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RESEARCH PAPER · Advanced Energy Materials · 2020

Recent Advances in Rechargeable Magnesium‐Based Batteries for High‐Efficiency Energy Storage

Ziqi Guo, Shuoqing Zhao, Tiexin Li, Dawei Su, Shaojun Guo, Guoxiu Wang

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Recent Advances in Rechargeable Magnesium‐Based Batteries for High‐Efficiency Energy StorageOriginalPrimary Sjogren's syndrome: rarity in India.20Advances in rechargeable Mg batteries148Nonaqueous Aluminum Ion Batteries: Recent Progress and Prospects88Progress on zinc ion hybrid supercapacitors: Insights and challenges234Ultrathin NixCoy-silicate nanosheets natively anchored on CNTs films for flexible lithium ion batteries36Designing interfacial chemical bonds towards advanced metal-based energy-storage/conversion materials62Practical energy densities, cost, and technical challenges for magnesium‐sulfur batteries28Magnesium batteries: Current picture and missing pieces of the puzzle114Hydrated MgxV5O12 Cathode with Improved Mg2+ Storage Performance58A flexible carbon nanotube@V2O5 film as a high-capacity and durable cathode for zinc ion batteries119Recent Progress of Carbon-Supported Single-Atom Catalysts for Energy Conversion and Storage335Cu-MOF-derived and porous Cu0.26V2O5@C composite cathode for aqueous zinc-ion batteries46General Liquid‐Driven Coaxial Flow Focusing Preparation of Novel Microcapsules for Rechargeable Magnesium Batteries34Recent Progress and Challenges in the Optimization of Electrode Materials for Rechargeable Magnesium Batteries90A new type of zinc ion hybrid supercapacitor based on 2D materials55Mitigating self-discharge and improving the performance of Mg–S battery in Mg[B(hfip) 4 ] 2 electrolyte with a protective interlayer22MOF-derived porous carbon inlaid with MnO 2 nanoparticles as stable aqueous Zn-ion battery cathodes22Progress of Non-Nucleophilic Electrolytes for Magnesium/Sulfur Battery4Recent advances in perovskite oxides as electrode materials for supercapacitors316The rational design of inorganic and organic material based nanocomposite hybrids as Na-ion battery electrodes9Advanced High‐Performance Potassium–Chalcogen (S, Se, Te) Batteries80The metamorphosis of rechargeable magnesium batteries271Additive Manufacturing of Electrochemical Energy Storage Systems Electrodes34An Overview on Anodes for Magnesium Batteries: Challenges towards a Promising Storage Solution for Renewables130Discharge performance of Mg–Al–Cd anode for Mg-air Battery7Nb-based compounds for rapid lithium-ion storage and diffusion20Organic Positive Materials for Magnesium Batteries: A Review35Polymers for aluminium secondary batteries: Solubility, ionogel formation and chloroaluminate speciation14Few-Layer Siloxene as an Electrode for Superior High-Rate Zinc Ion Hybrid Capacitors94Progress and Perspective on Rechargeable Magnesium–Sulfur Batteries41Assessing the Intrinsic Strengths of Ion–Solvent and Solvent–Solvent Interactions for Hydrated Mg2+ Clusters15Revisiting the degradation of solid/electrolyte interfaces of magnesium metal anodes: Decisive role of interfacial composition93The Quest for Functional Oxide Cathodes for Magnesium Batteries: A Critical Perspective77The applications of semiconductor materials in air batteries41Synergistic effect of structural stability and oxygen vacancies enabling long-life aqueous zinc-ion battery5Operando X-ray Diffraction Studies of the Mg-Ion Migration Mechanisms in Spinel Cathodes for Rechargeable Mg-Ion Batteries42Opportunities and Limitations of Ionic Liquid‐ and Organic Carbonate Solvent‐Based Electrolytes for Mg‐Ion‐Based Dual‐Ion Batteries37High-Specific-Capacity and High-Performing Post-Lithium-Ion Battery Anode over 2D Black Arsenic Phosphorus38Rechargeable Mg-Ion Full Battery System with High Capacity and High Rate35An Aqueous Mg2+‐Based Dual‐Ion Battery with High Power Density70Assembly of flexible nanohelix films: stress–exporting insights into the electrochemical performance of lithium–ion batteries13Recent progress of cathode materials for aqueous zinc-ion capacitors: Carbon-based materials and beyond137Reversible Magnesium Metal Anode Enabled by Cooperative Solvation/Surface Engineering in Carbonate Electrolytes45High-Energy Density Aqueous Zinc–Iodine Batteries with Ultra-long Cycle Life Enabled by the ZnI 2 Additive68MXene for aqueous zinc-based energy storage devices28Synergy Strategy of Electrical Conductivity Enhancement and Vacancy Introduction for Improving the Performance of VS4 Magnesium-Ion Battery Cathode37VS4 anchored on Ti3C2 MXene as a high-performance cathode material for magnesium ion battery76Aqueous zinc ion batteries based on sodium vanadate electrode materials with long lifespan and high energy density27Microwave-assisted synthesis of metallic V6O13 nanosheet as high-capacity cathode for magnesium storage12Review—Carbon Electrodes in Magnesium Sulphur Batteries: Performance Comparison of Electrodes and Future Directions15V-doped T-Nb 2 O 5 toward high-performance Mg 2+ /Li + hybrid ion batteries24First Principles Investigation of NASICON-Structured LiTi(PO) and MgTi(PO) Solid Electrolytes7Is proton a charge carrier for δ-MnO2 cathode in aqueous rechargeable magnesium-ion batteries?37Cathode Materials for Rechargeable Lithium‐Sulfur Batteries: Current Progress and Future Prospects20Cathode Materials for Rechargeable Magnesium-Ion Batteries: A Review17Challenges and opportunities for energy storage technologies2Hydrated eutectic electrolytes for high-performance Mg-ion batteries129Lattice Expanding by Te-Substitution to Boost Electrochemical Mg Storage of Cu7.2s4 Nanotube Cathode30Vo2/Graphene Oxide Composite as a Cathode Material with High Rate Performance for Hybrid Mg-Li Batteries0Anionic Te-Substitution Boosting the Reversible Redox in CuS Nanosheet Cathodes for Magnesium Storage113Strategy of cation/anion co-doping for potential elevating of VS4 cathode for magnesium ion batteries53Ether–Water Hybrid Electrolyte Contributing to Excellent Mg Ion Storage in Layered Sodium Vanadate98Rational Design Strategy of Novel Energy Storage Systems: Toward High‐Performance Rechargeable Magnesium Batteries100Understanding rechargeable magnesium ion batteries via first-principles computations: A comprehensive review64Tellurium: A High-Performance Cathode for Magnesium Ion Batteries Based on a Conversion Mechanism77Synergistic regulating the aluminum corrosion by ellagic acid and sodium stannate hybrid additives for advanced aluminum-air battery48Off-Planar, Two-Dimensional Polymer Cathode for High-Rate, Durable Rechargeable Magnesium Batteries24Switchable and Strain‐Releasable Mg‐Ion Diffusion Nanohighway Enables High‐Capacity and Long‐Life Pyrovanadate Cathode14Constructing Extended π-Conjugated Molecules with o-Quinone Groups as High-Energy Organic Cathode Materials49Core–Shell-Structured Carbon Nanotube@VS4 Nanonecklaces as a High-Performance Cathode Material for Magnesium-Ion Batteries38Advanced protective layer design on the surface of Mg-based metal and application in batteries: Challenges and progress51Modification of a Cu Mesh with Nanowires and Magnesiophilic Ag Sites to Induce Uniform Magnesium Deposition30A novel strategy to accelerate electrochemical kinetics in polymorphic Nb2O5 nanosheets for highly stable and rate-capable lithium storage11A VO2/graphene oxide composite as a cathode material with high rate performance for hybrid Mg-Li batteries24Electrolytes for Multivalent Metal‐Ion Batteries: Current Status and Future Prospect33Rechargeable Aqueous Aluminum‐Ion Battery: Progress and Outlook146Constructing robust polymer/two-dimensional Ti3C2TX solid-state electrolyte interphase via in-situ polymerization for high-capacity long-life and dendrite-free lithium metal anodes16Synthesis and characterization of Nb-doped strontium cobaltite@GQD electrodes for high performance supercapacitors49Phase Separation Induced Binary Core–Shell Alloy Nanoparticles Embedded in Carbon Sheets for Magnesium Storage14Eye Tear Activated Mg‐Air Battery Driven by Natural Eye Blinking for Smart Contact Lenses20Ionic liquid additive enabling anti-freezing aqueous electrolyte and dendrite-free Zn metal electrode with organic/inorganic hybrid solid electrolyte interphase layer160Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium95Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium3Controlling coordination environment and pore structure of Co/N-doped C host to enhance electrochemical performance of S cathode5Emerging rechargeable aqueous magnesium ion battery30Enhanced Elastic Migration of Magnesium Cations in alpha‐Manganese Dioxide Tunnels Locally Tuned by Aluminium Substitution38Magnesium storage enhancement of molybdenum dioxide in hybrid magnesium lithium batteries5The Conversion-Type Selenides as Potential High-Energy Cathode Materials for Mg-Based Batteries: A Review32Regulated electrochemical performance of manganese oxide cathode for potassium-ion batteries: A combined experimental and first-principles density functional theory (DFT) investigation56Fundamentals and advances of ligand field theory in understanding structure-electrochemical property relationship of intercalation-type electrode materials for rechargeable batteries106Microwave-anion-exchange route to spinel CuCo2S4 nanosheets as cathode materials for magnesium storage20Rechargeable batteries: Technological advancement, challenges, current and emerging applications309Emerging 2D Copper‐Based Materials for Energy Storage and Conversion: A Review and Perspective65Solvent Molecule Design Enables Excellent Charge Transfer Kinetics for a Magnesium Metal Anode112The Role of Polymer-Based Materials in Sustainable, Safe, and Efficient Metal Batteries2A comprehensive study of binder polymer for supercapattery electrode based on activated carbon and nickel-silicon composite11A practical perspective on the potential of rechargeable Mg batteries138Approaches to construct high-performance Mg–air batteries: from mechanism to materials design79Defect engineering of two-dimensional materials for advanced energy conversion and storage417Magnesium: properties and rich chemistry for new material synthesis and energy applications118Metal–iodine batteries: achievements, challenges, and future132Rational Design of Mg(Oh)2/Cu2(Oh)3(No3) Binary Heterostructure Based Electrode Material for Enhance Supercapacitors Performance0The origin of anode–electrolyte interfacial passivation in rechargeable Mg-metal batteries141Recent advances in manipulating strategy of aqueous electrolytes for Zn anode stabilization153What Would Battery Manufacturing Look Like on the Moon and Mars?27Cathode Electrolyte Interphase (CEI) Endows Mo 6 S 8 with Fast Interfacial Magnesium‐Ion Transfer Kinetics70Cathode Electrolyte Interphase (CEI) Endows Mo6S8 with Fast Interfacial Magnesium‐Ion Transfer Kinetics8Theoretical and experimental study of the titanium substituted Mg2-xTixNi alloys and Mg2-xTixNiH4 hydrides7How does fiscal decentralization lead to renewable energy transition and a sustainable environment? Evidence from highly decentralized economies96Cationic Co-doping in copper sulfide nanosheet cathodes for efficient magnesium storage41Advances in Cathodes for High-Performance Magnesium-Sulfur Batteries: A Critical Review17Bismuth Nanoparticle-Embedded Carbon Microrod for High-Rate Electrochemical Magnesium Storage20Recent progress in rechargeable calcium-ion batteries for high-efficiency energy storage56Copper Tetraselenophosphate Cathode for Rechargeable Magnesium Batteries: A Redox-Active Polyatomic Anion Strategy to Design the Cathode Material19A DFT study of COF-1 covalent organic framework as a disposable platform for rechargeable lithium-ion battery anodes11Cu+ redox activation and polyselenide stabilization via strong Se-C interaction for superior magnesium storage33First-Principles Study of FeB2Monolayers as High-Capacity Electrode Materials for Mg-Ion Batteries23Research development on electrolytes for magnesium-ion batteries157Layered Materials in the Magnesium Ion Batteries: Development History, Materials Structure, and Energy Storage Mechanism24Recent advancements and challenges in deploying lithium sulfur batteries as economical energy storage devices106Increasing the cell voltage of a magnesium ion battery with B 24 O 24 anode through encapsulating halides: a DFT study1Multiphase MoS2 monolayer: A promising anode material for Mg-Ion batteries16High Energy Density Aqueous Zinc–Chalcogen (S, Se, Te) Batteries: Recent Progress, Challenges, and Perspective104Bottom‐Up Magnesium Deposition Induced by Paper‐Based Triple‐Gradient Scaffolds toward Flexible Magnesium Metal Batteries62Single atom iron as an efficient electrocatalyst for enhanced kinetics in magnesium-sulfur batteries18Rational design of Mg(OH)2/Cu2(OH)3(NO3) binary heterostructure electrodes for enriched supercapacitors performance10Preparation of NiFe2O4@ slit modified hollow carbon fiber via electrospinning for supercapacitor electrode material33In-situ generated elemental selenium nanograins cooperated with NiSe2 microspheres for significantly enhanced magnesium-storage performance13Interlayer Engineering of VS2 Nanosheets via In Situ Aniline Intercalative Polymerization toward Long-Cycling Magnesium-Ion Batteries7Realizing horizontal magnesium platelet deposition and suppressed surface passivation for high-performance magnesium metal batteries70Facile preparation of bimetallic cobalt-copper selenide nanosheets as stable cathode materials for rechargeable magnesium batteries13Fast Mg-ion insertion kinetics in V 2 Se 97Noble metal catalysts for metal-air batteries: From nano-level to atom-level23Optimizing Coating Layer to Construct Corrosion Resistant Current Collectors for Highly Stable Magnesium-Air Batteries0Recent advances in rechargeable aqueous magnesium-ion batteries68Pillar‐Structured Ti 3 C 2 T x MXene with Engineered Interlayer Spacing for High‐Performance Magnesium Batteries23Unveiling the prospects of Y2O3-based nanocomposites: Synthesis, characterization, and electrochemical assessment for supercapacitor and biosensor applications20Accessing Mg‐Ion Storage in V2PS10 via Combined Cationic‐Anionic Redox with Selective Bond Cleavage5Accessing Mg‐Ion Storage in V2PS10 via Combined Cationic‐Anionic Redox with Selective Bond Cleavage2NiCo 2 O 4 Nanowires Immobilized on Nitrogen‐Doped Ti 3 C 2 T x for High‐Performance Wearable Magnesium–Air Batteries15Advances and Challenges in Electrolyte Development for Magnesium–Sulfur Batteries: A Comprehensive Review20Development of aqueous magnesium–air batteries: From structure to materials37Advances on lithium, magnesium, zinc, and iron-air batteries as energy delivery devices—a critical review36CuS-based composite for high-performance magnesium storage with a clarified charge-discharge mechanism9Bimetallic Selenide CuFeSe2 as Mg‐Storage Material for Rechargeable Magnesium Batteries7Preferentially in-situ generated copper nanograins boosting fast kinetic conversion magnesium storage of bimetallic copper-cobalt sulfide cathode15Highly cycle-stable VOPO4-based cathodes for magnesium ion batteries: Insight into the role of interlayer engineering in batteries performance17Machine learning molecular dynamics insight into high interface stability and fast kinetics of low-cost magnesium chloride amine electrolyte for rechargeable magnesium batteries23References0Synchronous regulation on solvation structure and interface engineering to enable reversible magnesium metal batteries16

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  49. Microwave-assisted synthesis of metallic V6O13 nanosheet as high-capacity cathode for magnesium storage

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