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RESEARCH PAPER · Science · 2024

Superionic lithium transport via multiple coordination environments defined by two-anion packing

Guopeng Han, Andrij Vasylenko, Luke M. Daniels, Christopher M. Collins, Lucia Corti, Ruiyong Chen, Hongjun Niu, Troy D. Manning, Dmytro Antypov, Matthew Stephen Dyer, Jungwoo Lim, Marco Zanella, Manel Sonni, Mounib Bahri, Hongil Jo, Yun Dang, Craig M. Robertson, Frédéric Blanc, Laurence J. Hardwick, Nigel D. Browning, John B. Claridge, Matthew J. Rosseinsky

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Superionic lithium transport via multiple coordination environments defined by two-anion packingOriginalAccelerating metal–organic framework discovery via synthesisability prediction: the MFD evaluation method for one-class classification models3Kinetic coefficients of ion transport in a porous medium based on the Enskog–Landau kinetic equation1Theoretical calculations of the performance of Li 7 NbO 6 and its doped Phases as solid electrolytes2Strategies for Enhancing the Stability of Lithium Metal Anodes in Solid-State Electrolytes14Critical Role of Framework Flexibility and Disorder in Driving High Ionic Conductivity in LiNbOCl 478Enhancement of Low Temperature Superionic Conductivity by Suppression of Li Site Ordering in Li 7 Si 2–x Ge x S 7 I8Enhancement of Low Temperature Superionic Conductivity by Suppression of Li Site Ordering in Li7Si2–xGexS7I0Lithium-ion rapid transport mechanism and channel design in solid electrolytes1Synthetic Design of Dual Polar Side Chain Polymers for Enhancing Electrochromic Performance17Microwave-Assisted Synthesis of Argyrodite Solid Electrolytes and Their Use in Solid-State Batteries94 V Na Solid State Batteries Enabled by a Scalable Sodium Metal Oxyhalide Solid Electrolyte62Revealing the Local Structure and Dynamics of the Solid Li Ion Conductor Li3P5O1402024 roadmap for sustainable batteries34Toward high performance all-solid-state lithium or sodium metal batteries: Potential application on Li/Na-rich antiperovskites (LiRAPs/NaRAPs) electrolyte for energy storage13Exploration of Chemical Space Through Automated Reasoning3Exploration of Chemical Space Through Automated Reasoning3Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges53A facile route to plastic inorganic electrolytes for all-solid state batteries based on molecular design43Cross‐Linked Polyamide‐Integrated Argyrodite Li 6 PS 5 Cl for All‐Solid‐State Lithium Metal Batteries15Fast‐Charging Solid‐State Li Batteries: Materials, Strategies, and Prospects44Digital features of chemical elements extracted from local geometries in crystal structures2Machine-learning-aided screening of inorganic lithium solid-state electrolytes with a wide electrochemical window7Solid-state electrolytes expediting interface-compatible dual-conductive cathodes for all-solid-state batteries15Tuning the band gap and structure from wide gap SrBi 3 O 4 Cl 3 to narrow gap Bi 4 O 4 SeCl 2 by aliovalent anion substitution2Vacuum evaporation-assisted reaction: sustainable solution for application of rare earth-based halide solid-state electrolytes4Discovering a Novel Cyan‐Light‐Emitting Thiosilicate Phosphor, Li 2 BaSiS 4 :Eu 2+ , via Experimental Active Learning4Ductile Inorganic Solid Electrolytes for All-Solid-State Lithium Batteries164All‐Solid‐State Lithium Metal Batteries with Microdomain‐Regulated Polycationic Solid Electrolytes57Strategies Toward Stable Anode Interface for Sulfide‐Based All‐Solid‐State Lithium Metal Batteries13Li 21 Ge 8 P 3 S 34 : New Lithium Superionic Conductor with Unprecedented Structural Type0Li 21 Ge 8 P 3 S 34 : New Lithium Superionic Conductor with Unprecedented Structural Type4Discovery of Crystalline Inorganic Solids in the Digital Age4Unraveling the Complexity of Divalent Hydride Electrolytes in Solid‐State Batteries via a Data‐Driven Framework with Large Language Model38Unraveling the Complexity of Divalent Hydride Electrolytes in Solid‐State Batteries via a Data‐Driven Framework with Large Language Model0Halide Chemistry Boosts All‐Solid‐State Li‐S Batteries9Proton-driven lithium separation using alkali-templated coordination cages12Accelerated discovery of solid-state battery properties enabled by active learning approaches10Silicon-nanoparticle-embedded hard carbon as high-capacity anode for all-solid-state lithium batteries24Understanding solid-state battery electrolytes using atomistic modelling and machine learning105A consistent description of the kinetic processes of electrolyte ion transport in a dynamic porous medium1Unveiling the Kinetics of Ion Transport in 2D Potassium Niobate by Raman Spectroscopy0Topology Augmented with Geometry in the Assembly of Structural Databases: Kagome Intermetallics3Optimizing one-dimensional ion conduction and interface stability in PEO electrolytes with PAN-coated palygorskite fibers1Lithium Lanthanum Titanate (LLTO) Solid Electrolyte with High Ionic Conductivity and Excellent Mechanical Properties Prepared by Aerodynamic Levitation Rapid Solidification5Strategies and Prospects for the Design of Inorganic Ceramic Electrolyte for High-Performance All-Solid-State Lithium-Ion Batteries9Anion sublattice design enables superionic conductivity in crystalline oxyhalides93Direct Lithium Harvesting via Superionic Conductor Membranes2State-independent ionic conductivity8Electrochemical Performance and Stability of Li 7 Si 2 S 7 I Solid Electrolytes in Solid-State Battery Cathode Composites1Highly Compressible Fast-Ion Conducting Catholyte LixNbOxCl5-x for Stable Dual Electrolyte Solid-State Batteries0Highly Compressible Fast-Ion Conducting Catholyte LixNbOxCl5-x for Stable Dual Electrolyte Solid-State Batteries0Next-Generation Electrolytes for Solid-State Batteries0Superionic lithium mobility in low symmetry Li 7 Si 2 S 7 I polymorph accessed via Si 2 S 7 dimer reorientation0Dynamic Li‐S Coordination Boosted Superionic Conduction in Cubic LiBS 2 Solid Electrolyte0Computational Discovery of Li 6 PO 5 I: An Oxide Argyrodite for Solid-State Electrolytes3Continuous ionic conductivity across phase boundaries in organic electrolytes1Featured Papers in Inorganic Materials 20250Collective anion rotation enabled superionic conduction in cubic Li imide1Structural Design Principles for Minimal‐Volume‐Change Anodes in Next‐Generation Sulfide Solid‐State Batteries0Reticular Assembly of Complex Cage-within-Cage Merged-Net MOFs for Lithium-Ion Conductivity2A high-entropy multicationic substituted Li10GeP2S12 solid electrolyte enabling stable all-solid-state batteries2Navigating polymorph generation and distilled-potential development via entropy-symmetry landscapes for metal plasticity mechanisms0Towards high-performance halide electrolytes: Data-driven approaches for materials design and synthesis2Generalized machine-learning descriptor for identifying superionic materials0Phonon-Activated Collective Hopping in a Superionic Phase0Molecular-Ratchet Like Cation–Anion Coupling Dynamics Assist Ion Migration in Room Temperature Ionic Conductors0HCl‐Free Mechanochemical Synthesis of Lithium Niobium Oxychlorides0Lipoic Acid-Derived Interphase for Stable Lithium Metal Anodes in High-Performance Lithium Metal Batteries0Electrochemical and Spectroscopic Evaluation of Li7Si2S7I Solid Electrolyte in All-Solid-State Batteries0Discovering solid-state superionic conductors with low Li-ion concentration assisted by artificial intelligence0PEO-based electrolyte with coordination-entropy-increase strategy for all-solid-state lithium metal batteries0Unraveling Lithium Dynamics in Solid Electrolyte Interphase: From Graph Contrastive Learning to Transport Pathways0Screening Lithium-Ion Conductors Based on Local and Global Topology0

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  2. Kinetic coefficients of ion transport in a porous medium based on the Enskog–Landau kinetic equation

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  3. Theoretical calculations of the performance of Li 7 NbO 6 and its doped Phases as solid electrolytes

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    Shihao Feng, Zhixing Wang, Guoshang Zhang, Pengfei Yue, Wengao Pan, Qiongqiong Lu, Huajun Guo, Xinhai Li, Guochun Yan, Jiexi Wang

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  4. Strategies for Enhancing the Stability of Lithium Metal Anodes in Solid-State Electrolytes

    Micromachines · 2024-03-28

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  5. Critical Role of Framework Flexibility and Disorder in Driving High Ionic Conductivity in LiNbOCl 4

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  6. Enhancement of Low Temperature Superionic Conductivity by Suppression of Li Site Ordering in Li 7 Si 2–x Ge x S 7 I

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  7. Enhancement of Low Temperature Superionic Conductivity by Suppression of Li Site Ordering in Li7Si2–xGexS7I

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  8. Lithium-ion rapid transport mechanism and channel design in solid electrolytes

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  9. Synthetic Design of Dual Polar Side Chain Polymers for Enhancing Electrochromic Performance

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  10. Microwave-Assisted Synthesis of Argyrodite Solid Electrolytes and Their Use in Solid-State Batteries

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  11. 4 V Na Solid State Batteries Enabled by a Scalable Sodium Metal Oxyhalide Solid Electrolyte

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  12. Revealing the Local Structure and Dynamics of the Solid Li Ion Conductor Li3P5O14

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  13. 2024 roadmap for sustainable batteries

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  14. Toward high performance all-solid-state lithium or sodium metal batteries: Potential application on Li/Na-rich antiperovskites (LiRAPs/NaRAPs) electrolyte for energy storage

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  17. Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges

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  19. Cross‐Linked Polyamide‐Integrated Argyrodite Li 6 PS 5 Cl for All‐Solid‐State Lithium Metal Batteries

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  20. Fast‐Charging Solid‐State Li Batteries: Materials, Strategies, and Prospects

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  29. Strategies Toward Stable Anode Interface for Sulfide‐Based All‐Solid‐State Lithium Metal Batteries

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  30. Li 21 Ge 8 P 3 S 34 : New Lithium Superionic Conductor with Unprecedented Structural Type

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  43. Optimizing one-dimensional ion conduction and interface stability in PEO electrolytes with PAN-coated palygorskite fibers

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  47. Direct Lithium Harvesting via Superionic Conductor Membranes

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  48. State-independent ionic conductivity

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  49. Electrochemical Performance and Stability of Li 7 Si 2 S 7 I Solid Electrolytes in Solid-State Battery Cathode Composites

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  50. Highly Compressible Fast-Ion Conducting Catholyte LixNbOxCl5-x for Stable Dual Electrolyte Solid-State Batteries

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