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Probing of the Noninnocent Role of P in Transition-Metal Phosphide Hydrogen Evolution Reaction Electrocatalysts via Replacement with Electropositive Si Seongyoung Kong , Prashant Kumar Singh , Georgiy Akopov , Dapeng Jing , Ryan C. Davis , Jorge E. Perez-Aguilar , Jiyun Hong , Shannon Lee , Gayatri Viswanathan , Ernesto Soto , Muhammad Azhan , Tiago Picolo Fernandes , Stasia Harycki , Alexander Gundlach‐Graham , Yury V. Kolen’ko , Duane D. Johnson , Kirill A. Kovnir
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