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RESEARCH PAPER · Nano Letters · 2015

Promotion of Oxygen Reduction by Exsolved Silver Nanoparticles on a Perovskite Scaffold for Low-Temperature Solid Oxide Fuel Cells

Yinlong Zhu, Wei Zhou, Ran Ran, Yubo Chen, Zongping Shao, Meilin Liu

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Promotion of Oxygen Reduction by Exsolved Silver Nanoparticles on a Perovskite Scaffold for Low-Temperature Solid Oxide Fuel CellsOriginalCO 2 -to-CO conversion on layered perovskite with in situ exsolved Co–Fe alloy nanoparticles: an active and stable cathode for solid oxide electrolysis cells148Smart utilization of cobaltite-based double perovskite cathodes on barrier-layer-free zirconia electrolyte of solid oxide fuel cells57Tuning layer-structured La 0.6 Sr 1.4 MnO 4+δ into a promising electrode for intermediate-temperature symmetrical solid oxide fuel cells through surface modification77Evaluation of the CO2 Poisoning Effect on a Highly Active Cathode SrSc0.175Nb0.025Co0.8O3-δ in the Oxygen Reduction Reaction137The Excellence of Both Worlds: Developing Effective Double Perovskite Oxide Catalyst of Oxygen Reduction Reaction for Room and Elevated Temperature Applications136Perovskite materials in energy storage and conversion122Recent development on perovskite‐type cathode materials based on SrCoO3 − δ parent oxide for intermediate‐temperature solid oxide fuel cells38Evaluation of A-site deficient Sr 1−x Sc 0.175 Nb 0.025 Co 0.8 O 3−δ (x=0, 0.02, 0.05 and 0.1) perovskite cathodes for intermediate-temperature solid oxide fuel cells32Phosphorus‐Doped Perovskite Oxide as Highly Efficient Water Oxidation Electrocatalyst in Alkaline Solution353An Aurivillius Oxide Based Cathode with Excellent CO2 Tolerance for Intermediate‐Temperature Solid Oxide Fuel Cells93An Aurivillius Oxide Based Cathode with Excellent CO2 Tolerance for Intermediate‐Temperature Solid Oxide Fuel Cells15New Opportunity for in Situ Exsolution of Metallic Nanoparticles on Perovskite Parent285Understanding the doping effect toward the design of CO2-tolerant perovskite membranes with enhanced oxygen permeability60Functionally graded doped lanthanum cobalt ferrite and ceria-based composite interlayers for advancing the performance stability in solid oxide fuel cell33Designing Fe-Based Oxygen Catalysts by Density Functional Theory Calculations70Nanomaterials for Advanced Electrode of Low Temperature Solid Oxide Fuel Cells (SOFCs)32La0.54Sr0.4Fe0.2Co0.8O3−δ@Co0.01Ce0.79Gd0.2O2−δ functional cathode material for solid oxide fuel cell application14Template-free and one-pot synthesis of N-doped hollow carbon tube @ hierarchically porous carbon supporting homogeneous AgNPs for robust oxygen reduction catalyst43An emerging platform for electrocatalysis: perovskite exsolution22Stability, compatibility and performance improvement of SrCo0.8Fe0.1Nb0.1O3− perovskite as a cathode for intermediate-temperature solid oxide fuel cells56Enhancing Electrode Performance by Exsolved Nanoparticles: A Superior Cobalt-Free Perovskite Electrocatalyst for Solid Oxide Fuel Cells119A novel fuel electrode enabling direct CO 2 electrolysis with excellent and stable cell performance180A review of high temperature co-electrolysis of H 2 O and CO 2 to produce sustainable fuels using solid oxide electrolysis cells (SOECs): advanced materials and technology782A single-/double-perovskite composite with an overwhelming single-perovskite phase for the oxygen reduction reaction at intermediate temperatures54Controlling cation segregation in perovskite-based electrodes for high electro-catalytic activity and durability376Developing metallic cathode for low-temperature solid oxide fuel cell applications0In situ growth of Pt 3 Ni nanoparticles on an A-site deficient perovskite with enhanced activity for the oxygen reduction reaction83La 1−x Ag x MnO 3 electrocatalyst with high catalytic activity for oxygen reduction reaction in aluminium air batteries52Nanocomposites for “nano green energy” applications1Validation and Electrochemical Characterization of LSCF Cathode Deposition on Metal Supported SOFC7Improved performance of a symmetrical solid oxide fuel cell by swapping the roles of doped ceria and La0.6Sr1.4MnO4+δ in the electrode37La0.7(Sr0.3-xPdx)MnO3 as a highly efficient electrocatalyst for oxygen reduction reaction in aluminum air battery45Perovskite/Carbon Composites: Applications in Oxygen Electrocatalysis393Promotion on electrochemical performance of a cation deficient SrCo 0.7 Nb 0.1 Fe 0.2 O 3−δ perovskite cathode for intermediate-temperature solid oxide fuel cells57A Highly Active Perovskite Cathode for Low‐Temperature Solid Oxide Fuel Cells: BaCo0.7Fe0.22Sc0.08O3–δ7High performance BaFe1−xBixO3−δ as cobalt-free cathodes for intermediate temperature solid oxide fuel cells60A rational design for enhanced oxygen reduction: Strongly coupled silver nanoparticles and engineered perovskite nanofibers71Recent Progress on Advanced Materials for Solid‐Oxide Fuel Cells Operating Below 500 °C390Enhancing Perovskite Electrocatalysis of Solid Oxide Cells Through Controlled Exsolution of Nanoparticles138Smart tuning of 3D ordered electrocatalysts for enhanced oxygen reduction reaction41Direct operation of Ag-based anode solid oxide fuel cells on propane56High‐Energy‐Density Metal–Oxygen Batteries: Lithium–Oxygen Batteries vs Sodium–Oxygen Batteries203Mass‐Production of Mesoporous MnCo 2 O 4 Spinels with Manganese(IV)‐ and Cobalt(II)‐Rich Surfaces for Superior Bifunctional Oxygen Electrocatalysis84Mass‐Production of Mesoporous MnCo2O4 Spinels with Manganese(IV)‐ and Cobalt(II)‐Rich Surfaces for Superior Bifunctional Oxygen Electrocatalysis256Demonstration of chemistry at a point through restructuring and catalytic activation at anchored nanoparticles166Direct Alcohol‐Fueled Low‐Temperature Solid Oxide Fuel Cells: A Review51Nanomaterials and technologies for low temperature solid oxide fuel cells: Recent advances, challenges and opportunities501Self-assembled alloy nanoparticles in a layered double perovskite as a fuel oxidation catalyst for solid oxide fuel cells104Silver-Perovskite Hybrid Electrocatalysts for Oxygen Reduction Reaction in Alkaline Media19Synergistically enhanced hydrogen evolution electrocatalysis by in situ exsolution of metallic nanoparticles on perovskites104Thermally driven in situ exsolution of Ni nanoparticles from (Ni, Gd)CeO 2 for high-performance solid oxide fuel cells50Transition metal oxide-based oxygen reduction reaction electrocatalysts for energy conversion systems with aqueous electrolytes236Material Discovery and Design Principles for Stable, High Activity Perovskite Cathodes for Solid Oxide Fuel Cells205Promotion of Oxygen Reduction with Both Amorphous and Crystalline MnOx through the Surface Engineering of La0.8Sr0.2MnO3‐δ Perovskite55Copper-based electrodes for IT-SOFC24Ferric ion pair mediated biomass redox flow fuel cell and related chemical reaction kinetics study32Fabrication of aligned porous LaNi0.6Fe0.4O3 perovskite by water based freeze casting19Enhancement of oxygen reduction reaction through coating a nano-web-structured La0.6Sr0.4Co0.2Fe0.8O3-δ thin-film as a cathode/electrolyte interfacial layer for lowering the operating temperature of solid oxide fuel cells29Recent Advances in Novel Nanostructuring Methods of Perovskite Electrocatalysts for Energy‐Related Applications407Silver-doped strontium niobium cobaltite as a new perovskite-type ceramic membrane for oxygen separation33Fabrication of integrated BZY electrolyte matrices for protonic ceramic membrane fuel cells by tape-casting and solid-state reactive sintering25Application of silver in microtubular solid oxide fuel cells35Energetics of Nanoparticle Exsolution from Perovskite Oxides96Nanoscale Architecture of RuO2/La0.9Fe0.92Ru0.08– x O3−δ Composite via Manipulating the Exsolution of Low Ru-Substituted A‑Site Deficient Perovskite58SDC-Infiltrated Microporous Silver Membrane with Superior Resistance to Thermal Agglomeration for Cathode-Supported Solid Oxide Fuel Cells7Enhanced electrochemical performance of Ca-doped NdBa1-xCaxCoCuO5+δ as cathode material for intermediate-temperature solid oxide fuel cells41Electrochemical Removal of NOx Using Oxide-Based Electrodes – A Review.7Improving the Electrocatalytic Activity and Durability of the La0.6Sr0.4Co0.2Fe0.8O3−δ Cathode by Surface Modification115In Situ Formation of Er0.4Bi1.6O3 Protective Layer at Cobaltite Cathode/Y2O3–ZrO2 Electrolyte Interface under Solid Oxide Fuel Cell Operation Conditions46Cation deficiency enabled fast oxygen reduction reaction for a novel SOFC cathode with promoted CO2 tolerance165A Nano-Architectured Metal-Oxide/Perovskite Hybrid Material as Electrocatalyst for the Oxygen Reduction Reaction in Aluminum–Air Batteries29Bimetallic nanoparticle decorated perovskite oxide for state-of-the-art trifunctional electrocatalysis106Enhancing the triiodide reduction activity of a perovskite-based electrocatalyst for dye-sensitized solar cells through exsolved silver nanoparticles44Fluid Mechanical Approaches for Rational Design of Infiltrated Electrodes of Solid Oxide Fuel Cells12Nickel-substituted Ba 0.5 Sr 0.5 Co 0.8 Fe 0.2 O 3−δ : a highly active perovskite oxygen electrode for reduced-temperature solid oxide fuel cells41Silver Modified Cathodes for Solid Oxide Fuel Cells23Unravelling inherent electrocatalysis of mixed-conducting oxide activated by metal nanoparticle for fuel cell electrodes129Heterostructured simple perovskite nanorod-decorated double perovskite cathode for solid oxide fuel cells: Highly catalytic activity, stability and CO2-durability for oxygen reduction reaction110The synergistic catalyst-carbonates effect on the direct bituminous coal fuel cell performance8Atomic Layer Deposition for Surface Engineering of Solid Oxide Fuel Cell Electrodes49Structural, morphological and optical properties and solar cell applications of thioglycolic routed nano cobalt oxide material46Nanoengineering of solid oxide electrochemical cell technologies: An outlook30Rational Design of a Metallic Functional Layer for High-Performance Solid Oxide Fuel Cells22Insight into the Electrochemical Processes of the Titanate Electrode with in Situ Ni Exsolution for Solid Oxide Cells28Enhanced overall water electrolysis on a bifunctional perovskite oxide through interfacial engineering56Enhancing NH3 sensing performance of mixed potential type sensors by chemical exsolution of Ag nanoparticle on AgNbO3 sensing electrode43BaCoxFe0.7-xZr0.3O3-δ(0.2≤x≤0.5) as cathode materials for proton-based SOFCs35Boosting the Activity of BaCo0.4Fe0.4Zr0.1Y0.1O3−δ Perovskite for Oxygen Reduction Reactions at Low‐to‐Intermediate Temperatures through Tuning B‐Site Cation Deficiency176Perovskite Structure Associated with Precious Metals: Influence on Heterogenous Catalytic Process36Ex-Solution Synthesis of Sub-5-nm FeOx Nanoparticles on Mesoporous Hollow N,O-Doped Carbon Nanoshells for Electrocatalytic Oxygen Reduction40In Situ Observation of Nanoparticle Exsolution from Perovskite Oxides: From Atomic Scale Mechanistic Insight to Nanostructure Tailoring276Exsolution of SrO during the Topochemical Conversion of LaSr3CoRuO8 to the Oxyhydride LaSr3CoRuO4H413Silver-Intermediated Perovskite La 0.9 FeO 3−δ toward High-Performance Cathode Catalysts for Nonaqueous Lithium–Oxygen Batteries63LaSrCoO4±@La0.5Sr0.5CoO3- core-shell hybrid as the cathode materials for solid oxide fuel cells6Nitrogen doped ultrathin calcium/sodium niobate perovskite nanosheets for photocatalytic water oxidation29Endogenous Nanoparticles Strain Perovskite Host Lattice Providing Oxygen Capacity and Driving Oxygen Exchange and CH 4 Conversion to Syngas21Endogenous Nanoparticles Strain Perovskite Host Lattice Providing Oxygen Capacity and Driving Oxygen Exchange and CH4 Conversion to Syngas98Cubic perovskite-type Sm 0.3 Sr 0.7 Nb 0.08 Co 0.92 O 3−δ as a novel cathode material for intermediate temperature solid oxide fuel cells14Pr 2 BaNiMnO 7−δ double-layered Ruddlesden–Popper perovskite oxides as efficient cathode electrocatalysts for low temperature proton conducting solid oxide fuel cells137Highly active self-assembled hybrid catalyst with multiphase heterointerfaces to accelerate cathodic oxygen reduction of intermediate-temperature solid oxide fuel cells34A hierarchical hybrid electrode for rapid oxygen reduction reaction below 800°C2Exploring Ni(Mn 1/3 Cr 2/3 ) 2 O 4 spinel-based electrodes for solid oxide cells46In Situ Investigation of Reversible Exsolution/Dissolution of CoFe Alloy Nanoparticles in a Co‐Doped Sr 2 Fe 1.5 Mo 0.5 O 6− δ Cathode for CO 2 Electrolysis340Overview of nanomaterials synthesis methods, characterization techniques and effect on seed germination24Facilitating oxygen reduction by silver nanoparticles on lanthanum strontium ferrite cathode15Exsolution of Nickel Nanoparticles from Mixed‐Valence Metal Oxides: A Quantitative Evaluation by Magnetic Measurements9Materials and nano-structural processes for use in solid oxide fuel cells: a review46Silver-Modified Ba 1– x Co 0.7 Fe 0.2 Nb 0.1 O 3−δ Perovskite Performing as a Cathodic Catalyst of Intermediate-Temperature Solid Oxide Fuel Cells35Activation-free supercapacitor electrode based on surface-modified Sr2CoMo1-xNixO6-δ perovskite64Progress and Opportunities for Exsolution in Electrochemistry26Review on exsolution and its driving forces in perovskites138Exceptional Tunability over Size and Density of Spontaneously Formed Nanoparticles via Nucleation Dynamics38Ex‐Solved Ag Nanocatalysts on a Sr‐Free Parent Scaffold Authorize a Highly Efficient Route of Oxygen Reduction87Atomic‐Scale Insight into Exsolution of CoFe Alloy Nanoparticles in La 0.4 Sr 0.6 Co 0.2 Fe 0.7 Mo 0.1 O 3− δ with Efficient CO 2 Electrolysis185Atomic‐Scale Insight into Exsolution of CoFe Alloy Nanoparticles in La0.4Sr0.6Co0.2Fe0.7Mo0.1O3−δ with Efficient CO2 Electrolysis6Development and application of ex-solution nanocatalyst0Toward Reducing the Operation Temperature of Solid Oxide Fuel Cells: Our Past 15 Years of Efforts in Cathode Development298Computational approaches to the exsolution phenomenon in perovskite oxides with a view to design highly durable and active anodes for solid oxide fuel cells13Shaping a Doped Perovskite Oxide with Measured Grain Boundary Defects to Catalyze Bifunctional Oxygen Activation for a Rechargeable Zn–Air Battery41Dopant‐Driven Positive Reinforcement in Ex‐Solution Process: New Strategy to Develop Highly Capable and Durable Catalytic Materials51A multiscale framework to predict electrochemical characteristics of yttrium doped Barium Zirconate based solid oxide cells11In situ and operando characterisation techniques for solid oxide electrochemical cells: recent advances30Organic Photochemistry-Assisted Nanoparticle Segregation on Perovskites14Modeling Exsolution of Pt from ATiO3 Perovskites (A = Ca/Sr/Ba) Using First-Principles Methods21Exploiting rare-earth-abundant layered perovskite cathodes of LnBa0.5Sr0.5Co1.5Fe0.5O5+δ (Ln=La and Nd) for SOFCs62Activity of layered swedenborgite structured Y 0.8 Er 0.2 BaCo 3.2 Ga 0.8 O 7+δ for oxygen electrode reactions in at intermediate temperature reversible ceramic cells66Efficient reversible CO/CO2 conversion in solid oxide cells with a phase-transformed fuel electrode53Nanoparticle Ex-solution for Supported Catalysts: Materials Design, Mechanism and Future Perspectives181Defect engineering of oxide perovskites for catalysis and energy storage: synthesis of chemistry and materials science335Direct alcohol-fed solid oxide fuel cells1Electrochemical energy storage devices working in extreme conditions345In Situ exsolved Au nanoparticles from perovskite oxide for efficient epoxidation of styrene25Coupling decreased polarization resistance Sr0.95Ti0.3Fe0.6Ni0.1O3-δ cathode with efficient metal supported Solid Oxide Fuel Cell31SrCo0.8Ti0.1Ta0.1O3-δ perovskite: A new highly active and durable cathode material for intermediate-temperature solid oxide fuel cells83Nanoparticle exsolution in perovskite oxide and its sustainable electrochemical energy systems43Introducing Ag in Ba0.9La0.1FeO3-δ: Combining cationic substitution with metal particle decoration123D GBM-supported Transition Metal Oxide Nanocatalysts and Heteroatom-doped 3D Graphene Electrocatalysts for Potential Application in Fuel Cells3Perovskite Cathode Materials for Low-Temperature Solid Oxide Fuel Cells: Fundamentals to Optimization99Effectively Promoting Activity and Stability of a MnCo2O4-Based Cathode by In Situ Constructed Heterointerfaces for Solid Oxide Fuel Cells50Silver decorated cobalt carbonate to enable high bifunctional activity for oxygen electrocatalysis and rechargeable Zn-air batteries28Computational Design and Experimental Validation of the Optimal Bimetal-Doped SrCoO3−δ Perovskite as Solid Oxide Fuel Cell Cathode104Computational discovery of energy materials in the era of big data and machine learning: A critical review60Cation-Deficient Perovskites for Clean Energy Conversion149Inkjet-printed Ag@SDC core-shell nanoparticles as a high-performance cathode for low-temperature solid oxide fuel cells13Theoretical insights on the exsolved behavior of ruthenium atom in titanate perovskite7Perovskite Oxides in Catalytic Combustion of Volatile Organic Compounds: Recent Advances and Future Prospects137Probing into the In-Situ Exsolution Mechanism of Metal Nanoparticles from Doped Ceria Host6Promoting exsolution of RuFe alloy nanoparticles on Sr2Fe1.4Ru0.1Mo0.5O6−δ via repeated redox manipulations for CO2 electrolysis268The Performance of Ruddlesden–Popper (R-P) Structured Pr2–xSrxNi0.2Mn0.8O4 for Reversible Single-Component Cells26Enhanced Electrochemical Performance and Durability of the BaCo0.4Fe0.4Zr0.1Y0.1O3−δ Composite Cathode of Protonic Ceramic Fuel Cells via Forming Nickel Oxide Nanoparticles49

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  44. Mass‐Production of Mesoporous MnCo2O4 Spinels with Manganese(IV)‐ and Cobalt(II)‐Rich Surfaces for Superior Bifunctional Oxygen Electrocatalysis

    Angewandte Chemie International Edition · 2017-10-11

    Wenhai Wang, Long Kuai, Wei Cao, Marko Huttula, Sami Ollikkala, Taru Ahopelto, A. Honkanen, Simo Huotari, Mengkang Yu, Baoyou Geng

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  45. Demonstration of chemistry at a point through restructuring and catalytic activation at anchored nanoparticles

    Nature Communications · 2017-11-24

    Dragos Neagu, Evangelos I. Papaioannou, Wan Khairunnisa Wan Ramli, David Miller, Billy J. Murdoch, Hervé Ménard, Ahmed Umar, Anders J. Barlow, Peter J. Cumpson, John T. S. Irvine, Ian S. Metcalfe

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  46. Direct Alcohol‐Fueled Low‐Temperature Solid Oxide Fuel Cells: A Review

    Energy Technology · 2017-12-26

    Byung Chan Yang, Junmo Koo, Jeong Woo Shin, Dohyun Go, Joon Hyung Shim, Jihwan An

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  47. Nanomaterials and technologies for low temperature solid oxide fuel cells: Recent advances, challenges and opportunities

    Nano Energy · 2017-12-29

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  48. Self-assembled alloy nanoparticles in a layered double perovskite as a fuel oxidation catalyst for solid oxide fuel cells

    Journal of Materials Chemistry A · 2018-01-01

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  49. Silver-Perovskite Hybrid Electrocatalysts for Oxygen Reduction Reaction in Alkaline Media

    Journal of The Electrochemical Society · 2018-01-01

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  50. Synergistically enhanced hydrogen evolution electrocatalysis by in situ exsolution of metallic nanoparticles on perovskites

    Journal of Materials Chemistry A · 2018-01-01

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