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RESEARCH PAPER · Chemical Reviews · 2025

Therapeutic Hydrogels: Properties and Biomedical Applications

Songtao Dong, Soohwan An, Qimanguli Saiding, Qian Chen, Bin Liu, Na Kong, Wei Chen, Wei Tao

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Therapeutic Hydrogels: Properties and Biomedical ApplicationsOriginalApplication and Prospects of Smart Dressings in Wound Healing26Near-infrared and pH dual-responsive chitosan/epigallocatechin gallate/hollow CuS hydrogel reprograms ROS dynamics for infected wound healing13Precision theranostics in cervical Cancer: Harnessing stimuli-responsive hydrogels for tumor microenvironment-targeted therapy and diagnosis8Alginate formulations with high loads of zebularine and retinoic acid promote tissue growth and innervation and induce extensive epigenetic repatterning1Recent Advances in Hydrogel‐Based Strategies for Promoting Wound Healing7Photo-crosslinkable hydrogel with programmable dual time-phase drug release for accelerated healing of infected diabetic wounds8Hydrogel-based tumor embolization and synergistic therapeutic strategies2Spatiotemporally controlled delivery of biomacromolecules via injectable hydrogels for precision modulation of the tumor immune microenvironment16Spatiotemporal controlled disintegration enabling injected magnetic hydrogel for percutaneous hepatocellular carcinoma treatment3Hydrogels for the cleaning of cultural heritage: A review of mechanisms, applications, and future perspectives5Bioinspired design of hierarchical structured hydrogels with extraordinary lubrication and load-bearing capacity0Cattail-inspired interfacial evaporation via porous thioctic acid-based hydrogels0Choline-based hydrogels and deep eutectic solvent systems for next-generation biomedical platforms: a review1Development of PVA-based hydrogels and e-spun nanofibers via boronic ester chemistry0Hybrid hydrogel system integrating thermoresponsive microspheres and KGN-loaded nanofibers enables efficient cartilage matrix regeneration0Hydrogel systems in orthopedics: delivery modality as a framework for translational design0Hydrogel-based delivery systems for cutaneous melanoma therapy: from chemical design and crosslinking strategies to structure–activity relationships5Hydrogels for in vivo biomedical applications: recent advances and future perspectives16Integration of sonosensitive nanomicelles and ultrasound for enhanced BBB penetration and targeted therapy against glioblastoma: intravenous injection vs. intranasal dripping0Intracellular gelation technology: frontier exploration in biomaterials and biomedical applications0Magnetite hybrid hydrogel of xanthan gum and poly( N -hydroxyethyl acrylamide): a cytocompatible vehicle for sustained oral dual delivery of 5-fluorouracil and curcumin0Mechanical and interfacial properties of zwitterionic hydrogels via a high-entanglement network design: a study of monomer and crosslinker synergy3Physicochemical foundations of biotribological biomaterials: Design, performance, and future horizons0Repurposing protein aggregation into a biofunctional BMP-2–hyaluronic acid hydrogel for sustained drug release and accelerated wound healing1Targeting calcium-crosslinked alginate hydrogel in a living subject using a synthetic anion receptor0The development of multifunctional polysuccinimide with programmable thermoresponsiveness by modulating the hydrophobic graft architecture for advanced drug delivery applications1Towards supramolecular regenerative medicine using low-molecular-weight gelator hydrogels for stem cell growth0Bioinspired and stimuli-responsive hydrogels for regenerative medicine: design principles and clinical translation4Intelligent drug delivery-wound healing integrated hydrogel dressing for Type 2 Diabetes Mellitus wounds with wound microenvironment modulation18Smart supramolecular hydrogels as a potential platform for wound dressings: Harnessing thiamine to boost neomycin efficacy1Tough and stretchable cellulose hydrogels engineered via the synergy of entanglements and cross-links7Advances in Damping Gel Materials: From Characterization and Design to Applications7Interphase-Centric and Mechanism-Driven Advances in Polymer Composites Reinforced with Nano-, Synthetic, and Inorganic Fillers47Applications of Multifunctional Hydrogel in Tissue Engineering and Regenerative Medicine11Electronic jelly: Engineering the mechanics of hydrogels for flexible electronics0Citric Acid–Mediated Crosslinking of Chia Seed Glucoxylan and Hydroxypropyl Cellulose: pH Responsiveness, Haemocompatibility and Sustained Drug Release0Hydrogels for Cancer Immunotherapy: Strategies From Construction to Application5Smart nanohydrogels for drug delivery: a comprehensive review0Hydrogel‐Based Implantable Medical Devices: Pioneering Therapies and Monitoring9Polyphenol-metal coordinated nanofiber-enhanced biopolymer hydrogels for sustainable full-thickness skin regeneration and defect repair4A Carboxymethyl Chitosan Hydrogel Loaded with Bacteriophage-Derived Bacteriostatic Peptide Exhibits Antibacterial, Hemostatic, and Wound-Healing Properties2A review on Janus biomaterials: Asymmetric design for advanced bone regeneration1Smart responsive hydrogels combined with AI design for tumor therapy5Advances in non-invasive delivery strategies for anti-cancer therapy0Bioinspired Keratin-Based Eutectic Hydrogels for Intelligent Health Monitoring and Photothermal Therapy2Safe polyacrylamide-based hydrogels with low monomer content achieved by using liquid metal nanoparticles or MoS2 nanosheets as efficient initiators1Pig skin-derived reconstituted lipid nanoparticles loaded sodium alginate hydrogel for wound healing1Recapitulation of human 3D colorectal cancer model using smart thermo-responsive hydrogel for monitoring angiogenesis1Emerging growth factor delivery hydrogel system for wound healing3Injectable Metal-Free Carbon Dot-Integrated Hydrogel for Regulating Inflammation via Macrophage Metabolic Reprograming in Spinal Cord Injury Therapy6Tunable microgel modulars for temporally coordinated combination therapy2Influence of process parameters on shape fidelity in extrusion-based bioprinting: a rheological perspective2Engineering multifunctional chitosan-based hydrogels for integrated antimicrobial therapy and endogenous stem cell-driven tissue repair in infectious keratitis3Cutting-Edge Smart Hydrogel Platforms for Improved Wound Healing7Electrically rewired healing of the infarcted heart via a smart bioadhesive patch targeting fibrosis and calcium imbalance0Leveraging Dynamic Electrostatic and Hydrophobic Interactions for Biomedical Hydrogels1A mechanoadaptive glycopeptide hydrogel alleviates intervertebral disc degeneration by targeting PPARα1Phase-separated hydrogels for advanced biomedical engineering: From material design to applications4High-performance hydrogels in orthopedics: Structural design, performance tuning, and clinical potential6Enhancing shape fidelity in bioprinting: Modeling die swell through rheological and process interaction analysis3An Iron-Scavenging and Hydrogen-Releasing Microneedle Patch Suppresses Ferroptosis and Promotes Spinal Cord Repair8A carboxymethyl chitosan-based responsive dual-crosslinked hydrogel loaded with diosmetin for traumatic wound healing1Semiclosed Cyclic Hemiaminal-Based Multistimuli- Responsive Hydrogels for Advanced Wound Dressings2Microenvironment engineering with injectable hydrogel-based biofunctional scaffolds for augmenting bone defect regeneration1A spatiotemporally enhanced polyanion hydrogel as a strategic trap for inflammatory signals in postoperative anti-adhesion0SA/HA double-network hydrogel combined with PVDF electret membrane enhances osteogenic differentiation of DPSCs and promotes mandibular bone defect repair0Coreopsis tinctoria -loaded gels for dermal delivery: development, optimization, retention capacity, and skin photoaging repair1Sonoimmunology in cancer therapy: expanding crosstalk among ultrasound-materials-immune system1Hydrogels for the treatment of spinal cord injury: progress and promise0AI-driven reconstruction of the evidence architecture of hydrogel-based intervertebral disc repair research0Vanadium-Doped Bioactive Glass-Modified GelMA/CMCS/HA Injectable Hydrogel for Osteosarcoma Postoperative Therapy and Bone Regeneration1Hydrophilic Anhydride-Containing Oligomers for Two-Component Hydrogels: From Biopolymer Compatibility to Cytocompatible Gelatin Bioinks0Biocompatible Interface for Organic Electrochemical Transistors Enables Bioadhesion and Over‐Swelling Suppression0Biocompatible Interface for Organic Electrochemical Transistors Enables Bioadhesion and Over‐Swelling Suppression0Development and Applications of Antifreeze Materials: From Nature to Design2Injectable Binary-Amplified Cascade Hydrogels Suppress Post-Incomplete Microwave Ablation Relapse via Integrated Metallo-Metabolic-Immunomodulation3Direct Ink Writing 3D Printing of Hydrogel Bioelectronics1Hydrogels for Healing Radiation-Injured Tissues and Organs2Functional Poly(allyl glycidyl ether)-PEG based hydrogels as a tunable platform for potential controlled release of therapeutics0Natural bioactive sericin-based hydrogel dressing for visual pH monitoring and infected wound therapy1Hydrogels form sustainable source for tendon-to-bone healing: Materials, mechanisms and translational design0Immunomodulatory effect of borophene grafted reinforced silk fibroin hydrogel scaffolds for promoting osteogenic biomineralization and macrophage polarization1Reprocessable and self-healing bio-based polyester via multiple dynamic networks for sustainable low-temperature sensor0Stimuli-responsive quantum-engineered polymeric networks: From molecular design and scalable manufacturing to high performance cargo loading systems0Photothermal and immunomodulatory chitosan composite hydrogel remodels the pathological microenvironment to accelerate infected diabetic wound healing2Platelet-rich plasma-loaded hydrogels: diffusivity and release of individual proteins in multicomponent complex environments0Frontal Polymerization-Enabled Rapid Fabrication of Gelatin-Containing Hydrogels with Good Mechanical and Biological Properties1Bio-recruiting hydrogel targeting mitochondrial homeostasis under neutrophil extracellular traps for diabetic wound repair0A Thermosensitive Hydroxybutyl Chitosan/Microalgae Hydrogel With Antibacterial and Antioxidant Activities for Accelerating Burn Wound Healing0Cyclic olefin copolymer (COC) incorporated triple-crosslinked composite hydrogels with enhanced mechanical properties and self-healing capacity0Engineered Mucoadhesive and Mucopenetrating Biomaterials for Ocular Drug Delivery1Innovative microneedle-integrated hydrogels: a promising strategy for diabetic foot ulcer management0Mechanically Stable Algal Biochar‐Alginate Hydrogels as Bio‐Based Adsorbents for Resource‐Efficient Heavy Metal Removal0Polysaccharide-based hydrogels as controlled-transport networks: Chemistry-to-performance design rules0Stimuli-Responsive Hydrogel Platforms for Cancer Immunotherapy: Advances in Design, Mechanisms, and Clinical Translation0Dynamic and adaptive self‐healing hydrogels: from network engineering to advanced functional systems2Mechanoregulative hydrogel enables scar-reduced and functional healing of infected diabetic mobile wounds0Alkali-triggered kinetic matching of polymerization and crosslinking enables hydrogels with programmable mechanics, flexible sensing, and dynamic information encryption0Biomimetic Redox-Mediated Proton Relay in Nanoreactors for Photocatalysis0Recent advances in two-dimensional material and nanocomposite-based surface plasmon resonance sensors for environmental, food, and biomedical applications0Development of a novel pH-responsive anti-caries nanocomposite hydrogel0Streptavidin functionalized hyaluronic acid hydrogels for controlled and customizable drug delivery0Guanine-Rich DNA Aptamers for Selective Binding to Agarose Hydrogels0Multifunctional Integrated Hydrogels for Tissue Regeneration and Repair0A recombinant collagen-based nanocomposite hydrogel for programmable full-cycle intelligent management of infected wounds0Co-delivery of NSC and metformin for efficient diabetic wound healing via coordination of immune-angiogenic-neural networks0Enzyme-Activated Near-Infrared Fluorescent Probe for Rapid and Precise Identification of Staphylococcus aureus -Induced Skin Infections0A phenylboronic-disulfide hybrid crosslinker for constructing multi-stimuli-responsive and self-healing hydrogels from diverse polysaccharides0Intra-Articularly Injectable Ion-Coordinated Bionic Lubricants Improve Rheumatoid Arthritis Recession via Pro-Regenerative Reprogramming of Synovial Macrophages0Bioinspired multifunctional microneedles assisted drug delivery for effective wound healing: A review0From Passive Cargo to Active Skeleton: A pH-Responsive Polysaccharide Hydrogel Integrating Dipotassium Glycyrrhizinate as a Dynamic Cross-Linking Node for Scarless Wound Healing0Injectable and thermosensitive poly(2-ethyl-2-oxazoline)-poly(L-alanine) hydrogel with enhanced mechanical performance and extended in vivo persistence0Quaternized chitosan-based double-network hydrogel for oral precise delivery of Sinapic acid in ulcerative colitis therapy0Artificial intelligence-driven 3D bioprinting hydrogels for wound healing: From design to closed-loop therapy2Shear‐Thinning Composite Hydrogel Incorporating Polycaprolactone ( PCL ) Short Nanofibers for Cell Therapy Applications0True Closed‐Loop Recyclable Hydrogels Enabled by Imine Boronic Ester Crosslinking1Overcoming Transmission Barriers: A Dual‐Functional Adhesive Hydrogel for Direct Monkeypox Virus Neutralization and Wound Healing0A Hierarchical Hydrogel Modulates Immune‐Mechanical Microenvironments to Spatiotemporally Reprogram Fibroblasts for Scarless Diabetic Wound Healing0Multifunctional Magnetothermo-Responsive Smart Hydrogel for On-Demand Controlled Drug Release in Cancer Therapy0Design, Properties and Applications of Multiple Dynamic Hydrogels0Low-Tortuosity Adsorption Networks Triggered by Micelle-Enhanced Swelling Enable Efficient Lithium Extraction from Seawater1Lysosome-targeted protein degradation platforms for spatiotemporally controlled degradation0Disguise strategy-adjusted controlled cleavage of DNA hydrogel for precision theranostics in colorectal cancer0Multifunctional high-strength adhesive hydrogels in wound dressings0Engineering oral hydrogels for versatile drug delivery: core technologies, disease applications, and industrial translation0Synergistic Performance Optimization of Polyvinyl Alcohol Hydrogels via Silica and Pluronic F127 Incorporation for Biomedical Applications0Advances in hydrogel for anticancer drug delivery0Multifunctional Hydrogels with Antibacterial, Fluorescent, and Conductive Properties via Acylhydrazone–Zn 2+ Coordination and Hydrophobic Association0Preferential Interfacial Engineering of Hydrogels via Interdigitated Nanoparticle Assembly0A self-administered long-acting AngioMatrix platform enables angiogenesis-driven drug delivery for chronic disease management0Wound healing potential of conductive hydrogels: Classification, mechanisms, applications, and clinical challenges0Glucose-rhythm gated Janus artificial enzymes for temporally adaptive treatment of infected diabetic wounds0Bioactive Hydrogel Patches: Polymer Network Design, Fabrication, Functional Regulation, and Biomedical Applications0Multifunctional Metal-Coordinated Hydrogels: Controlled Synthesis and Advances in Anti-Inflammatory, Anticancer, and Antibacterial Applications0Programmable crosslinking strategies for the rational design of engineered protein hydrogels0Coarse‐Grained Simulations Rationalize Thermosensitivity and Hydrolytic Degradation of Vinyl Copolymers Obtained by Radical Ring‐Opening Polymerization0Coarse‐Grained Simulations Rationalize Thermosensitivity and Hydrolytic Degradation of Vinyl Copolymers Obtained by Radical Ring‐Opening Polymerization0Multifunctional nucleic acid-based therapy in fibrosis-related diseases0Engineering oral biomaterials for overcoming gastrointestinal barriers0Enzymatically triggered in situ gelation of a multifunctional peptide for localized controlled release and conformal fracture repair0Evaluation of developmental toxicity of VTES-modified chitosan/PVA hydrogel in chick embryos0Hydrogel-based multifunctional biomaterials for glaucoma therapy: Emerging strategies in sustained delivery, anti-fibrotic regulation, and retinal neuroprotection0Twist‐Densified Collagen‐Silver Nanowire Hydrogel Yarns for Conductive, Bioactive Sutures and Smart Textiles0Engineering programmable peptide hydrogels for chronic refractory wounds: A mechanism‐driven framework0Ginsenoside Rd-functionalized hydrogel for immune modulation and enhanced diabetic wound healing0Dual-Crosslinked Sesbania Gum-Derived Antibacterial Hydrogel Enriched with Multiple Active Sites for Efficient Skin Tissue Engineering0Modulation of the TGF‐β/Smad Signaling Pathway by a Bioactive Oxidized Polygonati Rhizoma Polysaccharide Crosslinked Chitosan Hydrogel as Therapeutic Carrier for Parkinson's Disease Treatment0Recent progress of biomaterials-based hydrogels for wearable electronics and health monitoring0Efficient Separation of Exosomes by Aptamer‐Functionalized Polyacrylamide‐Polyacrylic Acid Hydrogel0Dual‐Targeting of ER Stress and the CD47‐SIRPα Axis via an In Situ Hydrogel Prevents Postoperative Glioblastoma Recurrence0

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