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RESEARCH PAPER · Angewandte Chemie International Edition · 2021

Introducing Intermolecular Cation‐π Interactions for Water‐Stable Low Dimensional Hybrid Lead Halide Perovskites

Tariq Sheikh, Shabnum Maqbool, Pankaj K. Mandal, Angshuman Nag

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Introducing Intermolecular Cation‐π Interactions for Water‐Stable Low Dimensional Hybrid Lead Halide PerovskitesOriginalChemically Spiraling CsPbBr3 Perovskite Nanorods88Third Harmonic Upconversion and Self-Trapped Excitonic Emission in 1D Pyridinium Lead Iodide29Te4+-doped Cs2InCl5·H2O single crystals for remote optical thermometry88“Plenty of Room” at the Interface of Hybrid Metal Halide Perovskite Single Crystals19Selective Luminescence Response of a Zero-Dimensional Hybrid Antimony(III) Halide to Solvent Molecules: Size-Effect and Supramolecular Interactions72Potential lead toxicity and leakage issues on lead halide perovskite photovoltaics359Force‐Reversible and Energetic Indole‐Mg‐Indole Cation‐π Interaction for Designing Toughened and Multifunctional High‐Performance Thermosets63Water-Molecule-Induced Emission Transformation of Zero-Dimension Antimony-Based Metal Halide79Iodine–Iodine Interactions Suppressing Phase Transitions of 2D Layered Hybrid (I-(CH 2 ) n -NH 3 ) 2 PbI 4 ( n = 2–6) Perovskites37Chiral 2D organic–inorganic hybrid perovskites based on l -histidine9Getting the details right: optical, dielectric, and vibrational outcomes of structural phase transition in one-dimensional pyrrolidinium lead iodide and the role of defects6Using chiral ammonium cations to modulate the structure of 1D hybrid lead bromide perovskites for linearly polarized broadband light emission at room temperature19Water-stable and hydrophobicity tunable organolead halide materials with Pb–N coordination for electrochemical CO 2 reduction12Triple Passivation Approach to Laminate Perovskite Layers for Augmented UV and Ambient Stable Photovoltaics12Robust Self‐Assembled Molecular Passivation for High‐Performance Perovskite Solar Cells54Robust Self‐Assembled Molecular Passivation for High‐Performance Perovskite Solar Cells19Zero‐Dimensional Organic Copper(I) Iodide Hybrid with High Anti‐Water Stability for Blue‐Light‐Excitable Solid‐State Lighting114Enhancing the Intrinsic and Extrinsic Stability of Halide Perovskite Nanocrystals for Efficient and Durable Optoelectronics112Challenges and Strategies to Design Phosphors for Future White Light Emitting Diodes105Bright Cyan‐Emissive Copper(I)‐Halide Single Crystals for Multi‐Functional Applications98The passage of alkali metal cations through the pores in phenine and N-doped phenine nanotubes4Ultrastable 0D Organic Zinc Halides with Highly Efficient Blue Light Emissions59Ultra‐Sensitive, Selective and Repeatable Fluorescence Sensor for Methanol Based on a Highly Emissive 0D Hybrid Lead‐Free Perovskite35Ultra‐Sensitive, Selective and Repeatable Fluorescence Sensor for Methanol Based on a Highly Emissive 0D Hybrid Lead‐Free Perovskite165Zero‐Dimensional Zn‐Based Halides with Ultra‐Long Room‐Temperature Phosphorescence for Time‐Resolved Anti‐Counterfeiting28Zero‐Dimensional Zn‐Based Halides with Ultra‐Long Room‐Temperature Phosphorescence for Time‐Resolved Anti‐Counterfeiting200Dibenzo‐18‐Crown‐6‐Assisted Inhibition of Cation Migration for Stable Perovskite Solar Cells16Picolylamine Isomers Trigger Multidimension Coupling Strategy toward Efficient and Stable Inorganic Perovskite Solar Cells4Advanced hydrogen adsorption on benzene: Cation-π interaction effects5Exciton Dynamics in Colloidal CdS Quantum Dots with Intense and Stokes Shifted Photoluminescence in a Single Decay Channel20Highly Stable and Moisture-Immune Monocomponent White Perovskite Phosphor by Trifluoromethyl (-CF3) Regulation11Releasable Water Charge‐Trapping and Water‐Resistant Photodetection using 1D Perovskitoid Hydrate Single Crystal28Expanding the absorption and photoresponse of 1D lead–halide perovskites via ultrafast charge transfer9Modulating Resonance Energy Transfer with Supramolecular Control in a Layered Hybrid Perovskite and Chromium Photosensitizer Assembly5Optimizing Broadband Emission in 2D Halide Perovskites43Organic‐inorganic Hybrid Perovskite‐Based Light‐Assisted Li‐oxygen Battery with Low Overpotential17Noncrystalline Hybrid Lead Halides with Liquid-Polymer Characteristics5[PPh 3 H] 2 [SbCl 5 ]: A Zero-Dimensional Hybrid Metal Halide with a Supramolecular Framework and Stable Dual-Band Emission54Enhanced power conversion efficiency of perovskite solar cells using dopant-free carbon nanotubes-Spiro-OMeTAD27Oxidation-induced phase transformations of hybrid tin bromide single crystals enable the occurrence of second-harmonic generation14Pivotal Role of A-Site Cations in Tailoring the Band-Edge States, Optical Properties, and Stability of 0D Hybrid Indium Chlorides212D nanosheets of layered double perovskites: synthesis, photostable bright orange emission and photoluminescence blinking9Fabricating a type II heterojunction by growing lead-free perovskite Cs 2 AgBiBr 6 in situ on graphite-like g-C 3 N 4 nanosheets for enhanced photocatalytic CO 2 reduction24Industrial perspectives on the upscaling of perovskite materials for photovoltaic applications and its environmental impacts3Recent advances in synthesis of water-stable metal halide perovskites and photocatalytic applications32Various approaches to synthesize water-stable halide PeNCs17Combining π-Conjugation and Cation−π Interaction for Water-Stable and Photoconductive One-Dimensional Hybrid Lead Bromide28Enhanced efficiency and stability of perovskite solar cells achieved by incorporating potassium cation-18-crown ether-6 complexes71D Diisopropylammonium Lead Iodide Perovskite Shows Exceptional Optical Stability and Third‐Order Nonlinearity16Non-covalent interactions involving π effect between organic cations in low-dimensional organic/inorganic hybrid perovskites20Layered B2O3/CsPbBr3 perovskite composite embedded using glass as microreactor with enhanced stability and high-efficiency light extraction23Novel 3D Cubic Topology in Hybrid Lead Halides with a Symmetric Aromatic Triammonium Exhibiting Water Stability4A step towards RoHS compliance for perovskite devices by using a novel lead-capturing encapsulant2A New Class of Donor‐π‐Acceptor Phosphonium Salt Exhibiting Intriguing Thermally Activated Delayed Fluorescence15All-Inorganic Lead-Free Doped-Metal Halides for Bright Solid-State Emission from Primary Colors to White Light20Understanding Microstructural Development of Perovskite Crystallization for High Performance Solar Cells29Intra- and Intermolecular Cation–π Interactions between Onium Salts and Alkynes/Acetylene: Experimental and Theoretical Insights5Guidelines for Designing Water‐Stable Hybrid Lead Bromide Perovskites with Broad Emission11Band Structure Optimized by Electron‐Acceptor Cations for Sensitive Perovskite Single Crystal Self‐Powered Photodetectors7Acquiring Bulk Photovoltaic Effect in One-Dimensional Sn-Based Perovskite Single Crystals by Nonlinear Organic Diamine14A resonance spacer cation-based heterostructure enables efficient and stable perovskite solar cells3Chemically driven dimensionality modulation of hybrid tin( ii ) halide perovskite microcrystals11Passivation Effect of Potassium Cation-18-Crownether-6 On Fapbi 3 (001) Perovskite Surface: A First-Principles Study0Recent advances in organolead halide crystalline materials for photocatalytic H 2 evolution and CO 2 reduction applications5Solvent assisted shape dependent MAPbI 3 /polyfluorene heterostructures with a larger surface area for improved photocatalytic H 2 evolution4The effect of precursor concentrations on the structure and optoelectronic properties of quasi low-dimensional hybrid 2-methylpyridinium lead bromide crystalline phases11Water-stable zero-dimensional hybrid zinc halide modulated by π–π interactions: efficient blue light emission and third-order nonlinear optical response11Cation-π interactions enabled water-stable perovskite X-ray flat mini-panel imager68Enhancing the Water‐Stability of 1D Hybrid Manganese Halides by a Cationic Engineering Strategy41Chlorophyl-Passivated Ytterbium-Doped Perovskite Quantum-Cutting Film for High-Performance Solar Energy Conversion and Near-Infrared Light-Emitting Diode Applications4Reversible CsPbBr 3 ↔ CsPb 2 Br 5 Transformation via Reverse Micellar Aqueous Solution12Harnessing strong aromatic conjugation in low-dimensional perovskite heterojunctions for high-performance photovoltaic devices60Halide Exchange in Perovskites Enables Bromine/Iodine Hybrid Cathodes for Highly Durable Zinc Ion Batteries67Harnessing Pb–S Interactions for Long‐Term Water Stability in Cesium Lead Halide Perovskite Nanocrystals29π–π Stacking at the Perovskite/C 60 Interface Enables High‐Efficiency Wide‐Bandgap Perovskite Solar Cells29Bulk Photovoltaic Effect Induced by Non‐Covalent Interactions in Bilayered Hybrid Perovskite for Efficient Passive X‐Ray Detection8Wafer-Scale Patterning Integration of Chiral 3D Perovskite Single Crystals toward High-Performance Full-Stokes Polarimeter90Crystal-Rigidifying Strategy in Hybrid Manganese Halide to Achieve Narrow Green Emission and High Structural Stability18Revival of Degraded CsPbI 3 Nanocrystals by Diselenide Ligand and Nanocrystal Self‐Assembly on Nanofibrilar Ligand Template8Unprecedented hybrid lead bromides featuring trivalent aromatic cation for potential photodetection0Exploring the Therapeutic Potential of 5-Fluorouracil-Loaded Calcium Carbonate Nanoparticles Combined with Natural Compound Thymoquinone for Colon Cancer Treatment28Organic–Inorganic Hybrid Halide X-ray Scintillator with High Antiwater Stability15Synchronously Improved Multiple Afterglow and Phosphorescence Efficiencies in 0D Hybrid Zinc Halides With Ultrahigh Anti‐Water Stabilities93Synchronously Improved Multiple Afterglow and Phosphorescence Efficiencies in 0D Hybrid Zinc Halides With Ultrahigh Anti‐Water Stabilities5Conjugated diamine cation based halide perovskitoid enables robust stability and high photodetector performance22One-Dimensional Red Light–Emissive Organic Manganese(II) Halides as X-Ray Scintillators17Dual-phase Cs4PbBr6/CsPbBr3 perovskite quantum dot borosilicate glass for WLED applications7Conformational Disordering of Organic Cations during Moisture-Induced Structural Collapse in Organic–Inorganic Hybrid Perovskites7Precise Modification of Organic Cations to Enhance the Moisture Stability and Luminescence Efficiency of Mn-Based Halides6Chiral Metal‐Free Anti‐Perovskite with Strong Chiroptical Nonlinearity13Chiral Metal‐Free Anti‐Perovskite with Strong Chiroptical Nonlinearity23Direct Crystallographic Observation of Obvious Structural Deformation in a Lead Halide Framework Induced by Host–Guest Interactions5Crucial impact of degrees of freedom on the pressure-induced optical properties of water-stable 1D perovskites0Effect of ring substituent position on the structural and optoelectronic properties of novel quasi low-dimensional hybrid 2-, 3-, and 4-(bromomethyl)pyridinium lead bromides9Ionothermal synthesis of a hybrid cuprous(I) iodide scintillator with efficient cyan emission and high antiwater stability23Passivation Effect of Potassium Cation-18-Crownether-6 On Fapbi 3 (001) Perovskite Surface: A First-Principles Study0A comprehensive SCAPS-1D simulation study on the photovoltaic properties and efficiency enhancement of CH3NH3PbCl3 perovskite solar cells27Broad‐Temperature Optical Thermometry via Dual Sensitivity of Self‐Trapped Excitons Lifetime and Higher‐Order Phonon Anharmonicity in Lead‐Free Perovskites22Broad‐Temperature Optical Thermometry via Dual Sensitivity of Self‐Trapped Excitons Lifetime and Higher‐Order Phonon Anharmonicity in Lead‐Free Perovskites6Ultra‐stable and Sensitive X‐ray Detectors Using 3D Hybrid Perovskitoid Single Crystals10Biomimetic Parallel Vein-like Two-Dimensional Supramolecular Layers Containing Embedded One-Dimensional Conduits Driven by Cation−π Interaction and Hydrogen Bonding to Promote Photocatalytic Hydrogen Evolution23Passivation effect of potassium cation-18-crownether-6 on FAPbI3(001) perovskite surface: a first-principles study4Chemical Composition Regulation for Tuning the Luminescent Properties of Organic–Inorganic Metal Halides7Broad Orange Emission from Piperazine-Based Layered Halide Perovskites0Chiral Perovskite Single Crystals: Toward Promising Design and Application7Hybrid Cuprous(I) Iodide Scintillator with Ultra-High Water Resistance for Underwater X-ray Imaging16Thermochromic Fluorescence of Bi 3+ /Sb 3+ Co‐Doped (Ph 3 S) 2 InCl 5 Flexible Composites for Optical Temperature Sensing12Bright luminescence from nontoxic Cs3Cu2X5 (X = Cl, Br, I) films prepared by chemical vapor deposition6Lattice Anchoring Stabilizes α-FAPbI3 Perovskite for High-Performance X-Ray Detectors19Enhancing Perovskite Solar Cell Stability and Performance via Bulk Passivation with Sulfonium‐Based Passivators4Cation‐π/π–π Synergy Induced Self‐Assembly of Semiconductor Spacers for High Efficiency and Stable 2D/3D Perovskite Solar Cells21Cation Engineering Enhanced Moisture Resistance in Centimeter‐Sized Lead‐Free Halide Perovskite Crystal for Ultrastable X‐Ray Detection0Highly Efficient Noble‐Metal Free Photocatalytic Hydrogen Generation Using Water‐Stable 4,4′‐Vinylenedipyridine‐Based Halide Perovskites2Manganese-Doped Low-Dimensional Cadmium Halide for Excitation-Dependent Multicolor Emitting8Structural Engineering for Chirality-Induced Spin Control in Metal–Halide Perovskites10Halogen-bond induced polar multilayer hybrid perovskites for efficient self-driven X-ray detection3Efficient visible-light photocatalytic degradation of rhodamine B dye based on water-stable (4,4′-VDP)Pb 2 Br 6 perovskites1Multi‐Level Waterproofing Strategy Toward an Ultra‐Water‐Stable 2D Luminescent Copper(I) Iodide: From Atomic‐Level Passivation to Surface‐Interface Hydrophobicity1How to Slow Down the Phase Transformation of CsPbBr 3 Nanocrystals in an Aqueous Medium? Playing with Metal-Ion Hydration Energy0Bonding Mechanisms Underpinning Structural and Electronic Properties of Halide Perovskites2Scaled synthesis, thin-film fabrication and photophysical characterization of a highly luminescent green-emitting hybrid Cu( i ) iodide0Structural and optoelectronic properties of quasi-1D hybrid 3-halogenopyridinium lead bromides0Tuning charge transfer in water-stable hybrid metal halide single crystals for high-efficiency X-ray scintillation through enhanced intracrystalline coordination interactions and π–π stacking0Phosphonium-Based Metal Halide Semiconductors: When a Single Atom Dictates Water and Thermal Stability2BiO(IO 3 ) with Ultrahigh Effective Atomic Number and Density for Sensitive and Stable Hard X‐Ray Detection0Photosensitive Halide Semiconductors Enabled by Electron Reservoirs From Extended Viologens0Halide Perovskite Photocatalysts in Action: Integrating Photostability, Solvent Robustness, and Surface Charge Management5Near-unity quantum yield blue hybrid cuprous halide with high water resistance for multiple applications5HI‐Mediated In Situ Nitro Reduction and Film Optimization Enable High‐Performance Water‐Stable Quasi‐1D Perovskite Photodetectors0Designing Stable Nanoarchitectonics of Metal Halide Perovskite‐Based Materials for Aqueous Electrocatalysis3Sulfonium-Ligand-Regulated Crystallization Interfacial Dynamics Enables Near-Infrared Perovskite Light-Emitting Diodes with 27% EQE0Cation-π anchoring enabled intimate interfacial coupling of 2D linear conjugated polymer/inorganic heterojunctions for efficient photocatalytic hydrogen evolution0Low-Dimensional Perovskites and Metal Halides across Structures and Functions: Connectivity, Dimensionality, and Emerging Principles1Strong Hydrogen Bond Interaction Induced Dimensional Evolution in Aromatic Diammonium-Based Perovskite/Perovskitoid for Achieving High-Performance X-ray Detection0Lateral Self-Assembly of 1D Supramolecular Columns into Ordered 2D Assemblies Enables In-Plane Hole Delocalization for Photocatalytic O2 Evolution0Exceptionally Water‐Stable Hybrid Metal Halides via Divide‐and‐Conquer Strategy for Anti‐Counterfeiting and X‐Ray Imaging0

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