Phosphors Enabled by Structural Regulation Toward Multi‐Functional Spectroscopy Applications51Near‐Infrared Broadband Emission for High Electroluminescence Efficiency by Cr3+/In3+‐Doped Germanate Phosphors0Persistent Luminescence for Night‐Time Individual Identification Based on Quantum Tunneling13Achieving Thermally Stable YAl3–xGax(BO3)4:Cr3+ Near-Infrared Emitting Phosphors via Chemical Substitution for Plant Growth LEDs23A Novel Multifunctional and Broadband Near‐Infrared Phosphor, Lu 3 MgGa 3 GeO 12 :Cr 3+ , Yb 3+ , Nd 3+ Achieved through a Chemical Unit Substitution and Energy Transfer Strategy23Enhancement of luminescence properties of broadband NIR Cr3+-activated phosphate phosphors through cationic substitution11Diving into the invisible region—a review of crystallographic-site-dependent ultraviolet and near-infrared luminescence of the garnet structure5Strategies for broadening the emission spectra of Cr 3+ -doped near-infrared emitting phosphors59Improving the near-infrared luminescence of Ca3MgSnGe3O12:Cr3+ using cation modulation and energy transfer for night-vision and nondestructive testing1Highly efficient and thermal stable near-infrared-emitting glass ceramic by optimizing Na2SrXGe5O14: Cr3+ (X = Si, Ge, Ti) phosphors4Chemical pressure effect on the magnetic properties of the S = 1 2 structural screw chain antiferromagnets A Co 2 ( Te 3 O 8 ) ( SO 4 ) ( A = Hg , Cd )1Simultaneous enhancement of quantum efficiency and thermal stability through double cation substitution (Sr2+→Lu3+, Ge4+→Al3+) in garnet structure for NIR pc-LED3Lithiation-Driven Phase Engineering Unlocking Broadband NIR Emission in Cr-Doped Zinc Tantalate1Efficient and broadband near-infrared emitting Ca2YHf2Ga3O12: Cr3+ phosphor for anti-counterfeiting applications8High purity red emitting CaLaGaO4:Eu3+ nanophosphors: Applications in w-LEDs and forensic fingerprint detection with YOLOv8x framework7Enhancement of NIR Luminescence Properties in Li 3 Cs 2 Sr 2 B 3 P 6 O 24 : Cr 3+ Phosphor via Yb 3+ Co‐Doping for Spectroscopy Applications3Chromium Ion Pairs Induce Highly Efficient and Thermostable Broadband NIR Phosphor for Plant Lighting and Night Vision12Structure and luminescence of Gd3Ga3MgSiO12:Cr3+ garnet phosphor with highly efficient broadband near-infrared emitting toward pc-LED application7Comparative Study of Cr 3+ -Activated Garnet Ca 2 YZnMGe 3 O 12 (M = Sc, In) Phosphors: Ultraefficient Near-Infrared Luminescence and Structure–Property Relationships1Dual‐Site Cooperative Regulation Strategy Enables High‐Performance Near‐Infrared Luminescence and Wireless Communication Applications of Cr 3+ Activated Garnet Phosphors9Multimode luminescence tailoring in Sb/Mn/Yb Co-doped scandium-based double perovskites exhibiting ultra-broadband warm white emission for multifunctional applications4Achieving high-performance near-infrared Cr3+-activated phosphor via A&C lattice sites cosubstitution strategy in garnet for plant lighting6Efficient and thermal stable broadband near-infrared emitting Gd2CaAl3GaZrO12:Cr3+ garnet phosphor: structure, luminescence, and pc-LED application9Growth, thermal, spectroscopy and mid-infrared laser performance of an Er:LuGSGG mixed crystal0Highly efficient and ultra-broadband visible to near-infrared luminescence in all-inorganic scandium-based double perovskite for multifunctional photoelectric applications0Dual-functional Cr 3+ -doped far-red to NIR broadband phosphors for high-fidelity white lighting and non-destructive detection0Garnet‐Structured Near‐Infrared Luminescent Materials: Luminescence Fundamentals, Regulation and Applications14Recent advances in Cr 3+ -doped near-infrared phosphors: preparation, luminescence, and LED applications5Ultra-efficient broadband NIR garnet phosphor via Ca2+-Sn4+/In3+-Al3+ double ion pair synergistical-substitution for multifunctional pc-LED applications in plant growth and night vision biological detection and information encryption0High‐Efficiency FWHM‐Variable NIR II Phosphor Mg 4 Al 4.5 Ga 2.45 B 1.05 O 16 : Cr 3+ with Excellent Thermal Stability6Structure-distortion-induced efficient and tunable NIR-II emission in Cr3+–Ni2+ co-doped garnet phosphor for pc-LED applications2Structure and Luminescence Regulation in Y 3 Al 5 O 12 :Cr 3+ via Cation Substitution to Achieve Broadband Near-Infrared Emitting Garnet Phosphor6Site Occupation Strategy for Tunable Ultra‐Broadband Emission in Cr 3+ ‐Doped Near‐Infrared Phosphors and High‐Efficiency Optoelectronic Applications1Thermodynamic Stabilization and Cr 3+ Luminescence Tuning in Gd 3 Al 5 O 12 Garnet Phosphor via Multi‐Cation Incorporation4Garnet-structured Y2CaGa4ZrO12:Cr3+ NIR phosphor with combined high efficiency and thermal stability toward constructing high-performance pc-NIR-LED1Near-infrared phosphor development and broad-range regulation of Cr3+ luminescence via Ca2+/Si4+ incorporation in Y3Ga3Al2O12 garnet0

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