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RESEARCH PAPER · Energy & Environmental Science · 2018

Cobalt-substituted SrTi 0.3 Fe 0.7 O 3−δ : a stable high-performance oxygen electrode material for intermediate-temperature solid oxide electrochemical cells

Shan-Lin Zhang, Hongqiang Wang, Matthew Y. Lu, Ai-Ping Zhang, Liliana Mogni, Qinyuan Liu, Chang‐Jiu Li, Chang‐Jiu Li, Chang-Jiu Li, Chang-Jiu Li, Scott Alexander Barnett

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Cobalt-substituted SrTi 0.3 Fe 0.7 O 3−δ : a stable high-performance oxygen electrode material for intermediate-temperature solid oxide electrochemical cellsOriginalCo and Fe co-doping influence on functional properties of SrTiO3 for use as oxygen transport membranes39Conditions for stable operation of solid oxide electrolysis cells: oxygen electrode effects115High stability SrTi 1−x Fe x O 3−δ electrodes for oxygen reduction and oxygen evolution reactions55Highly active and durable double-doped bismuth oxide-based oxygen electrodes for reversible solid oxide cells at reduced temperatures74Ta-doped PrBa0.94Co2-Ta O5+ as promising oxygen electrodes: A focused study on catalytic oxygen reduction reaction activity, stability and CO2-durability50Highly efficient reversible protonic ceramic electrochemical cells for power generation and fuel production764Metal‐Supported Solid Oxide Electrolysis Cell with Significantly Enhanced Catalysis45Electrochemical performance and stability of SrTi0.3Fe0.6Co0.1O3-δ infiltrated La0.8Sr0.2MnO3Zr0.92Y0.16O2-δ oxygen electrodes for intermediate-temperature solid oxide electrochemical cells40A 4 × 4 cm2 Nanoengineered Solid Oxide Electrolysis Cell for Efficient and Durable Hydrogen Production124High performance and stability of double perovskite-type oxide NdBa0.5Ca0.5Co1.5Fe0.5O5+ as an oxygen electrode for reversible solid oxide electrochemical cell73Heterointerface engineering for enhancing the electrochemical performance of solid oxide cells319Study of phase stability of SrTi0.3Fe0.7O3−δ perovskite in reducing atmosphere: Effect of microstructure22Mechanisms of PrOx performance enhancement of oxygen electrodes for low and intermediate temperature solid oxide fuel cells52In Situ Exsolved Ni-Decorated Ba(Ce0.9Y0.1)0.8Ni0.2O3−δ Perovskite as Carbon-Resistant Composite Anode for Hydrocarbon-Fueled Solid Oxide Fuel Cells15A Comprehensive Review and Technical Guideline for Optimal Design and Operations of Fuel Cell-Based Cogeneration Systems53Advanced oxygen-electrode-supported solid oxide electrochemical cells with Sr(Ti,Fe)O 3−δ -based fuel electrodes for electricity generation and hydrogen production43Boosting solid oxide fuel cell performance via electrolyte thickness reduction and cathode infiltration104Enhancement of Ni–(Y 2 O 3 ) 0.08 (ZrO 2 ) 0.92 fuel electrode performance by infiltration of Ce 0.8 Gd 0.2 O 2−δ nanoparticles61Isovalent doping: a new strategy to suppress surface Sr segregation of the perovskite O 2 -electrode for solid oxide fuel cells38Promotion of oxygen reduction and evolution by applying a nanoengineered hybrid catalyst on cobalt free electrodes for solid oxide cells40Tuning electrochemical and transport processes to achieve extreme performance and efficiency in solid oxide cells28Pr2NiO4-Pr0.2Ce0·8O1.9 composite cathode as a potential cathode material for intermediate temperature solid oxide fuel cells46Stable, efficient and cost-competitive Ni-substituted Sr(Ti,Fe)O3 cathode for solid oxide fuel cell: Effect of A-site deficiency52Large-area solid oxide cells with La0.6Sr0.4CoO3-δ infiltrated oxygen electrodes for electricity generation and hydrogen production73Tuning interfacial chemistry and electrochemical properties of solid oxide cells via cation interdiffusion6Effect of sintering temperature on electrochemical performance of porous SrTi1-xFexO3-δ (x = 0.35, 0.5, 0.7) oxygen electrodes for solid oxide cells10Study of oxygen electrode reactions on symmetrical porous SrTi0.30Fe0.70O3-δ electrodes on Ce0.8Gd0.2O1.9 electrolyte at 800 °C–500 °C13An efficient and durable perovskite electrocatalyst for oxygen reduction in solid oxide fuel cells51A mesoporous catalytic fiber architecture decorated by exsolved nanoparticles for reversible solid oxide cells20Efficient water splitting through solid oxide electrolysis cells with a new hydrogen electrode derived from A-site cation-deficient La0.4Sr0.55Co0.2Fe0.6Nb0.2O3-δ perovskite58High-temperature electrocatalysis and key materials in solid oxide electrolysis cells147Performance evaluation of highly active and novel La0.7Sr0.3Ti0.1Fe0.6Ni0.3O3-δ material both as cathode and anode for intermediate-temperature symmetrical solid oxide fuel cell74Surface Segregation in Solid Oxide Cell Oxygen Electrodes: Phenomena, Mitigation Strategies and Electrochemical Properties216A novel electrode with multifunction and regeneration for highly efficient and stable symmetrical solid oxide cell56Rare earth elements based oxide ion conductors52Sm 0.5 Sr 0.5 CoO 3− δ Surface Modification of La 0.6 Sr 0.4 Co 0.2 Fe 0.8 O 3− δ -Ce 0.9 Gd0.1 2− δ Composite Oxygen Electrodes for Solid Oxide Electrochemical Cells13A highly active CH 4 catalyst correlated with solid oxide fuel cell anode performance27A highly active perovskite anode with an in situ exsolved nanoalloy catalyst for direct carbon solid oxide fuel cells12Iron-based electrode materials for solid oxide fuel cells and electrolysers129Highly active and novel A-site deficient symmetric electrode material (Sr0.3La0.7)1−x (Fe0.7Ti0.3)0.9Ni0.1O3−δ and its effect on electrochemical performance of SOFCs36Towards understanding of oxygen electrode processes during solid oxide electrolysis operation to improve simultaneous fuel and oxygen generation43Achieving Strong Coherency for a Composite Electrode via One-Pot Method with Enhanced Electrochemical Performance in Reversible Solid Oxide Cells67Solid Oxide Electrolysis of H2O and CO2 to Produce Hydrogen and Low-Carbon Fuels164Perovskite Cathode Materials for Low-Temperature Solid Oxide Fuel Cells: Fundamentals to Optimization99Achieving exceptional activity and durability toward oxygen reduction based on a cobalt-free perovskite for solid oxide fuel cells35Characteristics of Oxygen Electrode Supported Reversible Solid Oxide Cells11Chromium evaporation and oxidation characteristics of alumina-forming austenitic stainless steels for balance of plant applications in solid oxide fuel cells26Simulation of the Electrochemical Impedance in a Three-Dimensional, Complex Microstructure of Solid Oxide Fuel Cell Cathode and Its Application in the Microstructure Characterization12Sintering behavior and electrochemical performance of A-site deficient SrxTi0.3Fe0·7O3-δ oxygen electrodes for solid oxide electrochemical cells27Vacuum cold sprayed nanostructured La0.6Sr0.4Co0.2Fe0.8O3−δ as a high-performance cathode for porous metal-supported solid oxide fuel cells operating below 600 °C10A promising strontium and cobalt-free air electrode Pr1-xCaxFeO3-δ for solid oxide electrolysis cell14Enhanced Electrochemical Performance of the Fe-Based Layered Perovskite Oxygen Electrode for Reversible Solid Oxide Cells57Effect of Pressurization on Solid Oxide Cell Oxygen Electrodes: the Role of PrO x Nanoparticle Infiltration16A highly efficient and durable air electrode for intermediate-temperature reversible solid oxide cells80Nitric oxide utilization for ammonia production using solid electrolysis cell at atmospheric pressure55Performance modulation through selective, homogenous surface doping of lanthanum strontium ferrite electrodes revealed by in situ PLD impedance measurements9Advances in Electrode Materials for Rechargeable Batteries4Effect of Gd-Doped Ceria Infiltration into Ni-Ysz on Reversible Solid Oxide Cell Operation33Tracking the nanoparticle exsolution/reoxidation processes of Ni-doped SrTi 0.3 Fe 0.7 O 3− δ electrodes for intermediate temperature symmetric solid oxide fuel cells47Progress and potential for symmetrical solid oxide electrolysis cells143Enhanced Long‐Term Cathode Stability by Tuning Interfacial Nanocomposite for Intermediate Temperature Solid Oxide Fuel Cells9Electrochemical Performance Investigation of Sr(Ti 1−x Fe x )O 3− δ Fuel Electrodes with Different Fe Contents for Solid Oxide Electrochemical Cells3The Influence of Cr-Additives on the Polarization Resistance of Praseodymium-Doped Ceria Cathodes for Solid Oxide Fuel Cells12Novel approach to integrate CO2 utilization coupled with direct methane conversion to C2 products using solid oxide electrolysis cell24Nanostructured spinel Mn1.3Co1.3Cu0.4O4 as a bifunctional electrocatalyst for high-performance solid oxide electrochemical cells at intermediate temperatures16A Novel Solid Oxide Electrolysis Cell with Micro‐/Nano Channel Anode for Electrolysis at Ultra‐High Current Density over 5 A cm −245Structural, Interfacial, and Electrochemical Stability of La0.3Ca0.7Fe0.7Cr0.3O3-δ Electrode Material for Application as the Oxygen Electrode in Reversible Solid Oxide Cells1A-site deficient Sr0.9Ti0.3Fe0.7O3−δ perovskite：A high stable cobalt-free oxygen electrode material for solid oxide electrochemical cells with excellent electrocatalytic activity and CO2 tolerance29High‐Performance and Durable Fuel Cells using Co/Sr‐Free Fluorite‐Based Mixed Conducting (Pr,Ce)O2‐δ Cathode20Comparative study on the electrochemical performance of Sr(Ti0.3Fe0.7)O3-δ fuel electrode in different fuel gases for solid oxide electrochemical cells11Fuel Cell Systems for Maritime: A Review of Research Development, Commercial Products, Applications, and Perspectives156Boosting the performance of reversible solid oxide electrochemical cells with a novel hybrid oxygen electrode, Pr 1.39 Ba 0.14 Sr 0.53 Co 1.48 Fe 0.76 O 6− δ -Ba 0.66 Sr 0.34 CoO 3− δ16Cation deficiency enables reversal of dopant segregation at perovskite oxide surfaces under anodic potential17Enhancing Sr-Deficient Sr(Ti0.3fe0.7)O3–Δ Cathode Performance Using a Nanoscale Sm0.5sr0.5coo3 –Δ Infiltrant0Fluorination Intensifying Oxygen Evolution Reaction for High-Temperature Steam Electrolysis16Nanoengineering of electrodes via infiltration: an opportunity for developing large-area solid oxide fuel cells with high power density13Realizing high-temperature steam electrolysis on tubular solid oxide electrolysis cells sufficing multiple and rapid start-up22Degradation and recovery of solid oxide fuel cell performance by control of cathode surface acidity: Case study – Impact of Cr followed by Ca infiltration29Figure‐of‐Merit Compatibility of Solid Oxide Fuel Cells10Boosting electrochemical CO2 directly electrolysis by tuning the surface oxygen defect of perovskite40Enhancing durability of solid oxide cells for hydrogen production from seawater by designing nano-structured Sm0.5Sr0.5Co3-δ infiltrated air electrodes21Rocking chair-like movement of ex-solved nanoparticles on the Ni-Co doped La0.6Ca0.4FeO3-δ oxygen carrier during chemical looping reforming coupled with CO2 splitting37Designing the nano-scale architecture of the air electrode for high-performance and robust reversible solid oxide cells34Electrochemical characteristics of Sr-deficient SrTi0.3Fe0.7O3−δ oxygen electrodes for solid oxide electrolyzers5Materials of solid oxide electrolysis cells for H 2 O and CO 2 electrolysis: A review177Impact of strontium non-stoichiometry of SrxTi0.3Fe0.7O3-δ on structural, electrical, and electrochemical properties for potential oxygen electrode of intermediate temperature solid oxide cells9Ethanol-induced formation of precursor for 8 mol% Yttria-stabilized zirconia: Towards the production of well-dispersed, easily sintering, and high-conductivity nano-powders5Chemistry and electrochemistry of CeO2-based interlayers: Prolonging the lifetime of solid oxide fuel and electrolysis cells41In situ synthesis of extremely small, thermally stable perovskite nanocatalysts for high-temperature electrochemical energy devices9Cobalt-free perovskite La0.6Ba0.4Ni0.2Fe0.8-xTixO3-δ(x=0–0.3) as cathode for intermediate-temperature solid oxide fuel cells28Structural Characterization of Multi-doped Barium Cerate as Perovskite for Solid Oxide Fuel Cells2Dense La0.3Sr0.7TiO3 interconnect sintered in air atmosphere at a reduced temperature with improved conductivity for solid oxide electrochemical cells8Improved bi-layer electrolytes of solid oxide cells: the role of a Sm 0.2 Ce 0.8 O 2− δ diffusion barrier layer3Performance deviation analysis and reliability improvement during experimental development of lab-scale solid oxide single cells21Enhancing Sr-deficient Sr(Ti0.3Fe0.7)O3–δ Cathode Performance through Sm0.5Sr0.5CoO3–δ Infiltration5Phase Stability of Perovskite Oxide Electrodes under Operating Condition in Solid Oxide Fuel Cell10Bismuth doped La0.5-xBixSr0.5Fe0.9Mo0.1O3-δ perovskite as high active oxygen electrode for solid oxide cells13Ce- and Ni-Codoped Double PrBaMn2O5 Perovskite as a Ceramic SOFC Anode18Reversal of chronic surface degradation of Sr(Ti,Fe)O3 perovskite-based fuel cell cathodes by surface acid/base engineering30Electrocatalysis in Solid Oxide Fuel Cells and Electrolyzers141A-site alkali metal-doped SrTi0.3Fe0.7O3-δ: A highly stable symmetrical electrode material for solid oxide electrochemical cells5Ni-doping influence on functional properties of SrTi0.65Fe0.35O3-δ for use as oxygen transport membranes4Sr(Ti0·3Fe0.7)O3−δ-based perovskite with in-situ exsolved Fe–Ru nanoparticles: A highly stable fuel electrode material for solid oxide electrochemical cells with efficient electrocatalytic CO2 reduction ability and preferential selectivity13Deciphering the enhanced oxygen reduction reaction activity of PrBa0.5Sr0.5Co1.5Fe0.5O5+δ via constructing negative thermal expansion offset for high-performance solid oxide fuel cell26Advanced design strategies for highly efficient and durable anodes in direct ammonia solid oxide fuel cells19Active and stable plasma-enhanced ALD Pt@Ni-YSZ hydrogen electrode for steam reversible solid oxide cells10Plasma-Sprayed La0.2Sr0.8MnO3-La0.3Sr0.7TiO3 Bilayer Coatings Along with the Interface Healing Processing Applied as the High Dense Interconnector for Tubular Solid Oxide Fuel Cells5Understanding delamination behavior of air electrode in solid oxide electrolysis cells through in situ monitoring of internal oxygen partial pressure10A comprehensive investigation of Sr segregation effects on the high-temperature oxygen evolution reaction rate39Enhanced oxygen electrode kinetics at low temperatures: an infiltrated Sr(Ti 0.3 Fe 0.55 Co 0.15 )O 3- δ –La 0.8 Sr 0.2 Ga 0.8 Mg 0.2 O 3- δ nanocomposite for solid oxide cells4Unveiling critical role of metal oxide infiltration in controlling the surface oxygen exchange activity and polarization of SrTi 1− x Fe x O 3− δ perovskite oxide electrodes10High-purity phase La0.8Sr0.2Ga0.8Mg0.2O3-δ electrolyte with superior ionic conductivity for solid oxide electrochemical cells fabricated by solid-state reaction via phase-forming additive6High-performance porous metal-supported solid oxide electrochemical cells with a reduction shrinkage optimized NiFe-based support6Understanding the degradation mechanisms of Ba-based double perovskite electrodes for solid oxide electrochemical cells6Strain evolution in La0.6Sr0.4CoO3−δ and SrTi0.3Fe0.7O3−δ multilayer systems1Targeted Co substitution at Fe/Ti sites in La0.1Sr1.9TiFeO6-δ double perovskite oxides to improve CO2 reduction activity4High activity and stability of calcium and nickel co-doped PrBaFe2O5+δ as a symmetrical electrode for solid oxide cells4Exploring the long-term stability of Pr0.25Nd0.25Ba0.25Sr0.25Fe0.75Ni0.25O3-δ electrodes in symmetrical solid oxide fuel cells0Advances in high-temperature solid oxide electrolysis technology for clean hydrogen and chemical production: materials, cells, stacks, systems and economics38Recent Advances in Solid Oxide Electrolysis Cells for Solar Energy Conversion24Real‐Time Analysis of Solid Oxide Electrolysis Cells Manufactured by Ceramic Sintering Process via Operando TEM and Electrochemical Impedance Spectroscopy2Advancements and Challenges in Iron Oxide and Ferrites Materials for Solid Oxide Fuel Cells: A Comprehensive Review2Solid oxide fuel cells using iron oxide-based materials0A-site element tuning in Nd2NiO4-based Ruddlesden-Popper cathodes: Enhanced electrochemical performance and stability for intermediate-temperature SOFCs6B‐Site Fe–Co–Ni Triple Doping for High‐Performance Oxygen Electrodes in Industrial‐sized Reversible Solid Oxide Cells0Trace vanadium doping triggers the additional oxygen vacancies in the oxygen electrode of solid oxide cells1A Novel Metal Foam‐Supported Solid Oxide Fuel Cell With High Specific Power0Enhancing perovskite oxygen electrode properties by in-situ constructed heterogeneous catalysts0Multi-factor optimization of Sc doping unravels enhanced CO2 adsorption and dissociation process for solid oxide electrolysis cells6Synergized Tri‐Phase Anode via Purposive Ba 2+ Doping at the La 3+ Site in LaFe 0.7 Ni 0.3 O 3‐δ for Improved SOFC Performance2High-stable direct methanol/ethanol solid oxide fuel cells via in-situ nanoparticle exsolved perovskite anode and internal reforming catalytic layer0

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  1. Co and Fe co-doping influence on functional properties of SrTiO3 for use as oxygen transport membranes

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  4. Highly active and durable double-doped bismuth oxide-based oxygen electrodes for reversible solid oxide cells at reduced temperatures

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  5. Ta-doped PrBa0.94Co2-Ta O5+ as promising oxygen electrodes: A focused study on catalytic oxygen reduction reaction activity, stability and CO2-durability

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  9. A 4 × 4 cm2 Nanoengineered Solid Oxide Electrolysis Cell for Efficient and Durable Hydrogen Production

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  10. High performance and stability of double perovskite-type oxide NdBa0.5Ca0.5Co1.5Fe0.5O5+ as an oxygen electrode for reversible solid oxide electrochemical cell

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  12. Study of phase stability of SrTi0.3Fe0.7O3−δ perovskite in reducing atmosphere: Effect of microstructure

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  13. Mechanisms of PrOx performance enhancement of oxygen electrodes for low and intermediate temperature solid oxide fuel cells

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  17. Boosting solid oxide fuel cell performance via electrolyte thickness reduction and cathode infiltration

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  19. Isovalent doping: a new strategy to suppress surface Sr segregation of the perovskite O 2 -electrode for solid oxide fuel cells

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  32. Performance evaluation of highly active and novel La0.7Sr0.3Ti0.1Fe0.6Ni0.3O3-δ material both as cathode and anode for intermediate-temperature symmetrical solid oxide fuel cell

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  34. A novel electrode with multifunction and regeneration for highly efficient and stable symmetrical solid oxide cell

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  35. Rare earth elements based oxide ion conductors

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  36. Sm 0.5 Sr 0.5 CoO 3− δ Surface Modification of La 0.6 Sr 0.4 Co 0.2 Fe 0.8 O 3− δ -Ce 0.9 Gd0.1 2− δ Composite Oxygen Electrodes for Solid Oxide Electrochemical Cells

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  37. A highly active CH 4 catalyst correlated with solid oxide fuel cell anode performance

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  39. Iron-based electrode materials for solid oxide fuel cells and electrolysers

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  40. Highly active and novel A-site deficient symmetric electrode material (Sr0.3La0.7)1−x (Fe0.7Ti0.3)0.9Ni0.1O3−δ and its effect on electrochemical performance of SOFCs

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  41. Towards understanding of oxygen electrode processes during solid oxide electrolysis operation to improve simultaneous fuel and oxygen generation

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