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RESEARCH PAPER · Chemical Reviews · 2019

Tuning the Luminescence of Layered Halide Perovskites

Matthew D. Smith, Bridget A. Connor, Hemamala I. Karunadasa

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Tuning the Luminescence of Layered Halide PerovskitesOriginalDirect emission from quartet excited states triggered by upconversion phenomena in solid-phase synthesized fluorescent lead-free organic–inorganic hybrid compounds73Two-dimensional lead-free halide perovskite materials and devices81Optically Modulated Ultra-Broad-Band Warm White Emission in Mn2+-Doped (C6H18N2O2)PbBr4 Hybrid Metal Halide Phosphor174Synthetic Variation and Structural Trends in Layered Two-Dimensional Alkylammonium Lead Halide Perovskites137Two-Dimensional Dion–Jacobson Hybrid Lead Iodide Perovskites with Aromatic Diammonium Cations386Lead-Free Halide Perovskites and Perovskite Variants as Phosphors toward Light-Emitting Applications159Seven-Layered 2D Hybrid Lead Iodide Perovskites105Orange to Red, Emission-Tunable Mn-Doped Two-Dimensional Perovskites with High Luminescence and Stability95Intrinsic Self‐Trapped Emission in 0D Lead‐Free (C 4 H 14 N 2 ) 2 In 2 Br 10 Single Crystal168Intrinsic Self‐Trapped Emission in 0D Lead‐Free (C4H14N2)2In2Br10 Single Crystal374Active meta-optics and nanophotonics with halide perovskites90Layered Lead Iodide of [Methylhydrazinium] 2 PbI 4 with a Reduced Band Gap: Thermochromic Luminescence and Switchable Dielectric Properties Triggered by Structural Phase Transitions108Single‐Component White‐Light Emission in 2D Hybrid Perovskites with Hybridized Halogen Atoms90Inorganic Cage Motion Dominates Excited-State Dynamics in 2D-Layered Perovskites (CxH2x+1NH3)2PbI4 (x = 4–9)64Multicolor Tunable Polymeric Nanoparticle from the Tetraphenylethylene Cage for Temperature Sensing in Living Cells1630D Cs 3 Cu 2 X 5 (X = I, Br, and Cl) Nanocrystals: Colloidal Syntheses and Optical Properties222Breaking Forbidden Transitions for Emission of Self-Trapped Excitons in Two Dimensional (F2CHCH2NH3)2CdBr4 Perovskite through Pb Alloying66Homo- and Heterovalent Doping-Mediated Self-Trapped Exciton Emission and Energy Transfer in Mn-Doped Cs2Na1–xAgxBiCl6 Double Perovskites151Origin of Broad-Band Emission and Impact of Structural Dimensionality in Tin-Alloyed Ruddlesden–Popper Hybrid Lead Iodide Perovskites792D layered all-inorganic halide perovskites: recent trends in their structure, synthesis and properties75Charge carrier dynamics in two-dimensional hybrid perovskites: Dion–Jacobson vs. Ruddlesden–Popper phases155Dimensional reduction of the small-bandgap double perovskite Cs 2 AgTlBr 665Materials chemistry and engineering in metal halide perovskite lasers411Rare-earth-containing perovskite nanomaterials: design, synthesis, properties and applications422What Defines a Halide Perovskite?509Inorganic Halide Double Perovskites with Optoelectronic Properties Modulated by Sublattice Mixing119Control of Crystal Symmetry Breaking with Halogen-Substituted Benzylammonium in Layered Hybrid Metal-Halide Perovskites135Charge Carrier Recombination Dynamics of Two-Dimensional Lead Halide Perovskites85Unveiling Mn2+ Dopant States in Two-Dimensional Halide Perovskite toward Highly Efficient Photoluminescence92Direct evidence of weakly dispersed and strongly anharmonic optical phonons in hybrid perovskites86Shining Light on the Photoluminescence Properties of Metal Halide Perovskites174Broad-band emission in metal halide perovskites: Mechanism, materials, and applications288Optoelectronic Properties of Two-Dimensional Bromide Perovskites: Influences of Spacer Cations74Polarons in Halide Perovskites: A Perspective172Three-Dimensional Perovskite Methylhydrazinium Lead Chloride with Two Polar Phases and Unusual Second-Harmonic Generation Bistability above Room Temperature173Highly Luminescent and Stable Green Quasi‐2D Perovskite‐Embedded Polymer Sheets by Inkjet Printing85Extrinsic nature of the broad photoluminescence in lead iodide-based Ruddlesden–Popper perovskites198Observation of Two Thresholds Leading to Polariton Condensation in 2D Hybrid Perovskites66Insight into the structural, electronic, mechanical and optical properties of inorganic lead bromide perovskite APbBr3 (A = Li, Na, K, Rb, and Cs)85Recent Progress in Engineering Metal Halide Perovskites for Efficient Visible‐Light‐Driven Photocatalysis135Tailorable Indirect to Direct Band-Gap Double Perovskites with Bright White-Light Emission: Decoding Chemical Structure Using Solid-State NMR86Establishing charge-transfer excitons in 2D perovskite heterostructures97Three‐Dimensional Cuprous Lead Bromide Framework with Highly Efficient and Stable Blue Photoluminescence Emission93Negative Pressure Engineering with Large Cage Cations in 2D Halide Perovskites Causes Lattice Softening144Bright Blue and Green Luminescence of Sb(III) in Double Perovskite Cs2MInCl6 (M = Na, K) Matrices372Supramolecular Approach for Fine-Tuning of the Bright Luminescence from Zero-Dimensional Antimony(III) Halides179Correlation of Dielectric Confinement and Excitonic Binding Energy in 2D Layered Hybrid Perovskites Using Temperature Dependent Photoluminescence116Enhancing Photoluminescence Quantum Yield in 0D Metal Halides by Introducing Water Molecules159Expanded Analogs of Three‐Dimensional Lead‐Halide Hybrid Perovskites65Narrow-band emitters in LED backlights for liquid-crystal displays217Efficient Lone-Pair-Driven Luminescence: Structure–Property Relationships in Emissive 5s2 Metal Halides416Self-trapped excitons in two-dimensional perovskites141Reaching 90% Photoluminescence Quantum Yield in One-Dimensional Metal Halide C 4 N 2 H 14 PbBr 4 by Pressure-Suppressed Nonradiative Loss244Halide Perovskite, a Potential Scintillator for X‐Ray Detection292Defect-Related Broadband Emission in Two-Dimensional Lead Bromide Perovskite Microsheets75Single Ensemble Non-exponential Photoluminescent Population Decays from a Broadband White-Light-Emitting Perovskite72Library of Two-Dimensional Hybrid Lead Halide Perovskite Scintillator Crystals141Organic-to-inorganic structural chirality transfer in a 2D hybrid perovskite and impact on Rashba-Dresselhaus spin-orbit coupling455Two Origins of Broadband Emission in Multilayered 2D Lead Iodide Perovskites98Solid-State NMR and NQR Spectroscopy of Lead-Halide Perovskite Materials140High energy X-ray radiation sensitive scintillating materials for medical imaging, cancer diagnosis and therapy250Heterogeneous Fenton catalysts: A review of recent advances878The Emergence of Halide Layered Double Perovskites161Conformational disorder of organic cations tunes the charge carrier mobility in two-dimensional organic-inorganic perovskites112Lead‐Free Halide Double Perovskites: Structure, Luminescence, and Applications131Lead‐Free Perovskite‐Inspired Absorbers for Indoor Photovoltaics184Alternative Organic Spacers for More Efficient Perovskite Solar Cells Containing Ruddlesden–Popper Phases111Boosting triplet self-trapped exciton emission in Te(IV)-doped Cs2SnCl6 perovskite variants239Recent Advances in Luminescent Zero‐Dimensional Organic Metal Halide Hybrids241Manipulation of Cl/Br transmutation in zero-dimensional Mn 2+ -based metal halides toward tunable photoluminescence and thermal quenching behaviors87Co-luminescence in a zero-dimensional organic–inorganic hybrid antimony halide with multiple coordination units67Overview of recent progress in electrohydrodynamic jet printing in practical printed electronics: focus on the variety of printable materials for each component90Recent progress of zero-dimensional luminescent metal halides873Role of spacer cations and structural distortion in two-dimensional germanium halide perovskites69Towards superior X-ray detection performance of two-dimensional halide perovskite crystals by adjusting the anisotropic transport behavior65Using steric hindrance to manipulate and stabilize metal halide perovskites for optoelectronics76Lead‐Free Halide Perovskites for Light Emission: Recent Advances and Perspectives335Dynamic Motion of Organic Spacer Cations in Ruddlesden–Popper Lead Iodide Perovskites Probed by Solid-State NMR Spectroscopy76The 2D Halide Perovskite Rulebook: How the Spacer Influences Everything from the Structure to Optoelectronic Device Efficiency1083Highly Efficient Halide Perovskite Light‐Emitting Diodes via Molecular Passivation87Tuning the Excitonic Properties of the 2D (PEA)2(MA)n−1PbnI3n+1Perovskite Family via Quantum Confinement83Doubling the Stakes: The Promise of Halide Double Perovskites159The photophysics of Ruddlesden-Popper perovskites: A tale of energy, charges, and spins73Unprecedented 2D Homochiral Hybrid Lead‐Iodide Perovskite Thermochromic Ferroelectrics with Ferroelastic Switching157A Review on X-ray Excited Emission Decay Dynamics in Inorganic Scintillator Materials98Distance Dependence of Förster Resonance Energy Transfer Rates in 2D Perovskite Quantum Wells via Control of Organic Spacer Length100Lead-Free Organic–Perovskite Hybrid Quantum Wells for Highly Stable Light-Emitting Diodes130[Methylhydrazinium]2PbBr4, a Ferroelectric Hybrid Organic–Inorganic Perovskite with Multiple Nonlinear Optical Outputs163Material exploration via designing spatial arrangement of octahedral units: a case study of lead halide perovskites87Two‐dimensional halide perovskite quantum‐well emitters: A critical review79Layered Double Perovskites75The Role of Dimensionality on the Optoelectronic Properties of Oxide and Halide Perovskites, and their Halide Derivatives179Polarons and Charge Localization in Metal‐Halide Semiconductors for Photovoltaic and Light‐Emitting Devices110Multimode dynamic luminescent switching of lead halide hybrids for anti-counterfeiting and encryption94An Overview for Zero‐Dimensional Broadband Emissive Metal‐Halide Single Crystals269Emerging Indoor Photovoltaic Technologies for Sustainable Internet of Things322Low‐Dimensional Metal Halide Perovskite Crystal Materials: Structure Strategies and Luminescence Applications281In Situ Phase-Transition Crystallization of All-Inorganic Water-Resistant Exciton-Radiative Heteroepitaxial CsPbBr 3 –CsPb 2 Br 5 Core–Shell Perovskite Nanocrystals81Structural descriptor for enhanced spin-splitting in 2D hybrid perovskites225Indium-antimony-halide single crystals for high-efficiency white-light emission and anti-counterfeiting252Advances in solution-processed near-infrared light-emitting diodes369Mechanics-coupled stability of metal-halide perovskites127Photoluminescent ionic metal halides based on s2 typed ions and aprotic ionic liquid cations87Molecular spectroscopy of hybrid organic–inorganic perovskites and related compounds68Ligand-Driven Grain Engineering of High Mobility Two-Dimensional Perovskite Thin-Film Transistors119Relationships between Distortions of Inorganic Framework and Band Gap of Layered Hybrid Halide Perovskites68Directed assembly of layered perovskite heterostructures as single crystals122Ultrafast Study of Exciton Transfer in Sb(III)-Doped Two-Dimensional [NH3(CH2)4NH3]CdBr4 Perovskite84Antimony‐Doped Lead‐Free Zero‐Dimensional Tin(IV)‐Based Organic–Inorganic Metal Halide Hybrids with High Photoluminescence Quantum Yield and Remarkable Stability72Cyan Emission in Two-Dimensional Colloidal Cs2CdCl4:Sb3+ Ruddlesden–Popper Phase Nanoplatelets67Alkyl–Aryl Cation Mixing in Chiral 2D Perovskites137Toward a General Understanding of Exciton Self-Trapping in Metal Halide Perovskites930D Perovskites: Unique Properties, Synthesis, and Their Applications386Exciton Self-Trapping for White Emission in 100-Oriented Two-Dimensional Perovskites via Halogen Substitution131Near-Infrared Phosphorescent Hybrid Organic–Inorganic Perovskite with High-Contrast Dielectric and Third-Order Nonlinear Optical Switching Functionalities72Zero-Dimensional Lead-Free Halide with Indirect Optical Gap and Enhanced Photoluminescence by Sb Doping76Color-tunable persistent luminescence in 1D zinc–organic halide microcrystals for single-component white light and temperature-gating optical waveguides103Regulation of the luminescence mechanism of two-dimensional tin halide perovskites149Ligand Control of Structural Diversity in Luminescent Hybrid Copper(I) Iodides66Recent progress of perovskite devices fabricated using thermal evaporation method: Perspective and outlook120Light Emission of Self‐Trapped Excitons in Inorganic Metal Halides for Optoelectronic Applications260Luminescent Organic‐Inorganic Hybrid Metal Halides: An Emerging Class of Stimuli‐Responsive Materials76Micro‐Nano Structure Functionalized Perovskite Optoelectronics: From Structure Functionalities to Device Applications78Bright Green Emission from Self-Trapped Excitons Triggered by Sb3+ Doping in Rb4CdCl6145Understanding Electron–Phonon Interactions in 3D Lead Halide Perovskites from the Stereochemical Expression of 6s 2 Lone Pairs116Reversible Triple-Mode Switching in Photoluminescence from 0D Hybrid Antimony Halides139Pressure-Driven Phase Transition in Two-Dimensional Perovskite MHy2PbBr469Structural Descriptors to Correlate Pb Ion Displacement and Broadband Emission in 2D Halide Perovskites121The Origin of Broad Emission in ⟨100⟩ Two-Dimensional Perovskites: Extrinsic vs Intrinsic Processes73Factors influencing self-trapped exciton emission of low-dimensional metal halides115Recent Advances on Mn2+‐Doping in Diverse Metal Halide Perovskites66Maximally Chiral Emission via Chiral Quasibound States in the Continuum72Achieving Near‐unity Photoluminescence Quantum Yields in Organic‐Inorganic Hybrid Antimony (III) Chlorides with the [SbCl 5 ] Geometry129Ultrabright Light Emission Properties of All-Inorganic and Hybrid Organic–Inorganic Copper(I) Halides121Carriers, Quasi-particles, and Collective Excitations in Halide Perovskites109Design Rules for Obtaining Narrow Luminescence from Semiconductors Made in Solution87Advances in the Application of Perovskite Materials460Reversible Triple-Mode Photo- and Radioluminescence and Nonlinear Optical Switching in Highly Efficient 0D Hybrid Cuprous Halides109Nature of Self-Trapped Exciton Emission in Zero-Dimensional Cs 2 ZrCl 6 Perovskite Nanocrystals78Pressure-Modulated Anomalous Organic–Inorganic Interactions Enhance Structural Distortion and Second-Harmonic Generation in MHyPbBr 3 Perovskite89Lead‐Free Halide Perovskite Materials and Optoelectronic Devices: Progress and Prospective326Accommodative Organoammonium Cations in A‐Sites of Sb─In Halide Perovskite Derivatives for Tailoring BroadBand Photoluminescence with X‐Ray Scintillation and White‐Light Emission75Multisite Fine‐Tuning in Hybrid Cadmium Halides Enables Wide Range Emissions for Anti‐Counterfeiting92Advances in Perovskite Nanocrystals and Nanocomposites for Scintillation Applications81Near‐infrared emitting metal halide materials: Luminescence design and applications78Exciton engineering of 2D Ruddlesden–Popper perovskites by synergistically tuning the intra and interlayer structures112Optical Phenomena in Molecule-Based Magnetic Materials154Self-Trapped Exciton Emission in Highly Polar 0D Hybrid Ammonium/Hydronium-Based Perovskites Triggered by Antimony Doping89Perovskite Solar Cells and Light Emitting Diodes: Materials Chemistry, Device Physics and Relationship71Diverse Perovskite Solar Cells: Progress, Challenges, and Perspectives74

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    Feng Jiang, Xingxing Jiang, Weihao Zheng, Yu Ouyang, Yushuang Zhang, Lihui Li, Peng Fan, Hepeng Zhao, Yang Li, Ying Xiang Jiang, Xiaoli Zhu, Xiujuan Zhuang, Yexin Feng, Anlian Pan

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  43. Charge carrier dynamics in two-dimensional hybrid perovskites: Dion–Jacobson vs. Ruddlesden–Popper phases

    Journal of Materials Chemistry A · 2020-01-01

    Dibyajyoti Ghosh, Debdipto Acharya, Laurent Pédesseau, Claudine Katan, Jacky Even, Sergei Tretiak, Amanda J. Neukirch

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  44. Chirality control in white-light emitting 2D perovskites

    Journal of Materials Chemistry C · 2020-01-01

    Karla Trujillo-Hernández, Germán Rodrı́guez-López, Arián Espinosa-Roa, Jesús González-Roque, A. Paulina Gómora‐Figueroa, Weiguo Zhang, P. Shiv Halasyamani, Vojtěch Jančík, Milan Gembický, Giuseppe Pirruccio, Diego Solís-Ibarra

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  45. Dimensional reduction of the small-bandgap double perovskite Cs 2 AgTlBr 6

    Chemical Science · 2020-01-01

    Bridget A. Connor, Raisa-Ioana Biega, Linn Leppert, Hemamala I. Karunadasa

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  46. Dual-source vacuum deposition of pure and mixed halide 2D perovskites: thin film characterization and processing guidelines

    Journal of Materials Chemistry C · 2020-01-01

    Maria‐Grazia La‐Placa, Dengyang Guo, Lidón Gil‐Escrig, Francisco Palazón, Michele Sessolo, Henk J. Bolink

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  47. Materials chemistry and engineering in metal halide perovskite lasers

    Chemical Society Reviews · 2020-01-01

    Haiyun Dong, Chunhuan Zhang, Xiaolong Liu, Jiannian Yao, Yong Sheng Zhao

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  48. Optically pumped white light-emitting diodes based on metal halide perovskites and perovskite-related materials

    APL Materials · 2020-01-01

    Michael Worku, Liang‐Jin Xu, Maya Chaaban, Azza Ben‐Akacha, Biwu Ma

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  49. Rare-earth-containing perovskite nanomaterials: design, synthesis, properties and applications

    Chemical Society Reviews · 2020-01-01

    Zhichao Zeng, Yueshan Xu, Zheshan Zhang, Zhansheng Gao, Meng Luo, Zongyou Yin, Chao Zhang, Jun Xu, Bolong Huang, Feng Chao Luo, Yaping Du, Chun‐Hua Yan

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  50. Solution-processed lead halide perovskite single crystal scintillators

    Unknown journal · 2020-01-01

    Aozhen Xie

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