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RESEARCH PAPER · Chemistry of Materials · 2019

Probing Electrochemical Mg-Ion Activity in MgCr 2– x V x O 4 Spinel Oxides

Bob Jin Kwon, Ka-Cheong Lau, Haesun Park, Yimin A. Wu, Krista L. Hawthorne, Haifeng Li, Soojeong Kim, Igor L. Bolotin, Timothy T. Fister, Peter Zapol, Robert F. Klie, Jordi Cabana, Chen Liao, Saul H. Lapidus, Baris Key, John T. Vaughey

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Probing Electrochemical Mg-Ion Activity in MgCr 2– x V x O 4 Spinel OxidesOriginalEnhanced charge storage of nanometric ζ-V 2 O 5 in Mg electrolytes23Energy storage emerging: A perspective from the Joint Center for Energy Storage Research344Phase evolution and microwave dielectric properties of the Li2(1+x)ZnGe3O8 spinel oxides6High Voltage Mg-Ion Battery Cathode via a Solid Solution Cr–Mn Spinel Oxide72Anion Association Strength as a Unifying Descriptor for the Reversibility of Divalent Metal Deposition in Nonaqueous Electrolytes42High Capacity for Mg2+ Deintercalation in Spinel Vanadium Oxide Nanocrystals67Electron-beam-induced Spinel to Defect Rocksalt Phase Transition in MgCrMnO42Influence of particle size on the structural and electrical properties of Mn1.1Co1.5Fe0.4O4 ceramics18High-Voltage Phosphate Cathodes for Rechargeable Ca-Ion Batteries121Control of crystal size tailors the electrochemical performance of α-V 2 O 5 as a Mg 2+ intercalation host12Phase Transition Behavior of MgMn 2 O 4 Spinel Oxide Cathode during Magnesium Ion Insertion44The Quest for Functional Oxide Cathodes for Magnesium Batteries: A Critical Perspective77Operando X-ray Diffraction Studies of the Mg-Ion Migration Mechanisms in Spinel Cathodes for Rechargeable Mg-Ion Batteries42Improving the microwave dielectric properties of Ga2[LiGa3]O8 inverse spinel by enhancing B-site ordering degree4Layered Transition Metal Oxides as Ca Intercalation Cathodes: A Systematic First‐Principles Evaluation24Synthesis and Characterization of Magnesium Vanadates as Potential Magnesium‐Ion Cathode Materials through an Ab Initio Guided Carbothermal Reduction Approach**3Synthesis and Characterization of Magnesium Vanadates as Potential Magnesium‐Ion Cathode Materials through an Ab Initio Guided Carbothermal Reduction Approach**13Solvation, Rational Design, and Interfaces: Development of Divalent Electrolytes6Facile Electrochemical Mg-Ion Transport in a Defect-Free Spinel Oxide14Recent advances in kinetic optimizations of cathode materials for rechargeable magnesium batteries56Unconventional Charge Transport in MgCr2O4 and Implications for Battery Intercalation Hosts26Room-Temperature Calcium Plating and Stripping Using a Perfluoroalkoxyaluminate Anion Electrolyte33A critical review of vanadium-based electrode materials for rechargeable magnesium batteries45Magnesium Battery Electrolytes with Improved Oxidative Stability Enabled by Selective Solvation in Fluorinated Solvents23Oxide Spinels with Superior Mg Conductivity15Electrolyte Reactivity on the MgV2O4 Cathode Surface10Design Strategies of Spinel Oxide Frameworks Enabling Reversible Mg-Ion Intercalation18Mixed-Anion Contact Ion-Pair Formation Enabling Improved Performance of Halide-Free Mg-Ion Electrolytes22Electrochemical reactivity and passivation of organic electrolytes at spinel MgCrMnO 4 cathode interfaces for rechargeable high voltage magnesium-ion batteries11Realization of Mg 2+ intercalation in a thermodynamically stable layer-structured oxide6Phase Transition Mechanism of ZnMn 2 O 4 Spinel Oxide with Electrochemical Magnesium-Ion Insertion3Monitoring Structural Changes during Electrochemical Cycling of Solid-Solution Spinel Oxide MgCrVO43Intercalation mechanism of solvated magnesium electrolytes on spinel cathode surfaces5Atomic-Scale Tracking of Beam-Induced Phase Transitions in MgCr1.5Mn0.5O44Demonstration of MgCr2–xMnxO4 Spinel Oxide Cathodes in High-Voltage Mg Batteries5First-Principles Investigation on MgMn2O4–yFy: Fluorine Doping as a Strategy for Magnesium-Ion Batteries beyond the Usual Cation Substitution3Exploration of Amorphous V 2 O 5 as Cathode for Magnesium Batteries10

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  1. Enhanced charge storage of nanometric ζ-V 2 O 5 in Mg electrolytes

    Nanoscale · 2020-01-01

    Ian D. Johnson, Gene M. Nolis, Liang Yin, Hyun Deog Yoo, Prakash Kumar Parajuli, Arijita Mukherjee, Justin L. Andrews, Mario Lopez, Robert F. Klie, Sarbajit Banerjee, Brian J. Ingram, Saul H. Lapidus, Jordi Cabana, Jawwad Arshad Darr

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  2. Energy storage emerging: A perspective from the Joint Center for Energy Storage Research

    Proceedings of the National Academy of Sciences · 2020-06-08

    Lynn Trahey, Fikile Richard Brushett, Nitash P. Balsara, Gerbrand Ceder, Lei Cheng, Yet‐Ming Chiang, Nathan T. Hahn, Brian J. Ingram, Shelley D. Minteer, Jeffrey S. Moore, Karl Todd Mueller, Linda F. Nazar, Kristin Aslaug Persson, Donald J. Siegel, Kang Xu, Kevin R. Zavadil, Venkat N. Srinivasan, G. W. Crabtree

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  3. Phase evolution and microwave dielectric properties of the Li2(1+x)ZnGe3O8 spinel oxides

    Journal of Materials Science Materials in Electronics · 2020-07-06

    Weishuang Fang, Laiyuan Ao, Ying Tang, Jie Li, Huaicheng Xiang, Zhiwei Zhang, Qianbiao Du, Liang Fang

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  4. High Voltage Mg-Ion Battery Cathode via a Solid Solution Cr–Mn Spinel Oxide

    Chemistry of Materials · 2020-07-14

    Bob Jin Kwon, Liang Yin, Haesun Park, Prakash Kumar Parajuli, Khagesh Kumar, Sang-Hyeon Kim, Mengxi Yang, Megan Murphy, Peter Zapol, Chen Liao, Timothy T. Fister, Robert F. Klie, Jordi Cabana, John T. Vaughey, Saul H. Lapidus, Baris Key

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  5. Anion Association Strength as a Unifying Descriptor for the Reversibility of Divalent Metal Deposition in Nonaqueous Electrolytes

    ACS Applied Materials & Interfaces · 2020-07-15

    Justin Grant Connell, Milena Zorko, Garvit Agarwal, Mengxi Yang, Chen Liao, Rajeev S. Assary, Dusan S. Strmcnik, Nenad M. Marković

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  6. High Capacity for Mg2+ Deintercalation in Spinel Vanadium Oxide Nanocrystals

    ACS Energy Letters · 2020-07-23

    Linhua Hu, Jacob R. Jokisaari, Bob Jin Kwon, Liang Yin, Soojeong Kim, Haesun Park, Saul H. Lapidus, Robert F. Klie, Baris Key, Peter Zapol, Brian J. Ingram, John T. Vaughey, Jordi Cabana

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  7. Electron-beam-induced Spinel to Defect Rocksalt Phase Transition in MgCrMnO4

    Microscopy and Microanalysis · 2020-07-30

    Prakash Kumar Parajuli, Bob Jin Kwon, Baris Key, Jordi Cabana, Brian J. Ingram, Robert F. Klie

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  8. Influence of particle size on the structural and electrical properties of Mn1.1Co1.5Fe0.4O4 ceramics

    Scripta Materialia · 2020-07-30

    Bing Wang, Aimin Chang, Junhua Wang, Jincheng Yao

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  9. High-Voltage Phosphate Cathodes for Rechargeable Ca-Ion Batteries

    ACS Energy Letters · 2020-09-14

    Sang-Hyeon Kim, Liang Yin, Myeong Hwan Lee, Prakash Kumar Parajuli, Lauren Blanc, Timothy T. Fister, Haesun Park, Bob Jin Kwon, Brian J. Ingram, Peter Zapol, Robert F. Klie, Kisuk Kang, Linda F. Nazar, Saul H. Lapidus, John T. Vaughey

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  10. Control of crystal size tailors the electrochemical performance of α-V 2 O 5 as a Mg 2+ intercalation host

    Nanoscale · 2021-01-01

    Ian D. Johnson, Natalie Stapleton, Gene M. Nolis, Dustin Bauer, Prakash Kumar Parajuli, Hyun Deog Yoo, Liang Yin, Brian J. Ingram, Robert F. Klie, Saul H. Lapidus, Jawwad Arshad Darr, Jordi Cabana

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  11. Phase Transition Behavior of MgMn 2 O 4 Spinel Oxide Cathode during Magnesium Ion Insertion

    Chemistry of Materials · 2021-01-29

    Feilure Tuerxun, Saeko Otani, Kentaro Yamamoto, Toshiyuki Matsunaga, Hiroaki Imai, Toshihiko Mandai, Toshiki Watanabe, Tomoki Uchiyama, Kiyoshi Kanamura, Yoshiharu Uchimoto

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  12. The Quest for Functional Oxide Cathodes for Magnesium Batteries: A Critical Perspective

    ACS Energy Letters · 2021-04-26

    Ian D. Johnson, Brian J. Ingram, Jordi Cabana

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  13. Operando X-ray Diffraction Studies of the Mg-Ion Migration Mechanisms in Spinel Cathodes for Rechargeable Mg-Ion Batteries

    Journal of the American Chemical Society · 2021-07-08

    Liang Yin, Bob Jin Kwon, Yunyeong Choi, Christopher J. Bartel, Mengxi Yang, Chen Liao, Baris Key, Gerbrand Ceder, Saul H. Lapidus

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  14. Improving the microwave dielectric properties of Ga2[LiGa3]O8 inverse spinel by enhancing B-site ordering degree

    Ceramics International · 2021-09-16

    Weishuang Fang, Laiyuan Ao, Ying Tang, Jie Li, Yihua Sun, Liang Fang

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  15. Layered Transition Metal Oxides as Ca Intercalation Cathodes: A Systematic First‐Principles Evaluation

    Advanced Energy Materials · 2021-11-06

    Haesun Park, Christopher J. Bartel, Gerbrand Ceder, Peter Zapol

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  16. Synthesis and Characterization of Magnesium Vanadates as Potential Magnesium‐Ion Cathode Materials through an Ab Initio Guided Carbothermal Reduction Approach**

    Angewandte Chemie · 2021-12-01

    Jeongjae Lee, Sunita Dey, Siân E. Dutton, Clare P. Grey

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  17. Synthesis and Characterization of Magnesium Vanadates as Potential Magnesium‐Ion Cathode Materials through an Ab Initio Guided Carbothermal Reduction Approach**

    Angewandte Chemie International Edition · 2021-12-02

    Jeongjae Lee, Sunita Dey, Siân E. Dutton, Clare P. Grey

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  18. Solvation, Rational Design, and Interfaces: Development of Divalent Electrolytes

    Frontiers in Energy Research · 2022-01-05

    Noel J. Leon, Mingfu He, Chen Liao

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  19. Facile Electrochemical Mg-Ion Transport in a Defect-Free Spinel Oxide

    Chemistry of Materials · 2022-04-07

    Bob Jin Kwon, Liang Yin, Indrani Roy, Noel J. Leon, Khagesh Kumar, Jae Jin Kim, Jinhyup Han, Jihyeon Gim, Chen Liao, Saul H. Lapidus, Jordi Cabana, Baris Key

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  20. Recent advances in kinetic optimizations of cathode materials for rechargeable magnesium batteries

    Coordination Chemistry Reviews · 2022-05-13

    Song Chen, Shuang Fan, Henan Li, Yumeng Shi, Hui Ying Yang

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  21. Unconventional Charge Transport in MgCr2O4 and Implications for Battery Intercalation Hosts

    Journal of the American Chemical Society · 2022-07-27

    Ian D. Johnson, Aashutosh N. Mistry, Liang Yin, Megan Murphy, Mark Wolfman, Timothy T. Fister, Saul H. Lapidus, Jordi Cabana, Venkat N. Srinivasan, Brian J. Ingram

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  22. Room-Temperature Calcium Plating and Stripping Using a Perfluoroalkoxyaluminate Anion Electrolyte

    The Journal of Physical Chemistry C · 2022-07-29

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  23. A critical review of vanadium-based electrode materials for rechargeable magnesium batteries

    Journal of Material Science and Technology · 2023-03-02

    Xiu‐Fen Ma, Hongyi Li, Weiwei Ren, Daibo Gao, Fuyu Chen, Jiang Diao, Bing Xie, Guangsheng Huang, Jingfeng Wang, Fusheng Pan

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  24. Magnesium Battery Electrolytes with Improved Oxidative Stability Enabled by Selective Solvation in Fluorinated Solvents

    ACS Applied Energy Materials · 2023-03-13

    Nathan T. Hahn, Ethan Phillip Kamphaus, Ying Chen, Vijayakumar Murugesan, Karl Todd Mueller, Lei Cheng, Kevin R. Zavadil

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  25. Oxide Spinels with Superior Mg Conductivity

    Chemistry of Materials · 2023-06-14

    Mohsen Sotoudeh, Manuel Dillenz, Johannes Döhn, Julian Hansen, Sonia Dsoke, Axel Groß

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  26. Electrolyte Reactivity on the MgV2O4 Cathode Surface

    ACS Applied Materials & Interfaces · 2023-10-08

    Heonjae Jeong, Dan Thien Nguyen, Yingjie Yang, D. Bruce Buchholz, Guennadi Evmenenko, Jinghua Guo, Feipeng Yang, Paul C. Redfern, Jian Zhi Hu, Karl Todd Mueller, Robert F. Klie, Vijayakumar Murugesan, Justin Grant Connell, Venkateshkumar Prabhakaran, Lei Cheng

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  27. Design Strategies of Spinel Oxide Frameworks Enabling Reversible Mg-Ion Intercalation

    Accounts of Chemical Research · 2023-12-19

    Bob Jin Kwon, Saul H. Lapidus, John T. Vaughey, Gerbrand Ceder, Jordi Cabana, Baris Key

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  28. Mixed-Anion Contact Ion-Pair Formation Enabling Improved Performance of Halide-Free Mg-Ion Electrolytes

    ACS Applied Materials & Interfaces · 2023-12-26

    Stefan Ilić, Sydney Nicole Lavan, Noel J. Leon, Haoyu Liu, Akash Jain, Baris Key, Rajeev S. Assary, Chen Liao, Justin Grant Connell

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  29. Electrochemical reactivity and passivation of organic electrolytes at spinel MgCrMnO 4 cathode interfaces for rechargeable high voltage magnesium-ion batteries

    Journal of Materials Chemistry A · 2024-01-01

    Zhenzhen Yang, Jiyu Cai, Evelyna Tsi Hsin Wang, Maksim A. Sultanov, Lihong Gao, Xianyang Wu, Chen Liao, Zonghai Chen, Jianguo Wen, Lynn Trahey, Brian J. Ingram

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  30. Realization of Mg 2+ intercalation in a thermodynamically stable layer-structured oxide

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    Junhao Zhang, Haotian Guan, Jili Yue, Yangfan Lu, Q. X. Li, Guangsheng Huang, Jingfeng Wang, Baihua Qu, Fusheng Pan

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  31. Phase Transition Mechanism of ZnMn 2 O 4 Spinel Oxide with Electrochemical Magnesium-Ion Insertion

    The Journal of Physical Chemistry C · 2024-01-26

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  32. Monitoring Structural Changes during Electrochemical Cycling of Solid-Solution Spinel Oxide MgCrVO4

    Inorganic Chemistry · 2024-01-31

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  33. Intercalation mechanism of solvated magnesium electrolytes on spinel cathode surfaces

    Journal of Power Sources · 2024-03-12

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  34. Atomic-Scale Tracking of Beam-Induced Phase Transitions in MgCr1.5Mn0.5O4

    Chemistry of Materials · 2025-02-10

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  35. Demonstration of MgCr2–xMnxO4 Spinel Oxide Cathodes in High-Voltage Mg Batteries

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  36. First-Principles Investigation on MgMn2O4–yFy: Fluorine Doping as a Strategy for Magnesium-Ion Batteries beyond the Usual Cation Substitution

    ACS Applied Energy Materials · 2025-07-03

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  37. Exploration of Amorphous V 2 O 5 as Cathode for Magnesium Batteries

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