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RESEARCH PAPER · Chemical Reviews · 2020

Chemistry of Quantum Spin Liquids

Juan R. Chamorro, Tyrel M. McQueen, Thao T. Tran

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Chemistry of Quantum Spin LiquidsOriginalMolecular quantum materials: electronic phases and charge dynamics in two-dimensional organic solids55Hexagonal Perovskites as Quantum Materials1163D supramolecular chiral crystal structures of radical anion salts of (−)-NDI-Δ and possible magnetic phase diagrams5Quantum materials with strong spin–orbit coupling: challenges and opportunities for materials chemists49First-principles characterization of the magnetic properties of Cu 2 ( OH ) 3 Br10Widely spaced planes of magnetic dimers in the Ba6Y2Rh2Ti2O17−δ hexagonal perovskite6Ferromagnetic Cr4PtGa17: A Half-Heusler-Type Compound with a Breathing Pyrochlore Lattice10Integer versus half-integer spin on an approximate honeycomb lattice2Universal fluctuating regime in triangular chromate antiferromagnets22Quantum spin fluctuations and hydrogen bond network in the antiferromagnetic natural mineral henmilite7Enhancement of Photoresponse on Narrow-Bandgap Mott Insulator α‑RuCl3 via Intercalation18Unraveling the Electrical and Magnetic Properties of Layered Conductive Metal‐Organic Framework With Atomic Precision80Unraveling the Electrical and Magnetic Properties of Layered Conductive Metal‐Organic Framework With Atomic Precision18Honeycomb‐Structure RuI3, A New Quantum Material Related to α‐RuCl343Disorder-Induced Structural Complexity in the Barlowite Family of S = 1/2 Kagomé Magnets8A cationic sulfur-hydrocarbon triradical with an excited quartet state15Nanocrystalline BaCo 3 (VO 4 ) 2 (OH) 2 with a kagome lattice of Co( ii ) ions: synthesis, crystal structure and magnetic properties5Three-Dimensional Critical Behavior and Nearly Isotropic Magnetic Entropy Change of Cr4ptga17: A Half-Heusler-Type Compound with Distorted Kagome Planes4Site-Selective d 10 /d 0 Substitution in an S = 1 / 2 Spin Ladder Ba 2 CuTe 1– x W x O 6 (0 ≤ x ≤ 0.3)12LaIr3Ga2: A Superconductor Based on a Kagome Lattice of Ir41Probing magnetic excitations in correlated electron materials using inelastic neutron and X-ray scattering2Structural, Thermodynamic, and Transport Properties of the Small-Gap Two-Dimensional Metal–Organic Kagomé Materials Cu 3 (hexaiminobenzene) 2 and Ni 3 (hexaiminobenzene) 214Interplay between External High Pressure and Intrinsic Jahn–Teller Effect in the Compression Behavior of Clinoatacamite14Magnetic order and spin liquid behavior in [Mo3]11+ molecular magnets12Eminuscent phase in frustrated magnets: a challenge to quantum spin liquids24LiYbSe2: Frustrated Magnetism in the Pyrochlore Lattice41Uncovering the S=12 Kagome Ferromagnet within a Family of Metal–Organic Frameworks12Structural Diversity in Oxoiridates with 1D Ir n O 3( n +1) Chain Fragments and Flat Bands3Possible realization of the Majumdar-Ghosh point in the mineral szenicsite1MnTa2N4: A Ternary Nitride Spinel with a Strong Magnetic Frustration14α-RuCl3 and other Kitaev materials35Optimization of PbTiO3 Single Crystals with Flux and Laser Floating Zone Method7The chemistry of quantum materials2Quantum critical spin-liquid-like behavior in the S=12 quasikagome-lattice compound CeRh1−xPdxSn investigated using muon spin relaxation and neutron scattering13Quantum spin liquids bootstrapped from Ising criticality in Rydberg arrays31Perspective on multiple degrees of freedom in crystal materials6Ln2(SeO3)2(SO4)(H2O)2 (Ln=Sm, Dy, Yb): A Mixed‐Ligand Pathway to New Lanthanide(III) Multifunctional Materials Featuring Nonlinear Optical and Magnetic Anisotropy Properties36Ln2(SeO3)2(SO4)(H2O)2 (Ln=Sm, Dy, Yb): A Mixed‐Ligand Pathway to New Lanthanide(III) Multifunctional Materials Featuring Nonlinear Optical and Magnetic Anisotropy Properties2A multiscale view in functional materials18Chemical Pressure Tuning Magnetism from Pyrochlore to Triangular Lattices5Two new cubic perovskite oxides Ba3CoSb2O9 and Ba2SrCoSb2O9: Syntheses, crystal structures and magnetic properties4Antiferromagnetic Order in the Rare-Earth Halide Perovskites CsEuBr3 and CsEuCl311Ground-State Spin Dynamics in d1 Kagome-Lattice Titanium Fluorides2Anomalously field-susceptible spin clusters emerging in the electric-dipole liquid candidate κ-(ET) 2 Hg(SCN) 2 Br8A Triply Negatively Charged Nanographene Bilayer with Spin Frustration22A Triply Negatively Charged Nanographene Bilayer with Spin Frustration4Ba 4 Ni 3 F 14 ·H 2 O: a ferrimagnetic compound with a staircase kagomé lattice4Microstructured layered-kagome BaCo 3 (VO 4 ) 2 (OH) 2 with variable crystallite size: alternative synthetic route and comparison with nanostructured samples2Zigzag magnetic order and possible Kitaev interactions in the spin-1 honeycomb lattice KNiAsO425Suppression of the antiferromagnetic order by Zn doping in a possible Kitaev material Na2Co2TeO68Chiral broken symmetry descendants of the kagome lattice chiral spin liquid9From spin liquid to magnetic ordering in the anisotropic kagome Y-kapellasite Y 3 Cu 9 ( OH ) 19 Cl 8 : A single-crystal study28van der Waals Heterostructures Based on Nanolayered Paramagnetic Tm(II) Compounds and Boron Nitride for Investigating Spin Frustration2Defect-manipulated magnetoresistance and above-room-temperature ferromagnetism in two-dimensional BaNi2V2O86Signatures of a gapless quantum spin liquid in the Kitaev material Na3Co2−xZnxSbO66Magnetic phase diagram of the breathing-kagome antiferromagnet Nd3BWO921What are the key degrees of freedom for the next generation of quantum functional materials?5Role of alkaline metal in the rare-earth triangular antiferromagnet KYbO210Design Principles for Noncentrosymmetric Materials23Crystal structure and properties of the magnetically frustrated B‐site ordered Sr2CaOsO6 double perovskite3A Dynamic Triradical: Synthesis, Crystal Structure, and Spin Frustration26Kanatzidisite: A Natural Compound with Distinctive van der Waals Heterolayered Architecture10Spin-Frustrated Trisradical Trication of PrismCage22Experimental Evidences for Quantum Spin Liquid Ground State in Layered Hexagonal Y2CuTiO66Classical spin liquid state in a rhombic lattice metal-organic framework4Diffuse spin waves and classical spin liquid behavior in the kagomé antiferromagnet chromium jarosite, KCr3(OD)6(SO4)21Magnetic order in the Seff=1/2 triangular-lattice compound NdCd3P38Spin Frustration in Organic Radicals26Spin Frustration in Organic Radicals4Superconductivity in a breathing kagome metals ROs2 (R = Sc, Y, Lu)15Physics-Inspired Quantum Simulation of Resonating Valence Bond States─A Prototypical Template for a Spin-Liquid Ground State2Honeycomb layered frameworks with metallophilic bilayers9Experimental signatures of quantum and topological states in frustrated magnetism56Robust Spin Liquidity in 2D Metal‐Organic Framework Cu3 (HHTP)2 with S=1/2 Kagome Lattice9Exploring the A -V-Sb landscape beyond AV3Sb5 : A case study on the KV6Sb6 Kagome compound9Quasi-one-dimensional Pb5Re3O15 : A 5d realization of the Heisenberg antiferromagnetic spin-1/2 chain1Structural approach to charge density waves in low-dimensional systems: electronic instability and chemical bonding27Possible Approaches to Studying the Influence of Magnetic Fields and Mechanical Effects on the Physicochemical Properties of Aqueous IgG Colloids1The pressure-stabilized polymorph of indium triiodide3Spinon Heat Transport in the Three-Dimensional Quantum Magnet PbCuTe 2 O 613Structure, Spin Correlations, and Magnetism of the S = 1/2 Square-Lattice Antiferromagnet Sr 2 CuTe 1– x W x O 6 (0 ≤ x ≤ 1)10Electronic, optical, and thermodynamic properties of a quantum spin liquid candidate NaRuO2: Ab-initio investigation21Spin-degree manipulation for one-dimensional room-temperature ferromagnetism in a haldane system1Possible quantum-spin-liquid state in van der Waals cluster magnet Nb3Cl811Synthesis and magnetic properties of the Shastry-Sutherland family R2Be2SiO7 (R=Nd,Sm,Gd-Yb)10Crystallographic Disorder and Strong Magnetic Anisotropy in Dy3Pt2Sb4.482Intertwining of Localized (d) and Delocalized (π) Spins in Magnetically Frustrated Two-Dimensional Metal–Organic Frameworks12Defect Engineering in Epitaxial Thin Films of the Pyrochlore Frustrated Magnet Tb2Ti2O710Heteropentanuclear {Ru(II)Cu(II)4} Kuratowski Complexes Assembled from a Ruthenium(II) Precursor Complex to Study Competing Exchange Interactions in M(II)(ta)2 Networks [ta(−) = 1,2,3-Triazolate]3Noncentrosymmetric Triangular Magnet CaMnTeO6: Strong Quantum Fluctuations and Role of s0 versus s2 Electronic States in Competing Exchange Interactions5Local distortion driven magnetic phase switching in pyrochlore Yb 2 ( Ti 1 − x Sn x ) 2 O 73Unique Hexanuclear Mixed Bimetallic MnIII2NiII4 Complex Possessing Both Jahn–Teller Tetragonally Elongated and Compressed MnIII Ions: Spin Frustration2Revisiting spin ice physics in the ferromagnetic Ising pyrochlore Pr2Sn2O75Possible gapless quantum spin liquid behavior in the triangular-lattice Ising antiferromagnet PrMgAl 11 O 1925N-Heterocyclic Carbene-Derived 1,3,5-Trimethylenebenzene: On-Surface Synthesis and Electronic Structure10Triangular Lattice of Ho 3+ with S eff = 1/2 in Antiferromagnetic KHoSe 22Pressure-induced insulator-to-metal transition in the quantum spin liquid candidate lithium ytterbium diselenide1Two-Dimensional Cobalt(II) Benzoquinone Frameworks for Putative Kitaev Quantum Spin Liquid Candidates4Quantum-centric supercomputing for materials science: A perspective on challenges and future directions87Interpenetrated Lattices of Quaternary Chalcogenides Displaying Magnetic Frustration, High Na-Ion Conductivity, and Cation Redox in Na-Ion Batteries1Unconventional Hole Doping of S = ½ Kagome Antiferromagnet CoCu3(OH)6Cl21Candidate for a quantum spin liquid ground state in the Shastry-Sutherland lattice material Yb 2 Be 2 GeO 722Synthesis, Structures, and Magnetic Investigations of Nickel Phosphates: Ni2(PO4)(OH), Ni7(PO4)3(HPO4)(OH)3, and NaNiPO4 Including Potential Haldane Behavior10Exploring new members of magnetoelectric materials in CuO–CuCl2–SeO2 system4Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er 2 Be 2 SiO 78Fantastic Frustrated Materials–and Where to Find Them1Signatures of spin-liquid-like state and spin-phonon coupling in square lattice Sr2CuTe0.5W0.5O62When van der Waals Met Kagome: A 2D Antimonide with a Vanadium-Kagome Network6Cascade of Phase Transitions and Large Magnetic Anisotropy in a Triangle-Kagome-Triangle Trilayer Antiferromagnet9Chemical Design of Spin Frustration to Realize Topological Spin Glasses7Nitrate‐Anion‐Induced Formation of a 2D Metal‐Organic Framework with an Unconventional Kagomé Lattice Exhibiting Methanol‐Mediated Ketone Catalysis3Characterizing the diffuse continuum excitations in the classical spin liquid h − YMnO 32Synthesis and characterization of a two-dimensional antiferromagnet KNiB4O6F3 with triangular spin lattice5Evolution of ferromagnetism and electrical resistivity in Sb-doped Cr4PtGa170Stable Mono‐Radical and Triplet Diradicals Based on Allylic Radical‐Embedded All‐Benzenoid Polycyclic Hydrocarbons22Stable Mono‐Radical and Triplet Diradicals Based on Allylic Radical‐Embedded All‐Benzenoid Polycyclic Hydrocarbons4Magnetic properties of R 2 O 2 CO 3 ( R = Pr, Nd, Gd, Tb, Dy, Ho, Er, Yb) with a rare earth-bilayer of triangular lattice2High-fidelity dimer excitations using quantum hardware5Ultralow-Temperature Heat Transport in Quantum Spin Liquid Candidates: A Brief Review4Two new tellurite compounds ACu 3 Te 2 O 8 (A = Ca, Cd) with ferromagnetic spin-1/2 kagomé layers2Hydroflux-controlled growth of magnetic K-Cu-Te-O(H) phases3Fragmenting the Kagomé Lattice: Pressure-Tuned Anisotropy of Cu2+ Triangles in a Novel Atacamite Relative CaCu(OH)3Cl0Experimental Testing of the Theoretically Predicted Magnetic Properties for Kagomé Compounds in the Li–Fe–Ge System3Frustrated Magnetism and Spin Anisotropy in a Buckled Square Net YbTaO45ASb3Mn9O19 (A = K or Rb): New Mn‐Based 2D Magnetoplumbites with Geometric and Magnetic Frustration4Kagomé lattice compounds and their related systems4Observation of competing magnetic phases, mechanical stability, electronic structure, magnetism, and remarkable thermoelectric aspects of Ba 2 GdRuO 615Short-range order and hidden energy scale in geometrically frustrated magnets10Spin reorientation and magnetic frustration in Fe 32+ δ Ge 35− x Si x with a kagome lattice broken by crystallographic intergrowth5Spin‐Frustrated Metal‐Organic Frameworks15Chemical and structural disorder in the kagome spin S = 1 2 systems ZnCu 3 ( OH ) 6 Cl 2 and YCu 3 ( OH ) 6 Br 2 [ Br x ( OH ) 1 − x ]6Structural Modulation and Enhanced Magnetic Ordering in Incommensurate K1–xCrSe2 Crystals8Pyrochlore NaYbO2: A Potential Quantum Spin Liquid Candidate8Tuning the Properties of Dodecylpyridinium Metallosurfactants: The Role of Iron-Based Counterions3Spin dynamics of an easy-plane Dirac spin liquid in a frustrated XY model: Application to honeycomb cobaltates3Emergent gauge fields in band insulators7Experimental evidence of crystal-field, Zeeman-splitting, and spin-phonon excitations in the quantum supersolid Na 2 BaCo ( PO 4 ) 25Indications of quantum fluctuations in magnetically frustrated Gd2GaSbO7 and Gd2InSbO7 pyrochlores3Magnetically disordered ground state in the triangular-lattice antiferromagnets Rb 3 Yb ( VO 4 ) 2 and Cs 3 Yb ( VO 4 ) 25Spin disorder state induced by Mg 2 + doping in the Kitaev material Na 3 Co 2 SbO 61Magnetic properties of Tm3+ in layered triangular lattices0Doping dependence of the magnetic ground state in the frustrated magnets Ba 2 M Te 1 − x W x O 6 ( M = Mn, Co)0Modified large- N approach to gapless spin liquids, magnetic orders, and dynamics: Application to triangular lattice antiferromagnets6Exerting chemical pressure on the kagome lattice as frustration control in the kapellasite family A Cu 3 ( OH ) 6 + x ( Cl , Br ) 3 − x1Synthesis and Characterization of Metastable Cobalt Honeycomb KCoAsO41Inductive-Effect-Driven Tunability of Magnetism and Luminescence in Triangular Layers ANd(SO4)2 (A = Rb, Cs)0Evolution from topological Dirac metal to flat-band-induced antiferromagnet in layered KxNi4S2 (0 ≤ x ≤ 1)0Structural constraint integration in a generative model for the discovery of quantum materials12Exactly solvable dissipative dynamics and one-form strong-to-weak spontaneous symmetry breaking in interacting two-dimensional spin systems2Hidden frustration in the triangular-lattice antiferromagnet NdCd 3 P 31

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  48. Microstructured layered-kagome BaCo 3 (VO 4 ) 2 (OH) 2 with variable crystallite size: alternative synthetic route and comparison with nanostructured samples

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