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RESEARCH PAPER · Materials Science and Engineering R Reports · 2020

Broad-band emission in metal halide perovskites: Mechanism, materials, and applications

Guojun Zhou, Binbin Su, Jinglong Huang, Qinyuan Zhang, Zhiguo Xia

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Broad-band emission in metal halide perovskites: Mechanism, materials, and applicationsOriginal2D layered perovskite containing functionalised benzothieno-benzothiophene molecules: formation, degradation, optical properties and photoconductivity29A zero-dimensional hybrid lead perovskite with highly efficient blue-violet light emission58Melt-grown large-sized Cs 2 TeI 6 crystals for X-ray detection45Role of specific distorted metal complexes in exciton self-trapping for hybrid metal halides13Tetrameric cluster assembled one-dimensional hybrid lead halides with broadband light emission3Pressure-Induced Enhancement of Broad-Band White Light Emission in Butylammonium Lead Bromide41Sb 3+ Dopant and Halogen Substitution Triggered Highly Efficient and Tunable Emission in Lead-Free Metal Halide Single Crystals331Perovskite Multiple Quantum Wells on Layered Materials toward Narrow-Band Green Emission for Backlight Display Applications19Reversible Release and Fixation of Bromine in Vacancy‐Ordered Bromide Perovskites39Supramolecular Approach for Fine-Tuning of the Bright Luminescence from Zero-Dimensional Antimony(III) Halides179Enhancing Photoluminescence Quantum Yield in 0D Metal Halides by Introducing Water Molecules159Synthesis, Crystal Structure and Green Luminescence in Zero-Dimensional Tin Halide (C8H14N2)2SnBr6110Unraveling the Near-Unity Narrow-Band Green Emission in Zero-Dimensional Mn 2+ -Based Metal Halides: A Case Study of (C 10 H 16 N) 2 Zn 1– x Mn x Br 4 Solid Solutions285Zero-Dimensional Organic-Inorganic Hybrid Material with Ultra-Narrow-Red Emission at Room Temperature0Lead-free violet-emitting K2CuCl3 single crystal with high photoluminescence quantum yield41Efficient Lone-Pair-Driven Luminescence: Structure–Property Relationships in Emissive 5s2 Metal Halides416Zero‐Dimensional Hybrid Cd‐Based Perovskites with Broadband Bluish White‐Light Emissions41Doped Zero‐Dimensional Cesium Zinc Halides for High‐Efficiency Blue Light Emission186Doped Zero‐Dimensional Cesium Zinc Halides for High‐Efficiency Blue Light Emission22Self-trapped excitons in two-dimensional perovskites141Mechanochemistry as a Green Route: Synthesis, Thermal Stability, and Postsynthetic Reversible Phase Transformation of Highly-Luminescent Cesium Copper Halides88Metal Halide Regulated Photophysical Tuning of Zero‐Dimensional Organic Metal Halide Hybrids: From Efficient Phosphorescence to Ultralong Afterglow206Metal Halide Regulated Photophysical Tuning of Zero‐Dimensional Organic Metal Halide Hybrids: From Efficient Phosphorescence to Ultralong Afterglow39Defect-Related Broadband Emission in Two-Dimensional Lead Bromide Perovskite Microsheets75One-Dimensional Face-Shared Perovskites with Broad-Band Bluish White-Light Emissions45Mn4+ doped zero-dimensional organic-inorganic hybrid material with narrow-red emission30Mn2+ doping enabled efficient high-color-rendering single-phase white-emitting lead halide perovskites13Pb alloying enables efficient broadband emission of two dimensional [NH3(CH2)4NH3]CdBr427Perovskite Quantum Dots for Application in High Color Gamut Backlighting Display of Light-Emitting Diodes265Pressure‐Engineered Photoluminescence Tuning in Zero‐Dimensional Lead Bromide Trimer Clusters104Pressure‐Engineered Photoluminescence Tuning in Zero‐Dimensional Lead Bromide Trimer Clusters21Size-dependent dark exciton properties in cesium lead halide perovskite quantum dots44Mechanism of transition metal cluster catalysts for hydrogen evolution reaction48Dielectric confinement for designing compositions and optoelectronic properties of 2D layered hybrid perovskites73Broadband white-light emission in a one-dimensional organic–inorganic hybrid cadmium chloride with face-sharing CdCl 6 octahedral chains88Mn 2+ ‐Doped Metal Halide Perovskites: Structure, Photoluminescence, and Application319Recent Advances in Luminescent Zero‐Dimensional Organic Metal Halide Hybrids241A Guanidinium-Based Mn4+-Doped Red-Emitting Hybrid Phosphor with High Stability35Anti-solvent mixture-mediated reduction of photocurrent hysteresis in high-impurity perovskite precursor based MAPbI3 solar cells22Chiral Switchable Low-Dimensional Perovskite Ferroelectrics99Long lifetime phosphorescence and X-ray scintillation of chlorobismuthate hybrids incorporating ionic liquid cations37Manipulation of Cl/Br transmutation in zero-dimensional Mn 2+ -based metal halides toward tunable photoluminescence and thermal quenching behaviors87A multiaxial electrical switching in a one-dimensional organic–inorganic (pyrrolidinium) 2 Cd 2 I 6 ferroelectric and photoluminescent crystal22Bulk assembly of a 0D organic tin( ii )chloride hybrid with high anti-water stability30Co-luminescence in a zero-dimensional organic–inorganic hybrid antimony halide with multiple coordination units67Highly efficient self-trapped exciton emission in a one-dimensional face-shared hybrid lead bromide45Lead-free Mn II -based red-emitting hybrid halide (CH 6 N 3 ) 2 MnCl 4 toward high performance warm WLEDs126Recent progress of zero-dimensional luminescent metal halides873Modulation of Metal Halide Structural Units for Light Emission112Combining Dual-Light Emissions to Achieve Efficient Broadband Yellowish-Green Luminescence in One-Dimensional Hybrid Lead Halides29Highly Efficient and Tunable Emission of Lead‐Free Manganese Halides toward White Light‐Emitting Diode and X‐Ray Scintillation Applications353Role of Metal–Chloride Anions in Photoluminescence Regulations for Hybrid Metal Halides40Tailoring the electron and hole dimensionality to achieve efficient and stable metal halide perovskite scintillators26Photoluminescence of Singlet/Triplet Self‐Trapped Excitons in Sb3+‐Based Metal Halides293Synthesis of Gram‐Scale Ultrastable Mn‐Doped 2D Perovskites for Light‐Emitting Diodes15Neural Networks for Analysis of Optical Properties in 2D Layered Hybrid Lead Halide Perovskites8Highly Efficient Cool-White Photoluminescence of (Gua) 3 Cu 2 I 5 Single Crystals: Formation and Optical Properties126Tunable White Light Emission in a Zero‐Dimensional Organic–Inorganic Metal Halide Hybrid with Ultra‐High Color Rendering Index61An efficient perovskite-type Rb2CaPO4F:Eu2+ phosphor with high brightness towards closing the cyan gap23Role of octahedral deformation in the broad-band emission in Mn-doped lead halide perovskite: First-principles investigation for the case of CsPbX3 (X = Cl, Br, I)18Controlled Structural Transformation in Sb‐Doped Indium Halides A3InCl6 and A2InCl5∙H2O Yields Reversible Green‐to‐Yellow Emission Switch86Strongly Luminescent Dion–Jacobson Tin Bromide Perovskite Microcrystals Induced by Molecular Proton Donors Chloroform and Dichloromethane43Systematic Approach of One-Dimensional Lead Perovskites with Face-Sharing Connectivity to Realize Efficient and Tunable Broadband Light Emission25Organic-inorganic hybrid manganese bromine single crystal with dual-band photoluminescence from polaronic and bipolaronic excitons196Multimode dynamic luminescent switching of lead halide hybrids for anti-counterfeiting and encryption94An Overview for Zero‐Dimensional Broadband Emissive Metal‐Halide Single Crystals269Ultra-Broad-Band-Excitable Cu(I)-Based Organometallic Halide with Near-Unity Emission for Light-Emitting Diode Applications168Structural Dimensionality Modulation toward Enhanced Photoluminescence Efficiencies of Hybrid Lead‐Free Antimony Halides164Introducing Intermolecular Cation‐π Interactions for Water‐Stable Low Dimensional Hybrid Lead Halide Perovskites136Introducing Intermolecular Cation‐π Interactions for Water‐Stable Low Dimensional Hybrid Lead Halide Perovskites7Tailoring of White Luminescence in a NaLi 3 SiO 4 :Eu 2+ Phosphor Containing Broad‐Band Defect‐Induced Charge‐Transfer Emission183Sb 3+ ‐Doping in Cesium Zinc Halides Single Crystals Enabling High‐Efficiency Near‐Infrared Emission370Highly Luminescent Zero-Dimensional Organic Copper Halides for X-ray Scintillation211Temperature‐Dependent Photoluminescence of Hexafluorobenzene‐Intercalated Phenethylammonium Tin Iodide 2D Perovskite4Unraveling the Ultrafast Self-assembly and Photoluminescence in Zero-Dimensional Mn 2+ -Based Halides with Narrow-Band Green Emissions39Low Dimensional, Broadband, Luminescent Organic‐Inorganic Hybrid Materials for Lighting Applications57Low pH-induced lone-pair activity in the hybrid (C6H10N2)[SnCl3]Cl: Chemical study and physical characterizations6Ultrafast Study of Exciton Transfer in Sb(III)-Doped Two-Dimensional [NH3(CH2)4NH3]CdBr4 Perovskite84Zero‐Dimensional Organic–Inorganic Hybrid Copper‐Based Halides with Highly Efficient Orange–Red Emission87Tin Halide Perovskites: From Fundamental Properties to Solar Cells333Rare-earth single atom based luminescent composite nanomaterials: Tunable full-color single phosphor and applications in WLEDs51Two SbX5-based isostructural polar 1D hybrid antimony halides with tunable broadband emission, nonlinear optics, and semiconductor properties34Structure‐Property Relationships and Idiosyncrasies of Bulk, 2D Hybrid Lead Bromide Perovskites25Multi-Dopant Engineering in Perovskite Cs2SnCl6: White Light Emitter and Spatially Luminescent Heterostructure58Selective Luminescence Response of a Zero-Dimensional Hybrid Antimony(III) Halide to Solvent Molecules: Size-Effect and Supramolecular Interactions72Double perovskite microcrystals-based white light-emitting diodes without reabsorption of multiphase phosphors13A Zero-Dimensional Hybrid Cadmium Perovskite with Highly Efficient Orange–Red Light Emission54Origin of Radioluminescence in Low-Dimensional Halide Perovskite Glass Ceramics under X-ray Excitation5Rubidium copper chloride scintillator for X-ray imaging screen7Unveiling White Light Emission of a One-Dimensional Cu(I)-Based Organometallic Halide toward Single-Phase Light-Emitting Diode Applications39Magnetic polaronic and bipolaronic excitons in Mn(II) doped (TDMP)PbBr4 and their high emission55Thermochromism Perovskite (COOH(CH2)3NH3)2PbI4 Crystals: Single-Crystal to Single-Crystal Phase Transition and Excitation-Wavelength-Dependent Emission28Air-grown hybrid copper( i ) halide single crystals: structural transformations and ultraviolet-pumped photoluminescence applications36Band gap modulation of organic–inorganic Sb( iii ) halide by molecular design17Bright tunable luminescence of Sb 3+ doping in zero-dimensional lead-free halide Cs 3 ZnCl 5 perovskite crystals26Centimeter-sized Cs3Cu2I5 Single Crystal: Synthesized by Low-cost Solution Method and Optical and Scintillation Properties8Coordination units of Mn 2+ modulation toward tunable emission in zero-dimensional bromides for white light-emitting diodes94Free and self-trapped exciton emission in perovskite CsPbBr 3 microcrystals49High-efficiency luminescent organic–inorganic hybrid manganese( ii ) halides applied to X-ray imaging70Modulating photoelectron localization degree to achieve controllable photoluminescence quenching and activation of 0D hybrid antimony perovskites53Structural distortion induced broad emission in vacancy-ordered halide triple perovskites17Triplet–triplet energy transfer from Bi 3+ to Sb 3+ in zero-dimensional indium hybrids via a B-site co-doping strategy toward white-light emission34Unveiling the uncommon blue-excitable broadband yellow emission from self-trapped excitons in a zero-dimensional hybrid tellurium-based double perovskite17Dual‐Band‐Tunable White‐Light Emission from Bi 3+ /Te 4+ Emitters in Perovskite‐Derivative Cs 2 SnCl 6 Microcrystals144Dual‐Band‐Tunable White‐Light Emission from Bi3+/Te4+ Emitters in Perovskite‐Derivative Cs2SnCl6 Microcrystals22Ternary zero-dimensional hybrid metal halides with dual emission10Unprecedented Self-Powered Visible–Infrared Dual-Modal Photodetection Induced by a Bulk Photovoltaic Effect in a Polar Perovskite23Temperature-Responsive Photoluminescence and Elastic Properties of 1D Lead Halide Perovskites R- and S-(Methylbenzylamine)PbBr36Inorganic halide perovskites for lighting and visible light communication41Effects of Electron–Phonon Coupling and Spin–Spin Coupling on the Photoluminescence of Low-Dimensional Metal Halides90Methanol-induced luminescence vapochromism based on a Sb3+-doped organic indium halide hybrid55Crystal structure and optical properties of in situ synthesized organic-inorganic hybrid metal halides13Recent Advances in Silver Nanowires Electrodes for Flexible Organic/Perovskite Light-Emitting Diodes29Tuning of emission by effect of local symmetry in BaLaLiWO6:Dy3+/Eu3+ for WLEDs41Highly efficient Sb3+ emitters in 0D cesium indium chloride nanocrystals with switchable photoluminescence through water-triggered structural transformation167Two-dimensional hybrid halide perovskites composed of mixed corner- and edge-shared octahedron as broadband yellow-light emissions3Solely 3-Coordinated Organic–Inorganic Hybrid Copper(I) Halide: Hexagonal Channel Structure, Turn-On Response to Mechanical Force, Moisture, and Amine11Highly stable metal halides Cs2ZnX4 (X = Cl, Br) with Sn2+ as dopants for efficient deep-red photoluminescence23Amino‐Acid‐Induced Circular Polarized Luminescence in One‐Dimensional Manganese(II) Halide Hybrid47Circularly Polarized Luminescence based on 0D Lead‐Free Antimony (III) Halide Hybrids63Ultra‐Sensitive, Selective and Repeatable Fluorescence Sensor for Methanol Based on a Highly Emissive 0D Hybrid Lead‐Free Perovskite35Ultra‐Sensitive, Selective and Repeatable Fluorescence Sensor for Methanol Based on a Highly Emissive 0D Hybrid Lead‐Free Perovskite165Temperature-Dependent Luminescence and Anisotropic Optical Properties of Centimeter-Sized One-Dimensional Perovskite Trimethylammonium Lead Iodide Single Crystals39Bright Green Emission from Self-Trapped Excitons Triggered by Sb3+ Doping in Rb4CdCl6145Highly Distorted Antimony(III) Chloride [Sb 2 Cl 8 ] 2− Dimers for Near‐Infrared Luminescence up to 1070 nm160Highly Distorted Antimony(III) Chloride [Sb2Cl8]2− Dimers for Near‐Infrared Luminescence up to 1070 nm25Halide Perovskites for X‑ray Detection: The Future of Diagnostic Imaging7Water Resistance and Flexible Cuprous Halide Composite Polysiloxane Luminescent Ceramics4Reversible Triple-Mode Switching in Photoluminescence from 0D Hybrid Antimony Halides139Water-Sensitive Mixed-Phase PEA6SnI8 Perovskite Derivative Single Crystal for Humidity Detection11Effect of Bimetallic and Halogen Ions on Performance in Inorganic Double Perovskites4High Quantum Efficiency of Stable Sb‐Based Perovskite‐Like Halides toward White Light Emission and Flexible X‐Ray Imaging83Synthetic-Method-Dependent Antimony Bromides and Their Photoluminescent Properties36Barrierless Exciton Self‐Trapping and Emission Mechanism in Low‐Dimensional Copper Halides76Metal halide perovskites-based white light-emitting diodes20Zero-dimensional rubidium zinc halide blue-emitting quantum dots for X-ray imaging9Structural, optical and dielectric properties of low temperature assisted grown crystals of CH3NH3Pb1-xCdxBr35Sequential and Reversible Phase Transformations in Zero‐Dimensional Organic‐Inorganic Hybrid Sb‐based Halides towards Multiple Emissions161Complete B-site cation regulation accomplish UV-excited red phosphors in double perovskite oxides13Sequential and Reversible Phase Transformations in Zero‐Dimensional Organic‐Inorganic Hybrid Sb‐based Halides towards Multiple Emissions19Molecular and Supramolecular Structure of a New Luminescent Hybrid Compound: (C5N2H14)2[BiBr6]Br·H2O8Solution growth and optical properties of lead-free highly efficient green-emitting [Emim]4[Cu4I8] single crystals with 0D structure11Regulation strategy of white emission from organic–inorganic hybrid metal halide perovskites67Mn 2+ -doped Cs 2 ZnBr 4 scintillator for X-ray imaging65Solid–liquid transitions in Mn-based ionic liquids [MeIM]2[MnBr4] and [EtIM]2[MnBr4] producing emission spectra with narrow green bands6Recent Advances on Mn2+‐Doping in Diverse Metal Halide Perovskites66Effects of Cl/Br substitution of antimony octahedra on photoluminescence and a new engineering strategy for performance optimization1Unraveling the Broadband Emission in Mixed Tin‐Lead Layered Perovskites27Single‐Component White Circularly Polarized Luminescence in Chiral 1D Double‐Chain Perovskites43Near-unity quantum yield in zero-dimensional lead-free manganese-based halides for flexible X-ray imaging with high spatial resolution116

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  4. Role of specific distorted metal complexes in exciton self-trapping for hybrid metal halides

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  5. Tetrameric cluster assembled one-dimensional hybrid lead halides with broadband light emission

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  9. Reversible Release and Fixation of Bromine in Vacancy‐Ordered Bromide Perovskites

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  10. Supramolecular Approach for Fine-Tuning of the Bright Luminescence from Zero-Dimensional Antimony(III) Halides

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  11. Enhancing Photoluminescence Quantum Yield in 0D Metal Halides by Introducing Water Molecules

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  30. Pressure‐Engineered Photoluminescence Tuning in Zero‐Dimensional Lead Bromide Trimer Clusters

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  31. Pressure‐Engineered Photoluminescence Tuning in Zero‐Dimensional Lead Bromide Trimer Clusters

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  32. Size-dependent dark exciton properties in cesium lead halide perovskite quantum dots

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  33. Mechanism of transition metal cluster catalysts for hydrogen evolution reaction

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  34. Dielectric confinement for designing compositions and optoelectronic properties of 2D layered hybrid perovskites

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  35. Broadband white-light emission in a one-dimensional organic–inorganic hybrid cadmium chloride with face-sharing CdCl 6 octahedral chains

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  36. Mn 2+ ‐Doped Metal Halide Perovskites: Structure, Photoluminescence, and Application

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  37. Recent Advances in Luminescent Zero‐Dimensional Organic Metal Halide Hybrids

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  38. A Guanidinium-Based Mn4+-Doped Red-Emitting Hybrid Phosphor with High Stability

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  39. Anti-solvent mixture-mediated reduction of photocurrent hysteresis in high-impurity perovskite precursor based MAPbI3 solar cells

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  40. Chiral Switchable Low-Dimensional Perovskite Ferroelectrics

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  41. Long lifetime phosphorescence and X-ray scintillation of chlorobismuthate hybrids incorporating ionic liquid cations

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