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RESEARCH PAPER · Chemical Science · 2023

The first polyanion-substitution-driven centrosymmetric-to-noncentrosymmetric structural transformation realizing an excellent nonlinear optical supramolecule [Cd 4 P 2 ][CdBr 4 ]

Zhixin Qiu, Zhe-Xiong Zheng, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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The first polyanion-substitution-driven centrosymmetric-to-noncentrosymmetric structural transformation realizing an excellent nonlinear optical supramolecule [Cd 4 P 2 ][CdBr 4 ]OriginalSalt-inclusion chalcogenides with d-orbital components: unveiling remarkable nonlinear optical properties and dual-band photoluminescence10KREP 2 S 6 (RE = Sm, Gd, Tb, Dy): A Series of Polar Rare-Earth Thiophosphates with High Laser-Induced Damage Thresholds and Moderate Nonlinear-Optical Responses Synergistically Contributed by Isolated P 2 S 6 Units and {[RE 2 S 15 ] 24– } ∞ Layers8EuSi7P10: An Inorganic Supramolecular Nonlinear Optical Crystal Exhibiting Strong Second-Harmonic Generation Response4La 3 (Ga 3 S 3 O 3 )(Si 2 O 7 ): An Oxychalcogenide Demonstrating Ultrawide Optical Bandgap and Favorable Birefringence Propelled by Divergent Anionic Groups6Non-centrosymmetric structures designed rationally via a “dimensionality addition” strategy toward the promising nonlinear optical family [A–X][In–Se] (A = K/Ba and Rb/Ba; X = Cl and Br)13Photoluminescent, dielectric, and magnetic responsivity to the humidity variation in SHG-active pyroelectric manganese( ii )-based molecular material9First-Principles High-Throughput Screening and Experimental Verification of III-VIB Transition Metal Chalcogenides Nonlinear Optical Crystals16Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 1131Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 116Alkali Metal Substitution-Induced Structural Transformation for RbREP2Se6 (RE = Gd, Tb, Dy) with Second-Harmonic Generation Responses6Structural Symmetry and Mixed‐anion Engineering in Halopnictides for Extraordinary Second‐Harmonic Generation6Structural Symmetry and Mixed‐anion Engineering in Halopnictides for Extraordinary Second‐Harmonic Generation4Rare-Earth Selenophosphates Cs 2 YP 2 Se 7 and KYP 2 Se 6 Synthesized by the RFMOBQ Routine: Structural Evolution and Nonlinear Optical Activity2Bonding-type-driven structural transformation toward novel fluoroiodosulfates: Achieving non-centrosymmetry and enhanced optical properties in K2(IO3F)SO30Nonlinear Optical-Active NaAlP 2 S 6 Synthesized by the MOBQ Method: Synthesis, Structure, and Optical Properties0Parallel arrangement of functional building blocks: toward performance synergy in oxalate borate ultraviolet nonlinear optical crystals0Beyond the bandgap bottleneck: structure–property design principles for infrared nonlinear optical phosphides0

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  1. Salt-inclusion chalcogenides with d-orbital components: unveiling remarkable nonlinear optical properties and dual-band photoluminescence

    Chemical Science · 2024-01-01

    Shao‐Min Pei, Ming‐Shu Zhang, Fan Wu, Yan Guo, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  2. KREP 2 S 6 (RE = Sm, Gd, Tb, Dy): A Series of Polar Rare-Earth Thiophosphates with High Laser-Induced Damage Thresholds and Moderate Nonlinear-Optical Responses Synergistically Contributed by Isolated P 2 S 6 Units and {[RE 2 S 15 ] 24– } ∞ Layers

    Inorganic Chemistry · 2024-02-17

    Chen‐Yi Zhao, Wen‐Dong Yao, Mingyang Li, Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

    Read original paper ↗ ·

  3. EuSi7P10: An Inorganic Supramolecular Nonlinear Optical Crystal Exhibiting Strong Second-Harmonic Generation Response

    Inorganic Chemistry · 2024-05-30

    Yunxia Song, Chensheng Lin, Chao Wang, Yuqiao Zhou, Shenghao Fang, Pengxiang Dong, Bingxuan Li, Ning Ye, Xin Lei Zhao, Min Luo

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  4. La 3 (Ga 3 S 3 O 3 )(Si 2 O 7 ): An Oxychalcogenide Demonstrating Ultrawide Optical Bandgap and Favorable Birefringence Propelled by Divergent Anionic Groups

    ACS Materials Letters · 2024-12-19

    Ming‐Shu Zhang, Shao‐Min Pei, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  5. Non-centrosymmetric structures designed rationally via a “dimensionality addition” strategy toward the promising nonlinear optical family [A–X][In–Se] (A = K/Ba and Rb/Ba; X = Cl and Br)

    Materials Horizons · 2025-01-01

    Shao‐Min Pei, Fan Wu, Ming‐Shu Zhang, Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  6. Photoluminescent, dielectric, and magnetic responsivity to the humidity variation in SHG-active pyroelectric manganese( ii )-based molecular material

    Chemical Science · 2025-01-01

    Aleksander Hoffman, Mikołaj Żychowicz, Junhao Wang, K. Matsuura, Fumitaka Kagawa, Jan Rzepiela, Michał Heczko, Sebastian Baś, Hiroko Tokoro, Shin‐ichi Ohkoshi, Szymon Chorąży

    Read original paper ↗ ·

  7. First-Principles High-Throughput Screening and Experimental Verification of III-VIB Transition Metal Chalcogenides Nonlinear Optical Crystals

    Chemistry of Materials · 2025-01-23

    Miao Song, Hongbo Huang, Baoli Gao, Yumiao Niu, Ying Wang, Daqing Yang, Bingbing Zhang

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  8. Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 11

    Angewandte Chemie International Edition · 2025-02-26

    Shao‐Min Pei, Ming‐Shu Zhang, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  9. Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 11

    Angewandte Chemie · 2025-02-26

    Shao‐Min Pei, Ming‐Shu Zhang, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

    Read original paper ↗ ·

  10. Alkali Metal Substitution-Induced Structural Transformation for RbREP2Se6 (RE = Gd, Tb, Dy) with Second-Harmonic Generation Responses

    Inorganic Chemistry · 2025-08-08

    Zongze Li, Zi-Nan Chen, Ning Wang, Mao‐Yin Ran, Wenlong Liu, Sheng‐Ping Guo

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  11. Structural Symmetry and Mixed‐anion Engineering in Halopnictides for Extraordinary Second‐Harmonic Generation

    Angewandte Chemie International Edition · 2025-12-18

    Yi‐Bing Huang, Bin‐Wen Liu, Wei Wu, Xiao‐Ming Jiang, Xiyue Cheng, Guo‐Qiang Wang, Guo‐Cong Guo

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  12. Structural Symmetry and Mixed‐anion Engineering in Halopnictides for Extraordinary Second‐Harmonic Generation

    Angewandte Chemie · 2025-12-18

    Yi‐Bing Huang, Bin‐Wen Liu, Wei Wu, Xiao‐Ming Jiang, Xiyue Cheng, Guo‐Qiang Wang, Guo‐Cong Guo

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  13. Rare-Earth Selenophosphates Cs 2 YP 2 Se 7 and KYP 2 Se 6 Synthesized by the RFMOBQ Routine: Structural Evolution and Nonlinear Optical Activity

    Inorganic Chemistry · 2026-01-14

    Zong-Ze Li, Ming-Yang Li, Ning Wang, Mao‐Yin Ran, Sheng‐Ping Guo

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  14. Bonding-type-driven structural transformation toward novel fluoroiodosulfates: Achieving non-centrosymmetry and enhanced optical properties in K2(IO3F)SO3

    Materials Today Chemistry · 2026-01-16

    Juhui Cui, Junwei Feng, Feng Xia Yu, Minqiang Gai

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  15. Nonlinear Optical-Active NaAlP 2 S 6 Synthesized by the MOBQ Method: Synthesis, Structure, and Optical Properties

    Inorganic Chemistry · 2026-07-04

    Zong-Ze Li, Zi-Nan Chen, Sheng‐Ping Guo

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  16. Parallel arrangement of functional building blocks: toward performance synergy in oxalate borate ultraviolet nonlinear optical crystals

    Science China Chemistry · 2026-07-13

    Juhui Cui, Minqiang Gai, Ke Li, Z L Yang, Xueling Hou, Shilie Pan, Miriding Mutailipu

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  17. Beyond the bandgap bottleneck: structure–property design principles for infrared nonlinear optical phosphides

    Coordination Chemistry Reviews · 2026-09-22

    Zichang Wang, Dajiang Mei, Ximeng Lv, Shuchang Wu, Yang Liu, Jingdong Yan, Xiangran Kong, Hongwei Leng, Zuotao Lei, Chunhui Yang

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