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RESEARCH PAPER · The Journal of Physical Chemistry B · 2001

Naturally Chiral Metal Surfaces as Enantiospecific Adsorbents

David S. Sholl, Aravind Asthagiri, Timothy D. Power

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Naturally Chiral Metal Surfaces as Enantiospecific AdsorbentsOriginalChemInform Abstract: Naturally Chiral Metal Surfaces as Enantiospecific Adsorbents0Induced Chiral Metal Surfaces in Asymmetric Hydrogenations?13From Local Adsorption Stresses to Chiral Surfaces: (R,R)-Tartaric Acid on Ni(110)196Effects of Surface Relaxation on Enantiospecific Adsorption on Naturally Chiral Pt Surfaces23Thermal Fluctuations in the Structure of Naturally Chiral Pt surfaces46Can Chiral Single Walled Carbon Nanotubes Be Used as Enantiospecific Adsorbents?63Enantiospecific Desorption of Chiral Compounds from Chiral Cu(643) and Achiral Cu(111) Surfaces153Atomically Detailed Models of the Effect of Thermal Roughening on the Enantiospecificity of Naturally Chiral Platinum Surfaces70Creating chiral architectures at metal surfaces41A computer simulation study of racemic mixtures12Heterogeneous asymmetric reactions, 33. Novel interpretation of the enantioselective hydrogenation of a-ketoesters on Pt/alumina-cinchona alkaloid catalyst system19Density Functional Theory Study of Enantiospecific Adsorption at Chiral Surfaces7322 Enantiospecific heterogeneous catalysis without a chiral modifier0Amplification of Chirality from Extremely Low to Greater than 99.5 % ee by Asymmetric Autocatalysis233Amplification of Chirality from Extremely Low to Greater than 99.5 % ee by Asymmetric Autocatalysis48Chiral expressions at metal surfaces47A comparative study of CO chemisorption on flat and stepped Ni surfaces using density functional theory53Chiral selection on inorganic crystalline surfaces488Complex organic molecules at metal surfaces: bonding, organisation and chirality741Enantiomeric electro-oxidation of d- and l-glucose on chiral gold single crystal surfaces39Enantiospecific electrodeposition of a chiral catalyst376Catalytic and Biological Activity of Organic Complexes of Precious Metals (A Review)5Naturally Chiral Surfaces85A new model of geometric chirality for two-dimensional continuous media and planar meta-materials38Assessment of heterochiral and homochiral glycine adlayers on Cu(110) using density functional theory99A simple model of enantioselective adsorption on chiral stationary phases20Chiral Crystal Faces of Common Rock-Forming Minerals65Direct STM Investigation of Cinchona Alkaloid Adsorption on Cu(111)10Chiral structures of lander molecules on Cu(100)15Enantioselectivity on Surfaces with Chiral Nanostructures3Highly enantioselective asymmetric autocatalysis induced by chiral ionic crystals of sodium chlorate and sodium bromate58Pt thin films on stepped SrTiO3 surfaces: SrTiO3(620) and SrTiO3(622)12Local and Global Chirality at Surfaces: Succinic Acid versus Tartaric Acid on Cu(110)145Molecular recognition in adsorption and electro-oxidation at chiral platinum surfaces50Ordered adsorption of ketones on Cu(643) revealed by scanning tunneling microscopy27Titration of chiral kink sites on Cu(643) using iodine adsorption13Adsorbate induced kink formation in straight step edges on Cu(533) and Cu(221)27Two-dimensional model for mixtures of enantiomers, bent hard needles: a Monte Carlo simulation20Amplification of Chirality from Molecules into Morphology of Crystals through Molecular Recognition105Expression of Molecular Chirality and Two-Dimensional Supramolecular Self-Assembly of Chiral, Racemic, and Achiral Monodendrons at the Liquid−Solid Interface37Chirally oriented heteroepitaxial thin films grown by pulsed laser deposition: Pt(621) on SrTiO3(621)22Enantiospecific Electrodeposition of Chiral CuO Films from Copper(II) Complexes of Tartaric and Amino Acids on Single-Crystal Au(001)53Adsorption-Induced Asymmetric Assembly from an Achiral Adsorbate31Enantioselective Separation on a Naturally Chiral Surface181Enantioselective synthesis induced by chiral epoxides in conjunction with asymmetric autocatalysis26Unequal-sphere packing model for the structural arrangement of the well-ordered adsorbate-substrate system7Structure of enantiopure and racemic alanine adlayers on Cu(110)100First-principles study of C adsorption, O adsorption, and CO dissociation on flat and stepped Ni surfaces51Structures Formed by the Chiral Assembly of Racemic Mixtures of Enantiomers: Iodination Products of Elaidic and Oleic Acids20Simulated Adsorption Properties and Synthesis Prospects of Homochiral Porous Solids Based on Their Heterochiral Analogs28Reflections on chiral metal surfaces and their potential for catalysis127Asymmetric Heterogeneous Catalysis: Science and Engineering249The symmetry and structure of crystalline surfaces46Interfacial Organization-Induced Supramolecular Chirality of the Langmuir−Schaefer Films of a Series of PPV Derivatives13Chemisorption and diffusion of hydrogen on surface and subsurface sites of flat and stepped nickel surfaces102Competition at Chiral Metal Surfaces: Fundamental Aspects of the Inversion of Enantioselectivity in Hydrogenations on Platinum95Surface Structure of Heterogeneous Catalysts: Cinchona and Tartaric Acid on Solid Surface7On the Separation of Nonadditive Symmetric Mixtures in Nanoscopic Slitlike Pores: A Simple Model for Racemic Fluids14Structures of Glycine, Enantiopure Alanine, and Racemic Alanine Adlayers on Cu(110) and Cu(100) Surfaces104Optical Recognition of Surface Chirality at Au(hkl) Single Crystalline Surfaces by Second Harmonic Generation Rotational Anisotropy16Chiral Symmetry Breaking in Two-Dimensional C60−ACA Intermixed Systems56Enantiospecific Chemisorption of Small Molecules on Intrinsically Chiral Cu Surfaces40Enantiospecific Chemisorption of Small Molecules on Intrinsically Chiral Cu Surfaces56Enantiospecific Adsorption of Cysteine at Chiral Kink Sites on Au(110)-(1×2)90First-principles studies of chiral step reconstructions of Cu(100) by adsorbed glycine and alanine47MCM-41-supported platinum carbonyl cluster-derived catalysts for asymmetric and nonasymmetric hydrogenation reactions49Bromine atom diffusion on stepped and kinked copper surfaces14Enantioselective Surface Chemistry of R-2-bromobutane on Cu(643)R&S and Cu(531)R&S37Enantioselective decomposition of chiral alkyl bromides on Cu(643)R&S: Effects of moving the chiral center24Structures of Dense Glycine and Alanine Adlayers on Chiral Cu(3,1,17) Surfaces37First principles study of the electronic and geometric structure of Cu(532)10Asymmetry Induction by Cooperative Intermolecular Hydrogen Bonds in Surface‐Anchored Layers of Achiral Molecules45Structure, dynamics and thermodynamics of a metal chiral surface: Cu(532)5Chiral Recognition of PVBA on Pd(111) and Ag(111) Surfaces5Surface Chirality of CuO Thin Films48Adsorption on nanostructured chiral surfaces studied by the Monte Carlo method13Enantiospecific electrodeposition of chiral CuO films on Cu(110) from aqueous Cu(II) tartrate and amino acid complexes11Chiral surfaces and metal/ceramic heteroepitaxy in the Pt/SrTiO3(621) system12Chiral crystallization of glutamic acid on self assembled films of cysteine39Anab initiostudy of adsorption of alanine on the chiral calcite surface36Enantioselective crystallization of histidine on chiral self-assembled films of cysteine21Chiral separation on a model adsorbent with periodic surface heterogeneity27Chirality Induction in Bulk Gold and Silver71Chirality at the Nano‐ and Micrometer Scale1Electrodeposition of Chiral Polymer–Carbon Nanotube Composite Films13Tuning Selectivity in Adsorption on Composite Chiral Surfaces15Theoretical studies of chiral adsorption on solid surfaces61Impact of Surface Symmetry on Growth-Induced Properties21Detection of Surface Chirality by Electrolyte Electroreflectance Rotational Anisotropy1Beyond the surface atlas: A roadmap and gazetteer for surface symmetry and structure110Asymmetric Catalysis at Chiral Metal Surfaces592Density functional theory study of β-hydride elimination of ethyl on flat and stepped Cu surfaces13Optical Recognition of Chirality at Surfaces by Vibrational Sum Frequency Generation Spectroscopy0Inducing enantioselectivity in electrodeposited CuO films by chiral etching14Chiral Surfaces and Enantioselective Catalysis7Spontaneous segregation on a hybrid chiral surface14Bridging the structure gap: Chemistry of nanostructured surfaces at well-defined defects123Enantioselective Chemisorption and Reactions on Model Chirally Modified Surfaces: 2-Butanol on l -Proline Templated Pd(111) Surfaces25The Chemistry of Intrinsically Chiral Surfaces41Characterization of enantiospecific chemisorption on chiral Cu surfaces vicinal to Cu(111) and Cu(100) using density functional theory25Enantiospecific Orientation of R–3-Methylcyclohexanone on the Chiral Cu(643)R/S Surfaces34Chiral nanopatterned surfaces as versatile enantiospecific adsorbents: A Monte Carlo model6First principles calculations of methylamine and methanol adsorption on hydroxylated quartz (0001)26Extended Surface Chirality for Enantiospecific Adsorption16Enantiospecific Adsorption of (R)-3-Methylcyclohexanone on Naturally Chiral Cu(531) R&S Surfaces34Monte Carlo Modeling of Chiral Adsorption on Nanostructured Chiral Surfaces and Slit Pores5Discrimination of Chiral Adsorption Configurations: Styrene on Germanium(100)10Surface Stress of Stepped Chiral Metal Surfaces9Facet enhanced photocatalytic effect with uniform single-crystalline zinc oxide nanodisks180Step decoration of chiral metal surfaces30Chirality induced by surface strain studied using scanning tunneling microscopy7Enantiospecific Adsorption of Amino Acids on Hydroxylated Quartz (0001)37Developing chiral surfaces for enantioselective chemical processing93Enantioselectivity on Naturally Chiral Metal Surfaces5Chirality at Metal Surfaces6Enantiospecific adsorption of amino acids on hydroxylated quartz (1010)33Chiral Surfaces: Accomplishments and Challenges178The effect of humic acid and ash on enantiomeric fraction change of chiral pollutants26Atomic Roughness of an Intrinsically Chiral Surface Orientation of an fcc Metal: Cu{531}29Mineral Surfaces, Geochemical Complexities, and the Origins of Life343Surface Chemistry Underpinning Enantioselective Heterogeneous Catalysis: Supramolecular Self-Assembly of Chiral Modifiers and Pro-Chiral Reagents on Ni{111}26Energetics of Chiral Imprinting of Cu(100) by Lysine45Adsorption Site Distributions on Cu(111), Cu(221), and Cu(643) as Determined by Xe Adsorption9Enantiospecific Wetting8XPS studies of the effects of modification pH on the interaction of methylacetoacetate with (S)-aspartic acid-modified Ni surfaces17Epitaxial electrodeposition of chiral CuO films from copper(ii) complexes of malic acid on Cu(111) and Cu(110) single crystals23Chiral Recognition at One-Dimensional Metal−Organic Coordination Networks Initiates the Ordering of Prochiral Catalytic Reagent Methylacetoacetate on Au{111}15Atomic and electronic structure of styrene on Ge(100)3Chemical speciation of adsorbed glycine on metal surfaces26Computational screening of homochiral metal–organic frameworks for enantioselective adsorption33Achiral Organic, Inorganic, and Metal Crystals as Auxiliaries for Asymmetric Transformations13Enantiospecific Adsorption of (R)-3-Methylcyclohexanone on Naturally Chiral Surfaces Vicinal to Cu(110)27Chirality in Amino Acid Overlayers on Cu Surfaces39Interaction of the Pro-Chiral Molecule, Methylacetoacetate, with (S)-Aspartic Acid Modified Ni{111}16Chiral biointerface materials221Enantiospecific Chemisorption of Amino Acids on Step Decorated Chiral Cu Surfaces24Chiral Surfaces Self-Assembling in One-Component Systems with Isotropic Interactions11Enantiospecific Desorption of R- and S-Propylene Oxide from d - or l -Lysine Modified Cu(100) Surfaces11Emerging chirality in nanoscience563Adsorption of lactic acid on chiral Pt surfaces: a density functional theory study13Enantioselectivity of (321) chiral noble metal surfaces: a density functional theory study of lactate adsorption5A Window on Surface Explosions: Tartaric Acid on Cu(110)44Enantioselective Separation on Naturally Chiral Metal Surfaces: d,l ‐Aspartic Acid on Cu(3,1,17)R&S Surfaces84Enantioselective Separation on Naturally Chiral Metal Surfaces: d,l ‐Aspartic Acid on Cu(3,1,17)R&S Surfaces6Adsorption of lactic acid on chiral Pt surfaces—A density functional theory study13Superenantioselective Chiral Surface Explosions74Enantioselectivity of (321) chiral noble metal surfaces: A density functional theory study of lactate adsorption6Enantioselective adsorption on rock-forming minerals: A thought experiment5The templated growth of a chiral transition metal chalcogenide5Investigation of the adsorption of amino acids on Pd(111): A density functional theory study15

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  1. ChemInform Abstract: Naturally Chiral Metal Surfaces as Enantiospecific Adsorbents

    ChemInform · 2001-08-07

    David S. Sholl, Aravind Asthagiri, Timothy D. Power

    Read original paper ↗ ·

  2. Induced Chiral Metal Surfaces in Asymmetric Hydrogenations?

    Reaction Kinetics and Catalysis Letters · 2001-11-01

    Antal Tungler

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  3. From Local Adsorption Stresses to Chiral Surfaces: (R,R)-Tartaric Acid on Ni(110)

    Journal of the American Chemical Society · 2001-12-22

    Vincent Humblot, Sam Haq, Christopher A. Muryn, Werner A. Hofer, Rasmita Raval

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  4. Effects of Surface Relaxation on Enantiospecific Adsorption on Naturally Chiral Pt Surfaces

    Topics in Catalysis · 2002-02-01

    Timothy D. Power, David S. Sholl

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  5. Thermal Fluctuations in the Structure of Naturally Chiral Pt surfaces

    Topics in Catalysis · 2002-02-01

    Aravind Asthagiri, Peter J. Feibelman, David S. Sholl

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  6. Can Chiral Single Walled Carbon Nanotubes Be Used as Enantiospecific Adsorbents?

    Journal of the American Chemical Society · 2002-02-09

    Timothy D. Power, Anastasios I. Skoulidas, David S. Sholl

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  7. Enantiospecific Desorption of Chiral Compounds from Chiral Cu(643) and Achiral Cu(111) Surfaces

    Journal of the American Chemical Society · 2002-02-13

    Joshua D. Horvath, Andrew J. Gellman

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  8. Atomically Detailed Models of the Effect of Thermal Roughening on the Enantiospecificity of Naturally Chiral Platinum Surfaces

    Langmuir · 2002-03-30

    Timothy D. Power, Aravind Asthagiri, David S. Sholl

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  9. Creating chiral architectures at metal surfaces

    Journal of Physics Condensed Matter · 2002-04-11

    Rasmita Raval

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  10. A computer simulation study of racemic mixtures

    Molecular Physics · 2002-08-10

    LARGO Lyndon, Carlos Vega, Luis G. MacDowell, J. R. Solana

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  11. Heterogeneous asymmetric reactions, 33. Novel interpretation of the enantioselective hydrogenation of a-ketoesters on Pt/alumina-cinchona alkaloid catalyst system

    Reaction Kinetics and Catalysis Letters · 2002-11-01

    Mihály Bartók, Katalin Balázsik, Ferenc Notheisz

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  12. Density Functional Theory Study of Enantiospecific Adsorption at Chiral Surfaces

    Journal of the American Chemical Society · 2002-11-13

    Željko Šljivančanin, Kurt V. Gothelf, Bjørk Hammer

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  13. 22 Enantiospecific heterogeneous catalysis without a chiral modifier

    Studies in surface science and catalysis · 2003-01-01

    Päivi Mäki‐Arvela, Tapio Salmi, Dmitry Yu. Murzin

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  14. Amplification of Chirality from Extremely Low to Greater than 99.5 % ee by Asymmetric Autocatalysis

    Angewandte Chemie International Edition · 2003-01-20

    Itaru Sato, Hiroki Urabe, Saori Ishiguro, Takanori Shibata, Kenso Soai

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  15. Amplification of Chirality from Extremely Low to Greater than 99.5 % ee by Asymmetric Autocatalysis

    Angewandte Chemie · 2003-01-20

    Itaru Sato, Hiroki Urabe, Saori Ishiguro, Takanori Shibata, Kenso Soai

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  16. Chiral expressions at metal surfaces

    Current Opinion in Solid State and Materials Science · 2003-02-01

    Rasmita Raval

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  17. A comparative study of CO chemisorption on flat and stepped Ni surfaces using density functional theory

    Surface Science · 2003-05-28

    Vaishali Shah, Tao Li, Kenneth L. Baumert, Hansong Cheng, David S. Sholl

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  18. Chiral selection on inorganic crystalline surfaces

    Nature Materials · 2003-05-30

    Robert M. Hazen, David S. Sholl

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  19. Complex organic molecules at metal surfaces: bonding, organisation and chirality

    Surface Science Reports · 2003-08-01

    S.M. Barlow, Rasmita Raval

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  20. Enantiomeric electro-oxidation of d- and l-glucose on chiral gold single crystal surfaces

    Electrochemistry Communications · 2003-09-01

    Ana C. Martins, Virginia C. Ferreira, A. Queirós, Ivo M. Aroso, Fernando Silva, Juan Miguel Feliu

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  21. Enantiospecific electrodeposition of a chiral catalyst

    Nature · 2003-10-01

    Jay A. Switzer, Hiten M. Kothari, Philippe Poizot, Shuji Nakanishi, Eric W. Bohannan

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  22. Catalytic and Biological Activity of Organic Complexes of Precious Metals (A Review)

    Pharmaceutical Chemistry Journal · 2003-11-01

    Rima P. Evstigneeva, Vasily P. Pchelkin

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  23. Naturally Chiral Surfaces

    Topics in Catalysis · 2003-11-01

    Joshua D. Horvath, Andrew J. Gellman

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  24. A new model of geometric chirality for two-dimensional continuous media and planar meta-materials

    Journal of Optics A Pure and Applied Optics · 2003-11-24

    A. Potts, Darren M. Bagnall, Nikolay I. Zheludev

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  25. Assessment of heterochiral and homochiral glycine adlayers on Cu(110) using density functional theory

    Surface Science · 2003-12-02

    Rees B. Rankin, David S. Sholl

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  26. A simple model of enantioselective adsorption on chiral stationary phases

    Applied Surface Science · 2003-12-31

    Paweł Szabelski

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  27. Chiral Crystal Faces of Common Rock-Forming Minerals

    Elsevier eBooks · 2004-01-01

    Robert M. Hazen

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  28. Direct STM Investigation of Cinchona Alkaloid Adsorption on Cu(111)

    Langmuir · 2004-03-19

    Qingmin Xu, Dong Wang, Mei‐Juan Han, Li‐Jun Wan, Chunli Bai

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  29. Chiral structures of lander molecules on Cu(100)

    Nanotechnology · 2004-03-24

    J Kuntze, X Ge, R Berndt

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  30. Enantioselectivity on Surfaces with Chiral Nanostructures

    CRC Press eBooks · 2004-03-31

    David M. Rampulla, Andrew J. Gellman

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  31. Highly enantioselective asymmetric autocatalysis induced by chiral ionic crystals of sodium chlorate and sodium bromate

    Journal of Molecular Catalysis A Chemical · 2004-04-26

    Itaru Sato, Kousuke Kadowaki, Yasushi Ohgo, Kenso Soai

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  32. Pt thin films on stepped SrTiO3 surfaces: SrTiO3(620) and SrTiO3(622)

    Journal of Molecular Catalysis A Chemical · 2004-04-29

    Aravind Asthagiri, David S. Sholl

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  33. Local and Global Chirality at Surfaces: Succinic Acid versus Tartaric Acid on Cu(110)

    Journal of the American Chemical Society · 2004-04-30

    Vincent Humblot, M. Ortega Lorenzo, Christopher J. Baddeley, Sam Haq, Rasmita Raval

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  34. Molecular recognition in adsorption and electro-oxidation at chiral platinum surfaces

    Journal of Molecular Catalysis A Chemical · 2004-05-08

    Omar Abdullah Hazzazi, Gary Anthony Attard, P.B. Wells

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  35. Ordered adsorption of ketones on Cu(643) revealed by scanning tunneling microscopy

    Journal of Molecular Catalysis A Chemical · 2004-05-11

    Xueying Zhao, Scott S. Perry

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  36. Titration of chiral kink sites on Cu(643) using iodine adsorption

    Surface Science · 2004-06-28

    Preeti Kamakoti, Joshua D. Horvath, Andrew J. Gellman, David S. Sholl

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  37. Adsorbate induced kink formation in straight step edges on Cu(533) and Cu(221)

    Surface Science · 2004-07-06

    Xueying Zhao, Scott S. Perry, Joshua D. Horvath, Andrew J. Gellman

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  38. Two-dimensional model for mixtures of enantiomers, bent hard needles: a Monte Carlo simulation

    Physica A Statistical Mechanics and its Applications · 2004-07-09

    Raúl A. Perusquı́a, Jörge Peón, Jacqueline Quintana

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  39. Amplification of Chirality from Molecules into Morphology of Crystals through Molecular Recognition

    Journal of the American Chemical Society · 2004-07-10

    Yuya Oaki, Hiroaki Imai

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  40. Expression of Molecular Chirality and Two-Dimensional Supramolecular Self-Assembly of Chiral, Racemic, and Achiral Monodendrons at the Liquid−Solid Interface

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    Wael Mamdouh, Hiroshi Uji‐i, Andrés E. Dulcey, Virgil Percec, Steven De Feyter, Frans Carl De Schryver

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  41. Chirally oriented heteroepitaxial thin films grown by pulsed laser deposition: Pt(621) on SrTiO3(621)

    Journal of Applied Physics · 2004-09-01

    Andrew J. Francis, Paul A. Salvador

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  42. Enantiospecific Electrodeposition of Chiral CuO Films from Copper(II) Complexes of Tartaric and Amino Acids on Single-Crystal Au(001)

    Chemistry of Materials · 2004-10-05

    Hiten M. Kothari, Elizabeth A. Kulp, Sansanee Boonsalee, Maxim P. Nikiforov, Eric W. Bohannan, Philippe Poizot, Shuji Nakanishi, Jay A. Switzer

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  43. Adsorption-Induced Asymmetric Assembly from an Achiral Adsorbate

    Journal of the American Chemical Society · 2004-10-07

    Yuguang Cai, Steven L. Bernasek

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  44. Enantioselective Separation on a Naturally Chiral Surface

    Journal of the American Chemical Society · 2004-10-26

    Joshua D. Horvath, Anjanette Koritnik, Preeti Kamakoti, David S. Sholl, Andrew J. Gellman

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  45. Enantioselective synthesis induced by chiral epoxides in conjunction with asymmetric autocatalysis

    Tetrahedron Asymmetry · 2004-11-01

    Tsuneomi Kawasaki, Masako Shimizu, Kenta Suzuki, Itaru Sato, Kenso Soai

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  46. Unequal-sphere packing model for the structural arrangement of the well-ordered adsorbate-substrate system

    Physical Review B · 2004-11-03

    Alexandre Tkatchenko, Nikola Batina

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  47. Structure of enantiopure and racemic alanine adlayers on Cu(110)

    Surface Science · 2004-11-05

    Rees B. Rankin, David S. Sholl

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  48. First-principles study of C adsorption, O adsorption, and CO dissociation on flat and stepped Ni surfaces

    The Journal of Chemical Physics · 2004-11-11

    Tao Li, Bhawna Bhatia, David S. Sholl

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  49. Structures Formed by the Chiral Assembly of Racemic Mixtures of Enantiomers: Iodination Products of Elaidic and Oleic Acids

    The Journal of Physical Chemistry B · 2004-12-10

    Yuguang Cai, Steven L. Bernasek

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  50. Simulated Adsorption Properties and Synthesis Prospects of Homochiral Porous Solids Based on Their Heterochiral Analogs

    Langmuir · 2004-12-16

    Louis A. Clark, Shaji Chempath, Randall Q. Snurr

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