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RESEARCH PAPER · Nature Chemistry · 2010

Selective incarceration of caesium ions by Venus flytrap action of a flexible framework sulfide

Nan Ding, Mercouri G. Kanatzidis

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Selective incarceration of caesium ions by Venus flytrap action of a flexible framework sulfideOriginalSeizing the caesium33Largest Molecular Clusters in the Supertetrahedral Tn Series104Syntheses and single-crystal structures of CsTh(MoO4)2Cl and Na4Th(WO4)410[(Me)2NH2]0.75[Ag1.25SnSe3]: A three-dimensionally microporous chalcogenide exhibiting framework flexibility upon ion-exchange70K+-recognition capsules with squirting release mechanisms61New compounds and structures in the solid state0Solid‐State Ion Channels for Potentiometric Sensing82Solid‐State Ion Channels for Potentiometric Sensing13Na5(Ga4S)(GaS4)3·6H2O: A three-dimensional thiogallate containing a novel octahedral building block8Metal encapsulation mediated planar to three dimensional structural transformation in Au-clusters: The venus flytrap effect24Stabilization of Noncondensed (AsIIIS3)3– Anions by Coordinating to [MnII(phen)]2+ Complex Cations: a Mixed-Valent Thioarsenate (III, V) {[Mn(phen)]3(AsVS4)(AsIIIS3)}n·nH2O Showing the Coexistence of Antiferromagnetic Order, Photoluminescence, and Nonlinear Optical Properties60[BMIm]4[Sn9Se20]: Ionothermal Synthesis of a Selenidostannate with a 3D Open-Framework Structure87Capture of Radioactive Cesium and Iodide Ions from Water by Using Titanate Nanofibers and Nanotubes254Capture of Radioactive Cesium and Iodide Ions from Water by Using Titanate Nanofibers and Nanotubes34Solvothermal synthesis of a bimetallic thiometallate containing germanium in two oxidation states20Layered indium chalcogenidoantimonates [Me 2 NH 2 ] 2 In 2 Sb 2 S 7-x Se x (x = 0, 2.20, 4.20, 7) with tunable band gaps and photocatalytic properties51Highly Efficient, Irreversible and Selective Ion Exchange Property of Layered Titanate Nanostructures263Structural Diversity, Optical and Magnetic Properties of a Series of Manganese Thioarsenates with 1,10-Phenanthroline or 2,2′-Bipyridine Ligands: Using Monodentate Methylamine as an Alkalinity Regulator47Synthesis and characterization of (H2dab)2Cu8Ge4S14·2H2O: An expanded framework based on icosahedral Cu8S12 cluster24Assembly of novel organic-decorated quaternary TM–Hg–Sb–Q compounds (TM = Mn, Fe, Co; Q = S, Se) by the combination of three types of metal coordination geometries72Size- and shape-controlled synthesis of Prussian Blue nanoparticles by a polyvinylpyrrolidone-assisted crystallization process203“Zeoball” [Sn36Ge24Se132]24–: A Molecular Anion with Zeolite-Related Composition and Spherical Shape146Ion-Exchange Characteristics of a Layered Metal Sulfide for Removal of Sr2+from Aqueous Solutions16ZnS Nanoparticle Gels for Remediation of Pb2+ and Hg2+ Polluted Water118Spatially controlled carbon sponge for targeting internalized radioactive materials in human body32Effects of Hydration during Strontium Exchange into Nanoporous Hydrogen Niobium Titanium Silicate8Copper‐Rich Framework Selenoarsenates Based on Icosahedral Cu8Se13 Clusters14On the Complexity of Crystallization of Thioantimonates: In‐situ Energy Dispersive X‐ray Diffraction (EDXRD) Studies of the Solvothermal Formation of the Isostructural Thioantimonates [TM(tren)Sb4S7] (TM = Fe, Zn)16[NH 3 CH 3 ] 4 [In 4 SbS 9 SH]: a novel methylamine-directed indium thioantimonate with Rb + ion-exchange property59[AEPH2][GeSb2S6]·CH3OH: a thiogermanate–thioantimonate featuring an infinite ribbon-like structure with an unusual {GeSb3S11} unit and exhibiting the ability of photocatalytic degradation of organic dye29Novel mercury selenidoantimonates with structures ranging from one-dimensional ribbon to three-dimensional open-framework17Silver oxide nanocrystals anchored on titanate nanotubes and nanofibers: promising candidates for entrapment of radioactive iodine anions72Titanate-based adsorbents for radioactive ions entrapment from water131Advances in Inorganic and Hybrid Ion Exchangers40Two novel one-dimensional mercury selenidostannates with transition metal complexes: [Fe(phen)3]Hg2Sn2Se7·1.5eta·0.25H2O and [Ni2(teta)2(μ-teta)]HgSn3Se922Synthesis of Cu2+ and Ag+ doped Na2Ti3O7 by a facile ion-exchange method as visible-light-driven photocatalysts44Changes in the Structural Dimensionality of Selenidostannates in Ionic Liquids: Formation, Structures, Stability, and Photoconductivity50Syntheses, crystal structures, and properties of two new one-dimensional heterometallic selenides: [DBNH]4[M3Sn4Se11(Se2)2] (M = Cd, Hg)14Selective anion exchange with nanogated isoreticular positive metal-organic frameworks370Surfactant–Thermal Method to Synthesize a Novel Two‐Dimensional Oxochalcogenide79In situ controllable synthesis of magnetic Prussian blue/graphene oxide nanocomposites for removal of radioactive cesium in water269Co-assembly of a three-dimensional open framework sulfide with a novel linkage between an oxygen-encapsulated T3 cluster and a supertetrahedral T2 cluster25Inclusion chemistry of a thiazyl radical in zeolite-Y13[(Me)2NH2][BiGeS4]: the first organically directed bismuth thiogermanate with Rb+ ion exchange property16Highly selective and efficient heavy metal capture with polysulfide intercalated layered double hydroxides206New strategies to prepare crystalline chalcogenides165Novel thioarsenates {[Mn(2,2′-bipy) 2 (SCN)][Mn(2,2′-bipy)](As V S 4 )} 2 and {[Mn(2,2′-bipy) 2 (SCN)] 2 [As III 2 (S 2 ) 2 S 2 ]}: introducing an anionic second ligand to modify Mn II complex cations of 2,2′-bipyridine20Magnetic prussian blue/graphene oxide nanocomposites caged in calcium alginate microbeads for elimination of cesium ions from water and soil204Atomically Precise Doping of Monomanganese Ion into Coreless Supertetrahedral Chalcogenide Nanocluster Inducing Unusual Red Shift in Mn2+ Emission172Characteristics of cesium ion sorption from aqueous solution on bentonite- and carbon nanotube-based composites116Mild Solvothermal Syntheses and Characterization of Layered Copper Thioantimonates(III) and Thioarsenate(III)44A Novel Vanadosilicate with Hexadeca‐Coordinated Cs + Ions as a Highly Effective Cs + Remover92A Novel Vanadosilicate with Hexadeca‐Coordinated Cs+ Ions as a Highly Effective Cs+ Remover20Synthesis and crystal structure of the bi-metallic hybrid compound {Mn4(2,2′-bipyridine)2Sb4S10}10{[M(NH3)6][Ag4M4Sn3Se13]}∞ (M=Zn, Mn): Three-dimensional chalcogenide frameworks constructed from quaternary metal selenide clusters with two different transition metals23Separate or Simultaneous Removal of Radioactive Cations and Anions from Water by Layered Sodium Vanadate-Based Sorbents77Surfactant-Thermal Syntheses, Structures, and Magnetic Properties of Mn–Ge–Sulfides/Selenides45Using solution- and solid-state S K-edge X-ray absorption spectroscopy with density functional theory to evaluate M–S bonding for MS 4 2− (M = Cr, Mo, W) dianions18Threading Chalcogenide Layers with Polymer Chains209Threading Chalcogenide Layers with Polymer Chains31New Members of the Family of In–Sb–S Compounds: Different Roles of Organic Amines20A crown-like heterometallic unit as the building block for a 3D In–Ge–S framework2A hybrid linkage mode between T2,2 and T3 selenide clusters14A two-dimensionally microporous thiostannate with superior Cs + and Sr 2+ ion-exchange property177Granulous KMS-1/PAN composite for Cs + removal21Nanolayered tin phosphate: a remarkably selective Cs ion sieve for acidic waste solutions14Selective chemical binding enhances cesium tolerance in plants through inhibition of cesium uptake36In situ growth of Prussian blue nanocrystal within Fe3+ crosslinking PAA resin for radiocesium highly efficient and rapid separation from water70Umbellate Distortions of the Uranyl Coordination Environment Result in a Stable and Porous Polycatenated Framework That Can Effectively Remove Cesium from Aqueous Solutions449Supercubooctahedron (Cs6Cl)2Cs5[Ga15Ge9Se48] Exhibiting Both Cation and Anion Exchange13Surfactants as Promising Media for the Preparation of Crystalline Inorganic Materials315Tenside als Reaktionsmedien zur Synthese von kristallinen anorganischen Materialien14Syntheses, Crystal Structures, Ion-Exchange, and Photocatalytic Properties of Two Amine-Directed Ge–Sb–S Compounds55Hydrazine-Hydrothermal Synthesis and Characterization of the Two New Quaternary Thioantimonates(III) BaAgSbS3 and BaAgSbS3·H2O40Porous Amorphous Chalcogenides as Selective Adsorbents for Heavy Metals47Preparation of Porous Three‐Dimensional Quaternary Thioantimonates(III) ACuSb2S4 (A=Rb, Cs) through a Surfactant‐Thermal Method29Facile surfactant-thermal syntheses and characterization of quaternary copper thioantimonates(III) ACu 2 SbS 3 (A = K, Rb, Cs)23Chemically derived optical sensors for the detection of cesium ions53Synthese kristalliner Chalkogenide in ionischen Flüssigkeiten43Synthesis of Crystalline Chalcogenides in Ionic Liquids150Efficient and selective heavy metal sequestration from water by using layered sulfide K 2x Sn 4−x S 8−x (x = 0.65–1; KTS-3)82Metal sulfide ion exchangers: superior sorbents for the capture of toxic and nuclear waste-related metal ions334Reinforced silica monoliths functionalised with metal hexacyanoferrates for cesium decontamination: a combination of a one-pot procedure and skeleton calcination16Combination of Metal Coordination Tetrahedra and Asymmetric Coordination Geometries of Sb(III) in the Organically Directed Chalcogenidometalates: Structural Diversity and Ion-exchange Properties25Highly Selective and Efficient Removal of Heavy Metals by Layered Double Hydroxide Intercalated with the MoS 4 2– Ion705Hydrazine-hydrothermal syntheses, characterizations and photoelectrochemical properties of two quaternary chalcogenidoantimonates(III) BaCuSbQ3 (Q = S, Se)51Facile Hydrazine‐Hydrothermal Syntheses and Characterizations of Two Quaternary Thioarsenates(III): Two‐Dimensional SrAg4As2S6⋅2 H2O and One‐Dimensional BaAgAsS320Organically directed heterometallic chalcogenidometalates containing group 12(II)/13(III)/14(IV) metal ions and antimony(III)68Synthesis, Structure, Band Gap, and Near-Infrared Photosensitivity of a New Chalcogenide Crystal, (NH4)4Ag12Sn7Se2215Effect of alkali cations on two-dimensional networks of two new quaternary thioarsenates (III) prepared by a facile surfactant-thermal method13Enhanced adsorption of cesium on PVA-alginate encapsulated Prussian blue-graphene oxide hydrogel beads in a fixed-bed column system143Cation-Dependent Gold Recovery with α-Cyclodextrin Facilitated by Second-Sphere Coordination89Efficient Removal and Recovery of Uranium by a Layered Organic–Inorganic Hybrid Thiostannate397Main group metal chalcogenidometalates with transition metal complexes of 1,10-phenanthroline and 2,2′-bipyridine59Highly Selective and Rapid Uptake of Radionuclide Cesium Based on Robust Zeolitic Chalcogenide via Stepwise Ion-Exchange Strategy151Selective and low temperature transition metal intercalation in layered tellurides17Multitopic ligand directed assembly of low-dimensional metal-chalcogenide organic frameworks5Removal of cadmium ions from wastewater by dithiocarbamate functionalized pyrrole based terpolymers43Inorganic layered ion-exchangers for decontamination of toxic metal ions in aquatic systems95Organically modified clay with potassium copper hexacyanoferrate for enhanced Cs + adsorption capacity and selective recovery by flotation76Syntheses, crystal structures, and photocatalytic properties of two ammonium-directed Ag–Sb–S complexes30Syntheses, Crystal Structures, and Optical and Photocatalytic Properties of Four Small-Amine-Molecule-Directed M–Sn–Q (M = Zn, Ag; Q = S, Se) Compounds49Facile synthesis of mesoporous magnetic AMP polyhedric composites for rapid and highly efficient separation of Cs+ from water49Layered A2Sn3S7·1.25H2O (A = Organic Cation) as Efficient Ion-Exchanger for Rare Earth Element Recovery142Layered Metal Chalcophosphate (K-MPS-1) for Efficient, Selective, and ppb Level Sequestration of Pb from Water46Effect of coexisting cations on the adsorption of cesium onto poly (β-cyclodextrin)/bentonite composite16Reversible and Efficient Sequestration of Cesium from Water by the Layered Metal Thiophosphate K 0.48 Mn 0.76 PS 3 ⋅H 2 O39Selective Ion Exchange and Photocatalysis by Zeolite‐Like Semiconducting Chalcogenide29Inorganic Ion Exchangers for Cesium Removal from Radioactive Wastewater104Recent developments in nanostructured inorganic materials for sorption of cesium and strontium: Synthesis and shaping, sorption capacity, mechanisms, and selectivity—A review295Towards magnetic responsive chalcogenides for efficient separation in water treatment: facile synthesis of magnetically layered chalcogenide Fe 3 O 4 /KMS-1 composite adsorbents and their zinc removal application in water10Extraction of rare earth elements using magnetite@MOF composites53Nanocomposite membrane for environmental remediation19Selective Binding and Precipitation of Cesium Ions from Aqueous Solutions: A Size‐Driven Supramolecular Reaction34[CH3NH3]4Ga4SbS9S0.28O0.72H: A Three‐Dimensionally Open‐Framework Heterometallic Chalcogenidoantimonate Exhibiting Ni2+ Ion‐Exchange Property19The adsorption of Cs+ from wastewater using lithium-modified montmorillonite caged in calcium alginate beads41Metal–Organic Frameworks for Separation1305Synergy between Zeolite Framework and Encapsulated Sulfur for Enhanced Ion-Exchange Selectivity to Radioactive Cesium71Efficient Removal of [UO2]2+, Cs+, and Sr2+ Ions by Radiation-Resistant Gallium Thioantimonates207A simple synthesis of magnetic ammonium 12-molybdophosphate/graphene oxide nanocomposites for rapid separation of Cs+ from water8Unusual Flexibility of Microporous Sulfides during Ion Exchange52Layered chalcogenide modified by Lanthanum, calcium and magnesium for the removal of phosphate from water34Alkylammonium thiostannate inorganic/organic hybrids as high-performance photocatalysts with a decoupled adsorption–photodegradation mechanism8Deep eutectic solvothermal synthesis of an open framework copper selenidogermanate with pH-resistant Cs + ion exchange properties33Disposal of cesium ion from wastewater using biocompatible titanate nanotube6Ionic liquid cations as methylation agent for extremely weak chalcogenido metalate nucleophiles38Highly Selective Radioactive 137Cs+ Capture in an Open-Framework Oxysulfide Based on Supertetrahedral Cluster42Composite hydrogel particles encapsulated ammonium molybdophosphate for efficiently cesium selective removal and enrichment from wastewater111Distinctive Two-Step Intercalation of Sr2+ into a Coordination Polymer with Record High 90Sr Uptake Capabilities184Removal of cesium ions from aqueous solutions using various separation technologies328Synthesis of a robust layered metal sulfide for rapid and effective removal of Sr2+ from aqueous solutions95Nano-sized Prussian blue immobilized costless agro-industrial waste for the removal of cesium-137 ions39Effective and Rapid Adsorption of Sr2+ Ions by a Hydrated Pentasodium Cluster Templated Zinc Thiostannate35Cesium separation from radioactive waste by extraction and adsorption based on crown ethers and calixarenes161Fast and Selective Removal of Aqueous Uranium by a K+-Activated Robust Zeolitic Sulfide with Wide pH Resistance40Adsorption of cesium on polyaniline montmorillonite nanotube-based composite from aqueous solution5Stimuli-Responsive Biopolymers: An Inspiration for Synthetic Smart Materials and Their Applications in Self-Controlled Catalysis18Hollow flower-like titanium ferrocyanide structure for the highly efficient removal of radioactive cesium from water73Construction of H 4x K 2x Sn 2−x S 4+x /TiO 2 nanocomposites with enhanced visible light-driven photocatalytic performance0Syntheses, structures, and photocatalytic properties of open-framework Ag–Sn–S compounds26Two new layered metal chalcogenide frameworks as photocatalysts for highly efficient and selective dye degradation6One-Dimensional Chains in Pentanary Chalcogenides A2Ba3Cu2Sb2S10 (A = K, Rb, Cs) Displaying a Photocurrent Response44Prussian blue-embedded carboxymethyl cellulose nanofibril membranes for removing radioactive cesium from aqueous solution72Facile Synthesis of Porous Polymer Using Biomass Polyphenol Source for Highly Efficient Separation of Cs+ from Aqueous Solution14Bio-Inspired Preparation of Clay–Hexacyanoferrate Composite Hydrogels as Super Adsorbents for Cs+67Novel montmorillonite-sulfur composite for enhancement of selective adsorption toward cesium32Rapid and selective removal of Cs+ from water by layered potassium antimony thiostannate44Macrocyclic Pyridone Pentamers for Highly Selective High‐Capacity Removal of Caesium Ions from Radioactive High‐Salinity Waste7Ultrafast and selective uptake of Eu3+ from aqueous solutions by two layered sulfides41Structural diversities in centrosymmetric La 8 S 4 Cl 8 La 12 S 8 Cl 4 [SbS 3 ] 8 and non-centrosymmetric Ln 12 S 8 Cl 8 [SbS 3 ] 4 (Ln = La and Ce): syntheses, crystal and electronic structures, and optical properties10

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  2. Largest Molecular Clusters in the Supertetrahedral Tn Series

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  3. Syntheses and single-crystal structures of CsTh(MoO4)2Cl and Na4Th(WO4)4

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  5. K+-recognition capsules with squirting release mechanisms

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  6. New compounds and structures in the solid state

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  10. Metal encapsulation mediated planar to three dimensional structural transformation in Au-clusters: The venus flytrap effect

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  11. Stabilization of Noncondensed (AsIIIS3)3– Anions by Coordinating to [MnII(phen)]2+ Complex Cations: a Mixed-Valent Thioarsenate (III, V) {[Mn(phen)]3(AsVS4)(AsIIIS3)}n·nH2O Showing the Coexistence of Antiferromagnetic Order, Photoluminescence, and Nonlinear Optical Properties

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  12. [BMIm]4[Sn9Se20]: Ionothermal Synthesis of a Selenidostannate with a 3D Open-Framework Structure

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  13. Capture of Radioactive Cesium and Iodide Ions from Water by Using Titanate Nanofibers and Nanotubes

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  20. Assembly of novel organic-decorated quaternary TM–Hg–Sb–Q compounds (TM = Mn, Fe, Co; Q = S, Se) by the combination of three types of metal coordination geometries

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  23. Ion-Exchange Characteristics of a Layered Metal Sulfide for Removal of Sr2+from Aqueous Solutions

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  25. Spatially controlled carbon sponge for targeting internalized radioactive materials in human body

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  27. Copper‐Rich Framework Selenoarsenates Based on Icosahedral Cu8Se13 Clusters

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  28. On the Complexity of Crystallization of Thioantimonates: In‐situ Energy Dispersive X‐ray Diffraction (EDXRD) Studies of the Solvothermal Formation of the Isostructural Thioantimonates [TM(tren)Sb4S7] (TM = Fe, Zn)

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  30. [AEPH2][GeSb2S6]·CH3OH: a thiogermanate–thioantimonate featuring an infinite ribbon-like structure with an unusual {GeSb3S11} unit and exhibiting the ability of photocatalytic degradation of organic dye

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  32. Silver oxide nanocrystals anchored on titanate nanotubes and nanofibers: promising candidates for entrapment of radioactive iodine anions

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  33. Titanate-based adsorbents for radioactive ions entrapment from water

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  34. Advances in Inorganic and Hybrid Ion Exchangers

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  35. Two novel one-dimensional mercury selenidostannates with transition metal complexes: [Fe(phen)3]Hg2Sn2Se7·1.5eta·0.25H2O and [Ni2(teta)2(μ-teta)]HgSn3Se9

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  36. Synthesis of Cu2+ and Ag+ doped Na2Ti3O7 by a facile ion-exchange method as visible-light-driven photocatalysts

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  37. Changes in the Structural Dimensionality of Selenidostannates in Ionic Liquids: Formation, Structures, Stability, and Photoconductivity

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  38. Syntheses, crystal structures, and properties of two new one-dimensional heterometallic selenides: [DBNH]4[M3Sn4Se11(Se2)2] (M = Cd, Hg)

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  39. Selective anion exchange with nanogated isoreticular positive metal-organic frameworks

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  40. Surfactant–Thermal Method to Synthesize a Novel Two‐Dimensional Oxochalcogenide

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  41. In situ controllable synthesis of magnetic Prussian blue/graphene oxide nanocomposites for removal of radioactive cesium in water

    Journal of Materials Chemistry A · 2013-10-17

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  42. Co-assembly of a three-dimensional open framework sulfide with a novel linkage between an oxygen-encapsulated T3 cluster and a supertetrahedral T2 cluster

    Chemical Communications · 2013-10-22

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  43. Inclusion chemistry of a thiazyl radical in zeolite-Y

    Dalton Transactions · 2013-10-30

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  44. [(Me)2NH2][BiGeS4]: the first organically directed bismuth thiogermanate with Rb+ ion exchange property

    Dalton Transactions · 2014-01-01

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  45. Highly selective and efficient heavy metal capture with polysulfide intercalated layered double hydroxides

    Journal of Materials Chemistry A · 2014-01-01

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  46. New strategies to prepare crystalline chalcogenides

    Inorganic Chemistry Frontiers · 2014-01-01

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  47. Novel thioarsenates {[Mn(2,2′-bipy) 2 (SCN)][Mn(2,2′-bipy)](As V S 4 )} 2 and {[Mn(2,2′-bipy) 2 (SCN)] 2 [As III 2 (S 2 ) 2 S 2 ]}: introducing an anionic second ligand to modify Mn II complex cations of 2,2′-bipyridine

    Dalton Transactions · 2014-01-01

    Guang‐Ning Liu, Guo‐Cong Guo, Ming‐Sheng Wang, Jin‐Shun Huang

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  48. Magnetic prussian blue/graphene oxide nanocomposites caged in calcium alginate microbeads for elimination of cesium ions from water and soil

    Chemical Engineering Journal · 2014-02-24

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  49. Atomically Precise Doping of Monomanganese Ion into Coreless Supertetrahedral Chalcogenide Nanocluster Inducing Unusual Red Shift in Mn2+ Emission

    Journal of the American Chemical Society · 2014-03-13

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  50. Characteristics of cesium ion sorption from aqueous solution on bentonite- and carbon nanotube-based composites

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