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RESEARCH PAPER · Journal of the American Chemical Society · 2025

Amorphous-Nanocrystalline Fluorinated Halide Electrolytes with High Ionic Conductivity and High-Voltage Stability

Lihai Zhou, Sidong Zhang, Weiping Li, Bing Li, Nicholas Spencer Grundish, Pengfei Ren, Xuefeng Wang, Nan Wu, Weidong Zhou, Yutao Li

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Amorphous-Nanocrystalline Fluorinated Halide Electrolytes with High Ionic Conductivity and High-Voltage StabilityOriginalHalide-based solid electrolytes: opportunities and challenges in the synergistic development of all-solid-state Li/Na batteries22Heterovalent doping of amorphous oxyhalide solid electrolytes for high-performance all-solid-state lithium batteries3Zr‐Doping Induced Complete Amorphization toward Highly Stable All‐Solid‐State Sodium Batteries10Advancing layered double hydroxides (LDHs) as the anodes for efficient anion-exchange-membrane water electrolyzers10Entropy‐Driven Electrolytes for Sodium‐Ion Batteries: From Liquid to Solid‐State Systems7An Oxychloride Solid Electrolyte with Superior Na-Ion Conductivity3Vacancy-mediated LaCl3-based superionic conductors for all-solid-state sodium batteries4Halide Solid-State Electrolytes for All-Solid-State Sodium Batteries: Progress and Perspectives30Multiscale structural engineering and electrochemical optimization of amorphous nanomaterials for advanced rechargeable batteries7Redox‐Active Halide Catholytes for Solid‐State Lithium Batteries4Halide solid electrolytes: composition tuning, structural design, and performance optimization for all-solid-state lithium batteries18Origin of Optimal Composition and Density for Li-Ion Diffusion in Amorphous Li–P–S Electrolytes3Crystalline-to-amorphous MOFs filler-modified polymer composite electrolytes enable high-performance solid-state Li-metal batteries4Synergistic Modulation of HOMO Energy Level and Electronic Structure in Phthalates Anodes Active Materials Enables High‐Performance of Li‐Ion Batteries4Fluorinated Halide Solid Electrolytes for High-Voltage All-Solid-State Sodium-Ion Batteries Enabling Reversible Oxygen Redox8Boosting ionic conductivity of fluoride electrolytes by polyanion coordination chemistry enabling 5 V-Class all-solid-state batteries13Aluminum chloride-based catholytes for stable high-voltage solid-state sodium batteries1Interface Engineering in Solid‐State Sodium Batteries: Advances in Materials Design, Interfacial Strategies, and Multiscale Characterization15Data and Physics-Informed Neural Network for Predicting Electrode Materials of Lithium-Ion Battery0Fluoridation-induced structural evolution and electrochemical performance on Zr-based halide solid electrolytes for high-voltage Li batteries1Halide solid-state electrolytes: structures, properties, anodic interfacial challenges and modification strategies0Navigating interfaces in solid-state sodium batteries: challenges, solutions, and future directions4Progress and Challenges of Solid Electrolytes for High-Performance Sodium Ion Batteries5Recent progress and perspectives of lithium-rich manganese-based cathodes for high-energy-density solid-state batteries0High Conductivity Zr-Rich Sodium Fluorochloride Catholytes for All Solid-State Sodium Batteries2Halide Electrolytes for All‐Solid‐State Sodium Batteries: From Fundamental Chemistry to Interface Engineering10Low-dimensional ruddlesden-popper anti-perovskites: a promising platform for flexible and high-performance solid-state batteries0Sodium halide solid electrolytes for all-solid-state sodium batteries: advances, challenges, strategies, and prospects3High‐Entropy Tailored UCl 3 ‐Type Halides With Enhanced Ionic Conduction and Stability for All‐Solid‐State Sodium Batteries0High‐Entropy Tailored UCl 3 ‐Type Halides With Enhanced Ionic Conduction and Stability for All‐Solid‐State Sodium Batteries0Amorphous Halide Solid-State Electrolytes: Synthesis Strategies, Ion Transport Mechanisms, and Application Progress0Ordered–Disordered Ionic Cocrystalline Solid-State Electrolytes for Rapid Ion Migration in Sodium Metal Batteries3Disorder and entropy engineering in solid-state electrolytes for fast Li⁺ and Na⁺ transport1Towards high-performance halide electrolytes: Data-driven approaches for materials design and synthesis2Bulk Na+ Transport and Interfacial Stability in Inorganic Solid Electrolytes for All-Solid-State Sodium-Metal Batteries2Chloride‐Regulated Depolymerization of Aluminosilicate Networks for Fast Ion Transport Compliant Interfaces in Sustainable All‐Solid‐State Sodium Batteries0Chloride‐Regulated Depolymerization of Aluminosilicate Networks for Fast Ion Transport Compliant Interfaces in Sustainable All‐Solid‐State Sodium Batteries0New High‐Entropy Zirconium‐Based Solid‐State Electrolyte: Balancing High Conductivity and High Voltage0Spatial Ion-Gradient Solid Polymer Electrolytes for Stable Solid-State Sodium Batteries0Halide Solid‐State Electrolytes for all‐Solid‐State Lithium Batteries: Structure, Transport, Interface Relationships and Design Principles0Dual Oxygen Precursors Boosting the Ionic Conductivity of Glassy Electrolytes for All‐Solid‐State Sodium Batteries1Solid Additive Engineering Breaks the Stability‐Conductivity Trade‐Off in Halide Electrolytes for Robust All‐Solid‐State Batteries0Solid Additive Engineering Breaks the Stability‐Conductivity Trade‐Off in Halide Electrolytes for Robust All‐Solid‐State Batteries0Sulfur-Enabled Structural Amorphization and Operando Interfacial Densification in Halide-Based Solid Electrolytes for Long-Lasting All-Solid-State Sodium Batteries0Synergistic dual-ion engineering strategy enhances ion transport and high-voltage stability for halide solid-state electrolytes0Anion-cation co-doping enhances the interfacial stability of halide electrolytes for high-voltage all-solid-state lithium batteries0

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  2. Heterovalent doping of amorphous oxyhalide solid electrolytes for high-performance all-solid-state lithium batteries

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  3. Zr‐Doping Induced Complete Amorphization toward Highly Stable All‐Solid‐State Sodium Batteries

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  4. Advancing layered double hydroxides (LDHs) as the anodes for efficient anion-exchange-membrane water electrolyzers

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  5. Entropy‐Driven Electrolytes for Sodium‐Ion Batteries: From Liquid to Solid‐State Systems

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  6. An Oxychloride Solid Electrolyte with Superior Na-Ion Conductivity

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  7. Vacancy-mediated LaCl3-based superionic conductors for all-solid-state sodium batteries

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  8. Halide Solid-State Electrolytes for All-Solid-State Sodium Batteries: Progress and Perspectives

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  9. Multiscale structural engineering and electrochemical optimization of amorphous nanomaterials for advanced rechargeable batteries

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  10. Redox‐Active Halide Catholytes for Solid‐State Lithium Batteries

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  11. Halide solid electrolytes: composition tuning, structural design, and performance optimization for all-solid-state lithium batteries

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  12. Origin of Optimal Composition and Density for Li-Ion Diffusion in Amorphous Li–P–S Electrolytes

    Advanced Energy Materials · 2025-11-21

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  13. Crystalline-to-amorphous MOFs filler-modified polymer composite electrolytes enable high-performance solid-state Li-metal batteries

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  14. Synergistic Modulation of HOMO Energy Level and Electronic Structure in Phthalates Anodes Active Materials Enables High‐Performance of Li‐Ion Batteries

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  15. Fluorinated Halide Solid Electrolytes for High-Voltage All-Solid-State Sodium-Ion Batteries Enabling Reversible Oxygen Redox

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  16. Boosting ionic conductivity of fluoride electrolytes by polyanion coordination chemistry enabling 5 V-Class all-solid-state batteries

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  17. Aluminum chloride-based catholytes for stable high-voltage solid-state sodium batteries

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  18. Interface Engineering in Solid‐State Sodium Batteries: Advances in Materials Design, Interfacial Strategies, and Multiscale Characterization

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  19. Data and Physics-Informed Neural Network for Predicting Electrode Materials of Lithium-Ion Battery

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  20. Fluoridation-induced structural evolution and electrochemical performance on Zr-based halide solid electrolytes for high-voltage Li batteries

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  24. Recent progress and perspectives of lithium-rich manganese-based cathodes for high-energy-density solid-state batteries

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  25. High Conductivity Zr-Rich Sodium Fluorochloride Catholytes for All Solid-State Sodium Batteries

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  27. Low-dimensional ruddlesden-popper anti-perovskites: a promising platform for flexible and high-performance solid-state batteries

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  29. High‐Entropy Tailored UCl 3 ‐Type Halides With Enhanced Ionic Conduction and Stability for All‐Solid‐State Sodium Batteries

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  32. Ordered–Disordered Ionic Cocrystalline Solid-State Electrolytes for Rapid Ion Migration in Sodium Metal Batteries

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  40. Halide Solid‐State Electrolytes for all‐Solid‐State Lithium Batteries: Structure, Transport, Interface Relationships and Design Principles

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  41. Dual Oxygen Precursors Boosting the Ionic Conductivity of Glassy Electrolytes for All‐Solid‐State Sodium Batteries

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  42. Solid Additive Engineering Breaks the Stability‐Conductivity Trade‐Off in Halide Electrolytes for Robust All‐Solid‐State Batteries

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  43. Solid Additive Engineering Breaks the Stability‐Conductivity Trade‐Off in Halide Electrolytes for Robust All‐Solid‐State Batteries

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  44. Sulfur-Enabled Structural Amorphization and Operando Interfacial Densification in Halide-Based Solid Electrolytes for Long-Lasting All-Solid-State Sodium Batteries

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