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RESEARCH PAPER · Small · 2024

Supramolecular/Dynamic Covalent Design of High‐Performance Pressure‐Sensitive Adhesive from Natural Low‐Molecular‐Weight Compounds

Sha Luo, Na Wang, Yanjuan Pan, Bo Zheng, Fenfang Li, Shengyi Dong

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Supramolecular/Dynamic Covalent Design of High‐Performance Pressure‐Sensitive Adhesive from Natural Low‐Molecular‐Weight CompoundsOriginalAn organic/inorganic hybrid soft material for supramolecular adhesion2Supramolecular control over the variability of color and fluorescence in low-molecular-weight glass14One-pot molten strategy to synthesize tough bio-derived lignin-based photothermal elastomers for photoelectric driven and programmable shape memory21Reusable soy protein derivative as sustainable adhesive4Controllable structure, super adhesion, multifunctional, conductive pressure-sensitive adhesive for electronic skin: Enhancing cohesion by cellulose-derived covalent crosslinking28Synthesis of highly transparent and fast-responding photochromic coating by template method with space-limited domains11Polyisoprene grafted white carbon black reinforced polyisobutylene‐based pressure‐sensitive adhesives: Comprehensive enhancement of adhesive performances3Natural cellulose reinforced multifunctional eutectogels for wearable sensors and epidermal electrodes27Harnessing dynamic covalent chemistry in sustainable biomass-based polymers: Synthesis, dynamic functionalities and potential of dithiolane-containing supramolecular polymers42Molecular engineering of supramolecular polymer adhesive with confined water and a single crown ether6Adhesion and affinity of supramolecular adhesives on fluorinated surfaces12An eco-friendly adhesive with ultra-strong adhesive performance12Long-term humid adhesion of sulfur thermoplastic polymers enabled by thioctic acid-initiated polymerization3Poly(ionic liquid) glass with high stiffness and toughness facilitated by supramolecular interactions3Reviving recovered carbon black as a reinforcement for natural rubber by utilizing acylhydrazine-functionalized polysulfide as an intelligent interfacial modifier19Visualization of different morphologies of block copolymer assemblies using various fluorescent colors via the introduction of solvent-responsive AIEgen3Facile synthesis amide‐functional anionic chain extenders for enhanced thermal stability and emulsion performance in waterborne polyurethanes4Enhanced adhesion to low-surface-energy substrates using polyurethane acrylate/polyacrylate interpenetrating network pressure-sensitive adhesives10Untying the Knot: A Fully Recyclable, Solvent‐Free, Wide‐Spectral Photocurable Thermoset Adhesive31A soft polyurethane foam adhesive with ultra-high and stable adhesion based on chemical coupling and mechanical interlocking8Photochromic Adhesives from One-Step Deep Eutectic Polymerization of Heteropoly Acids and Cyclodextrin0Thioctic acid driven chemical cross-linking of cellulose chains for fabricating high-performance cellulose films as food packaging11Robust and Reversible Supramolecular Adhesive via Dynamic Covalent Bond Crosslinking‐Induced Assembly of Metal‐Coordinated Nanoparticles11Thioctic Acid‐Enabled Melt Processing of Cyclodextrin‐Based Polyrotaxane into Functional Supramolecular Networks for Adhesives and Sensors13Sustainable and robust hot melt adhesives via non-covalent cross-linking of arginine and short-chain fatty acids4Spider Silk-Inspired Adhesion–Cohesion Synergistic Enhancement Strategy: Competitive Hydrogen-Bonding-Induced Crystallization Phase Separation for High-Performance, Recyclable, and Multifunctional Biobased Adhesives10Reactive Janus‐ SiO 2 Reinforced Acrylic‐Polyisobutylene Semi‐Interpenetrating Pressure‐Sensitive Adhesive: The Combined Effect of Crosslinking and Entanglement0Weaving-inspired asymmetric entangled nodes in multi-component polymer networks26Supramolecular Materials from Natural Thioctic Acid: Reconfigurable Design and Functional Applications13Developing α-lipoic acid-derived solvent-free bioadhesives via deep eutectic melting0Antibacterial Poly(disulfide) Elastomer Featuring High Metal Adhesion and Closed-Loop Recyclability1Honey-inspired thermally hysteretic adhesives for high strength and reversible underwater adhesion9Interfacial adhesive materials and chemistry in extreme/complex environments0α-Lipoic acid: from a mitochondrial cofactor to a versatile platform for dynamic biomaterials and translational biomedicine0Stuck on Repeat: Dynamic Liquid Crystal Elastomers as (Re)trainable Adhesives3In-situ preparation of uniform AgNPs/PVDF membrane with excellent photocatalytic and antibacterial properties3Design of a Hot-Melt Adhesive with Microphase-Separated Architecture Enabled by Hydrogen-Bond Engineering for Robust and Reversible Adhesion3Recent Progress in α-Lipoic Acid (Thioctic Acid)-Enabled Adhesives: Dynamic Disulfide Networks for Wet Adhesion, Self-Healing, and Circular Reuse1Tackifiers Regulate Interfacial Kinetics and Bonding Energy in Glycidyl Methacrylate‐Grafted Polyolefin/Aluminum Composites: A Multiscale Experimental and MD Study0Biobased Biomimetic Adhesive with Underwater Adhesion, Remolding, Degradation, and Closed-Loop Recycling1Bottom‐Up Molecular Engineering of Natural Thioctic Acid into Dual‐Crosslinked Covalent Adaptable Networks for Multi‐Functional Sustainable Structural Adhesive0Supramolecular Elastomer Based Switchable Adhesives Regulated by Soft Confinement Induced Nano‐Rod Crystals0Adhesion as a Quality Attribute of Transdermal Therapeutic Systems: Analysis of Requirements and Evaluation Methods0

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  1. An organic/inorganic hybrid soft material for supramolecular adhesion

    Soft Matter · 2024-01-01

    Yunfei Zhang, Wenchang Yi, Jia Pan, Song Liu, Shengyi Dong

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  2. Supramolecular control over the variability of color and fluorescence in low-molecular-weight glass

    Materials Horizons · 2024-01-01

    Yunfei Zhang, Changyong Cai, Fenfang Li, Xin Tan, Qing Li, Xin‐Long Ni, Shengyi Dong

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  3. One-pot molten strategy to synthesize tough bio-derived lignin-based photothermal elastomers for photoelectric driven and programmable shape memory

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    Zhiwen Sun, Zhiwen Sun, Changyou Shao, Sanwei Hao, Jifei Zhang, Jiaxuan Zhu, Wenfeng Ren, Jun Yang, Jun Yang, Run‐Cang Sun

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  4. Reusable soy protein derivative as sustainable adhesive

    Matter · 2024-10-01

    Changyong Cai, Zhijian Tan, Shengyi Dong

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  5. Controllable structure, super adhesion, multifunctional, conductive pressure-sensitive adhesive for electronic skin: Enhancing cohesion by cellulose-derived covalent crosslinking

    Chemical Engineering Journal · 2024-10-12

    Ji Qi, Tong Luo, Juan Yu, Chunpeng Wang, Fuxiang Chu, Jifu Wang

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  6. Synthesis of highly transparent and fast-responding photochromic coating by template method with space-limited domains

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    Yuting Tian, Weining Liu, Jun Hu, Zhiwei Li, Xiaoying Xin, Guodong Fu

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  7. Polyisoprene grafted white carbon black reinforced polyisobutylene‐based pressure‐sensitive adhesives: Comprehensive enhancement of adhesive performances

    Polymer Composites · 2024-10-29

    Yuanyi Kang, Xingzhen Feng, Yue Zhao, Jiawei Fang, Lifei Shui, Meng Xin, Chuncheng Hao

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  8. Natural cellulose reinforced multifunctional eutectogels for wearable sensors and epidermal electrodes

    Carbohydrate Polymers · 2024-11-04

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  9. Harnessing dynamic covalent chemistry in sustainable biomass-based polymers: Synthesis, dynamic functionalities and potential of dithiolane-containing supramolecular polymers

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    Peng Tan, Wenxi Gu, Yiwei Zou, Xiao Song, Zehuan Huang, Ji Liu, Iek Man Lei

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  10. Molecular engineering of supramolecular polymer adhesive with confined water and a single crown ether

    Chemical Science · 2024-12-23

    Qiangqiang Xu, Paulina Szymoniak, Mohamed Aejaz Kolmangadi, Zerui Yang, S Q Wang, Yurui Gao, Jie Shang, Johannes Hunger, Aitkazy Kaisha, Abdurakhman U. Aldiyarov, Andreas Schönhals, Yan Ge, Zhenhui Qi

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  11. Adhesion and affinity of supramolecular adhesives on fluorinated surfaces

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  12. An eco-friendly adhesive with ultra-strong adhesive performance

    Polymer Chemistry · 2025-01-01

    Zhenyu Yang, Xiaoting Ji, Xin-Long Sha, Jincheng Ding, Lin Cheng, Guangfeng Li

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  13. Long-term humid adhesion of sulfur thermoplastic polymers enabled by thioctic acid-initiated polymerization

    Polymer Chemistry · 2025-01-01

    Tongye Zhang, Zhiyue Fang, Shifang Luan, Lei Wang, Hengchong Shi

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  14. Poly(ionic liquid) glass with high stiffness and toughness facilitated by supramolecular interactions

    Chemical Engineering Journal · 2025-01-01

    Qianwen Lu, Hengfeng Li, Changyong Cai, Zhijian Tan

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  15. Reviving recovered carbon black as a reinforcement for natural rubber by utilizing acylhydrazine-functionalized polysulfide as an intelligent interfacial modifier

    Polymer Chemistry · 2025-01-01

    Senmao Yu, Zhenghai Tang, Dong Wang, Siwu Wu, Fei Chen, Baochun Guo, Liqun Zhang

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  16. Visualization of different morphologies of block copolymer assemblies using various fluorescent colors via the introduction of solvent-responsive AIEgen

    Science China Chemistry · 2025-04-23

    Shaoyu Xu, Mian Wang, Hui Liu, Jinsa Li, Renhua Deng, Xiaofan Ji

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  17. Facile synthesis amide‐functional anionic chain extenders for enhanced thermal stability and emulsion performance in waterborne polyurethanes

    Polymer Engineering and Science · 2025-04-28

    Ismail Omrani, R. Kiani, Hengameh Honarkar

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  18. Enhanced adhesion to low-surface-energy substrates using polyurethane acrylate/polyacrylate interpenetrating network pressure-sensitive adhesives

    Progress in Organic Coatings · 2025-05-16

    Yafang Han, Ziyang Gong, Renjie Zhou, Weile Li, Jun You Shi, Jiwen Hu

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  19. Untying the Knot: A Fully Recyclable, Solvent‐Free, Wide‐Spectral Photocurable Thermoset Adhesive

    Advanced Materials · 2025-05-16

    Natanel Jarach, Michal Cohen, Rivka Gitt, Hanna Dodiuk, Samuel Kenig, Shlomo Magdassi

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  20. A soft polyurethane foam adhesive with ultra-high and stable adhesion based on chemical coupling and mechanical interlocking

    Colloids and Surfaces A Physicochemical and Engineering Aspects · 2025-05-29

    Shengping Dai, Jingping Yao, Longhua Zeng, Jinlong Shuai, Yan Zhong, Hongmei Chen, Cheng Liu, Wen‐Tong Chen, Yan Sui

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  21. Photochromic Adhesives from One-Step Deep Eutectic Polymerization of Heteropoly Acids and Cyclodextrin

    Industrial & Engineering Chemistry Research · 2025-06-09

    Yanjuan Pan, Sha Luo, Xing Li, Xin Tan, Shengyi Dong

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  22. Thioctic acid driven chemical cross-linking of cellulose chains for fabricating high-performance cellulose films as food packaging

    International Journal of Biological Macromolecules · 2025-06-18

    Youjie Gao, Guozhuo Chen, Chao Wu, Junjie Zhou, Guojun Jin, Hou–Yong Yu

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  23. Robust and Reversible Supramolecular Adhesive via Dynamic Covalent Bond Crosslinking‐Induced Assembly of Metal‐Coordinated Nanoparticles

    Advanced Science · 2025-07-30

    Yanyan Guo, Mengran Zhang, Shuanggen Wu, Xunqiu Wang

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  24. Thioctic Acid‐Enabled Melt Processing of Cyclodextrin‐Based Polyrotaxane into Functional Supramolecular Networks for Adhesives and Sensors

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  25. Sustainable and robust hot melt adhesives via non-covalent cross-linking of arginine and short-chain fatty acids

    Chemical Engineering Journal · 2025-10-04

    Yuebo Meng, Xue Wang, Jun Fang, Guang Wen, Xinyan Wang, Wen Li

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  26. Spider Silk-Inspired Adhesion–Cohesion Synergistic Enhancement Strategy: Competitive Hydrogen-Bonding-Induced Crystallization Phase Separation for High-Performance, Recyclable, and Multifunctional Biobased Adhesives

    ACS Sustainable Chemistry & Engineering · 2025-10-28

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  27. Reactive Janus‐ SiO 2 Reinforced Acrylic‐Polyisobutylene Semi‐Interpenetrating Pressure‐Sensitive Adhesive: The Combined Effect of Crosslinking and Entanglement

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  28. Weaving-inspired asymmetric entangled nodes in multi-component polymer networks

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  29. Supramolecular Materials from Natural Thioctic Acid: Reconfigurable Design and Functional Applications

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  30. Developing α-lipoic acid-derived solvent-free bioadhesives via deep eutectic melting

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  31. Antibacterial Poly(disulfide) Elastomer Featuring High Metal Adhesion and Closed-Loop Recyclability

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  32. Honey-inspired thermally hysteretic adhesives for high strength and reversible underwater adhesion

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  33. Interfacial adhesive materials and chemistry in extreme/complex environments

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  34. α-Lipoic acid: from a mitochondrial cofactor to a versatile platform for dynamic biomaterials and translational biomedicine

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  35. Stuck on Repeat: Dynamic Liquid Crystal Elastomers as (Re)trainable Adhesives

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  36. In-situ preparation of uniform AgNPs/PVDF membrane with excellent photocatalytic and antibacterial properties

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  37. Design of a Hot-Melt Adhesive with Microphase-Separated Architecture Enabled by Hydrogen-Bond Engineering for Robust and Reversible Adhesion

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  38. Recent Progress in α-Lipoic Acid (Thioctic Acid)-Enabled Adhesives: Dynamic Disulfide Networks for Wet Adhesion, Self-Healing, and Circular Reuse

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  39. Tackifiers Regulate Interfacial Kinetics and Bonding Energy in Glycidyl Methacrylate‐Grafted Polyolefin/Aluminum Composites: A Multiscale Experimental and MD Study

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  40. Biobased Biomimetic Adhesive with Underwater Adhesion, Remolding, Degradation, and Closed-Loop Recycling

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  41. Bottom‐Up Molecular Engineering of Natural Thioctic Acid into Dual‐Crosslinked Covalent Adaptable Networks for Multi‐Functional Sustainable Structural Adhesive

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  42. Supramolecular Elastomer Based Switchable Adhesives Regulated by Soft Confinement Induced Nano‐Rod Crystals

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  43. Adhesion as a Quality Attribute of Transdermal Therapeutic Systems: Analysis of Requirements and Evaluation Methods

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