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RESEARCH PAPER · Annual Review of Materials Research · 2018

The Diversity of Layered Halide Perovskites

Matthew D. Smith, Ethan J. Crace, Adam Jaffé, Hemamala I. Karunadasa

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The Diversity of Layered Halide PerovskitesOriginalPromising photovoltaic and solid-state-lighting materials: two-dimensional Ruddlesden–Popper type lead-free halide double perovskites Cs n+1 In n/2 Sb n/2 I 3n+1 ( n = 3) and Cs n+1 In n/2 Sb n/2 Cl 3n+1 /Cs m+1 Cu m/2 Bi m/2 Cl 3m+1 ( n = 3, m = 1)31Completing the Picture of 2-(Aminomethylpyridinium) Lead Hybrid Perovskites: Insights into Structure, Conductivity Behavior, and Optical Properties42Structural evolution and photoluminescence properties of a 2D hybrid perovskite under pressure59General Synthesis Principles for Ruddlesden–Popper Hybrid Perovskite Halides from a Dynamic Equilibrium50Two-dimensional perovskite materials: From synthesis to energy-related applications172Effect of High Dipole Moment Cation on Layered 2D Organic–Inorganic Halide Perovskite Solar Cells167Low dimensional metal halide perovskites and hybrids489Doping Mn2+ in Single-Crystalline Layered Perovskite Microcrystals98A hybrid fluoride layered perovskite, ( en H 2 )MnF 410Designing a new family of oxonium-cation based structurally diverse organic–inorganic hybrid iodoantimonate crystals26Influence of organic cation planarity on structural templating in hybrid metal-halides19Searching for stability at lower dimensions: current trends and future prospects of layered perovskite solar cells194Structure-directing effects in (110)-layered hybrid perovskites containing two distinct organic moieties31White light emission in low-dimensional perovskites217The Role of Chloride Incorporation in Lead‐Free 2D Perovskite (BA)2SnI4: Morphology, Photoluminescence, Phase Transition, and Charge Transport64Tuning the Luminescence of Layered Halide Perovskites801Two‐Dimensional Halide Perovskites in Solar Cells: 2D or not 2D?287Excitonic states and structural stability in two-dimensional hybrid organic-inorganic perovskites49Small Cyclic Diammonium Cation Templated (110)-Oriented 2D Halide (X = I, Br, Cl) Perovskites with White-Light Emission130Melting Transitions of the Organic Subphase in Layered Two-Dimensional Halide Perovskites41Giant Nonlinear Optical Response in 2D Perovskite Heterostructures84Experiment Specification, Capture and Laboratory Automation Technology (ESCALATE): a software pipeline for automated chemical experimentation and data management73From 2D to 1D Electronic Dimensionality in Halide Perovskites with Stepped and Flat Layers Using Propylammonium as a Spacer128Green Emitting Single-Crystalline Bulk Assembly of Metal Halide Clusters with Near-Unity Photoluminescence Quantum Efficiency169Controlling Solvate Intermediate Growth for Phase-Pure Organic Lead Iodide Ruddlesden–Popper (C4H9NH3)2(CH3NH3)n−1PbnI3n+1 Perovskite Thin Films44Growth and morphology control of CH3NH3PbBr3 crystals5Two-dimensional hybrid organic-inorganic semiconductors deposited by resonant infrared, matrix-assisted pulsed laser evaporation2Ruddlesden–Popper Perovskites: Synthesis and Optical Properties for Optoelectronic Applications185Recent developments in emerging two-dimensional materials and their applications885Prediction of room-temperature half-metallicity in layered halide double perovskites35Bulk Assemblies of Lead Bromide Trimer Clusters with Geometry-Dependent Photophysical Properties74Crystallization of Ionically Bonded Organic Metal Halide Hybrids4Dual-source vacuum deposition of pure and mixed halide 2D perovskites: thin film characterization and processing guidelines29Function-oriented synthesis of two-dimensional (2D) covalent organic frameworks – from 3D solids to 2D sheets243Materials chemistry and engineering in metal halide perovskite lasers411Synthesis, modular composition, and electrochemical properties of lamellar iron sulfides15Understanding the Energetics in Two-dimensional Metal Halide Perovskite Quantum Wells0Two-Dimensional 111-Type In -Based Halide Perovskite Cs 3 In 2 X 9 ( X = Cl , Br , I ) with Optimal Band Gap for Photovoltaics and Defect-Insensitive Blue Emission28Bulk Assembly of Multicomponent Zero-Dimensional Metal Halides with Dual Emission94Band Alignment in Two-Dimensional Halide Perovskite Heterostructures: Type I or Type II?63From bulk to molecularly thin hybrid perovskites264Directional Anisotropy of the Vibrational Modes in 2D-Layered Perovskites144Organic Cation Alloying on Intralayer A and Interlayer A’ sites in 2D Hybrid Dion–Jacobson Lead Bromide Perovskites (A’)(A)Pb 2 Br 787Synthesis and Localized Photoluminescence Blinking of Lead‐Free 2D Nanostructures of Cs3Bi2I6Cl3 Perovskite44Synthesis and Localized Photoluminescence Blinking of Lead‐Free 2D Nanostructures of Cs3Bi2I6Cl3 Perovskite8Can Machines “Learn” Halide Perovskite Crystal Formation without Accurate Physicochemical Features?12Spin Correlated-Plasmons at Room Temperature Driven by Electronic Correlations in Lead-Free 2D Hybrid Organic–Inorganic Perovskites13Expanded Analogs of Three‐Dimensional Lead‐Halide Hybrid Perovskites65Expanded Analogs of Three‐Dimensional Lead‐Halide Hybrid Perovskites8Narrow-band emitters in LED backlights for liquid-crystal displays217Low-frequency Raman spectrum of 2D layered perovskites: Local atomistic motion or superlattice modes?48Structural Diversity in Layered Hybrid Perovskites, A2PbBr4 or AA′PbBr4, Templated by Small Disc-Shaped Amines39Molecular Engineering of Organic Spacer Cations for Efficient and Stable Formamidinium Perovskite Solar Cell83Solid-State NMR and NQR Spectroscopy of Lead-Halide Perovskite Materials140Photoluminescent and vapochromic properties of the Mn(II)-doped (C6H11NH3)2PbBr4 layered organic–inorganic hybrid perovskite3The Emergence of Halide Layered Double Perovskites161Electron tunneling at the molecularly thin 2D perovskite and graphene van der Waals interface64Lead‐Free Halide Double Perovskites: Structure, Luminescence, and Applications131Perovskite Puzzle for Revolutionary Functional Materials11Perovskite‐Related 2D Compounds in the System 5‐Amino Valerian Acid Cation/MA/Pb/X (X = Cl, Br) – Synthesis, Crystal Structures, and Optical Properties16Dual-color emitting Mn 2+ ion doped (PEA) 2 PbBr 4 perovskite towards white light-emitting diodes40Universal Strategy of 3D and 2D Hybrid Perovskites Single Crystal Growth via In Situ Solvent Conversion26Understanding and harnessing the potential of layered perovskite-based absorbers for solar cells19Organic–inorganic hybrid and inorganic halide perovskites: structural and chemical engineering, interfaces and optoelectronic properties49Etude des propriétés structurales, optiques et de la structure de bandes électroniques dans des halogénures de Plomb organiques : ABTPbCI3 et (Mélamine) PbCI40Effects of organic cations on optical properties and structural stability in two-dimensional hybrid perovskites1Role of spacer cations and structural distortion in two-dimensional germanium halide perovskites69Role of the spacer cation in the growth and crystal orientation of two-dimensional perovskites18The Dion–Jacobson perovskite CsSbCl 4 : a promising Pb-free solar-cell absorber with optimal bandgap ∼1.4 eV, strong optical absorption ∼10 5 cm −1 , and large power-conversion efficiency above 20%29The emergence and origin of broader light emission from two-dimensional layered (C 12 H 25 NH 3 ) 2 MnCl 4 at low-temperatures4Tuning the Interfacial Dipole Moment of Spacer Cations for Charge Extraction in Efficient and Ultrastable Perovskite Solar Cells99The 2D Halide Perovskite Rulebook: How the Spacer Influences Everything from the Structure to Optoelectronic Device Efficiency1083Laurionite Competes with 2D Ruddlesden–Popper Perovskites During the Saturation Recrystallization Process7Emerging Low‐Dimensional Crystal Structure of Metal Halide Perovskite Optoelectronic Materials and Devices60Probing Carrier Transport in Layered Perovskites with Nonlinear Optical and Photocurrent Spectroscopies9Layered Double Perovskites75Cation Dynamics in Hybrid Halide Perovskites40An Overview for Zero‐Dimensional Broadband Emissive Metal‐Halide Single Crystals269Ferroelectricity and Rashba effect in 2D organic–inorganic hybrid perovskites85Shedding Light on the Stability and Structure–Property Relationships of Two-Dimensional Hybrid Lead Bromide Perovskites51Structural chemistry of layered lead halide perovskites containing single octahedral layers592D Layered Dipeptide Crystals for Piezoelectric Applications46Structural diversity in hybrid lead halides templated by 4-methylimidazolium16Relationships between Distortions of Inorganic Framework and Band Gap of Layered Hybrid Halide Perovskites68Growth-Controlled Broad Emission in Phase-Pure Two-Dimensional Hybrid Perovskite Films13Magnetocaloric effect and critical behavior in arylamine-based copper chloride layered organic-inorganic perovskite172D Hybrid Halide Perovskites: Structure, Properties, and Applications in Solar Cells136Structure‐Property Relationships and Idiosyncrasies of Bulk, 2D Hybrid Lead Bromide Perovskites25PbS Nanocrystals Made Using Excess Lead Chloride Have a Halide-Perovskite-Like Surface22Surface Passivation Using 2D Perovskites toward Efficient and Stable Perovskite Solar Cells531Crystallization regulation of solution-processed two-dimensional perovskite solar cells22Lead-free layered Aurivillius-type Sn-based halide perovskite Ba 2 X 2 [Cs n −1 Sn n X 3 n +1 ] (X = I/Br/Cl) with an optimal band gap of ∼1.26 eV and theoretical efficiency beyond 27% for photovoltaics6Monochromatic light-enhanced photocatalytic CO 2 reduction based on exciton properties of two-dimensional lead halide perovskites16Unlocking surface octahedral tilt in two-dimensional Ruddlesden-Popper perovskites115Segmented Highly Reversible Thermochromic Layered Perovskite [(CH2)2(NH3)2]CuCl4 Crystal Coupled with an Inverse Magnetocaloric Effect22Active meta-learning for predicting and selecting perovskite crystallization experiments24The halogen chemistry of halide perovskites41Polar Ferromagnet Induced by Fluorine Positioning in Isomeric Layered Copper Halide Perovskites20Ruddlesden–Popper 2D perovskites of type (C6H9C2H4NH3)2(CH3NH3)n−1PbnI3n+1 (n = 1–4) for optoelectronic applications95Multifunctional Chiral 2D Lead Halide Perovskites with Circularly Polarized Photoluminescence and Piezoelectric Energy Harvesting Properties112Polarity and Ferromagnetism in Two-Dimensional Hybrid Copper Perovskites with Chlorinated Aromatic Spacers48Ligand Control of Structural Diversity in Luminescent Hybrid Copper(I) Iodides66(C 5 H 6 N)Pb 2 X 5 (X = Cl, Br): Hybrid Lead Halides Based on Seven-Coordinate Pb(II)15Thermochromic Phase Transitions of Long Odd-Chained Inorganic–Organic Layered Perovskite-Type Hybrids [(CnH2n+1NH3)2PbI4], n = 11, 13, and 1516Sub-angstrom noninvasive imaging of atomic arrangement in 2D hybrid perovskites13Effect of Stability of Two-Dimensional (2D) Aminoethyl Methacrylate Perovskite Using Lead-Based Materials for Ammonia Gas Sensor Application10Screening of Excitons by Organic Cations in Quasi-Two-Dimensional Organic–Inorganic Lead-Halide Perovskites58Probing Lattice Dynamics in Two-Dimensional Inorganic Pseudohalide Perovskites with Ultrafast Infrared Spectroscopy11Enhancing and Extinguishing the Different Emission Features of 2D (EA1−xFAx)4Pb3Br10 Perovskite Films3Engineering van der Waals Materials for Advanced Metaphotonics100Ordered Mixed-Spacer 2D Bromide Perovskites and the Dual Role of 1,2,4-Triazolium Cation38Serendipity based recommender system for perovskites material discovery: balancing exploration and exploitation across multiple models7Serendipity based recommender system for perovskites material discovery: balancing exploration and exploitation across multiple models5Chiral 2D Cu(I) Halide Frameworks52A practical guide to Three-dimensional halide perovskites: Structure, synthesis, and measurement3Efficient inorganic CsPbI2Br perovskite indoor photovoltaics demonstrated via slower crystallization by incorporated dimethylammonium iodide15Bandgap modification in 0D tellurium iodide perovskite derivatives via incorporation of polyiodide species14Broadband yellow and white emission from large octahedral tilting in (110)-oriented layered perovskites: imidazolium-methylhydrazinium lead halides24Challenges and future prospects2Does it mix? Insights and attempts to predict the formability of single phase mixed A-cation lead iodide perovskites8One-dimensional organic metal halide nanoribbons with dual emission11Emergence of Rashba-/Dresselhaus effects in Ruddlesden–Popper halide perovskites with octahedral rotations22Nanostructured Ruddlesden–Popper-Layered Lead Bromide Perovskites with Stable and Selected Wavelength for Photodetection Applications24Optoelectronic Properties of Expanded Halide Perovskite Analogs Enriched by Molecular Diversity0Organic Chain Length Effect on Trap States of Lead Halide Perovskite Scintillators23Carriers, Quasi-particles, and Collective Excitations in Halide Perovskites109Design Rules for Obtaining Narrow Luminescence from Semiconductors Made in Solution87Formamidine Engineering the Lattice Distortion of Chiral Halide Perovskites for Efficient Blue Circularly Polarized Emission28Right band gaps for the right reason at low computational cost with a meta-GGA36Meltable Hybrid Antimony and Bismuth Iodide One-Dimensional Perovskites16Energetic Stability and Band-Edge Orbitals of Layered Inorganic Perovskite Compounds for Solar Energy Applications2Clusterization-Triggered Emission Enhanced by Energy Transfer in the Layered Metal Halide Hybrid Material (TET)2[Pb4Cl16]11Impact of bromide incorporation on strain modulation in 2D Ruddlesden-Popper perovskite solar cells9First Principles Atomistic Theory of Halide Perovskites3Optical Characterizations for Broadening Emissions from Doping of the Two-Dimensional Tin–Lead Perovskite Films4An Air-Stable and Exfoliable Ferromagnetic Two-Dimensional Perovskite, (Phenethylammonium)2CrCl413Excitons in metal-halide perovskites from first-principles many-body perturbation theory25Unveiling the Influence of Organic Chain Length on the Physical Properties of Two-Dimensional Cobalt-Based Hybrid Perovskites2Extending the Family of Hybrid Layered Fluoride Perovskites2Halide perovskites from first principles: from fundamental optoelectronic properties to the impact of structural and chemical heterogeneity13Reversible Glass‐Crystal Transition in a New Type of 2D Metal Halide Perovskites19Rational Strategies to Improve the Efficiency of 2D Perovskite Solar Cells34Elucidating phonon dephasing mechanisms in layered perovskites with coherent Raman spectroscopies3Phonon Directionality Impacts Electron–Phonon Coupling and Polarization of the Band-Edge Emission in Two-Dimensional Metal Halide Perovskites9Pressure-controlled free exciton and self-trapped exciton emission in quasi-one-dimensional hybrid lead bromides50Advanced Organic–Inorganic Hybrid Materials for Optoelectronic Applications221Anion Exchange and Lateral Heterostructure Formation in Ferromagnetic PEA2Cr(Cl,Br)4 Two-Dimensional Perovskites8Leveraging ordered voids in microporous perovskites for intercalation and post-synthetic modification5Influence of organic cations on the structures of layered lead bromide perovskites1Raising the operating temperature of layered perovskite phase-change materials beyond 100 °C via alkylammonium extension2

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  1. Promising photovoltaic and solid-state-lighting materials: two-dimensional Ruddlesden–Popper type lead-free halide double perovskites Cs n+1 In n/2 Sb n/2 I 3n+1 ( n = 3) and Cs n+1 In n/2 Sb n/2 Cl 3n+1 /Cs m+1 Cu m/2 Bi m/2 Cl 3m+1 ( n = 3, m = 1)

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  2. Completing the Picture of 2-(Aminomethylpyridinium) Lead Hybrid Perovskites: Insights into Structure, Conductivity Behavior, and Optical Properties

    Chemistry of Materials · 2018-08-27

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  3. Structural evolution and photoluminescence properties of a 2D hybrid perovskite under pressure

    APL Materials · 2018-08-31

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  4. General Synthesis Principles for Ruddlesden–Popper Hybrid Perovskite Halides from a Dynamic Equilibrium

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  5. Two-dimensional perovskite materials: From synthesis to energy-related applications

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  6. Effect of High Dipole Moment Cation on Layered 2D Organic–Inorganic Halide Perovskite Solar Cells

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  7. Low dimensional metal halide perovskites and hybrids

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  8. Doping Mn2+ in Single-Crystalline Layered Perovskite Microcrystals

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  9. A hybrid fluoride layered perovskite, ( en H 2 )MnF 4

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  10. Designing a new family of oxonium-cation based structurally diverse organic–inorganic hybrid iodoantimonate crystals

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  12. Searching for stability at lower dimensions: current trends and future prospects of layered perovskite solar cells

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  13. Structure-directing effects in (110)-layered hybrid perovskites containing two distinct organic moieties

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  14. White light emission in low-dimensional perovskites

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  15. The Role of Chloride Incorporation in Lead‐Free 2D Perovskite (BA)2SnI4: Morphology, Photoluminescence, Phase Transition, and Charge Transport

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  16. Tuning the Luminescence of Layered Halide Perovskites

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  17. Two‐Dimensional Halide Perovskites in Solar Cells: 2D or not 2D?

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  18. Excitonic states and structural stability in two-dimensional hybrid organic-inorganic perovskites

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  19. Small Cyclic Diammonium Cation Templated (110)-Oriented 2D Halide (X = I, Br, Cl) Perovskites with White-Light Emission

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  20. Melting Transitions of the Organic Subphase in Layered Two-Dimensional Halide Perovskites

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  21. Giant Nonlinear Optical Response in 2D Perovskite Heterostructures

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  23. From 2D to 1D Electronic Dimensionality in Halide Perovskites with Stepped and Flat Layers Using Propylammonium as a Spacer

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  24. Green Emitting Single-Crystalline Bulk Assembly of Metal Halide Clusters with Near-Unity Photoluminescence Quantum Efficiency

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  25. Controlling Solvate Intermediate Growth for Phase-Pure Organic Lead Iodide Ruddlesden–Popper (C4H9NH3)2(CH3NH3)n−1PbnI3n+1 Perovskite Thin Films

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  26. Growth and morphology control of CH3NH3PbBr3 crystals

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  27. Two-dimensional hybrid organic-inorganic semiconductors deposited by resonant infrared, matrix-assisted pulsed laser evaporation

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  28. Ruddlesden–Popper Perovskites: Synthesis and Optical Properties for Optoelectronic Applications

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  29. Recent developments in emerging two-dimensional materials and their applications

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  30. Prediction of room-temperature half-metallicity in layered halide double perovskites

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  31. Bulk Assemblies of Lead Bromide Trimer Clusters with Geometry-Dependent Photophysical Properties

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  32. Crystallization of Ionically Bonded Organic Metal Halide Hybrids

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  33. Dual-source vacuum deposition of pure and mixed halide 2D perovskites: thin film characterization and processing guidelines

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  34. Function-oriented synthesis of two-dimensional (2D) covalent organic frameworks – from 3D solids to 2D sheets

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  35. Materials chemistry and engineering in metal halide perovskite lasers

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  37. Understanding the Energetics in Two-dimensional Metal Halide Perovskite Quantum Wells

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  38. Two-Dimensional 111-Type In -Based Halide Perovskite Cs 3 In 2 X 9 ( X = Cl , Br , I ) with Optimal Band Gap for Photovoltaics and Defect-Insensitive Blue Emission

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  39. Bulk Assembly of Multicomponent Zero-Dimensional Metal Halides with Dual Emission

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  40. Band Alignment in Two-Dimensional Halide Perovskite Heterostructures: Type I or Type II?

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  41. From bulk to molecularly thin hybrid perovskites

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  42. Directional Anisotropy of the Vibrational Modes in 2D-Layered Perovskites

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  43. Organic Cation Alloying on Intralayer A and Interlayer A’ sites in 2D Hybrid Dion–Jacobson Lead Bromide Perovskites (A’)(A)Pb 2 Br 7

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  45. Synthesis and Localized Photoluminescence Blinking of Lead‐Free 2D Nanostructures of Cs3Bi2I6Cl3 Perovskite

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  46. Can Machines “Learn” Halide Perovskite Crystal Formation without Accurate Physicochemical Features?

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  47. Spin Correlated-Plasmons at Room Temperature Driven by Electronic Correlations in Lead-Free 2D Hybrid Organic–Inorganic Perovskites

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  48. Expanded Analogs of Three‐Dimensional Lead‐Halide Hybrid Perovskites

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  49. Expanded Analogs of Three‐Dimensional Lead‐Halide Hybrid Perovskites

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  50. Narrow-band emitters in LED backlights for liquid-crystal displays

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