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RESEARCH PAPER · Inorganic Chemistry · 2023

Millimeter-Sized K2MnF6:Si4+, NH4+ Red-Luminescent Crystals with High Absorption Efficiency (AEmax of 93.5%) and External Quantum Efficiency (EQEmax of 68.9%) Grown by Cooling-Induced Crystallization

Wenrui Zhang, Zhaowu Wang, Shiyu Jia, Yayun Zhou, Haipeng Ji

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Millimeter-Sized K2MnF6:Si4+, NH4+ Red-Luminescent Crystals with High Absorption Efficiency (AEmax of 93.5%) and External Quantum Efficiency (EQEmax of 68.9%) Grown by Cooling-Induced CrystallizationOriginalK 2 SiF 6 :Mn 4+ red-luminescent crystals with high external quantum efficiency (EQE max of 78%) and high thermal quenching temperature ( T 1/2 > 500 K) enabling high brightness warm white LEDs20Millimeter-scale Na2SiF6:Mn4+ red-emitting crystals with intense zero phonon line at 617 nm and enhanced hydrolysis resistance8(NH 4 ) 2 MnF 6 : a highly soluble, K + -free Mn 4+ precursor for red fluoride phosphors1Large-sized K2SiF6:Mn4+ phosphor crystals up to 3 mm by seeded growth with near-unity quantum efficiency0NH 4 + ‐Induced Formation of Hexagonal‐K 1.5 (NH 4 + ) 0.5 SiF 6 :Mn 4+ with Polarized Zero‐Phonon Line Emission5Mn⁴⁺-doping-induced structural transformation and luminescence enhancement in bulk (NH₄)₂SiF₆: Mn⁴⁺ crystal grown via cooling crystallization0K 2 SiF 6 :Mn 4+ Red Phosphor Crystals: Near-Unity Quantum Efficiency, Size-Modulated Thermal Quenching, and Cooling-Crystallization Engineering of Millimeter Sizes for Crystal-to-Die Packaging7Achieving 57.15% EQE in Mn 4+ non-equivalent doped fluoride single crystals via a rapid synthesis for next-generation display lighting2A layer-stacking structure enabling K 2 TiF 6 :Mn 4+ platelet crystals for inorganic high-power WLED packaging0Low-temperature crystallization of the K 2 TiF 6 :Mn 4+ phosphor with near-unity quantum efficiency in dilute HF solution1Large-sized K2SiF6:Mn4+ phosphor crystals up to 3 mm grown by seeded growth with near-unity quantum efficiency2

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  1. K 2 SiF 6 :Mn 4+ red-luminescent crystals with high external quantum efficiency (EQE max of 78%) and high thermal quenching temperature ( T 1/2 > 500 K) enabling high brightness warm white LEDs

    Journal of Materials Chemistry C · 2024-11-29

    Wenrui Zhang, Yayun Zhou, Ce Shi, Jiajun Ren, Liying Zhang, Haipeng Ji

    Read original paper ↗ ·

  2. Millimeter-scale Na2SiF6:Mn4+ red-emitting crystals with intense zero phonon line at 617 nm and enhanced hydrolysis resistance

    Ceramics International · 2024-12-16

    Lulu He, Mingxin Zhang, Xiaoliang Dong, Liying Zhang, Ce Shi, Haipeng Ji

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  3. (NH 4 ) 2 MnF 6 : a highly soluble, K + -free Mn 4+ precursor for red fluoride phosphors

    Journal of Materials Chemistry C · 2025-01-01

    Mengyao Wang, Wenrui Zhang, Liying Zhang, Haipeng Ji

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  4. Large-sized K2SiF6:Mn4+ phosphor crystals up to 3 mm by seeded growth with near-unity quantum efficiency

    SSRN Electronic Journal · 2025-01-01

    Mingxin Zhang, Xiaoliang Dong, Dan Yue, Liying Zhang, Haipeng Ji

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  5. NH 4 + ‐Induced Formation of Hexagonal‐K 1.5 (NH 4 + ) 0.5 SiF 6 :Mn 4+ with Polarized Zero‐Phonon Line Emission

    Laser & Photonics Review · 2025-06-16

    Zeyu Lyu, Hao‐Ran Zhao, Hao Dong, Shuai Wei, Mingxiang You, Chunchun Chen, Ling‐Dong Sun, HongPeng You, Chun‐Hua Yan

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  6. Mn⁴⁺-doping-induced structural transformation and luminescence enhancement in bulk (NH₄)₂SiF₆: Mn⁴⁺ crystal grown via cooling crystallization

    Journal of Alloys and Compounds · 2025-07-15

    Zhaowu Wang, Zhiyu Min, Liping Tian, Wenrui Zhang, Hao Li, Jinlong Chen, Derong Zhu

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  7. K 2 SiF 6 :Mn 4+ Red Phosphor Crystals: Near-Unity Quantum Efficiency, Size-Modulated Thermal Quenching, and Cooling-Crystallization Engineering of Millimeter Sizes for Crystal-to-Die Packaging

    Inorganic Chemistry · 2025-11-17

    Xiaoliang Dong, Mingxin Zhang, Dan Yue, Liying Zhang, Haipeng Ji

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  8. Achieving 57.15% EQE in Mn 4+ non-equivalent doped fluoride single crystals via a rapid synthesis for next-generation display lighting

    Inorganic Chemistry Frontiers · 2025-11-22

    Ziang Peng, Yuanjing Wang, Chuang Zhang, Hong Ming, Zhen Chen, Renhua Guo, Enhai Song, Qinyuan Zhang

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  9. A layer-stacking structure enabling K 2 TiF 6 :Mn 4+ platelet crystals for inorganic high-power WLED packaging

    Journal of Materials Chemistry C · 2026-01-01

    Yusen Liu, Tianyue Shi, Mingxin Zhang, Dan Yue, Liying Zhang, Haipeng Ji

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  10. Low-temperature crystallization of the K 2 TiF 6 :Mn 4+ phosphor with near-unity quantum efficiency in dilute HF solution

    Journal of Materials Chemistry C · 2026-01-01

    Tianyue Shi, Yusen Liu, Dan Yue, Liying Zhang, Haipeng Ji

    Read original paper ↗ ·

  11. Large-sized K2SiF6:Mn4+ phosphor crystals up to 3 mm grown by seeded growth with near-unity quantum efficiency

    Journal of Alloys and Compounds · 2026-01-15

    Mingxin Zhang, Mingxin Zhang, Xiaoliang Dong, Dan Yue, Liying Zhang, Haipeng Ji

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