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RESEARCH PAPER · Advanced Science · 2017

Self‐Tuning n‐Type Bi2(Te,Se)3/SiC Thermoelectric Nanocomposites to Realize High Performances up to 300 °C

Yu Pan, Umut Aydemir, Fu‐Hua Sun, Chaofeng Wu, Thomas C. Chasapis, Gerald Jeffrey Snyder, Jing‐Feng Li

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Self‐Tuning n‐Type Bi2(Te,Se)3/SiC Thermoelectric Nanocomposites to Realize High Performances up to 300 °COriginalRemarkable Roles of Cu To Synergistically Optimize Phonon and Carrier Transport in n-Type PbTe-Cu 2 Te305Cost effective synthesis of p-type Zn-doped MgAgSb by planetary ball-milling with enhanced thermoelectric properties31Enhanced thermoelectric performance of Bi–Sb–Te/Sb 2 O 3 nanocomposites by energy filtering effect167Pressure-induced electrical transport properties, texture, and microstructure of the (Bi,Sb) 2 Te 3 alloys16Converting natural diatomite into nanoporous silicon for eco-friendly thermoelectric energy conversion20Enhancement of the Thermoelectric Figure of Merit in Blended Cu2Sn1–xZnxS3 Nanobulk Materials21Interfacial reactions in In/Bi2Se3, In/Bi2Te3 and In/Bi2(Se0.2Te0.8)3 couples6Attaining reduced lattice thermal conductivity and enhanced electrical conductivity in as-sintered pure n-type Bi2Te3 alloy32ZnO-Nanoparticle-Dispersed Cu11.5Ni0.5Sb4S13−δ Tetrahedrite Composites with Enhanced Thermoelectric Performance16Synergistic modulation of mobility and thermal conductivity in (Bi,Sb) 2 Te 3 towards high thermoelectric performance170Enhanced performance of thermoelectric nanocomposites based on Cu12Sb4S13 tetrahedrite65Local nanostructures enhanced the thermoelectric performance of n-type PbTe70Thermoelectric (Bi,Sb) 2 Te 3 –Ge 0.5 Mn 0.5 Te composites with excellent mechanical properties49Cation-anion codoping to enhance thermoelectric performance of BiSbSe 312Enhanced thermoelectric properties of the Lu-doped and CNT-dispersed Bi2Te3 alloy49Thermoelectric Performance of Rapidly Microwave-Synthesized α-MgAgSb with SnTe Nanoinclusions38Extraordinary thermoelectric performance in MgAgSb alloy with ultralow thermal conductivity94Amphoteric Indium Enables Carrier Engineering to Enhance the Power Factor and Thermoelectric Performance in n‐Type AgnPb100InnTe100+2n (LIST)77Thermoelectric Cu-doped (Bi,Sb)2Te3: Performance enhancement and stability against high electric current pulse78Complex Band Structures and Lattice Dynamics of Bi 2 Te 3 ‐Based Compounds and Solid Solutions228Energy Filtering of Charge Carriers: Current Trends, Challenges, and Prospects for Thermoelectric Materials539Simultaneous Enhancement of the Thermoelectric and Mechanical Performance in One-Step Sintered n-Type Bi2Te3-Based Alloys via a Facile MgB2 Doping Strategy88High‐Efficiency Thermoelectric Power Generation Enabled by Homogeneous Incorporation of MXene in (Bi,Sb)2Te3 Matrix1923D extruded composite thermoelectric threads for flexible energy harvesting81Microplastics and seafood: lower trophic organisms at highest risk of contamination592Possible Charge Density Wave and Enhancement of Thermoelectric Properties at Mild-Temperature Range in n-Type CuI-Doped Bi2Te2.1Se0.9 Compounds34Effects of Ni Magnetic Nanoparticles on Thermoelectric Properties of n-Type Bi2Te2.7Se0.3 Materials19A new defective 19-electron TiPtSb half-Heusler thermoelectric compound with heavy band and low lattice thermal conductivity37Rapid synthesis of PbSe by MA and HPS and its thermoelectric properties6Practical High-Performance (Bi,Sb)2Te3-Based Thermoelectric Nanocomposites Fabricated by Nanoparticle Mixing and Scrap Recycling42Half‐Heusler Thermoelectric Module with High Conversion Efficiency and High Power Density174Tuning Optimum Temperature Range of Bi2Te3‐Based Thermoelectric Materials by Defect Engineering92Thermoelectric Properties and Low-Energy Carrier Filtering by Mo Microparticle Dispersion in an n-Type (CuI)0.003Bi2(Te,Se)3 Bulk Matrix64Transport properties of AgPb16SbTe18 prepared by the inclusion of nano AgSbTe2 into PbTe matrix0Nanoparticle-modified thermoelectric tetrahedrite as an effective nucleating agent for sodium acetate trihydrate based phase change materials5Enhanced power factor and thermoelectric performance for n-type Bi2Te2.7Se0.3 based composites incorporated with 3D topological insulator nanoinclusions76Bismuth telluride2Defect engineering in thermoelectric materials: what have we learned?481Compensation of Zn substitution and secondary phase controls effective mass and weighted mobility in In and Ga co-doped ZnO material25Evolution of atomic structure and electronic transport properties in n-type Bi2Te3 films via Bi2 planar defects11Identifying the Manipulation of Individual Atomic-Scale Defects for Boosting Thermoelectric Performances in Artificially Controlled Bi2Te3 Films68Enhanced thermoelectric performance of Bi0.5Sb1.5Te3 via Ni-doping: A Shift of peak ZT at elevated temperature via suppressing intrinsic excitation30Simultaneous Regulation of Electrical and Thermal Transport Properties of N-Type Bi2Te3 via Adding Excessive Te Followed by Se Doping34The effects of structural integrity of graphene on the thermoelectric properties of the n-type bismuth-telluride alloy31Boosting Thermoelectric–Mechanical Properties of BiSb-Based Material by SiC Nanocomposites10Effects of SiC doping on the thermoelectric properties of Bi1.9Ba0.1Sr2Co2Oy ceramics15Enhanced thermoelectric performance and mechanical strength of n-type BiTeSe materials produced via a composite strategy62Boron‐Mediated Grain Boundary Engineering Enables Simultaneous Improvement of Thermoelectric and Mechanical Properties in N‐Type Bi2Te363Isotropic Thermoelectric Performance of Layer-Structured n-Type Bi2Te2.7Se0.3 by Cu Doping42Enhancing the thermoelectric performance of Sb 2 Si 2 Te 6 by germanium doping17A comprehensive review on the effects of doping process on the thermoelectric properties of Bi2Te3 based alloys102Mediating Point Defects Endows n‐Type Bi 2 Te 3 with High Thermoelectric Performance and Superior Mechanical Robustness for Power Generation Application135Modulation Doping Enables Ultrahigh Power Factor and Thermoelectric ZT in n‐Type Bi 2 Te 2.7 Se 0.384Temperature induced electrical transport in n-Bi2Te3/p-InAs thermoelectric heterojunctions2Tunable Electrical Conductivity and Simultaneously Enhanced Thermoelectric and Mechanical Properties in n‐type Bi2Te3107Microstructure design via novel thermodynamic route to enhance the thermoelectric performance of GeTe16Identifying polymorphic lattice positioning of copper and the effects on the thermoelectric performance of δ-LAST8A sound velocity method for determining isobaric specific heat capacity9Coupling modification of Fermi level, band flattening and lattice defects to approach outstanding thermoelectric performance of ZnO films via tuning In and Ga incorporation31Enhanced thermoelectric performance of Bi2Te3 by La2O3 dispersion9First principle analysis of the structural, electrical and thermoelectric properties of YTe (Y Si, pb, sn, ge) and PbX (X=O, S, se, te) nano-layers4Recent advances of electrodeposition of Bi 2 Te 3 and its thermoelectric applications in miniaturized power generation and cooling20Improving the thermoelectric properties of Bi2Te2.7Se0.3 through La2O3 dispersion17Design of N‐Type Textured Bi2Te3 with Robust Mechanical Properties for Thermoelectric Micro‐Refrigeration Application55Enhanced thermoelectric performance in Bi 0.5 Sb 1.5 Te 3 /SiC composites prepared by low-temperature liquid phase sintering28Oxygen vacancy engineered tin dioxide/tungsten disulfide heterostructure construction for effective NO sensing8Enhancing thermoelectric performance of n-type AgBi3S5 through synergistically optimizing the effective mass and carrier mobility27Advances in bismuth-telluride-based thermoelectric devices: Progress and challenges247Multi-scale hierarchical microstructure modulation towards high room temperature thermoelectric performance in n-type Bi2Te3-based alloys20Enhancing Thermoelectric and Mechanical Properties of p-Type (Bi, Sb)2Te3 through Rickardite Mineral (Cu2.9Te2) Incorporation16Gibbs Adsorption and Zener Pinning Enable Mechanically Robust High‐Performance Bi 2 Te 3 ‐Based Thermoelectric Devices60High Thermoelectric Performance of Large Size Bi2Te2.7Se0.3 Alloy Ingots17Nanostructuring and band engineering boosting thermoelectric performance of Bi-Sb-Te alloys via CsBr doping17Improved thermoelectric performance of n-type BiTeSe based composites incorporated with PEDOT: PSS polymer nanoinclusions7Advancing Thermoelectric Performance of Bi2Te3 below 400 K23Synergistic Tailoring of Electronic and Thermal Transports in Thermoelectric Se-Free n-Type (Bi,Sb)2Te36Regulation of dynamic recrystallization in p-type Bi2Te3-based compounds leads to high thermoelectric performance and robust mechanical properties22Improved Thermoelectric Performance in n–type Bi2(Te,Se)3 Alloys through the Incorporation of Fe Nanoparticles7Atomic insights into the sintering behaviour of Ag–Cu solid solution nanoparticles on Ag substrate8Synergistic effects lead to high thermoelectric performance of iodine doped pseudo-binary layered GeSb2Te47Advances and challenges in inorganic bulk-based flexible thermoelectric devices53Synergistic regulation of texture and low-angle grain boundaries enables mechanically robust p-type Bi2Te3- based compounds with superior thermoelectric performance10N-type Bi2Se2S materials with high ZT > 1 engineered by multi-scale second phases designing4Realizing p-type InSb with enhanced thermoelectric performance via Cd doping3Multi-dimensional interfaces significantly boost the thermoelectric performance of n-Bi2Te3 in a broad temperature range via electron and phonon transport modulation0Synergistically optimize thermoelectric and mechanical properties of cubic SnSe‐based alloys via nanocomposite engineering utilizing SiC nanoparticles as the dispersed phase4Ag and I co-doping realizes high ZT of In3.97Pb0.03Se3 thermoelectric materials0Synergistic optimization effects of energy band and interface engineering on the thermoelectric properties of Bi0.46Sb1.54Te37Optimizing the thermoelectric performance of Ti0.5Zr0.5NiSn0.98Sb0.02 by melt-spinning and MXene compositing4Point defect-driven switching of conductivity type in Bi 2 Te 3 films prepared by atomic layer deposition0Problems and Prospects of Using Solid Solutions Based on Bi2Te3–Bi2Se3 and Bi2Te3–Sb2Te3 to Create Thermoelements with Operating Temperatures of 300–600 K0

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  2. Cost effective synthesis of p-type Zn-doped MgAgSb by planetary ball-milling with enhanced thermoelectric properties

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  3. Enhanced thermoelectric performance of Bi–Sb–Te/Sb 2 O 3 nanocomposites by energy filtering effect

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  4. Pressure-induced electrical transport properties, texture, and microstructure of the (Bi,Sb) 2 Te 3 alloys

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  5. Converting natural diatomite into nanoporous silicon for eco-friendly thermoelectric energy conversion

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  7. Interfacial reactions in In/Bi2Se3, In/Bi2Te3 and In/Bi2(Se0.2Te0.8)3 couples

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  9. ZnO-Nanoparticle-Dispersed Cu11.5Ni0.5Sb4S13−δ Tetrahedrite Composites with Enhanced Thermoelectric Performance

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  13. Thermoelectric (Bi,Sb) 2 Te 3 –Ge 0.5 Mn 0.5 Te composites with excellent mechanical properties

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  14. Cation-anion codoping to enhance thermoelectric performance of BiSbSe 3

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  15. Enhanced thermoelectric properties of the Lu-doped and CNT-dispersed Bi2Te3 alloy

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  16. Thermoelectric Performance of Rapidly Microwave-Synthesized α-MgAgSb with SnTe Nanoinclusions

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  17. Extraordinary thermoelectric performance in MgAgSb alloy with ultralow thermal conductivity

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  18. Amphoteric Indium Enables Carrier Engineering to Enhance the Power Factor and Thermoelectric Performance in n‐Type AgnPb100InnTe100+2n (LIST)

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  19. Thermoelectric Cu-doped (Bi,Sb)2Te3: Performance enhancement and stability against high electric current pulse

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  23. High‐Efficiency Thermoelectric Power Generation Enabled by Homogeneous Incorporation of MXene in (Bi,Sb)2Te3 Matrix

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  31. Half‐Heusler Thermoelectric Module with High Conversion Efficiency and High Power Density

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  47. Enhanced thermoelectric performance and mechanical strength of n-type BiTeSe materials produced via a composite strategy

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  48. Boron‐Mediated Grain Boundary Engineering Enables Simultaneous Improvement of Thermoelectric and Mechanical Properties in N‐Type Bi2Te3

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  49. Isotropic Thermoelectric Performance of Layer-Structured n-Type Bi2Te2.7Se0.3 by Cu Doping

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  50. Enhancing the thermoelectric performance of Sb 2 Si 2 Te 6 by germanium doping

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