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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Enhanced Charge Transfer Process and Photocatalytic Activity over a Phosphonate‐based MOF via Amorphization Strategy

Honggang Zhang, Shaozhi Liu, Aili Zheng, Peng Wang, Zhaoke Zheng, Zeyan Wang, Hefeng Cheng, Ying Dai, Baibiao Huang, Yuanyuan Liu

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Enhanced Charge Transfer Process and Photocatalytic Activity over a Phosphonate‐based MOF via Amorphization StrategyOriginalAmorphous Strategy and Doping Copper on Metal-Organic Framework Surface for Enhanced Photocatalytic Co2 Reduction to C2h41In situ formation of a Co-MOF/Ti–Fe 2 O 3 photoanode for efficient photoelectrochemical water splitting9Metal–organic frameworks for organic transformations by photocatalysis and photothermal catalysis346Research progress on photocatalytic, electrocatalytic and photoelectrocatalytic selective oxidation of 5-hydroxymethylfurfural54Site-selective etching and conversion of bismuth-based Metal–Organic frameworks by oxyanions enables efficient and selective adsorption via robust coordination bonding12Optimal solutions and control strategies for photocatalytic conversion of toluene0Amorphous Strategy and Doping Copper on Metal–Organic Framework Surface for Enhanced Photocatalytic CO 2 Reduction to C 2 H 412Nano-photosensitizers with gallic acid-involved Fe–O–Cu “electronic storage station” bridging ligand-to-metal charge transfer for efficient catalytic theranostics19Rapid Hole Transfer and Molecular Enrichment at Amorphous‐Crystalline Interfaces of Pt0.25%/TO(B)‐FCP for Efficient Photocatalysis6Z‐Scheme Heterojunction of Hierarchical Cu 2 S/CdIn 2 S 4 Hollow Cubes to Boost Photoelectrochemical Performance30Enhancing Photoreduction of Cr(VI) through a Multivalent Manganese(II)-Organic Framework Incorporating Anthracene Moieties13Heterogeneous Nucleation and Enhanced Charge Transfer via Amorphous Metal‐Organic Frameworks for Efficient and Stable Perovskite Solar Cells28Disorder–order structure of a-CeO2/SnFe2O4 heterojunction with enhanced exciton dissociation for the NIR-driven photocatalysis13Interfacial modification of CuO/Ga2O3 by plasmonic Pt for high performance self-powered solar-blind UV photodetector10Photocatalytic Upcycling of Plastic Waste into Syngas by ZnS/Ga 2 O 3 Z‐Scheme Heterojunction15Crystal facet regulation enhances the photocatalytic performance for gaseous toluene degradation in BiOCl by promoting the activation of the methyl C(sp3)-H bond10Identifying and tuning coordinated water molecules for efficient electrocatalytic water oxidation16Controlled Phase and Structure Reconfiguration-Driven Anomalous Dielectric Behavior Enables Tailored Electromagnetic Attenuation0Coordination-driven assembly of a ferrocene-functionalized lead iodide framework with enhanced stability and charge transfer for photocatalytic CO 2 -to-CH 3 OH conversion5Lattice interconversion of 1D ferrocene-based perovskite induced by solvent molecules for selective photocatalytic toluene oxidation3High‐Performance Overall Water Splitting Dominated by Direct Ligand‐to‐Cluster Photoexcitation in Metal–Organic Frameworks1High‐Performance Overall Water Splitting Dominated by Direct Ligand‐to‐Cluster Photoexcitation in Metal–Organic Frameworks16Enhanced Selectivity of Photocatalytic CO2 Reduction to Formate via Tailoring the Metal Site43Selective heterogeneous photocatalytic activation for toluene oxidation: recent advances, challenges and perspective7Boosting Photocatalytic CO2 Cycloaddition with Epoxide over Facet-Dependent Cu2O@Cu3(HHTP)2 Heterojunctions2Breaking the crystalline barrier: Amorphous nanomaterials in advanced photocatalysis19Amorphous CuCoOx Boosts Active Hydrogen for High‐Rate Tandem Electroreduction of Nitrate to Ammonia10Making Photoresponsive Metal–Organic Frameworks an Effective Class of Heterogeneous Photocatalyst29Dual Z-scheme black phosphorus quantum dots (BPQDs)/ Cu2O crystalline/amorphous Ti, Fe-layered double hydroxides (LDH) heterojunction construction with enhanced electron transfer property for photocatalytic nitrogen fixation13The Cu─O─Co Asymmetric Bimetallic Sites Constructed by Ion‐Exchange for Efficient Oxygen Evolution Reaction28Dual‐Fluorinated Ni Single Atom Catalyst for Efficient Artificial Photosynthetic Diluted CO 2 Reduction22Constructing Matching Interfaces by Amorphous Engineering for Enhanced Lithium Ion Transport in Quasi‐Solid‐State Lithium–Iodine Batteries4Constructing Matching Interfaces by Amorphous Engineering for Enhanced Lithium Ion Transport in Quasi‐Solid‐State Lithium–Iodine Batteries25Tuning Bismuth Metal–Organic Framework Topology for Enhanced Photocatalytic NO Oxidation3Copper(I)-Based Coordination Polymers for Photocatalytic Benzylic C(sp 3 )–H-Oxidation via Energy Transfer5Modulating Order–Disorder Structures in Covalent Organic Frameworks for Photocatalytic CO2 Reduction to Propylene4Amorphous Metal–Organic Framework-Coated Halloysite Nanotubes as Efficient Sulfur Immobilizers for Lithium–Sulfur Batteries4Engineering Crystalline/Amorphous Interfaces for Enhanced CO 2 Electroreduction22Engineering Crystalline/Amorphous Interfaces for Enhanced CO 2 Electroreduction3Turning Defects Into Advantages: Structures, Synthesis, and Applications of 2D Amorphous Carbon12Amorphous metal-organic frameworks: From synthesis strategies to emerging applications16Interfacial Bi–O Bridge Elevated Bi p -Band Center Boosting Photocatalytic C( sp 3 )–H Bonds Oxidation40New Strategy for Cluster‐Based Covalent Organic Framework: Thermally Induced Covalent Crosslinking of Highly Stable Copper Clusters6g‐C 3 N 4 ‐Mediated Synthesis of Ru Crystalline/Amorphous Heterostructures on N‐Doped Carbon for Efficient and Chloride‐Resistant Alkaline HER13Integrated deep eutectic solvent with amorphous metal–organic framework for highly sensitive electrochemical determination of dicofol in milk and water14Spatially Separated Molecular Activation Over Dual Sites in Sn‐Doped ZnGa 2 O 4 /SnO 2 Photocatalysts Toward Complete VOCs Mineralization13Single-Particle Imaging Reveals Charge Redistribution on TiO 2 : Engineering Facets and Oxygen Vacancies for Photocatalytic Toluene Oxidation9Amorphous UiO-66-NH2 for next-generation interface engineering in perovskite solar cells5One Doping, Dual Amplification: A Spin State‐Charge Transfer Feedback in B‐Doped FeMOF for Synergistically Enhancing Both N 2 Activation and Its Conversion to Ammonia4Electron-Rich Macrocycle-Based Metal–Organic Frameworks for Efficient Photocatalytic CO 2 Reduction45Pathway modulation via directional radical regulation in Ov-rich Bi/BiOClBr solid solutions for enhanced photocatalytic mineralization of toluene5Voltage Regulation of Conjugated Coordination Polymer Electrodes via 3d Orbital Electron Control in Metal Ions4Sunlight Broad Spectrum-Capturing Nanophotofertilizer for Plant Growth Multiregulation and Second Near-Infrared Imaging7Orbital Hybridized MoO3/MoSe2 Heterojunction for Dual-Driven Interfacial Reaction and Charge Transfer Toward Enhanced Electrochemical Response12Directional Electron Transfer in Porphyrin‐Based Heteroleptic Metallacages for Enhanced Visible Light‐Driven Photocatalysis14The transformation of a bimetal carboxylate-MOF into a phosphonate-based MOF as a multifunctional photocatalyst4Controlled phase and structure engineering-driven unique dielectric behavior enabling tailored electromagnetic attenuation18Metal phosphonate frameworks as optical sensors0Ultralong Metal–Organic Framework Nanowires with Accelerated Reconstruction for Enhanced Oxygen Evolution Reaction3Ultrafast Adsorption of Strontium over β-Alanine-Coordinated 2D Derivatives of Amorphous ZIF-672Research Progress of Metal–Organic Radical Materials and Applications0Dynamic structural transformation of Ce-based bimetallic MOFs via kinetic trapping for enhanced pesticide residue sensing0Ligand-defect engineered amorphous MOFs via glycerol-assisted synthesis for efficient photo-Fenton degradation of fluoroquinolone antibiotics at neutral pH1Boosting Stabilized Pickering Emulsion via Janus Materials for Efficient Interfacial Photoreforming Hydrogen Evolution1Guest-Regulated Charge Separation in a Porphyrin Metallacage for Visible-Light Photocatalytic Oxidative Cyclization1Sulfur-induced deep reconstruction of nickel-cobalt-iron Prussian blue analogues for efficient 5-hydroxymethylfurfural electrooxidation0Tuning the Disordered Structure: Recent Advances in Amorphization Engineering for Enhanced Photocatalysis3Intrinsically Stable Amorphous Phases Unlock Sustainable Potassium Anodes0High-performance photocatalytic antibacterial technology: innovations, challenges, and future directions0An Oxygen‐Defect‐Induced Unsaturated Coordination Strategy Boosts High‐Selective PET Upcycling via Suppressing Oxygen Evolution1Utilizing Amorphous/Crystalline Interfaces in Bismuth Nanoparticles to Boost Hydrogen Peroxide Electrosynthesis0Prolonging the Triplet Excited‐State Lifetime via Tandem Through‐Space Conjugation in Tetracationic Cyclophanes for Efficient Metal‐Free Photoredox Catalysis1Engineering Metal-to-Metal Charge Transfer in Bimetallic CoFe-MOF-74 for Efficient Solar-Driven Photocatalytic Nitrogen Fixation0Unveiling Active Sites and Charge Carrier Dynamics in Copper–Phosphonobenzoate Photohybrids for Efficient H 2 O 2 Generation0Artemisinin‐Directed Crystallization of an Iron‐Sulfasalazine Coordination Polymer for Acne Synergistic Phototherapy With Sustained Antibacterial and Pro‐Regenerative Effects0Zr-Oxo Cluster-Based Metal–Organic Framework for Selective C(sp3)–H Bond Photooxidation0Heterogeneous Photocatalytic Oxidation of Toluene to Benzaldehyde over Nickel Coordinated Metatungstate, [Ni(dmbpy)3]2H2[H2W12O40]0Amorphous ZnWO4/CuIn4S6.5 with Intrinsic Sulfur Vacancies: Urbach Tail-Modulated Anomalous Charge Transfer toward Efficient Photocatalytic H2 Evolution0Fabrication of Bi2WO6-x@MOF via surface engineering for efficient photocatalytic degradation of fluoroquinolone antibiotics0Rare-earth metal–organic framework-based luminescent sensors for environmental and food safety: Recent progress in pesticide detection0

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