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RESEARCH PAPER · RSC Advances · 2016

Concentration dependent electrochemical properties and structural analysis of a simple magnesium electrolyte: magnesium bis(trifluoromethane sulfonyl)imide in diglyme

Niya Sa, Nav Nidhi Rajput, Hao Wang, Baris Key, Magali S. Ferrandon, Venkat N. Srinivasan, Kristin Aslaug Persson, Anthony K. Burrell, John T. Vaughey

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Concentration dependent electrochemical properties and structural analysis of a simple magnesium electrolyte: magnesium bis(trifluoromethane sulfonyl)imide in diglymeOriginalOdyssey of Multivalent Cathode Materials: Open Questions and Future Challenges1158Reversible S 0 /MgS x Redox Chemistry in a MgTFSI 2 /MgCl 2 /DME Electrolyte for Rechargeable Mg/S Batteries196Reversible S0/MgSx Redox Chemistry in a MgTFSI2/MgCl2/DME Electrolyte for Rechargeable Mg/S Batteries71Reducing Mg Anode Overpotential via Ion Conductive Surface Layer Formation by Iodine Additive153Elucidating Solvation Structures for Rational Design of Multivalent Electrolytes—A Review35Exploring the Liquid Structure and Ion Formation in Magnesium Borohydride Electrolyte Using Density Functional Theory1425Mg NMR and computational modeling studies of the solvation structures and molecular dynamics in magnesium based liquid electrolytes48Elucidating Zn and Mg Electrodeposition Mechanisms in Nonaqueous Electrolytes for Next-Generation Metal Batteries50Elucidating Solvation Structures for Rational Design of Multivalent Electrolytes—A Review94Rechargeable Magnesium Batteries using Conversion‐Type Cathodes: A Perspective and Minireview178Structural Study on Magnesium Ion Solvation in Diglyme-Based Electrolytes: IR Spectroscopy and DFT Calculations42The Joint Center for Energy Storage Research: A New Paradigm of Research, Development, and Demonstration1Перспективні матеріали та процеси в прикладній електрохімії - 20180Directing Mg-Storage Chemistry in Organic Polymers toward High-Energy Mg Batteries200Mg Cathode Materials and Electrolytes for Rechargeable Mg Batteries: A Review146Computational screening of electrolyte materials: status quo and open problems33Understanding Ca Electrodeposition and Speciation Processes in Nonaqueous Electrolytes for Next-Generation Ca-Ion Batteries100Structural and electrochemical studies of undoped and In3+-doped co-binary Cu2-xTe and Bi2Te3 thin films for aqueous Na–S batteries13“Ion Solvation Spectra”: Free Energy Analysis of Solvation Structures of Multivalent Cations in Aprotic Solvents32Modeling interfacial electrochemistry: concepts and tools50A Simple Halogen-Free Magnesium Electrolyte for Reversible Magnesium Deposition through Cosolvent Assistance69Electrolyte Reactivity in the Double Layer in Mg Batteries: An Interface Potential-Dependent DFT Study112Ion Pairing and Redissociaton in Low-Permittivity Electrolytes for Multivalent Battery Applications39Beyond Typical Electrolytes for Energy Dense Batteries33Modeling of Ion Agglomeration in Magnesium Electrolytes and its Impacts on Battery Performance25Kinetic- versus Diffusion-Driven Three-Dimensional Growth in Magnesium Metal Battery Anodes166Current-Density-Dependent Electroplating in Ca Electrolytes: From Globules to Dendrites84Ion Solvation Engineering: How to Manipulate the Multiplicity of the Coordination Environment of Multivalent Ions30Novel design concepts of efficient electrolytes and new organic materials for Magnesium batteries0Influence of Complexing Additives on the Reversible Deposition/Dissolution of Magnesium in an Ionic Liquid16The metamorphosis of rechargeable magnesium batteries271In Situ Probing of Mass Exchange at the Solid Electrolyte Interphase in Aqueous and Nonaqueous Zn Electrolytes with EQCM-D30Structure and Transport of Solvent Ligated Octahedral Mg-Ion in an Aqueous Battery Electrolyte7Poly(benzoquinonyldisulfide) as organic positve electrode for Mg and Li batteries10Advancing Electrolyte Solution Chemistry and Interfacial Electrochemistry of Divalent Metal Batteries32Critical Role of the Interphase at Magnesium Electrodes in Chloride-Free, Simple Salt Electrolytes203-V class Mg-based dual-ion battery with astonishingly high energy/power densities in common electrolytes19Modeling of Electron‐Transfer Kinetics in Magnesium Electrolytes: Influence of the Solvent on the Battery Performance41Solvation sheath reorganization enables divalent metal batteries with fast interfacial charge transfer kinetics604Modeling of Electron-Transfer Kinetics in Magnesium Electrolytes: Influence of the Solvent on the Battery Performance0The Effect of the Coordination Ability on the Mg Plating/Stripping Behavior in Mg(N(CF3SO2)2)2/Glyme Based Electrolytes2Interfaces and Interphases in Ca and Mg Batteries63Exploring hybrid Mg2+/H+ reactions of C@MgMnSiO4 with boosted voltage in magnesium-ion batteries23Investigating the abnormal conductivity behaviour of divalent cations in low dielectric constant tetraglyme-based electrolytes19Thermal stability and structural studies on the mixtures of Mg(BH 4 ) 2 and glymes3Effect of EtOMgCl Salt to Suppress Reductive Decomposition of TFSI− Anion in Electrolyte for Magnesium Rechargeable Battery7Electrolyte and Interphase Design for Magnesium Anode: Major Challenges and Perspectives79Electrochemical swelling induced high material utilization of porous polymers in magnesium electrolytes32Applying Classical, Ab Initio , and Machine-Learning Molecular Dynamics Simulations to the Liquid Electrolyte for Rechargeable Batteries561Efficacy of Stabilizing Calcium Battery Electrolytes through Salt-Directed Coordination Change22A Novel and Highly Efficient Indolyl‐Based Electrolyte for Mg Batteries7TFSI Anion Grafted Polymer as an Ion-Conducting Protective Layer on Magnesium Metal for Rechargeable Magnesium Batteries53Fast Magnesium Conducting Electrospun Solid Polymer Electrolyte16Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium95Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium3Gradient Perovskite Ionic–Electronic Heterointerphases for Deep Cycling Mg Metal Anodes17Chloride‐Free Electrolytes for High‐Voltage Magnesium Metal Batteries: Challenges, Strategies, and Perspectives21Deeping insight of Mg(CF3SO3)2 and comprehensive modified electrolyte with ionic liquid enabling high-performance magnesium batteries74Reversible Magnesium Metal Cycling in Additive-Free Simple Salt Electrolytes Enabled by Spontaneous Chemical Activation25Magnesiated Nafion-Based Gel Electrolytes: Structural and Electrochemical Characterization4Research development on electrolytes for magnesium-ion batteries157Research advances of the electrolytes for rechargeable magnesium ion batteries26Strong solvent coordination effect inducing gradient solid-electrolyte-interphase formation for highly efficient Mg plating/stripping102The Effect of Chlorides on the Performance of DME/Mg[B(HFIP)4]2 Solutions for Rechargeable Mg Batteries14Revealing the Structural Evolution of Electrode/Electrolyte Interphase Formation during Magnesium Plating and Stripping with operando EQCM‐D8Synergy between the coordination and trace ionization of co-solvents enables reversible magnesium electroplating/stripping behavior83Generalizable, tunable control of divalent cation solvation structure via mixed anion contact ion pair formation13Recent developments and future prospects of magnesium–sulfur batteries11Structure and chemical composition of the Mg electrode during cycling in a simple glyme electrolyte5Phase-field simulation of magnesium-metal anode interface growth in different electrolytes during electrodeposition2On the kinetics of electrodeposition in a magnesium metal anode24Advances in ionic-liquid-based eutectic electrolyte for high voltage rechargeable magnesium batteries4Review on dendrite formation of Mg metal anode and its prevention18Divalent Metal-Ion Batteries as Alternatives to Li-Ion Based Energy Storage0A solvation-driven reevaluation of organic electrolytes for zinc batteries19From Ab Initio to Instrumentation: A Field Guide to Characterizing Multivalent Liquid Electrolytes29Deciphering the interfacial electrochemistry of non-nucleophilic Mg(TFSI)2 as 4 V-class electrolyte for Mg batteries9Diethylene Glycol Diethyl Ether as Electrolyte Solvent for Reversible Electrochemical Magnesium Plating2Benchmarking Mg Electrolytes with Different Metal Plating/Stripping Protocols1A Dive into the Electrodeposition Kinetics and Mechanisms in Nonaqueous Magnesium Electrolytes2Reassessing Electrolyte Design for Non‐Aqueous Magnesium Batteries: Atomistic Structures and Performance Optimization14Hybrid ML–EIS framework for ionic conductivity prediction in solid-state battery electrolytes0Vanadium-Based Materials in Metal–Ion Hybrid Batteries─Beyond Conventional Lithium-Ion Storage: A Review and Perspectives2Synergistic effects of composite organic additives on the magnesium–ion battery performance0Deciphering the Halide Chemistry of Cl – and Br – in Enhancing Kinetics of Mg Plating/Stripping0A dual-function additive strategy for stabilizing magnesium metal interfaces0Countersolvent Relaxes Strong Mg−O Coulomb Force for Improved Rechargeable Magnesium Batteries0Progress in the molecular design of magnesium salts for high-performance rechargeable magnesium batteries0Electrochemical corrosion behavior of magnesium anodes0

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  2. Reversible S 0 /MgS x Redox Chemistry in a MgTFSI 2 /MgCl 2 /DME Electrolyte for Rechargeable Mg/S Batteries

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  3. Reversible S0/MgSx Redox Chemistry in a MgTFSI2/MgCl2/DME Electrolyte for Rechargeable Mg/S Batteries

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  4. Reducing Mg Anode Overpotential via Ion Conductive Surface Layer Formation by Iodine Additive

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  5. Elucidating Solvation Structures for Rational Design of Multivalent Electrolytes—A Review

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  6. Exploring the Liquid Structure and Ion Formation in Magnesium Borohydride Electrolyte Using Density Functional Theory

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  8. Elucidating Zn and Mg Electrodeposition Mechanisms in Nonaqueous Electrolytes for Next-Generation Metal Batteries

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  10. Rechargeable Magnesium Batteries using Conversion‐Type Cathodes: A Perspective and Minireview

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  11. Structural Study on Magnesium Ion Solvation in Diglyme-Based Electrolytes: IR Spectroscopy and DFT Calculations

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  17. Understanding Ca Electrodeposition and Speciation Processes in Nonaqueous Electrolytes for Next-Generation Ca-Ion Batteries

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  18. Structural and electrochemical studies of undoped and In3+-doped co-binary Cu2-xTe and Bi2Te3 thin films for aqueous Na–S batteries

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