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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2020

A Simple Halogen-Free Magnesium Electrolyte for Reversible Magnesium Deposition through Cosolvent Assistance

Shengqi Fan, Genevieve M. Asselin, Baofei Pan, Hao Wang, Yang Ren, John T. Vaughey, Niya Sa

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A Simple Halogen-Free Magnesium Electrolyte for Reversible Magnesium Deposition through Cosolvent AssistanceOriginalAdvances in rechargeable Mg batteries148Recent Advances in Non‐nucleophilic Mg Electrolytes16In Situ Probing of Mass Exchange at the Solid Electrolyte Interphase in Aqueous and Nonaqueous Zn Electrolytes with EQCM-D30A Systematic Electrochemical Investigation of a Dimethylamine Cosolvent-Assisted Nonaqueous Zinc(II) Bis(trifluoromethylsulfonyl)imide Electrolyte9Hybrid twin-metal aluminum–magnesium electrolytes for rechargeable batteries17Preparation and electrochemical characterization of magnesium gel electrolytes based on crosslinked Poly(tetrahydrofuran)7Advancing Electrolyte Solution Chemistry and Interfacial Electrochemistry of Divalent Metal Batteries32Chelated electrolytes for divalent metal ions9Probing a new halogen-free electrolyte and Ba0.85Sm0.1TiO3 cathode for Mg battery applications3The Role of Adding Naf to the Electrolyte in Constructing a Stable Anode/Electrolyte Interphase for Magnesium Battery Applications1Understanding the Solvation-Dependent Properties of Cyclic Ether Multivalent Electrolytes Using High-Field NMR and Quantum Chemistry23Electrolyte and Interphase Design for Magnesium Anode: Major Challenges and Perspectives79Probing the effect of the stoichiometric ratio of Mg(CF3SO3)2/AlCl3 on optimizing the electrolyte performance10A High Potential Polyanion Cathode Material for Rechargeable Mg‐Ion Batteries30Efficacy of Stabilizing Calcium Battery Electrolytes through Salt-Directed Coordination Change22Two-dimensional materials for aqueous zinc-ion batteries30Preparation of conductive Cu1.5Mn1.5O4 and Mn3O4 spinel mixture powders as positive active materials in rechargeable Mg batteries operative at room temperature2Evolution of the Dynamic Solid Electrolyte Interphase in Mg Electrolytes for Rechargeable Mg-Ion Batteries24The role of adding NaF to the electrolyte in constructing a stable anode/electrolyte interphase for magnesium battery applications18Non-nucleophilic electrolyte with non-fluorinated hybrid solvents for long-life magnesium metal batteries113On the Road to Stable Electrochemical Metal Deposition in Multivalent Batteries17Deeping insight of Mg(CF3SO3)2 and comprehensive modified electrolyte with ionic liquid enabling high-performance magnesium batteries74Probing the Functionality of Halogen-Free Electrolytes Using Succinonitrile Additive in Magnesium-Sulfur Batteries6Toward Improved Anodic Stability of Ether-Based Electrolytes for Rechargeable Magnesium Batteries24Succinonitrile as electrolyte-additive with modified separator and microwave-assisted synthesis of sulfur nanoparticles cathode for magnesium battery applications15A non-nucleophilic electrolyte based on all-inorganic salts with conditioning-free characteristic for rechargeable magnesium batteries11Constructing Efficient Mg(CF3SO3)2 Electrolyte via Tailoring Solvation and Interface Chemistry for High‐Performance Rechargeable Magnesium Batteries116Chloride-Free Electrolyte Based on Tetrabutylammonium Triflate Additive for Extended Anodic Stability in Magnesium Batteries35Synergy between the coordination and trace ionization of co-solvents enables reversible magnesium electroplating/stripping behavior83Toward high-energy magnesium battery anode: recent progress and future perspectives34Quantifying the Correlation between Coordination Chemistry, Interfacial Formation, and Electrochemical Performances for Mg Battery Electrolytes13Structure and chemical composition of the Mg electrode during cycling in a simple glyme electrolyte5References0Recent progress of magnesium electrolytes for rechargeable magnesium batteries62Solvation Structure Analysis by a Combination of Crystallography and Raman Spectroscopy, and Its Application to the Development of Functional Electrolytes for Next Generation Rechargeable Batteries0Activation mechanism of conventional electrolytes with amine solvents: Species evolution and hydride-containing interphase formation32Lithium fluoride additive helps construct stable electrode-electrolyte interfaces to boost the performance of Mg-S batteries10Divalent Metal-Ion Batteries as Alternatives to Li-Ion Based Energy Storage0Emerging amine-assisted electrolytes for rechargeable magnesium metal batteries: Current understanding and future direction13Tailoring the electrochemical performance of the polymer electrolyte using Na2H20B4O17 for magnesium sulfur battery applications6Dendritic Magnesium Formation in Conventional Electrolytes: Local Adsorption of Amine Solvents at Inner Helmholtz Plane Matters8Bridging Atomic Solvation Environment with Electrochemical Properties for the Bis(trifluoromethylsulfonyl)imide-Based Divalent Cation Electrolytes for the Next-Generation Energy Storage Systems3Critical Ingredients Revitalize Magnesium‐Metal Batteries: Rationality and Challenges32Mg Plating in Nonethereal Electrolyte Solutions: Fact or Misconception?6Co-solvent strategy for rechargeable post-lithium metal batteries65Decoding Cathode‐Electrolyte Interface Issues in Conventional Ethers Electrolytes‐Based Magnesium Rechargeable Batteries9Evolution of coordinated chemical innovations: A road to chlorine-free magnesium electrolyte system10Interfacial atomistic reactive mechanisms of magnesium batteries5Solvation Chemistry of Nonaqueous Electrolytes for Rechargeable Magnesium Batteries39Dual‐Site Modulation of Mg 2+ Desolvation Beyond the Primary Solvation Shell in Magnesium Battery Electrolytes3Dual‐Site Modulation of Mg 2+ Desolvation Beyond the Primary Solvation Shell in Magnesium Battery Electrolytes14Electrochemical Coinsertion of Magnesium and Lithium Ions with Silicon Anode: An Integrated Experiment and Finite Element Simulation Approach1Bulky Dimethyl Phosphate Anion-Based Ionic Liquid Enables Reversible Magnesium Electrodeposition2A Dive into the Electrodeposition Kinetics and Mechanisms in Nonaqueous Magnesium Electrolytes2Reassessing Electrolyte Design for Non‐Aqueous Magnesium Batteries: Atomistic Structures and Performance Optimization14Amine-based anion receptor enables an improved magnesium plating/stripping reversibility1A bromine-rich artificial interphase to regulate interfacial kinetics in boron-centered electrolytes for magnesium metal batteries4Dual-functional CF 3 SO 3 − /amine additives synergistically construct an MgF 2 /Mg 3 N 2 -rich interphase toward high-performance magnesium–sulfur batteries0Fundamental insights into magnesium electrodeposition through operando X-ray diffraction: crystal growth, orientation evolution, and interfacial dynamics0Development of a chloride-free dual-salt electrolyte based on Mg(NO3)2 and Mg(TFSI)2 for magnesium-sulfur batteries in a binary solvent system2Halogen-free electrolyte engineering and multifunctional sulfur cathodes for rechargeable Mg–S and Na–S batteries1Electrolytes for rechargeable magnesium batteries12Synergistic effects of composite organic additives on the magnesium–ion battery performance0A DFT Study on the Mechanism of Selective Formation of Substituted Azepines From 1‐Azabutadienes and Cyclopropanes2Advanced electrolyte design for high performance rechargeable magnesium batteries0Tackling the bottleneck in Mg anode/electrolyte interface1Probing compatibility of dual-salt ionic liquid electrolytes for rechargeable Mg-S batteries0Unsuccessful Coupling of Weakly Coordinating Anion–Based Mg Salts and Alkoxyalkylamine Solvents for Rechargeable Mg Battery Application: Trace Water‐Driven Interfacial Failure0Bridging Fundamentals and Practice: Advances in Electrolyte Chemistry for Rechargeable Magnesium‐Sulfur Batteries0

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  2. Recent Advances in Non‐nucleophilic Mg Electrolytes

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  3. In Situ Probing of Mass Exchange at the Solid Electrolyte Interphase in Aqueous and Nonaqueous Zn Electrolytes with EQCM-D

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  4. A Systematic Electrochemical Investigation of a Dimethylamine Cosolvent-Assisted Nonaqueous Zinc(II) Bis(trifluoromethylsulfonyl)imide Electrolyte

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  5. Hybrid twin-metal aluminum–magnesium electrolytes for rechargeable batteries

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  6. Preparation and electrochemical characterization of magnesium gel electrolytes based on crosslinked Poly(tetrahydrofuran)

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  9. Probing a new halogen-free electrolyte and Ba0.85Sm0.1TiO3 cathode for Mg battery applications

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  13. Probing the effect of the stoichiometric ratio of Mg(CF3SO3)2/AlCl3 on optimizing the electrolyte performance

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  18. Evolution of the Dynamic Solid Electrolyte Interphase in Mg Electrolytes for Rechargeable Mg-Ion Batteries

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  19. The role of adding NaF to the electrolyte in constructing a stable anode/electrolyte interphase for magnesium battery applications

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  20. Non-nucleophilic electrolyte with non-fluorinated hybrid solvents for long-life magnesium metal batteries

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  22. Deeping insight of Mg(CF3SO3)2 and comprehensive modified electrolyte with ionic liquid enabling high-performance magnesium batteries

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