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RESEARCH PAPER · Angewandte Chemie International Edition · 2017

Tailored Engineering of an Unusual (C 4 H 9 NH 3 ) 2 (CH 3 NH 3 ) 2 Pb 3 Br 10 Two‐Dimensional Multilayered Perovskite Ferroelectric for a High‐Performance Photodetector

Lina Li, Zhihua Sun, Peng Wang, Weida Hu, Sasa Wang, Chengmin Ji, Maochun Hong, Junhua Luo

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Tailored Engineering of an Unusual (C 4 H 9 NH 3 ) 2 (CH 3 NH 3 ) 2 Pb 3 Br 10 Two‐Dimensional Multilayered Perovskite Ferroelectric for a High‐Performance PhotodetectorOriginalLaryngeal Cancer In Children And Adolescents34(1,4-Butyldiammonium)CdBr 4 : a layered organic–inorganic hybrid perovskite with a visible-blind ultraviolet photoelectric response26A new antimony-based organic–inorganic hybrid absorber with photoconductive response15Chemically controlled crystal growth of (CH 3 NH 3 ) 2 AgInBr 629Interface engineering in solid state Li metal batteries by quasi-2D hybrid perovskites34Rational design of a triiodide-intercalated dielectric-switching hybrid for visible-light absorption20Switchable dielectric phase transition behaviors in two organic–inorganic copper( ii ) halides with distinct coordination geometries10Inch‐Size Single Crystal of a Lead‐Free Organic–Inorganic Hybrid Perovskite for High‐Performance Photodetector188Progress and Perspective in Low‐Dimensional Metal Halide Perovskites for Optoelectronic Applications132Guanidinium-Formamidinium Lead Iodide: A Layered Perovskite-Related Compound with Red Luminescence at Room Temperature153Semiconductive 1D nanobelt iodoplumbate hybrid with high humidity response12Novel Series of Quasi-2D Ruddlesden–Popper Perovskites Based on Short-Chained Spacer Cation for Enhanced Photodetection97Alloying n‐Butylamine into CsPbBr3 To Give a Two‐Dimensional Bilayered Perovskite Ferroelectric Material189Alloying n‐Butylamine into CsPbBr3 To Give a Two‐Dimensional Bilayered Perovskite Ferroelectric Material31Bilayered Hybrid Perovskite Ferroelectric with Giant Two-Photon Absorption242Exploring a Polar Two‐dimensional Multi‐layered Hybrid Perovskite of (C5H11NH3)2(CH3NH3)Pb2I7 for Ultrafast‐Responding Photodetection74Highly Efficient 2D/3D Hybrid Perovskite Solar Cells via Low‐Pressure Vapor‐Assisted Solution Process216Strain-Mediated Converse Magnetoelectric Coupling in La 0.7 Sr 0.3 MnO 3 /Pb(Mg 1/3 Nb 2/3 )O 3 –PbTiO 3 Multiferroic Heterostructures23Two-Dimensional Halide Perovskites Incorporating Straight Chain Symmetric Diammonium Ions, (NH3CmH2mNH3)(CH3NH3)n−1PbnI3n+1 (m = 4–9; n = 1–4)253Air‐Stable and Self‐Driven Perovskite Photodiodes with High On/Off Ratio and Swift Photoresponse46Series of 2D multilayered perovskites constructed by slicing the 3D [(CH3NH3)PbI3] with 4-fluorobenzylamine14Pervoskite-like hybrid lead bromides with bipyridine as structure-directing agent10Phase transition and switchable dielectric behaviours in an organic–inorganic hybrid compound: (3-nitroanilinium) 2 (18-crown-6) 2 (H 2 PO 4 ) 2 (H 3 PO 4 ) 3 (H 2 O)11Structural Phase Transition and Switchable Dielectric Properties of a Unique Two-Dimensional Organic–Inorganic Hybrid Perovskite Compound [C6H11NH2CH3]4Pb3I1043In‐Plane Ferroelectricity in Thin Flakes of Van der Waals Hybrid Perovskite115Towards a Spectrally Customized Photoresponse from an Organic–Inorganic Hybrid Ferroelectric22Towards a Spectrally Customized Photoresponse from an Organic–Inorganic Hybrid Ferroelectric3Two-Dimensional Hybrid Halide Perovskites: Principles and Promises1584Successive near-room-temperature dielectric phase transitions in a lead-free hybrid perovskite-like compound17Rational chemical doping of metal halide perovskites290Two-Dimensional Lead-Free Perovskite (C6H5C2H4NH3)2CsSn2I7 with High Hole Mobility49Enabling room-temperature processed highly efficient and stable 2D Ruddlesden–Popper perovskite solar cells with eliminated hysteresis by synergistic exploitation of additives and solvents64The First 2D Hybrid Perovskite Ferroelectric Showing Broadband White‐Light Emission with High Color Rendering Index178Low dimensional metal halide perovskites and hybrids489Constructing moisture-stable hybrid lead iodine semiconductors based on hydrogen-bond-free and dual-iodine strategies18High-temperature ferroelastic phase transition in a perovskite-like complex: [Et 4 N] 2 [PbBr 3 ] 217Hydrogen-bonded organo-amino phosphonium halides: dielectric, piezoelectric and possible ferroelectric properties12Incorporating mixed cations in quasi-2D perovskites for high-performance and flexible photodetectors49Tetradic phosphor white light with variable CCT and superlative CRI through organolead halide perovskite nanocrystals46The distinguishing of cis – trans isomers enabled via dielectric/ferroelectric signal feedback in a supramolecular Cu(1,10-phenanthroline) 2 SeO 4 ·(diol) system12Tunable optical absorption in lead-free perovskite-like hybrids by iodide management30Two-dimensional (PEA) 2 PbBr 4 perovskite single crystals for a high performance UV-detector210Quantum and Dielectric Confinement Effects in Lower-Dimensional Hybrid Perovskite Semiconductors864Two-Dimensional Hybrid Perovskite-Type Ferroelectric for Highly Polarization-Sensitive Shortwave Photodetection335Tuning the Luminescence of Layered Halide Perovskites802Two‐Step Structure Phase Transition, Dielectric Anomalies, and Thermochromic Luminescence Behavior in a Direct Band Gap 2D Corrugated Layer Lead Chloride Hybrid of [(CH3)4 N ]4Pb3Cl1022Unraveling the mechanochemical synthesis and luminescence in MnII-based two-dimensional hybrid perovskite (C4H9NH3)2PbCl433Hybrid organic-inorganic perovskites: Polar properties and applications130(C6H13NH3)2(NH2CHNH2)Pb2I7: A Two‐dimensional Bilayer Inorganic–Organic Hybrid Perovskite Showing Photodetecting Behavior24Tunable Ferroelectricity in Ruddlesden–Popper Halide Perovskites51Halide Perovskites for Nonlinear Optics355Highly Sensitive and Ultrafast Responding Array Photodetector Based on a Newly Tailored 2D Lead Iodide Perovskite Crystal57An above-room-temperature phosphonium-based molecular ferroelectric perovskite, [(CH3)4P]CdCl3, with Sb3+-doped luminescence61Controllable Growth of Centimeter-Sized 2D Perovskite Heterostructures for Highly Narrow Dual-Band Photodetectors141Ferroelectricity of the Orthorhombic and Tetragonal MAPbBr3 Single Crystal55Excitons in 2D Organic–Inorganic Halide Perovskites216High‐Temperature Reversible Phase‐Transition Behavior, Switchable Dielectric and Second Harmonic Generation Response of Two Homochiral Crown Ether Clathrates11Optically Modulated Ultra-Broad-Band Warm White Emission in Mn2+-Doped (C6H18N2O2)PbBr4 Hybrid Metal Halide Phosphor174Controlling the Property of Edges in Layered 2D Perovskite Single Crystals52Synthetic Variation and Structural Trends in Layered Two-Dimensional Alkylammonium Lead Halide Perovskites138High-Temperature Antiferroelectric of Lead Iodide Hybrid Perovskites159Highly Oriented Thin Films of 2D Ruddlesden‐Popper Hybrid Perovskite toward Superfast Response Photodetectors44Exploring Lead‐Free Hybrid Double Perovskite Crystals of (BA) 2 CsAgBiBr 7 with Large Mobility‐Lifetime Product toward X‐Ray Detection225Exploring Lead‐Free Hybrid Double Perovskite Crystals of (BA)2CsAgBiBr7 with Large Mobility‐Lifetime Product toward X‐Ray Detection32Bulk Photovoltaic Effect in a Pair of Chiral–Polar Layered Perovskite-Type Lead Iodides Altered by Chirality of Organic Cations193Intrinsic Strong Linear Dichroism of Multilayered 2D Hybrid Perovskite Crystals toward Highly Polarized‐Sensitive Photodetection52Plasmon‐Enhanced InGaZnO Ultraviolet Photodetectors Tuned by Ferroelectric HfZrO17Ferroelectricity and Rashba Effect in a Two-Dimensional Dion-Jacobson Hybrid Organic–Inorganic Perovskite188Designing and Constructing a High‐Temperature Molecular Ferroelectric by Anion and Cation Replacement in a Simple Crown Ether Clathrate19Room Temperature Lead-Free Multiaxial Inorganic–Organic Hybrid Ferroelectric44A Three‐Dimensional M3AB‐Type Hybrid Organic–Inorganic Antiperovskite Ferroelectric: [C3H7FN]3[SnCl6]Cl352D Hybrid Perovskite Ferroelectric Enables Highly Sensitive X‐Ray Detection with Low Driving Voltage199Plasmonic nanoprism enhanced quasi-2D Ruddlesden–Popper layered perovskite photodetectors26Dimensional Reduction of Cs2AgBiBr6: A 2D Hybrid Double Perovskite with Strong Polarization Sensitivity102Dimensional Reduction of Cs2AgBiBr6: A 2D Hybrid Double Perovskite with Strong Polarization Sensitivity21Ferroelectricity in Ethylammonium Bismuth-Based Organic–Inorganic Hybrid: (C2H5NH3)2[BiBr5]57Recent advances in solution-processed photodetectors based on inorganic and hybrid photo-active materials105Exploiting the Bulk Photovoltaic Effect in a 2D Trilayered Hybrid Ferroelectric for Highly Sensitive Polarized Light Detection180Exploiting the Bulk Photovoltaic Effect in a 2D Trilayered Hybrid Ferroelectric for Highly Sensitive Polarized Light Detection21A chiral lead-free photoactive hybrid material with a narrow bandgap20A two-dimensional bilayered Dion–Jacobson-type perovskite hybrid with a narrow bandgap for broadband photodetection30Bistable molecular materials with dynamic structures117Detection range extended 2D Ruddlesden–Popper perovskite photodetectors27Dielectric phase transition of an A 2 BX 4 -type perovskite with a pentahedral to octahedral transformation26Exploiting two-dimensional hybrid perovskites incorporating secondary amines for high-performance array photodetection17Ferroelectricity of trimethylammonium bromide below room temperature12Mn-doped 2D Sn-based perovskites with energy transfer from self-trapped excitons to dopants for warm white light-emitting diodes30Photo-induced PM 2.5 adsorption in molecular ferroelectric heterostructures6Properties and mechanism of strain and piezoelectricity of hybrid molecular ferroelectrics1Two-dimensional organic–inorganic hybrid Ruddlesden–Popper perovskite materials: preparation, enhanced stability, and applications in photodetection61A Potential Sn-Based Hybrid Perovskite Ferroelectric Semiconductor106Recent progress in molecular ferroelectrics with perovskite structure16Multilayered 2D Cesium‐Based Hybrid Perovskite with Strong Polarization Sensitivity: Dimensional Reduction of CsPbBr3252D organic‐inorganic hybrid perovskite materials for nonlinear optics131Low‐dimensional metal halide perovskites and related optoelectronic applications121Interlayer‐Sensitized Linear and Nonlinear Photoluminescence of Quasi‐2D Hybrid Perovskites Using Aggregation‐Induced Enhanced Emission Active Organic Cation Layers29Halide Double Perovskite Ferroelectrics104Halide Double Perovskite Ferroelectrics31From bulk to molecularly thin hybrid perovskites264Organic Cation Alloying on Intralayer A and Interlayer A’ sites in 2D Hybrid Dion–Jacobson Lead Bromide Perovskites (A’)(A)Pb 2 Br 787Room‐Temperature Ferroelectric Material Composed of a Two‐Dimensional Metal Halide Double Perovskite for X‐ray Detection186Room‐Temperature Ferroelectric Material Composed of a Two‐Dimensional Metal Halide Double Perovskite for X‐ray Detection37Local nearly non-strained perovskite lattice approaching a broad environmental stability window of efficient solar cells29Spontaneous Formation of 2D/3D Heterostructures on the Edges of 2D Ruddlesden–Popper Hybrid Perovskite Crystals73Ultrasensitive polarized-light photodetectors based on 2D hybrid perovskite ferroelectric crystals with a low detection limit91Dynamics of Chiral Cations in Two-Dimensional CuX4 and PbX4 Perovskites (X = Cl and Br)24In Situ Photosynthesis of an MAPbI3/CoP Hybrid Heterojunction for Efficient Photocatalytic Hydrogen Evolution149Ferroelectricity‐Driven Self‐Powered Ultraviolet Photodetection with Strong Polarization Sensitivity in a Two‐Dimensional Halide Hybrid Perovskite45Ferroelectricity‐Driven Self‐Powered Ultraviolet Photodetection with Strong Polarization Sensitivity in a Two‐Dimensional Halide Hybrid Perovskite164Giant and Broadband Multiphoton Absorption Nonlinearities of a 2D Organometallic Perovskite Ferroelectric74Two-dimensional hybrid organic–inorganic perovskites as emergent ferroelectric materials483D‐to‐2D Dimensional Reduction for Exploiting a Multilayered Perovskite Ferroelectric toward Polarized‐Light Detection in the Solar‐Blind Ultraviolet Region823D‐to‐2D Dimensional Reduction for Exploiting a Multilayered Perovskite Ferroelectric toward Polarized‐Light Detection in the Solar‐Blind Ultraviolet Region17A Three-Dimensional Molecular Perovskite Ferroelastic with Two-Step Switching of Quadratic Nonlinear Optical Properties Tuned by Molecular Chiral Design35A multiaxial lead-free two-dimensional organic-inorganic perovskite ferroelectric110New insights into the structure of two-dimensional lead iodide-based perovskites18A Multiaxial Layered Halide Double Perovskite Ferroelectric with Multiple Ferroic Orders69Solid-State NMR and NQR Spectroscopy of Lead-Halide Perovskite Materials1402D Perovskite Single Crystals with Suppressed Ion Migration for High‐Performance Planar‐Type Photodetectors103Surface structures and equilibrium shapes of layered 2D Ruddlesden-Popper perovskite crystals from density functional theory calculations9Self-Powered Photodetector Using Two-Dimensional Ferroelectric Dion–Jacobson Hybrid Perovskites161Acquiring High‐ T C Layered Metal Halide Ferroelectrics via Cage‐Confined Ethylamine Rotators76Acquiring High‐TC Layered Metal Halide Ferroelectrics via Cage‐Confined Ethylamine Rotators10Perovskite‐Related 2D Compounds in the System 5‐Amino Valerian Acid Cation/MA/Pb/X (X = Cl, Br) – Synthesis, Crystal Structures, and Optical Properties16Semiconductor physics of organic–inorganic 2D halide perovskites520Soft Ferroelectrics Enabling High‐Performance Intelligent Photo Electronics81Low‐Dimensional Metal Halide Perovskite Photodetectors574Cage-incorporation of secondary amine in Ruddlesden–Popper 2D hybrid perovskite with strong photoconductivity and polarization response19PFM (piezoresponse force microscopy)-aided design for molecular ferroelectrics143Research progress on two-dimensional (2D) halide organic–inorganic hybrid perovskites28Role of the spacer cation in the growth and crystal orientation of two-dimensional perovskites18Wafer-sized 2D perovskite single crystal thin films for UV photodetectors51Centimeter‐Sized Single Crystals of Two‐Dimensional Hybrid Iodide Double Perovskite (4,4‐Difluoropiperidinium) 4 AgBiI 8 for High‐Temperature Ferroelectricity and Efficient X‐Ray Detection203The 2D Halide Perovskite Rulebook: How the Spacer Influences Everything from the Structure to Optoelectronic Device Efficiency1085Spacer Cation Alloying of a Homoconformational Carboxylate trans Isomer to Boost in-Plane Ferroelectricity in a 2D Hybrid Perovskite156Oriented Perovskite Growth Regulation Enables Sensitive Broadband Detection and Imaging of Polarized Photons Covering 300–1050 nm78Reducing defect of inorganic perovskite film by sulphur-containing Lewis base for robust photodetectors33van der Waals Interaction-Induced Tunable Schottky Barriers in Metal–2D Perovskite Contacts26Harvesting High-Quality White-Light Emitting and Remarkable Emission Enhancement in One-Dimensional Halide Perovskites Upon Compression23Cooperative Nature of Ferroelectricity in Two-Dimensional Hybrid Organic–Inorganic Perovskites39Relationship Between Structure and Ferroelectric Properties1Relationship Between Structure and Ferroelectric Properties0The Relationship Between Structure and Electric Property0The Relationship Between Structure and Electric Property1The Relationship Between Structure and Electric Property0Progress and perspective in Dion-Jacobson phase 2D layered perovskite optoelectronic applications130Recent Progress on Electrical and Optical Manipulations of Perovskite Photodetectors315Ultra-Broad-Band-Excitable Cu(I)-Based Organometallic Halide with Near-Unity Emission for Light-Emitting Diode Applications169Ferroic Halide Perovskite Optoelectronics45Recent Advances in Synthesis, Properties, and Applications of Metal Halide Perovskite Nanocrystals/Polymer Nanocomposites214

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  39. Tetradic phosphor white light with variable CCT and superlative CRI through organolead halide perovskite nanocrystals

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  41. Tunable optical absorption in lead-free perovskite-like hybrids by iodide management

    Chemical Communications · 2019-01-01

    Bo Kou, Weichuan Zhang, Chengmin Ji, Zhenyue Wu, Shu‐Hua Zhang, Xitao Liu, Junhua Luo

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  42. Two-dimensional (PEA) 2 PbBr 4 perovskite single crystals for a high performance UV-detector

    Journal of Materials Chemistry C · 2019-01-01

    Yunxia Zhang, Yucheng Liu, Zhuo Xu, Haochen Ye, Qingxian Li, Mingxin Hu, Zhou Yang, Shengzhong Frank Liu

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  43. Quantum and Dielectric Confinement Effects in Lower-Dimensional Hybrid Perovskite Semiconductors

    Chemical Reviews · 2019-01-14

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  44. Two-Dimensional Hybrid Perovskite-Type Ferroelectric for Highly Polarization-Sensitive Shortwave Photodetection

    Journal of the American Chemical Society · 2019-01-20

    Lina Li, Xitao Liu, Yaobin Li, Zhiyun Xu, Zhenyue Wu, Shiguo Han, Kewen Tao, Maochun Hong, Junhua Luo, Zhihua Sun

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  45. Tuning the Luminescence of Layered Halide Perovskites

    Chemical Reviews · 2019-01-28

    Matthew D. Smith, Bridget A. Connor, Hemamala I. Karunadasa

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  46. Two‐Step Structure Phase Transition, Dielectric Anomalies, and Thermochromic Luminescence Behavior in a Direct Band Gap 2D Corrugated Layer Lead Chloride Hybrid of [(CH3)4 N ]4Pb3Cl10

    Chemistry - A European Journal · 2019-02-13

    Chen Xue, Shu Wang, Wen‐Long Liu, Xiao‐Ming Ren

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  47. Unraveling the mechanochemical synthesis and luminescence in MnII-based two-dimensional hybrid perovskite (C4H9NH3)2PbCl4

    Science China Materials · 2019-03-04

    Guojun Zhou, Shaoqiang Guo, Jing Wei Zhao, Мaxim S. Моlokeev, Quanlin Liu, Junying Zhang, Zhiguo Xia

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  48. Hybrid organic-inorganic perovskites: Polar properties and applications

    Coordination Chemistry Reviews · 2019-03-05

    Wei‐Jian Xu, Svitlana Kopyl, Andréi L. Kholkin, João Rocha

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  49. (C6H13NH3)2(NH2CHNH2)Pb2I7: A Two‐dimensional Bilayer Inorganic–Organic Hybrid Perovskite Showing Photodetecting Behavior

    Chemistry - An Asian Journal · 2019-03-06

    Yuyin Wang, Xitao Liu, Lina Li, Chengmin Ji, Zhihua Sun, Shiguo Han, Kewen Tao, Junhua Luo

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  50. Tunable Ferroelectricity in Ruddlesden–Popper Halide Perovskites

    ACS Applied Materials & Interfaces · 2019-03-11

    Qiannan Zhang, Ankur Solanki, Kaushik Parida, David Giovanni, Mingjie Li, Thomas L. C. Jansen, Maxim S. Pshenichnikov, Tze Chien Sum

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