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RESEARCH PAPER · ChemPhotoChem · 2017

Enhancing Charge Separation in Photocatalysts with Internal Polar Electric Fields

Zaizhu Lou, Peng Wang, Baibiao Huang, Ying Dai, Xiaoyan Qin, Xiaoyang Zhang, Zeyan Wang, Yuanyuan Liu

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Enhancing Charge Separation in Photocatalysts with Internal Polar Electric FieldsOriginalEnhancement of charge separation in ferroelectric heterogeneous photocatalyst Bi 4 (SiO 4 ) 3 /Bi 2 SiO 5 nanostructures30Charge transfer from internal electrostatic fields is superior to surface defects for 2,4-dichlorophenol degradation in K 3−x Na x B 6 O 10 Br photocatalysts16Enhanced visible-light-driven photocatalytic activities of Bi2Fe4O9/g-C3N4 composite photocatalysts41Realizing selective water splitting hydrogen/oxygen evolution on ferroelectric Bi3TiNbO9 nanosheets105The effect of pH on the photochemical reactivity of BaTiO313In Situ Raman Probing of Chlorphenol Degradation on Different Facets of K3B6O10Br Single Crystal8Charge Separation in a Multifunctionalized Framework of Hydrogen‐Bonded Periodic Mesoporous Organosilica5S, N Codoped Graphene Quantum Dots Embedded in (BiO)2CO3: Incorporating Enzymatic-like Catalysis in Photocatalysis64Facet, Junction and Electric Field Engineering of Bismuth‐Based Materials for Photocatalysis111Surface Strategies for Particulate Photocatalysts toward Artificial Photosynthesis208Influence of the Magnitude of Ferroelectric Domain Polarization on the Photochemical Reactivity of BaTiO 320A Full‐Spectrum Metal‐Free Porphyrin Supramolecular Photocatalyst for Dual Functions of Highly Efficient Hydrogen and Oxygen Evolution355Enhanced photocatalytic hydrogen evolution of CdWO4 through polar organic molecule modification19The Role of Polarization in Photocatalysis930The Role of Polarization in Photocatalysis60Calcination synthesis of N-doped BiOIO3 with high LED-light-driven photocatalytic activity30Enhancing oxygen evolution efficiency of multiferroic oxides by spintronic and ferroelectric polarization regulation117Spontaneous Polarization Effect and Photocatalytic Activity of Layered Compound of BiOIO373Exclusive enhancement of catalytic activity in Bi 0.5 Na 0.5 TiO 3 nanostructures: new insights into the design of efficient piezocatalysts and piezo-photocatalysts159Silver-based visible light–responsive photocatalysts10Superior adsorption capability and excellent photocatalytic activity derived from the ferroelectric external screening effect in Bi 3 TiNbO 9 single-crystal nanosheets20Improved Photoelectric Performance of UV Photodetector Based on ZnO Nanoparticle‐Decorated BiOCl Nanosheet Arrays onto PDMS Substrate: The Heterojunction and Ti3C2Tx MXene Conduction Layer122The mechanism of photodriven oxidation of CO over anatase and rutile TiO2 investigated from the hydrogen adsorption behavior37Piezocatalysis and Piezo‐Photocatalysis: Catalysts Classification and Modification Strategy, Reaction Mechanism, and Practical Application986Construction of an all-organic Z-scheme heterostructure based on 2D PDINH aggregates modified TCPP aggregates by co-assembly with enhanced photocatalytic performance24Photocatalysis Within Intrinsic Spontaneous Polarization Electric Field47Boosting charge spatial separation efficiency for catalytic H2 bubble evolution under macroscopic spontaneous polarization electric field7Photocatalytic activity of co-doped Janus monolayer MoSSe for solar water splitting: A computational investigation64High carrier separation efficiency for a defective g-C 3 N 4 with polarization effect and defect engineering: mechanism, properties and prospects41Regulating Electron-Hole Separation to Promote the Photocatalytic Property of BiOBr1−xIx/BiOBr Local Distorted Hierarchical Microspheres0Atomic‐Level Charge Separation Strategies in Semiconductor‐Based Photocatalysts505Designed Construction of SrTiO3/SrSO4/Pt Heterojunctions with Boosted Photocatalytic H2 Evolution Activity21Rationalize the Significantly Enhanced Photocatalytic Efficiency of In3+-doped α′-Ga2S3 by Bond Theory and Local Structural Distortion18Optically Induced Coherent Phonons in Bismuth Oxyiodide (BiOI) Nanoplatelets33Durable Metal Heteroanionic Photocatalysts24BaTi4O9 Photocatalysts with Variously Loaded Ag Cocatalyst for Highly Selective Photocatalytic CO2 Reduction with Water11Organic-inorganic complex nanoflake photocatalyst PDINH/Bi2WO6 with increased visible light catalytic performance6The asymmetrical-structure of supramolecular precursor to improve internal electric field for simultaneously enhancing contaminant degradation and H2O2 production performance32Enhancing an internal electric field by a solid solution strategy for steering bulk-charge flow and boosting photocatalytic activity of Bi24O31Cl Br10–34Regulating the Built-In Electric Field of BiOBr by a Piezoelectric Mineral Tourmaline and the Enhanced Photocatalytic Property31Electric Field Effects on Photoelectrochemical Water Splitting: Perspectives and Outlook4Photoinduced Surface Electric Fields and Surface Population Dynamics of GaP(100) Photoelectrodes8Enhanced piezo-photocatalytic performance of Ag@Na0.5Bi0.5TiO3 composites17Layered bismuth-based photocatalysts300Effects of coexistence of Mo and Zn vacancies with different valence states and interstitial H on the magneto-optical properties of ZnO: First-principles calculations2A perylenediimide modified SiO2@TiO2 yolk-shell light-responsive nanozyme: Improved peroxidase-like activity for H2O2 and sarcosine sensing59Improving charge separation efficiency and piezo-photodegradation properties in Na0.5Bi0.5TiO3 via lattice engineering14Spatial Separation of Electrons and Holes among ZnO Polar {0001} and {1010} Facets for Enhanced Photocatalytic Performance38Enhanced photocatalytic activity of MoS2 via N + F codoping and strain engineering: A first-principles investigation30Bi3O4Cl/Bi4NbO8Cl Z-scheme heterojunction catalysts for enhanced photocatalytic degradation of organic pollutants6Photocatalytic and Photocurrent Responses to Visible Light of the Lone-Pair-Based Oxysulfide Sr6Cd2Sb6S10O728Polar semiconductor photocatalysts with intrinsic electric fields for selective organic transformation8Silver niobate-based photocatalysts: Relevance in dye degradation13Building internal electric fields in porous ionic polymers for fast photocatalytic degradation of tetracycline hydrochloride6Facile synthesis of hierarchical CdS nanoflowers for efficient piezocatalytic hydrogen evolution22Influence of external electric field on electronic structure and optical properties of β-Ga 2 O 3 : a DFT study12Photocatalytic Water Splitting and Co2 Reduction with Internal Electric Field Modulation1Synergistic effect of exposed facets and surface defects of ZnO nanomaterials for photocatalytic ozonation of organic pollutants20A Review on Heteroanionic-Based Materials for Photocatalysis Applications37Molten Salts‐Driven Discovery of a Polar Mixed‐Anion 3D Framework at the Nanoscale: Zn4Si2O7Cl2, Charge Transport and Photoelectrocatalytic Water Splitting1Molten Salts‐Driven Discovery of a Polar Mixed‐Anion 3D Framework at the Nanoscale: Zn4Si2O7Cl2, Charge Transport and Photoelectrocatalytic Water Splitting0Proton transport controlled at surface layer of CeO2 by gradient-doping with a built-in-field effect1Photocatalytic reduction of uranium (VI) by 2D-perylene diimide with surface cross-linked polyethyleneimine21Progress in wastewater treatment via organic supramolecular photocatalysts under sunlight irradiation20Towards the design of oxychalcogenide materials as candidates for solar water- splitting photocatalysis0Low Carrier Effective Masses in Photoactive Sr2Sb2O2Q3 (Q = S, Se): The Role of the Lone Pair17Activating black phosphorene's inert basal plane via nonprecious metal–nonmetal co-doping for visible-light-driven photocatalytic H 2 evolution3Effective solar light-driven isothiazolinone degradation by morphology- and oxygen vacancy-modified Gd-doped BiOCl5Multiple Enhancement Effects of Dipoles within Polyimide Cathode Promoting Highly Efficient Energy Storage of Lithium-Ion Battery0Prospects for the application of nanostructures of bismuth oxychloride (BiOCl) towards the degradation of organic compounds in an aqueous solution3Recent Progress in Charge Separation of Photocatalysts Facilitated by Polarization1Strong thickness dependence in thin film photocatalytic heterojunctions: the ZnO–Bi 2 O 3 case study9Iron Oxychalcogenides and Their Photocurrent Responses16Photocatalytic H2O splitting and CO2 reduction with internal electric field modulation23Surface states of photoelectrodes by surface-specific steady-state and time-resolved sum frequency spectroscopies2Molecular modification: A promising strategy for the design of donor-acceptor-type organic polymers photocatalyst56BiOBr/Bi 2 O 2 CO 3 Heterojunction Photocatalyst for the Degradation of Tetracycline38Partial MOF-derived BiFeO3 from Fe/Bi-BDC framework for efficient piezo-photocatalytic reduction of Cr(VI) and N2 fixation under visible light17Significantly enhanced catalytic performance of solid-state-synthesized Na0.5Bi0.5TiO3 nanoparticles by piezo-phototronic coupling effect8Boosting BaTi4O9 photocatalytic H2 evolution activity by functionalized CuNi alloy5Co-doped bismuth vanadate/zinc tungstate heterojunction with dual internal electric fields for efficient photocatalytic reduction of carbon dioxide31Impact of {100} polar surfaces of α-Bi2O3 on photocatalytic dye degradation and hydrogen production7Modeling heterojunctions: a computational chemistry perspective9Impact of Molecular Structure on Reactive Oxygen Species Generation in D–A Heterojunction Photocatalysts for Efficient Dye Degradation under Weak Light34Inorganic–Organic Bi 4 Nb 1– x Ta x O 8 Cl/rGO/SA-PTA Z-Scheme Heterojunction with a Third-Order Polarized Electric Field and a Fast Electron Transfer Channel for Photocatalytic Overall Water Splitting37Application of Molecular Ferroelectric in Photocatalytic Selective Oxidization of C(sp 3 )─H Bonds9Application of Molecular Ferroelectric in Photocatalytic Selective Oxidization of C(sp 3 )─H Bonds0Optical fiber triethylamine room temperature gas sensor based on HMS platform with DFT calculation and Experimental Demonstration11From micro to subnano scale: Insights into the dielectric properties of BiOI nanoplates1Spontaneous Electric Field Directionality in One-Dimensional Semiconductors: Key to Efficient Charge Migration, Minimizing Recombination, and Enhancing Photocatalytic Performance8Defect‐driven innovations in photocatalysts: Pathways to enhanced photocatalytic applications127Multifunctional PVDF based composite for sustainable catalysis: Insights into piezo-photocatalytic environmental and energy application24Bismuth-Based Oxyfluorides as Emergent Photocatalysts: A Review4Design of LaFeO₃/CuBi₂O₄ composite for enhanced visible-light photocatalytic degradation of atrazine: Insights into activity, stability, and mechanism7Advances in the study of unconventional BixMoyOz photocatalysts for energy and environmental applications0Modulating Surface Band Bending and Redox Site Spacing in Metal–Organic Frameworks for Boosting Methanol Photosynthesis from CO 2 and H 2 O17Synergistic One-Dimensional Conductive Pathways and Local Polarization Fields for Intrinsic Bulk Charge Separation in Nonpolar Oxide Photocatalysts0Recent advances in transition metal oxide-based photocatalysis for the treatment of agricultural wastewater: A review1Multi-field-enhanced photocatalysis and electrocatalysis for energy and environment application1P–N Junction-Based Photocatalysts: Synthesis, Mechanism, and Their Applications0

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  1. Enhancement of charge separation in ferroelectric heterogeneous photocatalyst Bi 4 (SiO 4 ) 3 /Bi 2 SiO 5 nanostructures

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  2. Charge transfer from internal electrostatic fields is superior to surface defects for 2,4-dichlorophenol degradation in K 3−x Na x B 6 O 10 Br photocatalysts

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  3. Enhanced visible-light-driven photocatalytic activities of Bi2Fe4O9/g-C3N4 composite photocatalysts

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  4. Realizing selective water splitting hydrogen/oxygen evolution on ferroelectric Bi3TiNbO9 nanosheets

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  6. In Situ Raman Probing of Chlorphenol Degradation on Different Facets of K3B6O10Br Single Crystal

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  12. A Full‐Spectrum Metal‐Free Porphyrin Supramolecular Photocatalyst for Dual Functions of Highly Efficient Hydrogen and Oxygen Evolution

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  13. Enhanced photocatalytic hydrogen evolution of CdWO4 through polar organic molecule modification

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  14. The Role of Polarization in Photocatalysis

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  17. Enhancing oxygen evolution efficiency of multiferroic oxides by spintronic and ferroelectric polarization regulation

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  18. Spontaneous Polarization Effect and Photocatalytic Activity of Layered Compound of BiOIO3

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