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RESEARCH PAPER · Journal of the American Chemical Society · 2024

Dimensional Regulation from 1D/3D to 2D/3D of Perovskite Interfaces for Stable Inverted Perovskite Solar Cells

Ting Wang, Leyu Bi, Yang Liu, Zixin Zeng, Xiaofei Ji, Ziyang Hu, Sai‐Wing Tsang, Hin‐Lap Yip, Qiang Fu, Alex K.‐Y. Jen, Yongsheng Liu

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Dimensional Regulation from 1D/3D to 2D/3D of Perovskite Interfaces for Stable Inverted Perovskite Solar CellsOriginalAir-fabricated CsPbIBr 2 perovskite film for efficient and stable solar cells by a triacetyl resveratrol additive3Interface passivation strategies for high-performance perovskite solar cells using two-dimensional perovskites32Multifunctional Buffer Layer Engineering for Efficient and Stable Wide‐Bandgap Perovskite and Perovskite/Silicon Tandem Solar Cells42Multifunctional Buffer Layer Engineering for Efficient and Stable Wide‐Bandgap Perovskite and Perovskite/Silicon Tandem Solar Cells7Unprecedented Richness of Temperature‐ and Pressure‐Induced Polymorphism in 1D Lead Iodide Perovskite10Anions Regulation of 1D Perovskite Intrusion-Behavior for Efficient and Stable Perovskite Solar Cells15Recent development in solid additives enables high-performance organic solar cells65Non‐Fullerene Organic Electron Transport Materials toward Stable and Efficient Inverted Perovskite Photovoltaics31Methods for Passivating Defects of Perovskite for Inverted Perovskite Solar Cells and Modules213From Chalcogen Bonding to S–π Interactions in Hybrid Perovskite Photovoltaics14Minimizing Interfacial Energy Loss and Volatilization of Formamidinium via Polymer‐Assisted D–A supramolecular Self‐Assembly Interface for Inverted Perovskite Solar Cells with 25.78% Efficiency50Ionic liquid engineering enables 1D/3D perovskite photovoltaics with > 25 % efficiency: A real-time study exploring formation mechanism of 1D perovskites13Imidazole derivative spacers functional-group-induced regulation of interfacial recrystallization and defect passivation ability for high-performance perovskite solar cells7Perovskite solar cells: Organic-based molecules for electron and hole transport materials with machine learning insights11Bilayer interface engineering through 2D/3D perovskite and surface dipole for inverted perovskite solar modules115Enhancing perovskite solar cell efficiency to 28.17% by Integrating Dion-Jacobson 2D and 3D phase perovskite Absorbers18Regulating crystallization and retarding oxidation in Sn-Pb perovskite via 1D cation engineering for high performance all-perovskite tandem solar cells21Phenanthroline-Based Low-Cost and Efficient Small-Molecule Cathode Interfacial Layer Enables High-Performance Inverted Perovskite Solar Cells via Doctor-Blade Coating9Rational Engineering of Phase‐Pure 2D Perovskite Solar Cells20Surface Planarization‐Epitaxial Growth Enables Uniform 2D/3D Heterojunctions for Efficient and Stable Perovskite Solar Modules22Enhancing the Efficiency and Stability of Inverted Perovskite Solar Cells and Modules through Top Interface Modification with N‐type Semiconductors5Enhancing the Efficiency and Stability of Inverted Perovskite Solar Cells and Modules through Top Interface Modification with N‐type Semiconductors27Boosting Carrier Transport in Quasi‐2D/3D Perovskite Heterojunction for High‐Performance Perovskite/Organic Tandems66Sustainable Green Solvents for Lead Halide Perovskites14Suppressing non-radiative recombination for efficient and stable perovskite solar cells235Effect of 2D layer preparation on the performance of 2D/3D heterojunction perovskite solar cells1Resolving interfacial challenges in perovskite solar cells: From defect control to energy band optimization33Lock FA/MA Cations by Constructing Multiple Hydrogen Bonds for Efficient and Stable 2D/3D Perovskite Solar Cells16MAPbI3 perovskite inverted solar cell with bottom interface defects passivation via 2-thiophenemethylammonium bromide9A Systematic Analysis of The Current 2D Perovskite Engineering Approach and Future Prospects0Anti-solvent engineering for efficient and stable perovskite solar cells with preferentially orientated 2-dimensional/3-dimensional heterojunctions32Decoding recombination dynamics in perovskite solar cells: an in-depth critical review76Efficiently screening organic ligands by machine learning for stabilizing 2D/3D perovskites5Faceted Growth of 1D Perovskite Layers via Ionic Liquid Control for Efficient and Stable Inverted Perovskite Solar Cells0Molecular interactions and excited-state dynamics in MA free efficient and stable 2D/3D perovskite solar cells3Synchronous dimension-crystallization engineering enables highly efficient 2D/3D tin perovskite solar cells43Tailored Multisite Rigid Conjugated Molecules to Anchor Perovskite for Comprehensive Management of Perovskite Crystallization and Defects15DMSO‐Assisted Control Enables Highly Efficient 2D/3D Hybrid Perovskite Solar Cells13Rationally designed universal passivator for high-performance single-junction and tandem perovskite solar cells82Stable and Efficient Perovskite Photovoltaics via a Three‐In‐One Passivating Approach by Aminoacetonitrile Hydrochloride16Self-Assembled Monolayer Materials with Multifunction for Antimony Selenosulfide Solar Cells5Multi‐Functional Interface Engineering for Monolithic Perovskite/Perovskite/Crystalline Silicon Triple‐Junction Tandem Solar Cells10Pushing the certified efficiency of inverted perovskite solar cells beyond 24 %: A review16Alkyl Fluorination Aromatic Acetamidine Cation Enhances the Lattice Stability and Performance of 2D Ruddlesden‐Popper Perovskite Solar Cells7Recent Advances in the Development of Efficient Tin Halide Perovskite Solar Cells: Interface Engineering, Crystallization Kinetics, and Stability Optimization5A Soft Nonpolar‐Soluble Two‐Dimensional Perovskite for General Construction of Mixed‐Dimensional Heterojunctions8Fully Conjugated Co‐Self‐Assembled Monolayers for Efficient and Stable Inverted Perovskite Solar Cells28A 2D/3D Heterostructure Perovskite Solar Cell with a Phase‐Pure and Pristine 2D Layer39Triphenylamine-Based Hole-Transporting Ligands for 2D/3D FAPbI3 Perovskite Solar Cells29How to Make Over 25% Efficient Perovskite Solar Cells1Photogenerated Holes Induced Deep Sodium Storage of TiO 2 /CdSe/NFPP Cathode for High‐Efficiency Photorechargeable Sodium Batteries2Photogenerated Holes Induced Deep Sodium Storage of TiO 2 /CdSe/NFPP Cathode for High‐Efficiency Photorechargeable Sodium Batteries16Bilayer interfacial engineering with PEAI/OAI for synergistic defect passivation in high-performance perovskite solar cells14Synergistic Effect of Cation and Anion Passivation Defects and Suppression of Phase Transition Enhance the Performance and Stability of Inverted Perovskite Solar Cells9Unraveling the thermodynamic origins and kinetic pathways of intermediate phase engineering in perovskite solar cells11Rational design of methylthio-based self-assembled molecule for buried interface engineering in perovskite solar cells16Perovskite solar modules with high efficiency exceeding 20%: From laboratory to industrial community45Surface Impurity Healing by the Formation of 1D/3D Perovskite Heterojunctions for Inverted Perovskite Solar Cells6Molecular Engineering of Terminus, Conjugation, and Energetics for Thermally Stable Inverted Perovskite Solar Cells18Molecular‐Perspective Insights into Top Interface Passivation in Inverted Perovskite Solar Cells11Regulating perovskite crystallization via tailoring chemical interactions for printing high-efficiency 30 cm × 30 cm solar modules6Multi-Step Spin-Coating with In Situ Crystallization for Growing 2D/3D Perovskite Films1Benzylhydrazinium Chloride Interface Engineering Boosts Performance of Wide‐Bandgap Perovskite and Tandem Solar Cells2Fully-ambient-air processed perovskite solar cells with 24.38 % efficiency through passivation at buried interface by multifunctional molecule5Multidimensional Perovskite Solar Cells: What's Next after 3D/2D?12Core Extended Conjugation in Thiophene‐Based Cations Enables Open‐Circuit Voltage Improvement in Inverted Perovskite Solar Cells2Deprotonation‐Resistant Bimolecular Passivation Strategy for 26% Efficient and Stable Inverted Perovskite Solar Cells5Minimizing interfacial energy losses via multifunctional cage-like diammonium molecules for efficient perovskite/silicon tandem solar cells23Upper Interface Engineering Between Perovskite and Electron Transport Layer Toward Efficient and Stable Inverted Perovskite Solar Cells33In Situ Polymerization‐Assisted Crystallization of Open‐Air Blade‐Coated Perovskite Films for Efficient Solar Cells and Mini‐Modules1In Situ Polymerization‐Assisted Crystallization of Open‐Air Blade‐Coated Perovskite Films for Efficient Solar Cells and Mini‐Modules6Direct versus indirect 2D/3D heterojunction engineering: Ordered interface design for ultastable perovskite solar cells2Universal 3D/2D Surface Heterojunction‐Based Piperidine Derivatives for Efficient Inverted Perovskite Solar Cells14Dimensionality engineering of perovskites for stable heterojunction-based photovoltaics30Perovskite materials for multifaceted energy applications: From fundamental properties to industrialization challenges4Nanoscale soft interaction-engineered perovskite heterojunctions for highly efficient and reproducible solar cells11Stability of Tin–Lead Mixed Perovskite Solar Cells: Challenges, Strategies, and Future Prospects0Biological Zwitterion Betaine‐Assisted Wide Voltage Window and Freeze‐Resistance Hydrogel Electrolyte for Flexible Supercapacitor1Solvated-intermediate-driven surface transformation of lead halide perovskites46Turning off 2D reconstruction with a sulfone-modified passivator for efficient and stable inverted perovskite solar cells0Chiral ligand-assisted interface modulation for reduced voltage loss in perovskite solar cells10D perovskite directing oriented crystallization toward high-performance perovskite solar cells and modules0A synergistic molecular lock strategy enables efficient and durable wide bandgap perovskite/TOPCon tandem solar cells1Bifacial carbodithioate-lead chelating for efficient and robust inverted perovskite solar cells27Interfacial Regulation Strategy of 2D/3D Heterojunction Perovskite for Efficient Inverted Solar Cells0Synergistic regulation of crystallization and the buried interface in Cs x FA 1− x PbI 3 perovskite photovoltaics using a multifunctional sulfonyl–ammonium additive3Multifunctional Thiazolidine Derivatives Synergistic Regulation of Charge Transport Interface for Inverted Perovskite Solar Cells5Multivalent ligands regulate dimensional engineering for inverted perovskite solar modules29Meso ‐Crowned Porphyrin as a Dual Cavity Hybrid Macrocycle for Improving the Efficiency and Stability of Perovskite Solar Cells9Faceted growth of 1D perovskite layers via ionic liquid control for efficient and stable inverted perovskite solar cells2Dynamic Iodide Regeneration Enabled by Piperazine‐Tailored PCBM Interfaces for Photothermally Stable and Efficient Inverted Perovskite Photovoltaics4Dynamic Iodide Regeneration Enabled by Piperazine‐Tailored PCBM Interfaces for Photothermally Stable and Efficient Inverted Perovskite Photovoltaics2In Situ Postsynthesis of 2D/3D Bilayer Structured All-Inorganic Perovskites: Elucidating the Cation Exchange Mechanism0Construction of 2D-3D Halide Perovskite Heterojunctions with the Amine Vapor Replacement Reaction0Recent Advances in Interface Engineering to Stabilize Formamidinium‐Based Perovskite Solar Cells3Imide‐Based Molecular Passivation Enables Efficient Wide‐Bandgap Perovskite and Perovskite/Silicon Tandem Solar Cells8Gemini quaternary ammonium salt-enabled efficient interface and bulk engineering for inverted perovskite solar cells1Controlling Top‐Interface Reconstruction in Perovskite Solar Cells via Molecular Design of Dual‐Functional Ammonium Salts4Dimensional control of low-dimensional perovskite hybrids for photovoltaics6Interfacial Energetics Reconstruction via Bridging Engineering for Efficient Inverted Perovskite Solar Cells and Modules7Interfacial Energetics Reconstruction via Bridging Engineering for Efficient Inverted Perovskite Solar Cells and Modules1Mechanism study on performance enhancement of inverted perovskite solar cells via 5-nitro-2-(3-pyridyl)benzimidazole molecular interface modification0Ambient-compatible precursor engineering for efficient perovskite photovoltaics3Synergistic enhancement of defect passivation and energy-level alignment via fluorine-substitution driven coordination engineering for high-performance inverted perovskite solar cells1Recent progress in enhancing built-in electric fields of perovskite solar cells via junction engineering1Designed Lewis Acid–Base Passivation for High Performance Perovskite Solar Cells1High-performance flexible 2D perovskite solar cells with novel spacer cation0Integrated bulk-interface defect management via grain-boundary-mediated 2D reconstruction enables durable 2D/3D perovskite solar cells1A unified ligand-dimensional design to halt cation migration in perovskite photovoltaics0Thermodynamically Matched Molten‐Salt‐Assisted Phase Engineering of 2D/3D Perovskite Heterostructures for Efficient and Stable Solar Cells0Thermally Independent Interfacial Reconstruction for Phase‐Pure n = 1 2D Perovskites With Mixed‐Orientation Surface Architecture0Modification with simple molecular 4-tert-butylbenzenethiol for high-performance antimony sulfide indoor photovoltaics0Modulating p–n transition of two-dimensional perovskites for efficient and stable perovskite/Si tandem photovoltaics0Crystallization Modulation for Stable Wide‐Bandgap Perovskite Solar Cells and Modules1Modulation on energy band bending for balanced charge transport in high-efficiency perovskite solar cells0Mixed-Ligand-Driven Phase-Pure 2D Perovskite for Interfacial Passivation of Perovskite Photovoltaics0Lead carboxylates passivation for metre-scale perovskite solar modules2Polyfluorinated‐Regulator‐Assisted Scaffold‐Directed Tilted 1D/3D Heterointerfaces for High‐Voltage and Stable Perovskite Solar Cells0Polyfluorinated‐Regulator‐Assisted Scaffold‐Directed Tilted 1D/3D Heterointerfaces for High‐Voltage and Stable Perovskite Solar Cells0All-Perovskite Low-Dimensional/Quantum Dot Heterojunctions for Long-Term Efficient Quantum Dot Solar Cells0Air‐Processed Perovskite/Silicon Tandem Solar Cells via Iodide Oxidation Suppression0Atomic-level interface engineering for optoelectronic devices: structure–property relationships and multi-mechanism synergy0Performance enhancement of perovskite solar cells for energy storage applications: Materials and device engineering0Noncovalently functionalized conjugated polymers with conjugation-headed poly(ethylene glycol) as efficient hole-transport materials for nanocrystal photovoltaics0Regioisomer‐Induced In Situ Construction of 1D/3D Perovskite Heterojunctions for Efficient and Stable Solar Cells0Active acylation-induced ionic reconstruction enables efficient and stable oxidation of Spiro-OMeTAD0Compact Multifunctional Cation Regulating 1D/3D Heterointerface for High‐Performance Inverted Perovskite Solar Cells0Compatibility of Low‐Dimensional Perovskites in n–i–p and p–i–n Perovskite Solar Cells0Phase‐Pure 2D/3D Perovskite Heterojunctions Enabled by n ‐Specific Nanocrystal Templates for High‐Efficiency and Stable Solar Cells0

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  18. Phenanthroline-Based Low-Cost and Efficient Small-Molecule Cathode Interfacial Layer Enables High-Performance Inverted Perovskite Solar Cells via Doctor-Blade Coating

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  27. Resolving interfacial challenges in perovskite solar cells: From defect control to energy band optimization

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  28. Lock FA/MA Cations by Constructing Multiple Hydrogen Bonds for Efficient and Stable 2D/3D Perovskite Solar Cells

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  29. MAPbI3 perovskite inverted solar cell with bottom interface defects passivation via 2-thiophenemethylammonium bromide

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  33. Efficiently screening organic ligands by machine learning for stabilizing 2D/3D perovskites

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  35. Molecular interactions and excited-state dynamics in MA free efficient and stable 2D/3D perovskite solar cells

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  36. Synchronous dimension-crystallization engineering enables highly efficient 2D/3D tin perovskite solar cells

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  37. Tailored Multisite Rigid Conjugated Molecules to Anchor Perovskite for Comprehensive Management of Perovskite Crystallization and Defects

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  38. DMSO‐Assisted Control Enables Highly Efficient 2D/3D Hybrid Perovskite Solar Cells

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  39. Rationally designed universal passivator for high-performance single-junction and tandem perovskite solar cells

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  40. Stable and Efficient Perovskite Photovoltaics via a Three‐In‐One Passivating Approach by Aminoacetonitrile Hydrochloride

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