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RESEARCH PAPER · Nature Materials · 2003

Chiral selection on inorganic crystalline surfaces

Robert M. Hazen, David S. Sholl

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Chiral selection on inorganic crystalline surfacesOriginalCreating chiral architectures at metal surfaces41Naturally Chiral Surfaces85Chiral Crystal Faces of Common Rock-Forming Minerals65Highly enantioselective asymmetric autocatalysis induced by chiral ionic crystals of sodium chlorate and sodium bromate58Preface to special issue on heterogeneous chiral catalysis2Pt thin films on stepped SrTiO3 surfaces: SrTiO3(620) and SrTiO3(622)12Molecular recognition in adsorption and electro-oxidation at chiral platinum surfaces50Step dynamics and step–step interactions on the chiral Cu(5 8 90) surface31Chiral indices of crystalline surfaces as a measure of enantioselective potential49Titration of chiral kink sites on Cu(643) using iodine adsorption13Correlation of pH-dependent surface interaction forces to amino acid adsorption: Implications for the origin of life112Amplification of Chirality from Molecules into Morphology of Crystals through Molecular Recognition105Chirally oriented heteroepitaxial thin films grown by pulsed laser deposition: Pt(621) on SrTiO3(621)22Enantioselective Separation on a Naturally Chiral Surface181Structure of enantiopure and racemic alanine adlayers on Cu(110)100Simulated Adsorption Properties and Synthesis Prospects of Homochiral Porous Solids Based on Their Heterochiral Analogs28Chirality in the RNA world and beyond24Reflections on chiral metal surfaces and their potential for catalysis127Isomer-Selective Adsorption of Amino Acids by Components of Natural Sediments24DFT study of Pt adsorption on low index SrTiO3 surfaces: SrTiO3(100), SrTiO3(111) and SrTiO3(110)45Interfacial Organization-Induced Supramolecular Chirality of the Langmuir−Schaefer Films of a Series of PPV Derivatives13Synthesis, Structure, and Stereochemistry of Trinuclear Metal Complexes Formed from the Phosphorus-Based Achiral Tripodal Ligand {P(S)[N(Me)NCHC6H4-o-OH]3} (LH3): Luminescent Properties of L2Cd3·2H2O29Genesis: Rocks, Minerals, and the Geochemical Origin of Life43Structures of Glycine, Enantiopure Alanine, and Racemic Alanine Adlayers on Cu(110) and Cu(100) Surfaces104The Hierarchical Architecture of Nacre and Its Mimetic Material237The Hierarchical Architecture of Nacre and Its Mimetic Material38Stochastic “Mirror Symmetry Breaking” via Self-Assembly, Reactivity and Amplification of Chirality: Relevance to Abiotic Conditions155Enantiospecific Chemisorption of Small Molecules on Intrinsically Chiral Cu Surfaces40Enantiospecific Chemisorption of Small Molecules on Intrinsically Chiral Cu Surfaces56A Supramolecular Chiroptical Switch Exclusively from an Achiral Amphiphile84Robert Boyle's chiral crystal chemistry: Computational re‐evaluation of enantioselective adsorption on quartz14Enantiospecific Adsorption of Cysteine at Chiral Kink Sites on Au(110)-(1×2)90Enantioselective Photooxidation of a Sulfide by a Chiral Ruthenium(II) Complex Immobilized on a Montmorillonite Clay Surface: The Role of Weak Interactions in Asymmetric Induction55The Role of the Chiral Modifier on the Enantioselective Hydrogenation of Methyl Pyruvate on Pt(111)14Enantiodiscrimination between an N‐Acetyl‐ L ‐cysteine SAM and Proline: An In Situ Spectroscopic and Computational Study20First-principles studies of chiral step reconstructions of Cu(100) by adsorbed glycine and alanine47Supramolecular Surface Chirality216Ab initiostudies of phonon softening and high-pressure phase transitions of α -quartz SiO263Chiral Templating of Surfaces: Adsorption of (S)-2-Methylbutanoic Acid on Pt(111) Single-Crystal Surfaces57With a Grain of Salt: What Halite Has to Offer to Discussions on the Origin of Life24Structures of Dense Glycine and Alanine Adlayers on Chiral Cu(3,1,17) Surfaces37Direction Specific Interactions of 1,4-Dicarboxylic Acid with Calcite Surfaces42Presidential Address to the Mineralogical Society of America, Salt Lake City, October 18, 2005: Mineral surfaces and the prebiotic selection and organization of biomolecules133Definitely Life but not Definitively46A Biomimetic Approach for Hierarchically Structured Inorganic Crystals through Self-Organization132Sub-micrometer polarimetry of chiral surfaces using near-field scanning optical microscopy11Stereospecific Interaction between Immune Cells and Chiral Surfaces148Chiral surfaces and metal/ceramic heteroepitaxy in the Pt/SrTiO3(621) system12Chiral crystallization of glutamic acid on self assembled films of cysteine39Probing Enantioselectivity with X-Ray Photoelectron Spectroscopy and Density Functional Theory69Anab initiostudy of adsorption of alanine on the chiral calcite surface36Enantioselective crystallization of histidine on chiral self-assembled films of cysteine21Stereospecific Morphogenesis of Aspartic Acid Helical Crystals through Molecular Recognition25Enhancing Enantioselectivity of Electrodeposited CuO Films by Chiral Etching13Intrinsic asymmetries of amino acid enantiomers and their peptides: A possible role in the origin of biochirality45Tuning Selectivity in Adsorption on Composite Chiral Surfaces15Direct Visualization of Enantiospecific Substitution of Chiral Guest Molecules into Heterochiral Molecular Assemblies at Surfaces45Direct Visualization of Enantiospecific Substitution of Chiral Guest Molecules into Heterochiral Molecular Assemblies at Surfaces16Theoretical studies of chiral adsorption on solid surfaces61Asymmetric Catalysis at Chiral Metal Surfaces592Electrochemical Biomineralization: The Deposition of Calcite with Chiral Morphologies43Characteristics of Amino Acids in the Atmospheric and Marine Environment3Complete asymmetric amplification of ethylenediammonium sulfate using an abrasion/grinding technique78Fabrication of Si(110)-16×2 Single-domain Surface0Inducing enantioselectivity in electrodeposited CuO films by chiral etching14Dendritic crystal growth, differential circular scattering, and the origin of biomolecular homochirality17The first contribution of capillary electrophoresis to the study of abiotic origins of homochirality: Investigation of the enantioselective adsorption of 3‐carboxy adipic acid on minerals11The Chemistry of Intrinsically Chiral Surfaces41Characterization of enantiospecific chemisorption on chiral Cu surfaces vicinal to Cu(111) and Cu(100) using density functional theory25Controlling the surface chirality of Si(110)20Chiral nanopatterned surfaces as versatile enantiospecific adsorbents: A Monte Carlo model6First principles calculations of methylamine and methanol adsorption on hydroxylated quartz (0001)26Supramolecular Chiroptical Switches Based on Achiral Molecules65Crystallization of Sodium Chlorate with d -Glucose Co-Solute Is Not Enantioselective22Extended Surface Chirality for Enantiospecific Adsorption16Stereoselective Interaction between DNA and Chiral Surfaces85Monte Carlo Modeling of Chiral Adsorption on Nanostructured Chiral Surfaces and Slit Pores5Manipulating Crystal Orientation in Nanoscale Cylindrical Pores by Stereochemical Inhibition94Postsynthetic Modification of Gold Nanoparticles with Calix[4]arene Enantiomers: Origin of Chiral Surface Plasmon Resonance74Biomimetic Modelling of Copper Enzymes: Synthesis, Characterization, EPR Analysis and Enantioselective Catalytic Oxidations by a New Chiral Trinuclear Copper(II) Complex28Amino acid directed mirror symmetry breaking and chiral amplification of ethylenediammonium sulfate crystals27Chiral expression from molecular assemblies at metal surfaces: insights from surface science techniques291Surface Stress of Stepped Chiral Metal Surfaces9Nanoscale Exploration of Molecular and Supramolecular Chirality at Metal Surfaces under Ultrahigh‐Vacuum Conditions2SiC(0001) 3 × 3 Heterochirality Revealed by Single-Molecule STM Imaging19Turiner Stereochemie: Eligio Peruccas Enantioselektivität und Primo Levis Asymmetrie6Turinese Stereochemistry: Eligio Perucca's Enantioselectivity and Primo Levi's Asymmetry19Chiral Assembly from Achiral Rod−Coil Molecules Triggered by Compression at the Air−Water Interface36Selective Adsorption of DNA on Chiral Surfaces: Supercoiled or Relaxed Conformation48Selective Adsorption of DNA on Chiral Surfaces: Supercoiled or Relaxed Conformation19The adsorption and stability of sulfur containing amino acids on Cu{531}47Step decoration of chiral metal surfaces30Enantiospecific Adsorption of Amino Acids on Hydroxylated Quartz (0001)37Nucleotide‐Catalyzed Conversion of Racemic Zeolite‐Type Zincophosphate into Enantioenriched Crystals55Nucleotide‐Catalyzed Conversion of Racemic Zeolite‐Type Zincophosphate into Enantioenriched Crystals9Fundamental Aspects of the Chiral Modification of Platinum with Peptides: Asymmetric Induction in Hydrogenation of Activated Ketones16Absolute Asymmetric Reduction Based on the Relative Orientation of Achiral Reactants40Absolute Asymmetric Reduction Based on the Relative Orientation of Achiral Reactants11Developing chiral surfaces for enantioselective chemical processing93Emergence and the experimental pursuit of the origin of life3Enantioselectivity on Naturally Chiral Metal Surfaces5Reversible Mechanical Induction of Optical Activity in Solutions of Soft‐Matter Nanophases37Asymmetric Autocatalysis Induced by Chiral Crystals of Achiral Tetraphenylethylenes50Chiral Biases in Solids by Effect of Shear Gradients: A Speculation on the Deterministic Origin of Biological Homochirality13Chirality at Metal Surfaces6Amplification of chirality as a pathway to biological homochirality42Concept of Absolute Enantioselective Separation1Separation of chiral molecules by temperature programmed desorption2Chiral supramolecular self-assembly of rubrene14Emergence of helical morphologies with crystals: twisted growth under diffusion-limited conditions and chirality control with molecular recognition42Enantiospecific adsorption of amino acids on hydroxylated quartz (1010)33Single-stranded DNA adsorption on chiral molecule coated Au surface: a molecular dynamics study12Stereochemistry triggered differential cell behaviours on chiral polymer surfaces88Chiral Surfaces: Accomplishments and Challenges178The effect of humic acid and ash on enantiomeric fraction change of chiral pollutants26Asymmetric Amplification and Autocatalysis24Generation of Absolute Controlled Crystal Chirality by the Removal of Crystal Water from Achiral Crystal of Nucleobase Cytosine65The Silicate-Mediated Formose Reaction: Bottom-Up Synthesis of Sugar Silicates181Mineral Surfaces, Geochemical Complexities, and the Origins of Life343Circular Dichroism Tensor of a Triarylmethyl Propeller in Sodium Chlorate Crystals27Recognition behavior of chiral nanocomposites toward biomolecules and its application in electrochemical immunoassay6Zucker an Kieselsäure präbiotisch0Possible origin of life between mica sheets81Mechanical resolution of chiral objects in achiral media: Where is the size limit?16Adsorption Site Distributions on Cu(111), Cu(221), and Cu(643) as Determined by Xe Adsorption9Enantioselective Recognition between Polydiacetylene Nucleolipid Monolayers and Complementary Oligonucleotides18Linking Surface Potential and Deprotonation in Nanoporous Silica: Second Harmonic Generation and Acid/Base Titration62Chiral Molecules on Surfaces10Chiral Poly(fluorene-alt-benzothiadiazole) (PFBT) and Nanocomposites with Gold Nanoparticles: Plasmonically and Structurally Enhanced Chirality138Enantiospecific Wetting8Generation of Chirality by Crystallization of Achiral Organic Compounds and Asymmetric Autocatalysis Induced by Chiral Organic Crystals0On the Origin of Biological Functions3STM Characterization of Supramolecular Materials with Potential for Organic Electronics and Nanotechnology0Crystalline Architectures as Templates of Relevance to the Origins of Homochirality283Controlling Chiral Organization of Molecular Rods on Au(111) by Molecular Design34Biomimetic Smart Interface Materials for Biological Applications261Enantioselective Synthesis Induced by Chiral Crystal Composed of dl -Serine in Conjunction with Asymmetric Autocatalysis34Chiral Optical Films Based on Achiral Chromophore Guests40Chiral Design for Polymeric Biointerface: The Influence of Surface Chirality on Protein Adsorption116Amino Acids Functionalized Heterogeneous Chiral Catalyst0Chemical speciation of adsorbed glycine on metal surfaces26Chiral Induction by Seeding Surface Assemblies of Chiral Switches55Asymmetric Induction Arising from Enantiomerically Enriched Carbon-13 Isotopomers and Highly Sensitive Chiral Discrimination by Asymmetric Autocatalysis65Achiral Organic, Inorganic, and Metal Crystals as Auxiliaries for Asymmetric Transformations13Control over the crystal phase, crystallinity, morphology of AgVO3 via protein inducing process20Chiral Symmetry Breaking Observed for Cysteine on the Au(110)-(1×2) Surface21The Study of Chiral Adsorption Systems Using Synchrotron-Based Structural and Spectroscopic Techniques: Stereospecific Adsorption of Serine on Au-Modified Chiral Cu{531} Surfaces27Determining the Orientation of a Chiral Substrate Using Full-Hemisphere Angle-Resolved Photoelectron Spectroscopy5Enantioselective recognition of mandelic acid based on γ-globulin modified glassy carbon electrode34Two-Dimensional Chiral Molecular Networks from Achiral Building Blocks: A Computational Study13

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  2. Naturally Chiral Surfaces

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  3. Chiral Crystal Faces of Common Rock-Forming Minerals

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  4. Highly enantioselective asymmetric autocatalysis induced by chiral ionic crystals of sodium chlorate and sodium bromate

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  5. Preface to special issue on heterogeneous chiral catalysis

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  6. Pt thin films on stepped SrTiO3 surfaces: SrTiO3(620) and SrTiO3(622)

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  7. Molecular recognition in adsorption and electro-oxidation at chiral platinum surfaces

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  8. Step dynamics and step–step interactions on the chiral Cu(5 8 90) surface

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  9. Chiral indices of crystalline surfaces as a measure of enantioselective potential

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  10. Titration of chiral kink sites on Cu(643) using iodine adsorption

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  11. Correlation of pH-dependent surface interaction forces to amino acid adsorption: Implications for the origin of life

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  12. Amplification of Chirality from Molecules into Morphology of Crystals through Molecular Recognition

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  13. Chirally oriented heteroepitaxial thin films grown by pulsed laser deposition: Pt(621) on SrTiO3(621)

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  14. Enantioselective Separation on a Naturally Chiral Surface

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  15. Structure of enantiopure and racemic alanine adlayers on Cu(110)

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  16. Simulated Adsorption Properties and Synthesis Prospects of Homochiral Porous Solids Based on Their Heterochiral Analogs

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  17. Chirality in the RNA world and beyond

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  18. Reflections on chiral metal surfaces and their potential for catalysis

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  19. Isomer-Selective Adsorption of Amino Acids by Components of Natural Sediments

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  20. DFT study of Pt adsorption on low index SrTiO3 surfaces: SrTiO3(100), SrTiO3(111) and SrTiO3(110)

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  21. Interfacial Organization-Induced Supramolecular Chirality of the Langmuir−Schaefer Films of a Series of PPV Derivatives

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  22. Synthesis, Structure, and Stereochemistry of Trinuclear Metal Complexes Formed from the Phosphorus-Based Achiral Tripodal Ligand {P(S)[N(Me)NCHC6H4-o-OH]3} (LH3): Luminescent Properties of L2Cd3·2H2O

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  23. Genesis: Rocks, Minerals, and the Geochemical Origin of Life

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  24. Structures of Glycine, Enantiopure Alanine, and Racemic Alanine Adlayers on Cu(110) and Cu(100) Surfaces

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  25. The Hierarchical Architecture of Nacre and Its Mimetic Material

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  26. The Hierarchical Architecture of Nacre and Its Mimetic Material

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  27. Stochastic “Mirror Symmetry Breaking” via Self-Assembly, Reactivity and Amplification of Chirality: Relevance to Abiotic Conditions

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  28. Enantiospecific Chemisorption of Small Molecules on Intrinsically Chiral Cu Surfaces

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  29. Enantiospecific Chemisorption of Small Molecules on Intrinsically Chiral Cu Surfaces

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  30. A Supramolecular Chiroptical Switch Exclusively from an Achiral Amphiphile

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  31. Robert Boyle's chiral crystal chemistry: Computational re‐evaluation of enantioselective adsorption on quartz

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  32. Enantiospecific Adsorption of Cysteine at Chiral Kink Sites on Au(110)-(1×2)

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  33. Enantioselective Photooxidation of a Sulfide by a Chiral Ruthenium(II) Complex Immobilized on a Montmorillonite Clay Surface: The Role of Weak Interactions in Asymmetric Induction

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  34. The Role of the Chiral Modifier on the Enantioselective Hydrogenation of Methyl Pyruvate on Pt(111)

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  35. Enantiodiscrimination between an N‐Acetyl‐ L ‐cysteine SAM and Proline: An In Situ Spectroscopic and Computational Study

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  36. First-principles studies of chiral step reconstructions of Cu(100) by adsorbed glycine and alanine

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  37. Supramolecular Surface Chirality

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  38. Ab initiostudies of phonon softening and high-pressure phase transitions of α -quartz SiO2

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  39. Chiral Templating of Surfaces: Adsorption of (S)-2-Methylbutanoic Acid on Pt(111) Single-Crystal Surfaces

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  40. With a Grain of Salt: What Halite Has to Offer to Discussions on the Origin of Life

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  41. Structures of Dense Glycine and Alanine Adlayers on Chiral Cu(3,1,17) Surfaces

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  42. Direction Specific Interactions of 1,4-Dicarboxylic Acid with Calcite Surfaces

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  43. Presidential Address to the Mineralogical Society of America, Salt Lake City, October 18, 2005: Mineral surfaces and the prebiotic selection and organization of biomolecules

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  44. Definitely Life but not Definitively

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  45. A Biomimetic Approach for Hierarchically Structured Inorganic Crystals through Self-Organization

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  46. Sub-micrometer polarimetry of chiral surfaces using near-field scanning optical microscopy

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  47. Stereospecific Interaction between Immune Cells and Chiral Surfaces

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  48. Chiral surfaces and metal/ceramic heteroepitaxy in the Pt/SrTiO3(621) system

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    Andrew J. Francis, Anjanette Koritnik, Andrew J. Gellman, Paul A. Salvador

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  49. Chiral crystallization of glutamic acid on self assembled films of cysteine

    Chirality · 2007-03-12

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  50. Probing Enantioselectivity with X-Ray Photoelectron Spectroscopy and Density Functional Theory

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