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RESEARCH PAPER · Inorganic Chemistry · 2020

From S–O–S to B–O–S to B–O–B Bridges: Ba[B(S2O7)2]2 as a Model System for the Structural Diversity in Borosulfate Chemistry

Philip Netzsch, Florian Pielnhofer, Henning A. Höppe

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From S–O–S to B–O–S to B–O–B Bridges: Ba[B(S2O7)2]2 as a Model System for the Structural Diversity in Borosulfate ChemistryOriginalDie ersten zwei Bismutborosulfate – eines davon enthält Oxonium und ein tektosilicatanaloges Anion8The First Bismuth Borosulfates Comprising Oxonium and a Tectosilicate‐Analogous Anion27Sr[B2(SO4)3(S2O7)]: A Borosulfate with an Unprecedented Chain Structure Comprising Disulfate Groups18Ag[B(S2O7)2]: The First Transition Metal Borosulfate Featuring Disulfate Groups13Starke Lewis‐ und Brønsted‐saure Zentren im Borosulfat Mg3[H2O→B(SO4)3]26Strong Lewis and Brønsted Acidic Sites in the Borosulfate Mg3[H2O→B(SO4)3]218Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units102Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units9Ba 2 B 5 O 8 (OH) 2 (NO 3 )·3H 2 O: the design of an alkaline earth metal borate-nitrate optimized from a hydroxylic borate4Polymorphism and optical, magnetic and thermal properties of the either phyllo- or inosilicate-analogous borosulfate Cu[B 2 (SO 4 ) 4 ]8Targeting Diverse Bridging Motifs within Actinide Borosulfates and Establishing an Unconventional Structural Hierarchy1The Unconventional Cadmium Borosulfates Cd[B2O(SO4)3] and Cd4[B2O(SO4)6]4Metal to non-metal sites of metallic sulfides switching products from CO to CH4 for photocatalytic CO2 reduction267A review of photocatalytic CO2 reduction: exploring sustainable carbon emission mitigation from thermodynamics to kinetics and strategies for enhanced efficiency30Li2NaB3S2O12: A Deep-UV Transparent Borosulfate with Moderate Birefringence Derived from the [B3S2O12]∞ Infinite Chain Designed by the High Boron-to-Sulfur Ratio Strategy6Na 2 PbB 6 O 10 SO 4 and Ca 2.58 Pb 0.42 B 6 O 11 SO 4 : first borate–sulfates featuring 3D porous borate anionic frameworks0Die ersten Antimon‐Borosulfate offenbaren das Baukastensystem M III M I [B(SO 4 ) 2 ] 4 (M III =Bi 3+ , Sb 3+ , Lu 3+ ; M I =H 3 O + , NO 2 + , Li + , Na + , K + , Rb + , Cs + )0The First Antimony Borosulfates Unveil a Modular System M III M I [B(SO 4 ) 2 ] 4 (M III =Bi 3+ , Sb 3+ , Lu 3+ ; M I =H 3 O + , NO 2 + , Li + , Na + , K + , Rb + , Cs + )7Low-temperature oxidation of hexagonal boron nitride during oxidative dehydrogenation reactions7Covalent oxygen BO -M catalysts for the oxidative dehydrogenation of propane3Variability of a Non‐Centrosymmetric Tecto‐Borosulfate: Introduction of Various Molecular Cations into BiX[B(SO 4 ) 2 ] 4 (X = H 3 O + , NO 2 + , NH 4 + , NO + )5Synthesis and Crystal Structure of Rb[B(SO 4 ) 2 ]: A Borosulfate Obtained from a Reaction with Chlorosulfuric Acid0Mössbauer Spectroscopy on Antimony Borosulfates Reveals Weak Coordination Behavior1Mößbauer‐Spektroskopie an Antimon‐Borosulfaten belegt deren schwache Koordinationskraft1Significant Enhancement of Birefringence Resulting from the Introduction of [BO 2 (OH)] Groups into Borosulfates0Gas-phase BOx species govern oxidative dehydrogenation of propane over boron-based catalysts0Borosulfates Hosting Se 4 2+ Ions—Crystal Structures, Chemical Bonding, Optical Spectroscopy, and Magnetism0Borosulfates Hosting Se 4 2+ Ions—Crystal Structures, Chemical Bonding, Optical Spectroscopy, and Magnetism0

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  1. Die ersten zwei Bismutborosulfate – eines davon enthält Oxonium und ein tektosilicatanaloges Anion

    Angewandte Chemie · 2020-10-07

    Matthias Hämmer, Lkhamsuren Bayarjargal, Henning A. Höppe

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  2. The First Bismuth Borosulfates Comprising Oxonium and a Tectosilicate‐Analogous Anion

    Angewandte Chemie International Edition · 2020-10-07

    Matthias Hämmer, Lkhamsuren Bayarjargal, Henning A. Höppe

    Read original paper ↗ ·

  3. Sr[B2(SO4)3(S2O7)]: A Borosulfate with an Unprecedented Chain Structure Comprising Disulfate Groups

    Inorganic Chemistry · 2020-11-26

    Philip Netzsch, Henning A. Höppe

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  4. Ag[B(S2O7)2]: The First Transition Metal Borosulfate Featuring Disulfate Groups

    European Journal of Inorganic Chemistry · 2020-12-30

    Philip Netzsch, Henning A. Höppe

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  5. Starke Lewis‐ und Brønsted‐saure Zentren im Borosulfat Mg3[H2O→B(SO4)3]2

    Angewandte Chemie · 2021-03-10

    Philip Netzsch, Regina Stroh, Florian Pielnhofer, Ingo Krossing, Henning A. Höppe

    Read original paper ↗ ·

  6. Strong Lewis and Brønsted Acidic Sites in the Borosulfate Mg3[H2O→B(SO4)3]2

    Angewandte Chemie International Edition · 2021-03-10

    Philip Netzsch, Regina Stroh, Florian Pielnhofer, Ingo Krossing, Henning A. Höppe

    Read original paper ↗ ·

  7. Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units

    Angewandte Chemie International Edition · 2021-10-09

    Zi‐Jian Li, Wenqi Jin, Fangfang Zhang, Zilong Chen, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  8. Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units

    Angewandte Chemie · 2021-10-09

    Zi‐Jian Li, Wenqi Jin, Fangfang Zhang, Zilong Chen, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  9. Ba 2 B 5 O 8 (OH) 2 (NO 3 )·3H 2 O: the design of an alkaline earth metal borate-nitrate optimized from a hydroxylic borate

    Dalton Transactions · 2021-12-20

    Huaiyu Hu, Junben Huang, Zhiyong Guo, Min Zhang, Zhihua Yang, Shilie Pan

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  10. Polymorphism and optical, magnetic and thermal properties of the either phyllo- or inosilicate-analogous borosulfate Cu[B 2 (SO 4 ) 4 ]

    Dalton Transactions · 2022-01-01

    Matthias Hämmer, Florian Pielnhofer, Oliver Janka, Hirotaka Takahashi, Peter Groß, Rainer Pöttgen, Henning A. Höppe

    Read original paper ↗ ·

  11. Targeting Diverse Bridging Motifs within Actinide Borosulfates and Establishing an Unconventional Structural Hierarchy

    Inorganic Chemistry · 2022-09-01

    Teagan F. M. Sweet, Daniel E. Felton, Jennifer E. S. Szymanowski, Peter Carman Burns

    Read original paper ↗ ·

  12. The Unconventional Cadmium Borosulfates Cd[B2O(SO4)3] and Cd4[B2O(SO4)6]

    Zeitschrift für anorganische und allgemeine Chemie · 2022-09-02

    Matthias Hämmer, Henning A. Höppe

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  13. Metal to non-metal sites of metallic sulfides switching products from CO to CH4 for photocatalytic CO2 reduction

    Nature Communications · 2023-10-04

    Yao Chai, Yuehua Kong, Min Lin, Wei Lin, Jinni Shen, Jinlin Long, Rusheng Yuan, Wenxin Dai, Xuxu Wang, Zizhong Zhang

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  14. A review of photocatalytic CO2 reduction: exploring sustainable carbon emission mitigation from thermodynamics to kinetics and strategies for enhanced efficiency

    Journal of the Korean Ceramic Society · 2024-02-21

    Hassan Akbar, Muhammad Subhan Javed, Syeda Tehreem Iqbal, Muhammad Iftikhar Khan, Tauseef Anwar, Faiza Anjum, Ashfaq Ahmad, Muhammad Muneeb, Asghar Ali, Won‐Chun Oh

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  15. Li2NaB3S2O12: A Deep-UV Transparent Borosulfate with Moderate Birefringence Derived from the [B3S2O12]∞ Infinite Chain Designed by the High Boron-to-Sulfur Ratio Strategy

    Inorganic Chemistry · 2024-10-07

    Zichang Wang, Jianyi Zuo, Qing‐Yu Liu, Xueling Hou, Minqiang Gai

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  16. Na 2 PbB 6 O 10 SO 4 and Ca 2.58 Pb 0.42 B 6 O 11 SO 4 : first borate–sulfates featuring 3D porous borate anionic frameworks

    Inorganic Chemistry Frontiers · 2025-01-01

    Huan Pei, Zi‐Jian Li, Shaohuan Liu, Xueling Hou, Fangfang Zhang

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  17. Die ersten Antimon‐Borosulfate offenbaren das Baukastensystem M III M I [B(SO 4 ) 2 ] 4 (M III =Bi 3+ , Sb 3+ , Lu 3+ ; M I =H 3 O + , NO 2 + , Li + , Na + , K + , Rb + , Cs + )

    Angewandte Chemie · 2025-02-12

    Erich Turgunbajew, Henning A. Höppe

    Read original paper ↗ ·

  18. The First Antimony Borosulfates Unveil a Modular System M III M I [B(SO 4 ) 2 ] 4 (M III =Bi 3+ , Sb 3+ , Lu 3+ ; M I =H 3 O + , NO 2 + , Li + , Na + , K + , Rb + , Cs + )

    Angewandte Chemie International Edition · 2025-02-12

    Erich Turgunbajew, Henning A. Höppe

    Read original paper ↗ ·

  19. Low-temperature oxidation of hexagonal boron nitride during oxidative dehydrogenation reactions

    Scientific Reports · 2025-07-01

    Mehran Sajad, Kateřina Knotková, Roman Bulánek, Ota Bludský, Miroslav Rubeš

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  20. Covalent oxygen BO -M catalysts for the oxidative dehydrogenation of propane

    Journal of the Taiwan Institute of Chemical Engineers · 2025-09-11

    Xiaoqing Xu, Yuhan Sun, Xiangze Yu, Rui Huang, Renjie Ji, Jiale Xu, Jianxiang Li, Ruifan Zhou, Qiang Zhang, Xiaoyu Yan

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  21. Variability of a Non‐Centrosymmetric Tecto‐Borosulfate: Introduction of Various Molecular Cations into BiX[B(SO 4 ) 2 ] 4 (X = H 3 O + , NO 2 + , NH 4 + , NO + )

    Chemistry - A European Journal · 2025-10-05

    Erich Turgunbajew, Matthias Hämmer, Lkhamsuren Bayarjargal, Florian Pielnhofer, Henning A. Höppe

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  22. Synthesis and Crystal Structure of Rb[B(SO 4 ) 2 ]: A Borosulfate Obtained from a Reaction with Chlorosulfuric Acid

    Zeitschrift für anorganische und allgemeine Chemie · 2025-10-11

    Jasper Nickelsen, Arthur Edelmann, Marios Symeonidis, Jörn Bruns

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  23. Mössbauer Spectroscopy on Antimony Borosulfates Reveals Weak Coordination Behavior

    Angewandte Chemie International Edition · 2025-12-12

    Erich Turgunbajew, Gwendolyn Buchner, Aylin Koldemir, Theresa Block, Rainer Pöttgen, David Hemker, Richard Dronskowski, Henning A. Höppe

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  24. Mößbauer‐Spektroskopie an Antimon‐Borosulfaten belegt deren schwache Koordinationskraft

    Angewandte Chemie · 2025-12-12

    Erich Turgunbajew, Gwendolyn Buchner, Aylin Koldemir, Theresa Block, Rainer Pöttgen, David Hemker, Richard Dronskowski, Henning A. Höppe

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  25. Significant Enhancement of Birefringence Resulting from the Introduction of [BO 2 (OH)] Groups into Borosulfates

    Chemistry of Materials · 2026-03-04

    Luyong Zhang, Jianyi Zuo, Guangsheng Xu, Jinbin Fan, Xue Bai, Zhihua Yang, Fangfang Zhang, Shilie Pan

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  26. Gas-phase BOx species govern oxidative dehydrogenation of propane over boron-based catalysts

    Journal of Catalysis · 2026-07-16

    Roman Bulánek, Kateřina Knotková, Mehran Sajad, Jhonatan Rodríguez‐Pereira, Viktor Johánek, Ota Bludský, Miroslav Rubeš

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  27. Borosulfates Hosting Se 4 2+ Ions—Crystal Structures, Chemical Bonding, Optical Spectroscopy, and Magnetism

    Angewandte Chemie International Edition · 2026-09-19

    Erich Turgunbajew, Marios Symeonidis, Jörn Bruns, S. N. Özbay, Jan Langwald, Mathias Siegfried Wickleder, Robert E. Dinnebier, Linda S. Reitz, Richard Dronskowski, Lars Schumacher, Rainer Pöttgen, Henning A. Höppe

    Read original paper ↗ ·

  28. Borosulfates Hosting Se 4 2+ Ions—Crystal Structures, Chemical Bonding, Optical Spectroscopy, and Magnetism

    Angewandte Chemie · 2026-09-19

    Erich Turgunbajew, Marios Symeonidis, Jörn Bruns, S. N. Özbay, Jan Langwald, Mathias Siegfried Wickleder, Robert E. Dinnebier, Linda S. Reitz, Richard Dronskowski, Lars Schumacher, Rainer Pöttgen, Henning A. Höppe

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