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RESEARCH PAPER · Inorganic Chemistry · 2018

Tunable Optical Properties and Enhanced Thermal Quenching of Non-Rare-Earth Double-Perovskite (Ba1–xSrx)2YSbO6:Mn4+ Red Phosphors Based on Composition Modulation

Jiasong Zhong, Daqin Chen, Shuo Yuan, Meijiao Liu, Yongjun Yuan, Yiwen Zhu, Xinyue Li, Zhenguo Ji

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Tunable Optical Properties and Enhanced Thermal Quenching of Non-Rare-Earth Double-Perovskite (Ba1–xSrx)2YSbO6:Mn4+ Red Phosphors Based on Composition ModulationOriginalHighly efficient rare-earth-free deep red emitting phosphor La 2 Li 1−y Sb 1−x O 6 : x Mn 4+ , y Mg 2+ : application in high-power warm w-LEDs63Photoluminescence tuning in a novel Bi 3+ /Mn 4+ co-doped La 2 ATiO 6 :(A = Mg, Zn) double perovskite structure: phase transition and energy transfer78Preparation, characterization, and luminescence properties of double perovskite SrLaMgSbO 6 :Mn 4+ far-red emitting phosphors for indoor plant growth lighting29Synthesis, structure, and luminescence characteristics of far-red emitting Mn 4+ -activated LaScO 3 perovskite phosphors for plant growth15Luminescence properties of a non-rare-earth doped oxyfluoride LiAl4O6F:Mn4+ red phosphor for solid-state lighting72A novel rare-earth free red-emitting Li3Mg2SbO6:Mn4+ phosphor-in-glass for warm w-LEDs: Synthesis, structure, and luminescence properties101Structure and luminescence properties of Zn3V2O8 yellow phosphor for white light emitting diodes36Luminescence quenching properties of Sr2Ga2GeO7: Pr3+ with and without traps participation18Double perovskite A 2 LaNbO 6 :Mn 4+ ,Eu 3+ (A = Ba, Ca) phosphors: potential applications in optical temperature sensing121Enhanced deep-red emission from Mn 4+ /Mg 2+ co-doped CaGdAlO 4 phosphors for plant cultivation63Enhanced photoluminescence and thermal properties due to size mismatch in Mg 2 Ti x Ge 1−x O 4 :Mn 4+ deep-red phosphors44Facile preparation of Eu 3+ -activated Ca 7 (VO 4 ) 4 O nanoparticles: a blue light-triggered red-emitting platform for indoor solid-state lighting35Highly efficient red-emitting Ca 2 YSbO 6 :Eu 3+ double perovskite phosphors for warm WLEDs48Insight into emission-tuning and luminescence thermal quenching investigations in NaLa 1−x Gd x Ca 4 W 2 O 12 :Mn 4+ phosphors via the ionic couple substitution of Na + + Ln 3+ (Ln = La, Gd) for 2Ca 2+ in Ca 6 W 2 O 12 :Mn 4+ for plant-cultivation LED applications14Luminescent perovskites: recent advances in theory and experiments259Mn 4+ -activated BaLaMgSbO 6 double-perovskite phosphor: a novel high-efficiency far-red-emitting luminescent material for indoor plant growth lighting42Morphology evolution of Eu 3+ -activated NaTbF 4 nanorods: a highly-efficient near-ultraviolet light-triggered red-emitting platform towards application in white light-emitting diodes93Novel bismuth activated blue-emitting phosphor Ba 2 Y 5 B 5 O 17 :Bi 3+ with strong NUV excitation for WLEDs82Review—Tanabe−Sugano Energy-Level Diagram and Racah Parameters in Mn4+-Activated Red and Deep Red-Emitting Phosphors78Simultaneously enhanced far-red luminescence and thermal stability in Ca3Al4ZnO10:Mn4+ phosphor via Mg2+ doping for plant growth lighting69CaYAlO4:Mn4+,Mg2+: An efficient far-red-emitting phosphor for indoor plant growth LEDs58Synthesis and photoluminescence properties of novel Sr3LiSbO6:Mn4+ red phosphor for indoor plant growth51Low temperature synthesis and photoluminescence properties of Mn4+-doped La2MgTiO6 deep-red phosphor with a LiCl flux24Rare‐earth‐free Li 5 La 3 Ta 2 O 12 :Mn 4+ deep‐red‐emitting phosphor: Synthesis and photoluminescence properties40Luminescence property improvement of Ba2LaSbO6:Mn4+ phosphor by using Dy3+ or H3BO311Deep-red-emitting SrLa2Sc2O7:Mn4+ phosphor: Synthesis and photoluminescence properties52Local Structure Modulation Induced Highly Efficient Far-Red Luminescence of La 1– x Lu x AlO 3 :Mn 4+ for Plant Cultivation89Cation vacancy repair towards a new yellow Ca7Sr3Na(PO4)7:Eu2+ phosphor15Enhancing quantum efficiency and tuning photoluminescence properties in far-red-emitting phosphor Ca14Ga10Zn6O35:Mn4+ based on chemical unit engineering142Enhancing photoluminescence properties of Mn 4+ ‐activated Sr 4− x Ba x Al 14 O 25 red phosphors for plant cultivation LEDs20Novel cyan‐emitting KBaScSi 2 O 7 :Eu 2+ phosphors with ultrahigh quantum efficiency and excellent thermal stability for WLEDs57Non-radiative processes and luminescence quenching in Mn4+ doped phosphors27Deep-red-emitting Ca2LuSbO6:Mn4+ phosphors for plant growth LEDs: Synthesis, crystal structure, and photoluminescence properties69Multicolour emission from thermally stable Tb3+/Eu3+ co-doped CaLa4Si3O13 phosphors for single-component w-LEDs application61Review—Mn 4+ -Activated Red and Deep Red-Emitting Phosphors193Ammonium salt conversion towards Mn4+ doped (NH4)2NaScF6 narrow-band red-emitting phosphor15Novel Intense Emission-Tunable Li1.5La1.5WO6:Mn4+,Nd3+,Yb3+ Material with Good Luminescence Thermal Stability for Potential Applications in c-Si Solar Cells and Plant-Cultivation Far-Red-NIR LEDs36Sm3+-activated Y2Mo4O15 red-emitting microparticles with admirable luminescent performance for indoor illumination25Effects of Al3+-substitution on photoluminescence properties of Sr2YNbO6:Mn4+ far-red phosphor for plant cultivation28Synthesis and luminescence properties of CaLaMgNbO6:Mn4+ red phosphor for UV-based w-LEDs3NaLa2SbO6:Mn4+ far-red phosphor: Synthesis, luminescence properties and emission enhancement by Al3+ ions15A novel Mn4+-activated garnet-type Li5La3Nb2O12 far red-emitting phosphor with high thermal stability for plant cultivation31Synthesis and luminescent properties of a novel deep-red phosphor Sr2GdNbO6:Mn4+ for indoor plant growth lighting48Rare-earth-containing perovskite nanomaterials: design, synthesis, properties and applications422Mn4+ doped tetratungstate Sr9Gd2W4O24 far-red phosphor: Synthesis, luminescence properties, and potential applications in indoor plant cultivation30Far red-emitting double perovskite phosphors Ca2(1-x)Sr2xGdSbO6:Mn4+: Luminescence improvement based on composition modulation39UVB-emitting gadolinium-doped Ba2YZrO6 perovskite ceramic phosphor8Plant habitat-conscious phosphors: Tuneable luminescence properties of Dy3+-doped Ca8ZnY(PO4)7 phosphors by co-dopants Mg2+ and B3+31Sr2LaSbO6:Mn4+ far-red phosphor for plant cultivation: Synthesis, luminescence properties and emission enhancement by Al3+ ions47Tuning the luminescence properties of Mn 4+ ‐activated CaYAlO 4 phosphor by co‐doping cations for indoor plant cultivation27Investigations of crystal-field energy levels and microscopic spin-Hamiltonian parameters of Mn 4+ ions in pyrochlore hosts Y 2 Ti 2 O 7 and Y 2 Sn 2 O 77A double perovskite-based red-emitting phosphor with robust thermal stability for warm WLEDs31A new strategy to the NaY(MoO4)2:Eu3+ phosphors modified by tetraethyl orthosilicate for LEDs: Photoludminescence properties and morphology10Structure analysis, tuning photoluminescence and enhancing thermal stability on Mn4+-doped La2-xYxMgTiO6 red phosphor for agricultural lighting78Optical properties of deep-red-emitting Ca2YTaO6:Mn4+ phosphors for LEDs applications37A new strategy to the phosphors for plant growth LEDs: Far red emission from the Ca9MY0.667 (PO4)7 (M = Li, Na):Eu3+ phosphors due to the Eu3+: 5D0 → 7F4 transition42Achieving Efficient Red-Emitting Sr2Ca1−δLnδWO6:Mn4+ (Ln = La, Gd, Y, Lu, δ = 0.10) Phosphors with Extraordinary Luminescence Thermal Stability for Potential UV-LEDs Application via Facile Ion Substitution in Luminescence-Ignorable Sr2CaWO6:Mn4+52Charge compensation assisted enhanced photoluminescence derived from Al3+-codoped NaLaMgWO6:Mn4+ phosphors for plant growth lighting applications22A red phosphor LaSc3(BO3)4:Eu3+ with zero-thermal-quenching and high quantum efficiency for LEDs251Exploiting the diverse photoluminescence behaviors of NaLuF4:xEu3+ nanoparticles and g-C3N4 to realize versatile applications in white light-emitting diode and optical thermometer161Enhancement of luminescence and thermal stability in Sr 2.92-x Tm x SiO 5 :Eu 2+ for white LEDs3A novel inequivalent double-site substituted red phosphor Li 4 AlSbO 6 :Mn 4+ with high color purity: its structure, photoluminescence properties, and application in warm white LEDs43Enhanced luminescence properties of Ca 1+x Sr 2−x Al 2 O 6 :Eu 3+ (0 ≤ x ≤ 1) red phosphors based on composition modulation6Local Structure Modulation Induced Highly Efficient Red-Emitting Ba 2Gd 1-xY xNbO 6:Mn 4+ Phosphors for Warm WLEDs0Structure and luminescence behaviour of a novel red-emitting fluoroperovskite for display backlight application7Perovskite tungstate Ba2La2ZnW2O12:Mn4+ phosphor: Synthesis, energy transfer and tunable emission53Cyan-emitting Ba0.45Ca2.5La6(SiO4)6: 0.05 Eu2+ and Ba1.45Ca1.5La6(SiO4)6:0.05 Eu2+ solid-solution phosphors for white light-emitting diodes19Synthesis and luminescent properties of new green Li2Mg1-xSiO4:xMn2+ phosphors16Development of red-emitting Ba2LaSbO6:Mn4+ phosphors for latent fingerprint detection66Deep‐red‐emitting SrLaLiTeO 6 : Mn 4+ double perovskites: Correlation between Mn 4+ ‐O 2− bonding and photoluminescence62Equivalent cation substitution-triggered highly efficient Mn4+ red emission in double-perovskite type (Ba, Sr)2(Gd, La, Y, Lu)(Nb, Sb)O6:Mn4+ solid solution phosphors and photophysical studies62Luminescence studies of CaLa4Si3O13 doped with Er3+ ions5Enhancing emission property of red phosphor Sr2MgGe2O7:Mn4+ via Ba2+ doping7Realization of non-rare earth doped blue-emitting phosphor Ba2Y5B5O17: Sb by selective site excitation, and its application in n-UV excited wLEDs3Excitation selective thermal characteristics of Mg28Ge7.55−xGaxO32F15.04: Mn4+ and application in single/dual-mode optical thermometry15Preparation, crystal structure and photoluminescence properties of novel red-emitting phosphor Mg3Gd2Ge3O12: RE3+ (RE=Sm, Eu) with high thermal stability23A Novel Ba 2 LuNbO 6 :Mn 4+ Double-Perovskite Far-Red Phosphor for Indoor Plant Cultivation8Enhanced self-activated far-red photoluminescence from Sr3LiSbO6 phosphors by Gd3+ doping for plant growth20Efficient luminescence lifetime thermometry with enhanced Mn4+-activated BaLaCa1−xMgxSbO6 red phosphors142Local Structure Modulation-Induced Highly Efficient Red-Emitting Ba 2 Gd 1– x Y x NbO 6 :Mn 4+ Phosphors for Warm WLEDs45Surface engineered environment-stable red-emitting fluorides for white light emitting diodes12Chemical unit co-substitution for a new far-red-emitting phosphor Ca3-6(NaLu)3LiSbO6:Mn4+ to achieve high quantum efficiency and superb thermal stability12Emerging near-unity internal quantum efficiency and color purity from red-emitting phosphors for warm white LED with enhanced color rendition33Solid state reaction preparation of an efficient rare-earth free deep-red Ca2YNbO6:Mn4+ phosphor46Analysis of crystal-field effect on luminescence spectra of Mn 4+ (3d 3 ) ion-doped double perovskite La 2 ZnTiO 6 phosphor by semiempirical computations: exchange charge model and superposition model19Presence of the irregular oxidation state of Bi 4+ and single-element white emission in YAl 3 (BO 3 ) 4 :Bi0Synergistic luminescent thermometer using co-doped Ca 2 GdSbO 6 :Mn 4+ /(Eu 3+ or Sm 3+ ) phosphors77Suppression of charge imbalance via Li+-Mn4+ co-incorporated Sr2YSbO6 red phosphors for warm w-LEDs43A new series of long wavelength red phosphors BaLaLiTe1-xO6:xMn4+ for plant cultivation LED13Mn4+-activated double perovskite red phosphor for multifunctional applications26Effects of activated Sr 2+ ion content on strong blue‐emitting Ca 2 Sb 2 O 7 materials for high‐quality WLED devices5Novel Findings on the Optical Properties of Mn4+‐Doped (Rb,K)2Ge4O9 Phosphors5Emission color shift from green yellow to reddish orange in Eu2+-activated Ca6BaP4O17 by doping high amount of activator ion9Synthesis and characterization of Cu–doped Cs2KBiBr6 double perovskite phosphors for photoluminescent applications11A Mn4+ activated (Gd,La)2(Zn,Mg)TiO6 deep-red emission phosphor: The luminescence properties and potential application for full-spectrum pc-LEDs14Highly efficient and thermally stable red emitting CaGdMgNbO6:Mn4+ double perovskites for indoor plant growth LEDs13Accessing deep-red emission using chemical units cosubstituted LaTiSbO6:Mn4+ phosphor38A highly intense double perovskite BaSrYZrO5.5: Eu3+ phosphor for latent fingerprint and security ink applications61Improving the emission intensity and broadening spectrum of borate NaSrBO 3 blue phosphor by double ion doping1Polyhedron engineering by chemical unit co-substitution in LaAlO3:0.02Pb2+ to generate multimode and condition-sensitive luminescence for dynamic anticounterfeiting34Systemic development of Mn4+-activated double perovskite red phosphors for plant growth applications16Synthesis and optical properties of far-red dual perovskite Sr2InTaO6: Mn4+ phosphors for indoor plant lighting LED31Fluorescence Lifetime-Based Luminescent Thermometry Material with Lifetime Varying over a Factor of 5044Analysis of crystal-field effects on the energy levels of Mn4+ ions doped in different photoluminescent host lattices, exhibiting lowering of site symmetry: Exchange charge and superposition model calculations, for potential applications21Enhanced luminescence of Mn4+ equivalently doped fluoride phosphors by reducing defects and impurities16A Novel Double-Perovskite Mn4+-Doped Sr2scnbo6 Phosphor for Indoor Plant Growth Lighting0Equivalent chemical substitution in double–double perovskite-type ALaLiTeO 6 :Mn 4+ (A = Ba 2+ , Sr 2+ , Ca 2+ ) phosphors enabling wide range crystal field strength regulation and efficient far-red emission17Phosphors Ba2LaTaO6:Mn4+ and its alkali metal charge compensation for plant growth illumination9Customizing dual-functional platforms for solid-state lighting and luminescence lifetime thermometry with high sensing sensitivity3Synthesis and characterization of a far-red-emitting Sr2ScNbO6: Mn4+ phosphor for short-day plant cultivation28Luminescence properties and energy-transfer behavior of Y2-x-yBixEuyMgTiO6 phosphors11A double-perovskite Mn4+-doped Sr2ScNbO6 phosphor for indoor plant growth lighting20Influence of Ga Substitution on the Local Structure and Luminescent Properties of Eu-Doped CaYAlO4 Phosphors4Mn4+ activated phosphors in photoelectric and energy conversion devices56Eu3+-Doped Ca2GdSbO6 Double Perovskite Phosphor for Solid-State Lighting Applications0Luminescence and temperature sensing properties of Y2--Tm Sm MgTiO6 phosphors9Compositional modulation induced broadband NIR luminescence enhancement in A2ScNbO6:Cr3+ (A = Ba, Sr)12An efficient rare-earth free deep red-emitting GdGeSbO 6 :Mn 4+ phosphor for white light-emitting diodes21Analysis of crystal-field effects on the energy levels of Mn4+ ions doped in Gd2MgTiO6 phosphor using exchange charge model and superposition model1Novel red emitting Phosphor-in-Glass (PiG) based on Na6CaP2O9: Eu3+ phosphor as an inorganic colour converter for w-LED applications23Novel Sm3+-Mn4+ co-activated CaGdMgNbO6 red phosphor with anomalous thermal quenching for plant growth lighting6The nephelauxetic function he: A tool to locate the emission of Mn4+ in oxides and fluorides3Mn4+-activated NaSr10Y5W4O30 far-red emitting luminescent material for plant growth lighting4Preparation, Characterization, Photoluminescence and Thermoluminescence Studies of Li2−3xLnxGeTeO6 (Ln = Eu3+, Tb3+; x = 0.0, 0.02, 0.05, 0.075 and 0.1)0Enhanced luminescence performance in double perovskite CaSrLaSbO6: Mn4+ red emission phosphors for indoor plant growth via cation doping17Cool white light emitting Dy3+ activated KNaCa2(PO4)2 phosphor for outdoor lighting and optical thermometric applications9Novel efficient deep-red emitting phosphor SrCa 2 Ga 2 O 6 :Mn 4+ with tululite-related structure12Dual green and red emitting Mn-doped MgAl2O4 phosphors for WLED and plant growth LED applications31Enhancing Mn4+ luminescence via Y3+ substitution in Sr0.1La0.9Mg0.45Ti0.55O3 double perovskite for advanced horticultural lighting1Structural, dielectric, and impedance studies of Ta5+ substituted Sr0.6Mg0.4Nb2(1-x)Ta2xO6 (0.00 ≤ x ≤ 0.06) lead-free ceramics2Engineering the optoelectronic properties of lead-free Rb2B’BiCl6 (B = K, Li) double perovskites: highly efficient blue light emission1Study on the luminescence enhancement of NaLaMgWO 6 : Eu phosphors1Boosting luminescence of Ca2GdTaO6: Mn4+ red phosphors via Li+ charge compensation for plant growth LEDs1Sb5+-Nb5+ substitution driven structural tuning and luminescence enhancement of Mn4+-activated double perovskite phosphors1Preparation and characterization of a novel far-red phosphor powder SrBaGdNbO6: Mn4+ for indoor plant cultivation lighting0

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  3. Preparation, characterization, and luminescence properties of double perovskite SrLaMgSbO 6 :Mn 4+ far-red emitting phosphors for indoor plant growth lighting

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  4. Synthesis, structure, and luminescence characteristics of far-red emitting Mn 4+ -activated LaScO 3 perovskite phosphors for plant growth

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  5. Luminescence properties of a non-rare-earth doped oxyfluoride LiAl4O6F:Mn4+ red phosphor for solid-state lighting

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  7. Structure and luminescence properties of Zn3V2O8 yellow phosphor for white light emitting diodes

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  9. Double perovskite A 2 LaNbO 6 :Mn 4+ ,Eu 3+ (A = Ba, Ca) phosphors: potential applications in optical temperature sensing

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  19. Review—Tanabe−Sugano Energy-Level Diagram and Racah Parameters in Mn4+-Activated Red and Deep Red-Emitting Phosphors

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  30. Enhancing photoluminescence properties of Mn 4+ ‐activated Sr 4− x Ba x Al 14 O 25 red phosphors for plant cultivation LEDs

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  31. Novel cyan‐emitting KBaScSi 2 O 7 :Eu 2+ phosphors with ultrahigh quantum efficiency and excellent thermal stability for WLEDs

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  32. Non-radiative processes and luminescence quenching in Mn4+ doped phosphors

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  33. Deep-red-emitting Ca2LuSbO6:Mn4+ phosphors for plant growth LEDs: Synthesis, crystal structure, and photoluminescence properties

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  34. Multicolour emission from thermally stable Tb3+/Eu3+ co-doped CaLa4Si3O13 phosphors for single-component w-LEDs application

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  35. Review—Mn 4+ -Activated Red and Deep Red-Emitting Phosphors

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  36. Ammonium salt conversion towards Mn4+ doped (NH4)2NaScF6 narrow-band red-emitting phosphor

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  37. Novel Intense Emission-Tunable Li1.5La1.5WO6:Mn4+,Nd3+,Yb3+ Material with Good Luminescence Thermal Stability for Potential Applications in c-Si Solar Cells and Plant-Cultivation Far-Red-NIR LEDs

    ACS Sustainable Chemistry & Engineering · 2019-09-05

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  38. Sm3+-activated Y2Mo4O15 red-emitting microparticles with admirable luminescent performance for indoor illumination

    Optical Materials · 2019-09-18

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  39. Effects of Al3+-substitution on photoluminescence properties of Sr2YNbO6:Mn4+ far-red phosphor for plant cultivation

    Journal of Luminescence · 2019-10-19

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  40. Synthesis and luminescence properties of CaLaMgNbO6:Mn4+ red phosphor for UV-based w-LEDs

    Modern Physics Letters B · 2019-11-01

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  41. NaLa2SbO6:Mn4+ far-red phosphor: Synthesis, luminescence properties and emission enhancement by Al3+ ions

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  42. A novel Mn4+-activated garnet-type Li5La3Nb2O12 far red-emitting phosphor with high thermal stability for plant cultivation

    Journal of Luminescence · 2019-11-08

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  43. Synthesis and luminescent properties of a novel deep-red phosphor Sr2GdNbO6:Mn4+ for indoor plant growth lighting

    Journal of Luminescence · 2019-12-19

    Ya-jie Han, Shuang Wang, Han Liu, Lei Shi, Jiaying Zhang, Zhenni Zhang, Zhenni Zhang, Zhiyong Mao, Dajian Wang, Zhongfei Mu, Zhi‐wei Zhang, Zhi‐wei Zhang, Ying Gang Zhao

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  44. Rare-earth-containing perovskite nanomaterials: design, synthesis, properties and applications

    Chemical Society Reviews · 2020-01-01

    Zhichao Zeng, Yueshan Xu, Zheshan Zhang, Zhansheng Gao, Meng Luo, Zongyou Yin, Chao Zhang, Jun Xu, Bolong Huang, Feng Chao Luo, Yaping Du, Chun‐Hua Yan

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  45. Mn4+ doped tetratungstate Sr9Gd2W4O24 far-red phosphor: Synthesis, luminescence properties, and potential applications in indoor plant cultivation

    Journal of Luminescence · 2020-01-07

    Ya-jie Han, Shuang Wang, Han Liu, Lei Shi, Wenxin Zhang, Lin-ke Cai, Zhiyong Mao, Dajian Wang, Zhongfei Mu, Zhi‐wei Zhang, Ying Gang Zhao

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  46. Far red-emitting double perovskite phosphors Ca2(1-x)Sr2xGdSbO6:Mn4+: Luminescence improvement based on composition modulation

    Ceramics International · 2020-01-20

    Ya-jie Han, Shuang Wang, Han Liu, Lei Shi, Chang Liu, Shi Xiao-fan, Shumin Yang, Minglu Tang, Lulu Zhao, Zhi‐wei Zhang, Ying Gang Zhao

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  47. UVB-emitting gadolinium-doped Ba2YZrO6 perovskite ceramic phosphor

    Optik · 2020-01-20

    Vijay Pal Singh, Sumandeep Kaur, Allam Srinivasa Rao, N. Singh, J.L. Rao, Muhammad Irfan

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  48. Plant habitat-conscious phosphors: Tuneable luminescence properties of Dy3+-doped Ca8ZnY(PO4)7 phosphors by co-dopants Mg2+ and B3+

    Ceramics International · 2020-01-24

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  49. Sr2LaSbO6:Mn4+ far-red phosphor for plant cultivation: Synthesis, luminescence properties and emission enhancement by Al3+ ions

    Journal of Luminescence · 2020-02-05

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  50. Tuning the luminescence properties of Mn 4+ ‐activated CaYAlO 4 phosphor by co‐doping cations for indoor plant cultivation

    Journal of the American Ceramic Society · 2020-03-16

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